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Yamashita, Kiyoto; Maki, Shota; Yokosuka, Kazuhiro; Fukui, Masahiro; Iemura, Keisuke
JAEA-Technology 2023-023, 97 Pages, 2024/03
The incinerator adopted to incineration room, Plutonium Waste Treatment Facility had been demonstrated since 2002 for developing technologies to reduce the volume of fire-resistant wastes such as vinyl chloride (represented by Polyvinyl chloride bags) and rubber gloves for Radio Isotope among radioactive solid wastes generated by the production of mixed oxide fuels. The incinerator, cooling tower, and processing pipes were replaced with a suspension period from 2018 to 2022, which fireproof materials on the inner wall of the incinerator was cracked and grown caused by hydrogen chloride generated when disposing of fire-resistant wastes. This facility consists of the waste feed process, the incineration process, the waste gas treatment process, and the ash removal process. We replaced the cooling tower in the waste gas treatment process from March 2020 to March 2021, and the incinerator in the incineration process from January 2021 to February 2022. In addition, samples were collected from the incinerator and the cooling tower during the removing and dismantling of the replaced devices, observed by Scanning Electron Microscope and X-ray microanalyzer, and analyzed by X-ray diffraction to investigate the corrosion and deterioration of them. This report describes the method of setting up the green house, the procedure for replacing them, and the results from analysis in corrosion and deterioration of the cooling tower and incinerator.
Hirano, Tatsumi*; Maeda, Takehiro*; Murata, Tetsuyuki*; Yamaki, Takahiro*; Matsubara, Eiichiro*; Shobu, Takahisa; Shiro, Ayumi*; Yasuda, Ryo*; Takamatsu, Daiko*
SPring-8/SACLA Riyo Kenkyu Seikashu (Internet), 11(1), p.49 - 57, 2023/02
Yamashita, Kiyoto; Yokoyama, Aya*; Takagai, Yoshitaka*; Maki, Shota; Yokosuka, Kazuhiro; Fukui, Masahiro; Iemura, Keisuke
JAEA-Technology 2022-020, 106 Pages, 2022/10
Radioactive solid wastes generated by Fukushima Daiichi Nuclear Power Station disaster may contain high levels of salt from the tsunami and seawater deliberately released into the area. It is assumed that polyvinyl chloride (PVC) products may be used for decommissioning work and for containment of radioactive wastes in the future. Among the method of handling them, incineration is one method that needs to be investigated as it is good method for reduction and stabilization of wastes. But in order to dispose of Trans-Uranic (TRU) solid waste containing chlorides, it is necessary to select the structure and materials of the facility based on the information such as the movement of nuclides and chlorides in the waste gas treating system and the corrosion of equipment due to chlorides. Therefore, we decided to get various data necessary to design a study of the incineration facilities. And we decided to examine the transfer behavior of chlorides to the waste gas treatment system, the corrosion-resistance of materials in the incineration facilities, and the distribution survey of plutonium in them obtained using the Plutonium-contaminated Waste Treatment Facility (PWTF), Nuclear Fuel Cycle Engineering Laboratories, which is a unique incinerating facility in Japan. This report describes the transfer behavior of chlorides in the waste gas treatment system, the evaluation of corrosion-resistance materials and the distribution survey of plutonium in the incineration facilities obtained by these tests using the Plutonium-contaminated Waste Treatment Facility, Nuclear Fuel Cycle Engineering Laboratories.
Zheng, X.; Tamaki, Hitoshi; Takahara, Shogo; Sugiyama, Tomoyuki; Maruyama, Yu
Proceedings of Probabilistic Safety Assessment and Management (PSAM16) (Internet), 10 Pages, 2022/09
Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.
Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03
Times Cited Count:44 Percentile:96.93(Astronomy & Astrophysics)Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.
Tanaka, Taiki*; Narikiyo, Yoshihiro*; Morita, Kosuke*; Fujita, Kunihiro*; Kaji, Daiya*; Morimoto, Koji*; Yamaki, Sayaka*; Wakabayashi, Yasuo*; Tanaka, Kengo*; Takeyama, Mirei*; et al.
