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Journal Articles

Current status of decommissioning and waste management at the Ningyo-Toge Environmental Engineering Center

Ohashi, Yusuke; Shimaike, Masamitsu; Matsumoto, Takashi; Takahashi, Nobuo; Yokoyama, Kaoru; Morimoto, Yasuyuki

Nuclear Technology, 209(5), p.777 - 786, 2023/05

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

At the Ningyo-Toge Center, technical development related to uranium refining conversion and enrichment has been completed, and decommissioning of these facilities has begun. The error between the quantity of dismantled materials estimated from the facility design drawings and the actual quantity of dismantled materials was minimal when averaging over the entire Uranium Refining and Conversion Plant and Uranium Enrichment Engineering Facility, which results indicated that the preliminary estimate of the quantity of dismantled materials for decommissioning was reasonable. Most of the dismantled materials, which have no contamination history and are properly managed were able to be carried out to recyclers as non-radioactive waste (NR). In addition, the possibility of evaluating the uranium concentration of clearance level in dismantled objects was confirmed through gamma-ray measurement tests using mock-up waste.

JAEA Reports

Separation/removal of steel surface coating film by laser cleaning

Yamane, Ikumi; Takahashi, Nobuo; Sawayama, Kengo; Nishiwaki, Hiroki; Matsumoto, Takashi; Ogawa, Jumpei; Nomura, Mitsuo; Arima, Tatsumi*

JAEA-Technology 2021-038, 18 Pages, 2022/02

JAEA-Technology-2021-038.pdf:1.61MB

We have dismantled uranium enrichment facilities in Ningyo-toge Environmental Engineering Center since their operation finished in 2001, and the total amount of metallic wastes is estimated to be about 130 thousand tons. Eighty percent of them can be disposed as nonradioactive waste (NR), but there are some steel parts possibly uranium-contaminated. We need removing painted surface of such steels and radiologically surveying to dispose them as NRs. Though painted surfaces have been conventionally removed through hand working with grinders, this manual work requires installation of green house, protective clothing, and full-face mask, in order to prevent dispersion and inhalation of airborne dusts. We desire further developments of surface cleaning techniques to reduce time, cost, workload, and secondary waste generation caused by excessive grinding. Therefore, in this study, we focused on the laser cleaning technology used for the separation and removal of paint films at construction sites. In order to improve the coating separation and removal technology for NR objects, we evaluated the coating separation and removal performance of NR steel surface by laser cleaning system, observed the coating scattering behavior by high-speed camera and investigated the coating recovery method, evaluated the laser separation and removal performance of steel surface powder, and thermodynamically evaluated the uranium compounds on steel surface. We additionally evaluated the feasibility of laser cleaning techniques in our works basing on these results, and discussed future work plans for further developments of laser cleaning techniques.

Journal Articles

PSTEP: Project for solar-terrestrial environment prediction

Kusano, Kanya*; Ichimoto, Kiyoshi*; Ishii, Mamoru*; Miyoshi, Yoshizumi*; Yoden, Shigeo*; Akiyoshi, Hideharu*; Asai, Ayumi*; Ebihara, Yusuke*; Fujiwara, Hitoshi*; Goto, Tadanori*; et al.

Earth, Planets and Space (Internet), 73(1), p.159_1 - 159_29, 2021/12

 Times Cited Count:6 Percentile:52.8(Geosciences, Multidisciplinary)

The PSTEP is a nationwide research collaboration in Japan and was conducted from April 2015 to March 2020, supported by a Grant-in-Aid for Scientific Research on Innovative Areas from the Ministry of Education, Culture, Sports, Science and Technology of Japan. It has made a significant progress in space weather research and operational forecasts, publishing over 500 refereed journal papers and organizing four international symposiums, various workshops and seminars, and summer school for graduate students at Rikubetsu in 2017. This paper is a summary report of the PSTEP and describes the major research achievements it produced.

