PANDORA Project for the study of photonuclear reactions below

Tamii, Atsushi*; Pellegri, L.*; Sderstrm, P.-A.*; Allard, D.*; Goriely, S.*; Inakura, Tsunenori*; Khan, E.*; Kido, Eiji*; Kimura, Masaaki*; Litvinova, E.*; et al.

European Physical Journal A, 59(9), p.208_1 - 208_21, 2023/09

https://doi.org/10.1140/epja/s10050-023-01081-w

no abstracts in English

Hydrogen absorption and diffusion behaviors in cube-shaped palladium nanoparticles revealed by ambient-pressure X-ray photoelectron spectroscopy

Tang, J.*; Seo, O.*; Rivera Rocabado, D. S.*; Koitaya, Takanori*; Yamamoto, Susumu*; Namba, Yusuke*; Song, C.*; Kim, J.*; Yoshigoe, Akitaka; Koyama, Michihisa*; et al.

Applied Surface Science, 587, p.152797_1 - 152797_8, 2022/06

https://doi.org/10.1016/j.apsusc.2022.152797

The hydrogen absorption and diffusion mechanisms on cube-shaped Pd nanoparticles (NPs) which are important hydrogen-storage materials were studied using X-ray photoelectron spectroscopy and DFT calculations. In the surface region, hydrogen absorption showed almost similar behavior regardless of the NPs size. It was found that the octahedral sites are more favorable than the tetrahedral sites for hydrogen occupation. We also clarified that the hydrogen atoms absorbing on the smaller-sized Pd NPs diffuse to the subsurface more actively because of the weakened Pd-H bond by the surface disordering, which plays an important role in hydrogen adsorption at a low H pressure.

A Modeling study on the oceanic dispersion and sedimentation of radionuclides off the coast of Fukushima

Kamidaira, Yuki; Uchiyama, Yusuke*; Kawamura, Hideyuki; Kobayashi, Takuya; Otosaka, Shigeyoshi*

Journal of Environmental Radioactivity, 238-239, p.106724_1 - 106724_16, 2021/11

https://doi.org/10.1016/j.jenvrad.2021.106724

A three-dimensional oceanic dispersion model considering the migration of radionuclides between seawater and sediments was developed. The migration mechanism of dissolved Cs-137 originating from the Fukushima Daiichi Nuclear Power Plant accident to sediments was investigated. The comparison between the model and the observed data showed that the model can adequately reproduce the ocean structure and the concentration of Cs-137 in seawater and sediments. Cs-137 distribution in the sediment off the Fukushima coast was formed mainly owing to adsorption from the dissolved phase by June 2011, when the impact of the direct oceanic Cs-137 release from FNPP1 was remarkable.

Development of regional downscaling capability in STEAMER ocean prediction system based on multi-nested ROMS model

Kamidaira, Yuki; Kawamura, Hideyuki; Kobayashi, Takuya; Uchiyama, Yusuke*

Journal of Nuclear Science and Technology, 56(8), p.752 - 763, 2019/08

https://doi.org/10.1080/00223131.2019.1613269

Oceanic regional downscaling capability was implemented into Short-Term Emergency Assessment system of Marine Environmental Radioactivity (STEAMER) developed by Japan Atomic Energy Agency to enable us to predict more realistically the oceanic dispersion of radionuclides at higher spatiotemporal resolutions for broader applications. The system consisted of a double-nested oceanic downscaling circulation model with tidal forcing and an oceanic radionuclide dispersion model. This system was used to comparatively examine downscaling and tidal effects on the dispersion of radionuclides hypothetically released from the Fukushima Daiichi Nuclear Power Plant in the colder season. The simulated dissolved Cs distribution was different from that obtained using coarser-resolution models because downscaling enhanced both horizontal and vertical mixing. The suppression of horizontal mixing and the promotion of vertical mixing by tidal forcing synergistically reduced offshore Cs transport. In addition, the submesoscale effects strengthened the three-dimensional Cs fluctuations by 10 times, while the tidal effects promoted slightly increased the intensity of three-dimensional Cs fluctuations by approximately 3%. This indicated that the submesoscale effects substantially surpassed tidal forcing in oceanic mixing in the coastal margin off Fukushima in the colder season.

Verification of alternative dew point hygrometer for CV-LRT in MONJU; Short- and long-term verification for capacitance-type dew point hygrometer (Translated document)

Ichikawa, Shoichi; Chiba, Yusuke; Ono, Fumiyasu; Hatori, Masakazu; Kobayashi, Takanori; Uekura, Ryoichi; Hashiri, Nobuo*; Inuzuka, Taisuke*; Kitano, Hiroshi*; Abe, Hisashi*

JAEA-Research 2017-001, 40 Pages, 2017/03

JAEA-Research-2017-001.pdf:5.19MB

In order to reduce the influence on a plant schedule of the MONJU by the maintenance of dew point hygrometers, The JAEA examined a capacitance type dew point hygrometer as an alternative dew point hygrometer for a lithium-chloride type dew point hygrometer which had been used at the CV-LRT in the MONJU. As a result of comparing a capacitance type dew point hygrometer with a lithium-chloride type dew point hygrometer at the CV-LRT (Atmosphere: nitrogen, Testing time: 24 hours), there weren't significant difference between a capacitance type dew point hygrometer and a lithium-chloride type dew point hygrometer. As a result of comparing a capacitance dew point hygrometer with a high-mirror-surface type dew point hygrometer for long term verification (Atmosphere: air, Testing time: 24 months), the JAEA confirmed that a capacitance type dew point hygrometer satisfied the instrument specification (2.04C) required by the JEAC4203-2008.