Journal of the Physical Society of Japan, 87(1), p.014201_1 - 014201_9, 2018/01
Times Cited Count:18 Percentile:74.47(Physics, Multidisciplinary)Excitation functions of quasielastic scattering cross sections for the Ca + Pb, Ti + Pb, and Ca + Cm reactions were successfully measured by using the gas-filled recoil-ion separator GARIS. Fusion barrier distributions were extracted from these data, and compared with the coupled-channels calculations. It was found that the peak energies of the barrier distributions for the Ca + Pb and Ti + Pb systems coincide with those of the 2n evaporation channel cross sections for the systems, while that of the Ca + Cm is located slightly below the 4n evaporation ones. This results provide us helpful information to predict the optimum beam energy to synthesize superheavy nuclei.
Kimata, Tetsuya*; Kato, Sho*; Yamaki, Tetsuya; Yamamoto, Shunya; Kobayashi, Tomohiro*; Terai, Takayuki*
Surface & Coatings Technology, 306(Part A), p.123 - 126, 2016/11
Times Cited Count:13 Percentile:52.49(Materials Science, Coatings & Films)Platinum (Pt) nanoparticle catalysts with oxygen reduction reaction (ORR) activity are required for practical applications of polymer electrolyte fuel cells. We prepared Pt nanoparticles on an Ar-irradiated glassy carbon (GC) surface by a radio-frequency magnetron sputtering method to investigate the influence of the ion-induced lattice defects in GC on the ORR activity of the deposited Pt nanoparticles. Interestingly, the Pt nanoparticles on the irradiated surface exhibited ca. 2.5 times higher specific activity than those on the non-irradiated one. X-ray photoelectron spectroscopy suggested the interfacial Pt-C interaction occurring between the irradiated GC and Pt nanoparticles, which should be a reason for improvement of the ORR activity.
Shibama, Yusuke; Okano, Fuminori; Yagyu, Junichi; Kaminaga, Atsushi; Miyo, Yasuhiko; Hayakawa, Atsuro*; Sagawa, Keiich*; Mochida, Tsutomu*; Morimoto, Tamotsu*; Hamada, Takashi*; et al.
Fusion Engineering and Design, 98-99, p.1614 - 1619, 2015/10
Times Cited Count:4 Percentile:33.25(Nuclear Science & Technology)The JT-60SA vacuum vessel (150 tons) is a double wall torus structure and the maximum major radius of 5.0 m and height of 6.6 m. The manufacturing design concept is that the vessel is split in the 10 toroidal sectors manufactured at factory, and assembled on-site; seven of the 40-degree sectors, two of the 30-degree beside final one, and the final of the 20-degree. The final sector is assembled with the VV thermal shield and toroidal field magnets into the 340-degree as prepared in one sector. Sectors are temporally fitted on-site and adjusted one over the other before the assembly. After measurement of the dimensions and the reference, these sectors are transferred onto the cryostat base. First, three 80-degree sectors are manufactured with mating each 40-degree sector by direct joint welding. The rest sectors including the final sector are jointed with splice plates. Welding manipulator and its guide rails are used for these welding. In this paper, the detail of the VV sectors assembly including the final sector is explained. Welding technologies to joint the two of 40-degree sectors are reported with the present manufacturing status and the welding trial on the vertical stub with the partial mock-up of the final sector are discussed with the assembly process.
Yoshihara, Toshihiro*; Suzui, Nobuo; Ishii, Satomi; Kitazaki, Mayu*; Yamazaki, Haruaki*; Kitazaki, Kazuyoshi*; Kawachi, Naoki; Yin, Y.-G.; Tanabata, Sayuri*; Hashida, Shinnosuke*; et al.
Plant, Cell & Environment, 37(5), p.1086 - 1096, 2014/05
Times Cited Count:24 Percentile:65.61(Plant Sciences)Kato, Sho; Yamaki, Tetsuya; Yamamoto, Shunya; Hakoda, Teruyuki; Kawaguchi, Kazuhiro; Kobayashi, Tomohiro*; Suzuki, Akihiro*; Terai, Takayuki*
Nuclear Instruments and Methods in Physics Research B, 314, p.149 - 152, 2013/11
Times Cited Count:2 Percentile:19.73(Instruments & Instrumentation)We implanted 100 keV W in unpolished GC substrates at nominal fluences up to ions/cm. The implanted samples were electrochemically anodized in a NaOH aqueous solution to etch the surface layer. The analyses were performed by X-ray photoelectron spectroscopy (XPS), Rutherford backscattering spectrometry (RBS), and transmission electron microscopy (TEM). XPS W 4f spectra indicated the formation of carbides as reported previously. The electrochemical etching clearly increased the W concentration on the surface. According to the RBS results, half of the implanted W atoms were retained in the substrate, while the rest should escape to the etching solution. The cross-sectional TEM image revealed a uniform distribution of WC particles with a diameter of less than 10 nm just near the surface region.