Journal Articles

Quantum proton entanglement on a nanocrystalline silicon surface

Matsumoto, Takahiro*; Sugimoto, Hidehiko*; Ohara, Takashi; Tokumitsu, Akio*; Tomita, Makoto*; Ikeda, Susumu*

Physical Review B, 103(24), p.245401_1 - 245401_9, 2021/06

 Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)

Journal Articles

Determination of localized surface phonons in nanocrystalline silicon by inelastic neutron scattering spectroscopy and its application to deuterium isotope enrichment

Matsumoto, Takahiro*; Nomata, Ikumi*; Ohara, Takashi; Kanemitsu, Yoshihiko*

Physical Review Materials (Internet), 5(6), p.066003_1 - 066003_9, 2021/06

 Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)

Journal Articles

High-temperature antiferromagnetism in Yb based heavy fermion systems proximate to a Kondo insulator

Suzuki, Shintaro*; Takubo, Ko*; Kuga, Kentaro*; Higemoto, Wataru; Ito, Takashi; Tomita, Takahiro*; Shimura, Yasumichi*; Matsumoto, Yosuke*; Bareille, C.*; Wadachi, Hiroki*; et al.

Physical Review Research (Internet), 3(2), p.023140_1 - 023140_12, 2021/05

We report our experimental discovery of the transition temperature reaching 20 K in a Yb-based compound at ambient pressure. The Mn substitution at the Al site in an intermediate valence state of $$alpha$$-YbAlB$$_4$$ not only induces antiferromagnetic transition at a record high temperature of 20 K but also transforms the heavy-fermion liquid state in $$alpha$$-YbAlB$$_4$$ into a highly resistive metallic state proximate to a Kondo insulator.

Journal Articles

Visualization of the boron distribution in core material melting and relocation specimen by neutron energy resolving method

Abe, Yuta; Tsuchikawa, Yusuke; Kai, Tetsuya; Matsumoto, Yoshihiro*; Parker, J. D.*; Shinohara, Takenao; Oishi, Yuji*; Kamiyama, Takashi*; Nagae, Yuji; Sato, Ikken

JPS Conference Proceedings (Internet), 33, p.011075_1 - 011075_6, 2021/03

Journal Articles

Development of three-dimensional distribution visualization technology for boron using energy resolved neutron-imaging system (RADEN)

Abe, Yuta; Tsuchikawa, Yusuke; Kai, Tetsuya; Matsumoto, Yoshihiro*; Parker, J. D.*; Shinohara, Takenao; Oishi, Yuji*; Kamiyama, Takashi*; Nagae, Yuji; Sato, Ikken

Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 6 Pages, 2020/08

Journal Articles

The Energy-resolved neutron imaging system, RADEN

Shinohara, Takenao; Kai, Tetsuya; Oikawa, Kenichi; Nakatani, Takeshi; Segawa, Mariko; Hiroi, Kosuke; Su, Y. H.; Oi, Motoki; Harada, Masahide; Iikura, Hiroshi; et al.

Review of Scientific Instruments, 91(4), p.043302_1 - 043302_20, 2020/04

 Times Cited Count:42 Percentile:96.38(Instruments & Instrumentation)

Journal Articles

Structural characterization and magnetic behavior of uranium compound U$$_2$$Pt$$_6$$Al$$_{15}$$

Haga, Yoshinori; Sugai, Takashi*; Matsumoto, Yuji*; Yamamoto, Etsuji

JPS Conference Proceedings (Internet), 29, p.013003_1 - 013003_5, 2020/02

Journal Articles

Quantum twin spectra in nanocrystalline silicon

Matsumoto, Takahiro*; Ohara, Takashi; Sugimoto, Hidehiko*; Bennington, S. M.*; Ikeda, Susumu*

Physical Review Materials (Internet), 1(5), p.051601_1 - 051601_6, 2017/10

 Times Cited Count:2 Percentile:7.84(Materials Science, Multidisciplinary)

