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JAEA Reports

Carrying-out of whole nuclear fuel materials in Plutonium Research Building No.1

Inagawa, Jun; Kitatsuji, Yoshihiro; Otobe, Haruyoshi; Nakada, Masami; Takano, Masahide; Akie, Hiroshi; Shimizu, Osamu; Komuro, Michiyasu; Oura, Hirofumi*; Nagai, Isao*; et al.

JAEA-Technology 2021-001, 144 Pages, 2021/08

JAEA-Technology-2021-001.pdf:12.98MB

Plutonium Research Building No.1 (Pu1) was qualified as a facility to decommission, and preparatory operations for decommission were worked by the research groups users and the facility managers of Pu1. The operation of transportation of whole nuclear materials in Pu1 to Back-end Cycle Key Element Research Facility (BECKY) completed at Dec. 2020. In the operation included evaluation of criticality safety for changing permission of the license for use nuclear fuel materials in BECKY, cask of the transportation, the registration request of the cask at the institute, the test transportation, formulation of plan for whole nuclear materials transportation, and the main transportation. This report circumstantially shows all of those process to help prospective decommission.

JAEA Reports

Data on plutonium sorption onto rock; Results of the experiment for data on plutonium sorption onto tuff under conditions of reducing and of presence of nitrate

Suguro, Toshiyasu; Nishikawa, Yoshiaki*; Komuro, Takashi*; Kagawa, Akio; Kashiwazaki, Hiroshi; Yamada, Kazuo

JAEA-Technology 2007-058, 20 Pages, 2007/11

JAEA-Technology-2007-058.pdf:3.26MB

For safety assessment of TRU waste disposal, data on sorption data of plutonium on Tuff have been obtained by a static batch-type experiment. Because the repository condition will be reducing and be affected by considerable amount of nitrate in waste, the authors carried out the experiments using Tuff under the reducing (Na$$_{2}$$S$$_{2}$$O$$_{4}$$ as added as reductant) and anoxic condition (O$$_{2}$$$$leq$$1 ppm) and solution of 0 to 0.5 M NaNO$$_{3}$$. The experimental results suggest that distribution coefficient (Kd) ranges 0.2 to 0.7 m$$^{3}$$ kg$$^{-1}$$ in case of L/S=0.1 m$$^{3}$$ kg$$^{-1}$$. Similarly the Kd ranges, 1 to 7 m$$^{3}$$ kg$$^{-1}$$ at L/S=1 m$$^{3}$$ kg$$^{-1}$$. However, almost samples of the solution after experiments were plutonium solubility less than detection limit(10$$^{-13}$$mol/dm$$^{3}$$) of alpha spectrometer. The reason, it is guessed plutonium coprecipitation with calcium hydroxide, because experiments using saturated calcium hydroxide in the liquid.

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