Shibanuma, Kiyoshi; Arai, Takashi; Hasegawa, Koichi; Hoshi, Ryo; Kamiya, Koji; Kawashima, Hisato; Kubo, Hirotaka; Masaki, Kei; Saeki, Hisashi; Sakurai, Shinji; et al.
Fusion Engineering and Design, 88(6-8), p.705 - 710, 2013/10
Times Cited Count:10 Percentile:61.16(Nuclear Science & Technology)Kato, Sho; Yamaki, Tetsuya; Yamamoto, Shunya; Hakoda, Teruyuki; Kawaguchi, Kazuhiro; Kobayashi, Tomohiro*; Suzuki, Akihiro*; Terai, Takayuki*
Transactions of the Materials Research Society of Japan, 38(1), p.81 - 84, 2013/03
Nanoparticles were formed by 100 keV tungsten-ion implantation in unpolished glassy carbon substrates at nominal fluences of - ions/cm. The implanted samples were analyzed by Rutherford backscattering spectrometry, X-ray photoelectron spectroscopy, hydrodynamic voltammetry using a rotating disk electrode, and field emission scanning electron microscopy. A significant sputtering effect changed the depth profile during the course of irradiation and limited the amount of tungsten retainable in the substrate in agreement with our calculated distributions. The nanoparticles were composed of tungsten carbide and dispersed uniformly with diameters of around 10 nm.
Kamiya, Koji; Onishi, Yoshihiro; Ichige, Toshikatsu; Furukawa, Masato; Murakami, Haruyuki; Kizu, Kaname; Tsuchiya, Katsuhiko; Yoshida, Kiyoshi; Mizumaki, Shoichi*
Proceedings of 24th International Cryogenic Engineering Conference (ICEC 24) and International Cryogenic Materials Conference 2012 (ICMC 2012) (CD-ROM), p.587 - 590, 2012/05
The JT-60 plans to be upgraded to a full-superconducting tokamak referred as the JT-60 Super Advance (JT-60SA) as one of the JA-EU broader approach projects. In the JT-60SA, the superconducting magnets are surrounded by thermal shield cooled at 80 K, which is categorized into 3 groups; the vacuum vessel thermal shield (VVTS), the port thermal shield (PTS) and the cryostat thermal shield (CTS). In this study, seismic analysis was conducted for the thermal shield to confirm the soundness of the latest design, taking the dynamical analysis into account. Trial manufacturing of a 10 degree outer VVTS was also conducted. The outer VVTS was subsequently assembled with already existing inner VVTS to measure the total tolerance (manufacturing plus assembly). It was found that the total tolerance was 5.2 mm which is less than the target tolerance of 10 mm. Finally, concept and the current status of the JT-60SA cryodistribution design are reported.
Asano, Shiro*; Okuyama, Toshihisa*; Onawa, Toshio*; Yanagi, Yutaka*; Ejiri, Mitsuru*; Kanahara, Toshio*; Ichihashi, Koji*; Kikuchi, Atsushi*; Mizumaki, Shoichi*; Masaki, Kei; et al.
Fusion Engineering and Design, 86(9-11), p.1816 - 1820, 2011/10
Times Cited Count:12 Percentile:66.82(Nuclear Science & Technology)The real vacuum vessel (VV) manufacturing of JT-60SA has started since Nov. 2009 at Toshiba. Prior to starting manufacturing, fundamental welding R&Ds had been performed by three stages. In the first stage, primary tests for screening welding method were performed. In the second stage, the trial welding for 1m-long straight and curved double shell samples were conducted. The dependences of welding quality and distortion on the welding conditions, such as arc voltage and current, setting accuracy, welding sequence, the shape of grooves, etc. were measured. In addition, welding condition with low heat input was explored. In the last stage, fabrication sequence was confirmed and established by the trial manufacturing of the 20 upper half mock-up. This poster presents the R&D results obtained in the first and second stages.
Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Aramaki, Y.*; et al.
Physical Review C, 83(4), p.044912_1 - 044912_16, 2011/04
Times Cited Count:9 Percentile:49.7(Physics, Nuclear)Measurements of electrons from the decay of open-heavy-flavor mesons have shown that the yields are suppressed in Au+Au collisions compared to expectations from binary-scaled collisions. Here we extend these studies to two particle correlations where one particle is an electron from the decay of a heavy flavor meson and the other is a charged hadron from either the decay of the heavy meson or from jet fragmentation. These measurements provide more detailed information about the interaction between heavy quarks and the quark-gluon matter. We find the away-side-jet shape and yield to be modified in Au+Au collisions compared to collisions.