Journal Articles

Experimental analysis of neutron and background $$gamma$$-ray energy spectra of 80-400 MeV $$^{7}$$Li(p,n) reactions under the quasi-monoenergetic neutron field at RCNP, Osaka University

Iwamoto, Yosuke; Sato, Tatsuhiko; Satoh, Daiki; Hagiwara, Masayuki*; Yashima, Hiroshi*; Masuda, Akihiko*; Matsumoto, Tetsuro*; Iwase, Hiroshi*; Shima, Tatsushi*; Nakamura, Takashi*

EPJ Web of Conferences, 153, p.08019_1 - 08019_3, 2017/09

 Times Cited Count:0 Percentile:0.03

To develop 100-400 MeV quasi-monoenergetic neutron field, we measured neutron and unexpected $$gamma$$-ray energy spectra of the $$^{7}$$Li(p,n) reaction with 80-389 MeV protons in the 100-m time-of-flight (TOF) tunnel at the Research Center for Nuclear Physics (RCNP). Neutron energy spectra with energies above 3 MeV were measured by the TOF method and $$gamma$$ energy spectra with energies above 0.1 MeV were measured by the automatic unfolding function of the radiation dose monitor DARWIN. For neutron spectra, the contribution of peak intensity to the total intensity integrated with energies above 3 MeV varied between 0.38 and 0.48. For $$gamma$$-ray spectra, high-energetic $$gamma$$-rays at around 70 MeV originated from the decay of $$pi$$$$^{0}$$ were observed over 200 MeV. For the 246-MeV proton incident reaction, the contribution of $$gamma$$-ray dose to neutron dose is negligible because the ratio of $$gamma$$-ray to neutron is 0.014.

Journal Articles

Characterization of the PTW 34031 ionization chamber (PMI) at RCNP with high energy neutrons ranging from 100 - 392 MeV

Theis, C.*; Carbonez, P.*; Feldbaumer, E.*; Forkel-Wirth, D.*; Jaegerhofer, L.*; Pangallo, M.*; Perrin, D.*; Urscheler, C.*; Roesler, S.*; Vincke, H.*; et al.

EPJ Web of Conferences, 153, p.08018_1 - 08018_5, 2017/09

 Times Cited Count:0 Percentile:0.03

At CERN, gas-filled ionization chambers PTW-34031 (PMI) are commonly used in radiation fields including neutrons, protons and $$gamma$$-rays. A response function for each particle is calculated by the radiation transport code FLUKA. To validate a response function to high energy neutrons, benchmark experiments with quasi mono-energetic neutrons have been carried out at RCNP, Osaka University. For neutron irradiation with energies below 200 MeV, very good agreement was found comparing the FLUKA simulations and the measurements. In addition it was found that at proton energies of 250 and 392 MeV, results calculated with neutron sources underestimate the experimental data due to a non-negligible gamma component originating from the target $$^{7}$$Li(p,n)Be reaction.

Journal Articles

Shielding experiments of concrete and iron for the 244 MeV and 387 MeV quasi-mono energetic neutrons using a Bonner sphere spectrometer (at RCNP, Osaka Univ.)

Matsumoto, Tetsuro*; Masuda, Akihiko*; Nishiyama, Jun*; Iwase, Hiroshi*; Iwamoto, Yosuke; Satoh, Daiki; Hagiwara, Masayuki*; Yashima, Hiroshi*; Yashima, Hiroshi*; Shima, Tatsushi*; et al.

EPJ Web of Conferences, 153, p.08016_1 - 08016_3, 2017/09

 Times Cited Count:0 Percentile:61.28

Neutron energy spectra behind concrete and iron shields were measured for quasi-monoenergetic neutrons above 200 MeV using a Bonner sphere spectrometer (BSS). Quasi-monoenergetic neutrons were produced by the $$^{7}$$Li(p,xn) reaction with 246-MeV and 389-MeV protons. The response function of BSS was also measured at neutron energies from 100 MeV to 387 MeV. In data analysis, the measured response function was used and the multiple neutron scattering effect between the BSS and the shielding material was considered. The neutron energy spectra behind the concrete and iron shields were obtained by the unfolding method using the MAXED code. Ambient dose equivalents were obtained as a function of a shield thickness successfully. For the case of the 244 MeV neutron incidence, the multiple neutron scattering effect on the effective dose is large under 50 cm thickness of the concrete shield.