Constitutive modeling for compacted bentonite buffer materials as unsaturated and saturated porous media

Takayama, Yusuke; Tachibana, Shinya*; Iizuka, Atsushi*; Kawai, Katsuyuki*; Kobayashi, Ichizo*

Soils and Foundations, 57(1), p.80 - 91, 2017/02

https://doi.org/10.1016/j.sandf.2017.01.006

Bentonite has remarkable swelling characteristics and low permeability that makes it a suitable buffer material in a purpose built repository for the geological disposal of radioactive waste. It is necessary to use reliable numerical simulation techniques to demonstrate that the repository is safe and mechanically stable for tens of thousands of years. Constitutive model that describes the mechanical behavior of bentonite is a key technique in such numerical simulations. The current paper proposes a constitutive model for bentonite, which treats bentonite as an unsaturated elasto-plastic material that changes its mechanical properties as it becomes saturated. In the proposed model, the swelling index and an expression formula for negative dilatancy are treated as functions of degree-of-saturation. Montmorillonite content is used as an input parameter in the proposed model and so is applicable to a variety of bentonite based materials of varying montmorillonite content. Experimental results from swelling volume and swelling pressure tests taken from the literature are shown to be satisfactorily predicted by the proposed model.

Three-dimensional stress analysis of reflooding tunnel during submerging process using crack tensor model at Mizunami Underground Research Laboratory

Ozaki, Yusuke; Matsui, Hiroya; Kuwabara, Kazumichi; Tada, Hiroyuki*; Sakurai, Hideyuki*; Kumasaka, Hiroo*; Goke, Mitsuo*; Kobayashi, Shinji*

JAEA-Research 2016-007, 125 Pages, 2016/06

JAEA-Research-2016-007.pdf:34.66MB

In Mizunami Underground Research Laboratory (MIU), the stress analysis of fractured rock have been performed with crack tensor model. In MIU, a reflooding test is performed at 500m stage. In this study, stress analysis of rock during submerging process of the tunnel is performed by using crack tensor model. The deformation of the rock under different water levels in the tunnel is simulated. The stress condition by high pressure due to inflow of groundwater into tunnel is also estimated. These simulation are performed under assumption that groundwater does not permeate into rock for the estimation of maximum pressure acting on the rock. The stress analysis with consideration of permeation of groundwater into rock is also conducted for the estimation of stress condition after the diffusion of water pressure in tunnel. The results of these analyses lead the conclusion that the pressure of the rock reaches the groundwater pressure near the face of tunnel when the tunnel is submerged.

Three-dimensional excavation analysis based on crack tensor model at the Mizunami Underground Research Laboratory

Takayama, Yusuke; Sato, Toshinori; Sanada, Hiroyuki; Tada, Hiroyuki*; Kumasaka, Hiroo*; Fukuda, Tsuyoshi*; Kobayashi, Shinji*

JAEA-Research 2015-003, 102 Pages, 2015/07

JAEA-Research-2015-003.pdf:20.21MB

In the rock mechanical study in the Mizunami Underground Research Laboratory Project, the development of the evaluation method for the excavation damaged zone due to excavation of shafts and research galleries is one of the important issues. In this study, three-dimensional excavation analysis is conducted. Crack tensor used in these analysis were measured using the data collected in wall surface observation in study tunnels such as the horizontal tunnels to a depth of 500 m. The results of analysis were compared with existing measurements at a depth of 500 m obtained using in-situ strain meters. The excavation analysis using crack tensor and initial stress obtained from the Phase I and Phase II were carried out to examine the influence of crack tensor and initial stress on the results of analysis.

Observation of ion cyclotron emission owing to DD fusion product H ions in JT-60U

Sato, Shoichi*; Ichimura, Makoto*; Yamaguchi, Yusuke*; Katano, Makoto*; Imai, Yasutaka*; Murakami, Tatsuya*; Miyake, Yuichiro*; Yokoyama, Takuro*; Moriyama, Shinichi; Kobayashi, Takayuki; et al.

Plasma and Fusion Research (Internet), 5, p.S2067_1 - S2067_4, 2010/12

https://doi.org/10.1585/pfr.5.S2067

Ion cyclotron emissions (ICEs) due to deuterium-deuterium fusion-product (FP) ions on JT-60U are studied. ICE due to H-ions is identified from the difference of the toroidal wave number of 2nd ICE(D). The parameter dependence for the appearance of ICE(H) is investigated from the experimental conditions and also is studied by using "Escape Particle Orbit analysis Code (EPOC)".

Isotope fractionation due to sedimentation of atoms in centrifuged indium-lead alloy

Ono, Masao; Iguchi, Yusuke*; Okayasu, Satoru; Esaka, Fumitaka; Kobayashi, Katsura*; Hao, T.; Bagum, R.*; Osawa, Takahito; Fujii, Kimio; Nakamura, Eizo*; et al.

Defect and Diffusion Forum, 289-292, p.63 - 68, 2009/04

The atomic-scale graded structure of In-Pb alloy was formed by an ultracentrifuge experiment under conditions that a gravitational field of 0.8110 G for 100 hours at 150 C in solid state in our previous study. The isotope ratio measurements were performed on the centrifuged sample with secondary ion mass spectrometer (SIMS). Pb/Pb and Pb/Pb isotope ratio changed with negative gradient in the direction of centrifugal force approximately 1.5% and 0.8%, respectively. And three-isotope diagram of Pb/Pb versus Pb/Pb proved that the isotope fluctuation depends on isotopic mass difference. These results showed that the strong gravitational field not only affected on the inter-diffusion but also on self-diffusion in this alloy as causing isotope fractionation effect, and the isotope fractionation was dependent on mass-difference.