Fujita, Satoshi*; Kuma, Kenshi*; Ishikawa, Satoko*; Nishimura, Shotaro*; Nakayama, Yuta*; Ushizaka, Satomi*; Isoda, Yutaka*; Otosaka, Shigeyoshi; Aramaki, Takafumi*
Journal of Geophysical Research, 115(C12), p.C12001_1 - C12001_12, 2010/12
Times Cited Count:16 Percentile:38.53(Oceanography)Vertical distributions of dissolved iron (D-Fe, less than 0.22 micrometer fraction), total iron (T-Fe, unfiltered), and chemical and biological components (e.g., nutrients) in seawater were determined at seven stations in the Japan Sea to understand the mechanisms that control iron behavior. Distributions of the D-Fe were characterized by surface depletion, mid-depth maxima, then slight decrease with depth in deep water and uniform concentration in bottom water because of biological uptake in the surface water and release from microbial decomposition of sinking organic matter in mid-depth water. The T-Fe concentrations in the deep-water column were variable with different T-Fe levels among stations and depths. We found a significant relationship of the exponential increase in the T-Fe concentrations with decreasing water transmittance, resulting from the iron supply into the deep and bottom waters due to the lateral transport of resuspended sediment from the continental slope.
Matsumura, Hiroyoshi*; Adachi, Motoyasu; Sugiyama, Shigeru*; Okada, Shino*; Yamakami, Megumi*; Tamada, Taro; Hidaka, Koshi*; Hayashi, Yoshio*; Kimura, Toru*; Kiso, Yoshiaki*; et al.
Acta Crystallographica Section F, 64(11), p.1003 - 1006, 2008/11
Times Cited Count:17 Percentile:77.92(Biochemical Research Methods)This paper reports the crystallization and preliminary neutron diffraction measurements of HIV-1 protease, a potential target for anti-HIV therapy, complexed with an inhibitor (KNI-272). The aim of this neutron diffraction study is to obtain structural information about the H atoms and to determine the protonation states of the residues within the active site. The crystal was grown to a size of 1.4 mm by repeated macroseeding and a slow-cooling method using a two-liquid system. Neutron diffraction data were collected at room temperature using a BIX-4 diffractometer at the JRR-3 research reactor of the Japan Atomic Energy Agency (JAEA). The data set was integrated and scaled to 2.3 resolution in space group P2(1)2(1)2, with unit-cell parameters a = 59.5, b = 87.4, c = 46.8 .
Sekimoto, Hitoshi*; Kawachi, Naoki; Honda, Shuzo*; Yamaguchi, Yoshie*; Kato, Shota*; Yoneyama, Kaori*; Fujimaki, Shu; Suzui, Nobuo; Ishii, Satomi; Watanabe, Satoshi; et al.
JAEA-Review 2007-060, JAEA Takasaki Annual Report 2006, P. 124, 2008/03
no abstracts in English
Sekimoto, Hitoshi; Honda, Shuzo*; Kato, Shota*; Ochiai, Yukiko*; Yoneyama, Kaori*; Yoneyama, Koichi*; Takeuchi, Yasutomo*; Kawachi, Naoki; Fujimaki, Shu; Suzui, Nobuo; et al.
JAEA-Review 2006-042, JAEA Takasaki Annual Report 2005, P. 125, 2007/02
Tomita, Yutaka; Morihira, Masayuki; Tamaki, Yoshihisa*; Nishimura, Kazuhisa*; Shoji, Shuichi*; Kihara, Yoshiyuki; Kase, Takeshi; Koizumi, Tsutomu
JAEA-Research 2006-088, 95 Pages, 2007/01
JAEA has developed sphere-pac fuels in the feasibility study on commercialized FBR cycle systems as one of the candidates for low decontamination TRU fuels. Optimization of the fabrication condition for coarse spheres, development of an improved external gelation process, and examination of peculiar problems for the low decontamination fuel were carried out in Phase II. The results are shown as follows. (1) Fabrication condition of coarse spheres was optimized. (2) Feasibility of the improved external gelation process was confirmed. (3) Rare earth elements did not bring any problem for the characteristic of spheres and fabrication condition. (4) Radiation resistant data of the feed solution was acquired. Results of tests show the feasibility of the external gelation process for the low decontamination TRU fuel microsphere fabrication.