Journal Articles

Neutron spectrometry and dosimetry in 100 and 300 MeV quasi-mono-energetic neutron field at RCNP, Osaka University, Japan

Mares, V.*; Trinkl, S.*; Iwamoto, Yosuke; Masuda, Akihiko*; Matsumoto, Tetsuro*; Hagiwara, Masayuki*; Satoh, Daiki; Yashima, Hiroshi*; Shima, Tatsushi*; Nakamura, Takashi*

EPJ Web of Conferences, 153, p.08020_1 - 08020_3, 2017/09

 Times Cited Count:5 Percentile:94.1

To validate response of an extended range Bonner Sphere Spectrometer (ERBSS) with $$^{3}$$He proportional counter, neutron energy spectra were measured using an ERBSS in the quasi-mono-energetic neutron field at the Research Center for Nuclear Physics (RCNP). Using 100 MeV and 296 MeV proton beams, neutron fields with nominal peak energies of 96 MeV and 293 MeV were generated via $$^{7}$$Li(p,n)$$^{7}$$Be reactions. The energy spectra were measured at a distance of 35 m from the target. To deduce the corresponding neutron spectra from thermal to the nominal maximum energy, the ERBSS data were unfolded using the MSANDB unfolding code. At high energies, the neutron spectra were also measured by means of the TOF method using NE213 organic liquid scintillators. The agreement between ERBSS and TOF neutron spectra above 5 MeV is very good. Comparison in terms of ambient dose equivalent, H$$^{*}$$(10) between ERBSS and TOF values for both proton energies shows very good agreement.

Journal Articles

Non-aqueous selective synthesis of orthosilicic acid and its oligomers

Igarashi, Masayasu*; Matsumoto, Tomohiro*; Yagihashi, Fujio*; Yamashita, Hiroshi*; Ohara, Takashi; Hanashima, Takayasu*; Nakao, Akiko*; Moyoshi, Taketo*; Sato, Kazuhiko*; Shimada, Shigeru*

Nature Communications (Internet), 8, p.140_1 - 140_8, 2017/07

 Times Cited Count:25 Percentile:64.44(Multidisciplinary Sciences)

Journal Articles

Applicability of the two-angle differential method to response measurement of neutron-sensitive devices at the RCNP high-energy neutron facility

Masuda, Akihiko*; Matsumoto, Tetsuro*; Iwamoto, Yosuke; Hagiwara, Masayuki*; Satoh, Daiki; Sato, Tatsuhiko; Iwase, Hiroshi*; Yashima, Hiroshi*; Nakane, Yoshihiro; Nishiyama, Jun*; et al.

Nuclear Instruments and Methods in Physics Research A, 849, p.94 - 101, 2017/03

 Times Cited Count:0 Percentile:10.71(Instruments & Instrumentation)

Quasi-monoenergetic high-energy neutron fields induced by $$^{7}$$Li(p,n) reactions are used for the response evaluation of neutron-sensitive devices. The quasi-monoenergetic high-energy field consists of high-energy monoenergetic peak neutrons and unwanted continuum neutrons down to the low-energy region. A two-angle differential method has been developed to compensate for the effect of the continuum neutrons in the response measurements. In this study, the two-angle differential method was demonstrated for Bonner sphere detectors, which are typical examples of moderator-based neutron-sensitive detectors, to investigate the method's applicability and its dependence on detector characteristics. Through this study, the adequacy of the two-angle differential method was experimentally verified, and practical suggestions were made pertaining to this method.

JAEA Reports

Current status of a decommissioning project in the Enrichment Engineering Facility; Results in the second-half of the fiscal year of 2014

Matsumoto, Takashi; Takahashi, Nobuo; Hayashibara, Kenichi; Ishimori, Yuu; Mita, Yutaka; Kakiya, Hideyoshi

JAEA-Technology 2016-020, 80 Pages, 2016/11

JAEA-Technology-2016-020.pdf:17.8MB

The Enrichment Engineering Facility of the Ningyo-toge Environmental Engineering Center was constructed in order to establish the technological basis of plant engineering for uranium enrichment in Japan. Uranium enrichment tests, using natural and reprocessed uranium, were carried out from 1979 to 1989 with two types of centrifuges in the facility. According to the decommissioning plan of the facility, UF$$_{6}$$ handling equipment and supplemental equipment in these plants are intended to be dismantled by 2019 in order to make vacant spaces for future projects use, for example, inventory investigation, precipitation treatment, etc. This report shows the current state of the decommissioning project in the second-half of the fiscal year of 2014.

JAEA Reports

Current status of a decommissioning project in the Enrichment Engineering Facilities; Results in the first-half of the fiscal year of 2014

Matsumoto, Takashi; Morimoto, Yasuyuki; Takahashi, Nobuo; Takata, Masaharu; Yoshida, Hideaki; Nakashima, Shinichi; Ishimori, Yuu

JAEA-Technology 2015-036, 60 Pages, 2016/01

JAEA-Technology-2015-036.pdf:9.15MB

The Enrichment Engineering Facilities of the Ningyo-toge Environmental Engineering Center was constructed in order to establish the technical basis of the uranium enrichment plant in Japan. Uranium enrichment tests, using natural and reprocessed uranium, were carried out from 1979 to 1990 at two types of plants in the facilities. UF$$_{6}$$ handling equipment and Supplemental equipment in these plants are intended to be dismantled by 2019 in order to make places for future projects, for example, inventory investigation, precipitation treatment, etc. This report shows the basic plan of this decommissioning project and presents the current state of dismantling in the first-half of the fiscal year of 2014, with indicating its schedule, procedure, situation, results, and so on. The dismantled materials generated amounted to 37 mesh containers and 199 drums, and the secondary waste generated amounted to 271.4 kg.

Journal Articles

Characterization of high-energy quasi-monoenergetic neutron energy spectra and ambient dose equivalents of 80-389 MeV $$^{7}$$Li(p,n) reactions using a time-of-flight method

Iwamoto, Yosuke; Hagiwara, Masayuki*; Satoh, Daiki; Araki, Shohei*; Yashima, Hiroshi*; Sato, Tatsuhiko; Masuda, Akihiko*; Matsumoto, Tetsuro*; Nakao, Noriaki*; Shima, Tatsushi*; et al.

Nuclear Instruments and Methods in Physics Research A, 804, p.50 - 58, 2015/12

 Times Cited Count:22 Percentile:87.32(Instruments & Instrumentation)

We have measured neutron energy spectra for the 80, 100 and 296 MeV proton incident reactions at the RCNP cyclotron facility using time-of-flight method. The neutron energy spectrum consisted of the peak and continuum parts and the peak intensity was 0.9-1.1 $$times$$ 10$$^{10}$$ neutrons/sr/$$mu$$C. The ratio of peak intensity of the spectrum to the total intensity was between 0.38 and 0.48. To consider the correction required to derive a response in the peak region from the measured total response for neutron monitors, we proposed the subtraction method using energy spectra between 0$$^{circ}$$ and 25$$^{circ}$$. The normalizing factor k against the 25$$^{circ}$$ neutron fluence that equalizes the 0$$^{circ}$$ neutron fluence in the continuum region was from 0.74 to 1.02. With our previous results, we have obtained data for characterization of monoenergetic neutron field for the $$^{7}$$Li(p,n) reaction with 80$$sim$$389 MeV protons at the RCNP cyclotron facility.

110 (Records 1-20 displayed on this page)