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JAEA Reports

Analysis work report on removal of spent fuel sheared powder for decommissioning of main plant

Aoya, Juri; Mori, Amami; Sato, Hinata; Kono, Soma; Morokado, Shiori; Horigome, Kazushi; Goto, Yuichi; Yamamoto, Masahiko; Taguchi, Shigeo

JAEA-Technology 2023-008, 34 Pages, 2023/06

JAEA-Technology-2023-008.pdf:1.92MB

Flush-out, by which nuclear materials in the Tokai Reprocessing Plant process are recovered, has been started in June 2022 as the first step of decommissioning. Flush-out consists of removal of spent fuel sheared powder, plutonium solution, uranium solution, and the other nuclear materials. Removal of spent fuel sheared powder has been completed in September 2022. During removal of spent fuel sheared powder, uranium concentration, plutonium concentration, acid concentration, radioactivity concentration, and solution density have been analyzed for process control. For nuclear material accountancy, uranium concentration, plutonium concentration, isotope ratio, and solution density have been analyzed. Analysis work including sample pretreatment before transportation to IAEA analytical facility for safeguards, and the other operations related to Flush-out such as calibration of analytical instruments, education, and training of operators are reported.

Journal Articles

Study on actinide burning core concepts for the future phaseout of a fast reactor fuel cycle

Mori, Tetsuya; Naganuma, Masayuki; Oki, Shigeo

Nuclear Technology, 209(4), p.532 - 548, 2023/04

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

This paper deals with a conceptual study on a plutonium (Pu) and minor actinide (MA) burning fast reactor core for the distant future phaseout of a fast-reactor fuel cycle after it is commercialized and used for a long time. This burning core aims to reduce the Pu and MA inventories contained in the fuel cycle through multiple recycling. A key point for the core design is the degradation of Pu and MA during multiple recycling. This degradation affects the core feasibility by increasing the sodium void reactivity and decreasing the absolute value of the Doppler constant. A feasible core concept was found by incorporating the following three factors to improve the reactivity coefficients: core flattening, fuel burnup reduction, and the use of silicon carbide (SiC) in the cladding and wrapper tubes. Notably, softening the neutron spectrum using the SiC structural material not only improved the reactivity coefficients but also indirectly mitigated the degradation of Pu and MA. Consequently, the designed core allowed for multiple recycling to continue until the Pu and MA reduced significantly, particularly by about 99% in a phaseout scenario starting from a fast-reactor fleet of 30-GWe nuclear power capacity. Fast reactors were found to have the potential to become self-contained energy systems that can minimize the inventories of Pu they produced themselves, as well as long-lived MA. Fast reactors can be among the important options for environmental burden reduction in the future.

Journal Articles

Local structure analysis of BiFeO$$_3$$-BaTiO$$_3$$ solid solutions

Yoneda, Yasuhiro; Kim, S.*; Mori, Shigeo*; Wada, Satoshi*

Japanese Journal of Applied Physics, 61(SN), p.SN1022_1 - SN1022_10, 2022/11

 Times Cited Count:1 Percentile:17.38(Physics, Applied)

Local structural analysis of the (1-${it x}$) BiFeO$$_3$$-${it x}$BaTiO$$_3$$ solid solution was performed by PDF analysis of the data obtained in the synchrotron radiation high-energy X-ray diffraction experiment. First, when XAFS experiments were performed and sample screening was performed, it was found that structural fluctuations were large in the BiFeO$$_3$$-rich composition. Therefore, PDF analysis of a sample with BiFeO$$_3$$-rich composition was performed. As a result, it was found that although the average structure is a cubic structure, the local structure can be reproduced with a rhombohedral crystal structure, and there is a displacement that breaks the symmetry of the rhombohedral structure in a composition with a large fluctuation.

Journal Articles

Partial breakdown of translation symmetry at a structural quantum critical point associated with a ferroelectric soft mode

Ishii, Yui*; Yamamoto, Arisa*; Sato, Naoki*; Nambu, Yusuke*; Kawamura, Seiko; Murai, Naoki; Ohara, Koji*; Kawaguchi, Shogo*; Mori, Takao*; Mori, Shigeo*

Physical Review B, 106(13), p.134111_1 - 134111_7, 2022/10

 Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)

Journal Articles

Development of ARKADIA for the innovation of advanced nuclear reactor design process (Overview of optimization process development in design optimization support tool, ARKADIA-Design)

Tanaka, Masaaki; Doda, Norihiro; Yokoyama, Kenji; Mori, Takero; Okajima, Satoshi; Hashidate, Ryuta; Yada, Hiroki; Oki, Shigeo; Miyazaki, Masashi; Takaya, Shigeru

Dai-26-Kai Doryoku, Enerugi Gijutsu Shimpojiumu Koen Rombunshu (Internet), 5 Pages, 2022/07

To assist conceptual studies of various reactor systems conducted by private sectors in nuclear power innovation, development of an innovative design system named ARKADIA (Advanced Reactor Knowledge- and AI-aided Design Integration Approach through the whole plant lifecycle) is undergoing to achieve the design of an advanced nuclear reactor as a safe, economic, and sustainable carbon-free energy source. In this paper, focusing on the ARKADIA-Design as a part of it, the progress in the development of optimization processes on the representative problems in the fields of the core design, the plant structure design, and the maintenance schedule planning are introduced.

Journal Articles

Sodium-cooled Fast Reactors

Ohshima, Hiroyuki; Morishita, Masaki*; Aizawa, Kosuke; Ando, Masanori; Ashida, Takashi; Chikazawa, Yoshitaka; Doda, Norihiro; Enuma, Yasuhiro; Ezure, Toshiki; Fukano, Yoshitaka; et al.

Sodium-cooled Fast Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.3, 631 Pages, 2022/07

This book is a collection of the past experience of design, construction, and operation of two reactors, the latest knowledge and technology for SFR designs, and the future prospects of SFR development in Japan. It is intended to provide the perspective and the relevant knowledge to enable readers to become more familiar with SFR technology.

Journal Articles

PSTEP: Project for solar-terrestrial environment prediction

Kusano, Kanya*; Ichimoto, Kiyoshi*; Ishii, Mamoru*; Miyoshi, Yoshizumi*; Yoden, Shigeo*; Akiyoshi, Hideharu*; Asai, Ayumi*; Ebihara, Yusuke*; Fujiwara, Hitoshi*; Goto, Tadanori*; et al.

Earth, Planets and Space (Internet), 73(1), p.159_1 - 159_29, 2021/12

 Times Cited Count:6 Percentile:51.19(Geosciences, Multidisciplinary)

The PSTEP is a nationwide research collaboration in Japan and was conducted from April 2015 to March 2020, supported by a Grant-in-Aid for Scientific Research on Innovative Areas from the Ministry of Education, Culture, Sports, Science and Technology of Japan. It has made a significant progress in space weather research and operational forecasts, publishing over 500 refereed journal papers and organizing four international symposiums, various workshops and seminars, and summer school for graduate students at Rikubetsu in 2017. This paper is a summary report of the PSTEP and describes the major research achievements it produced.

Journal Articles

Quantifying the dislocation structures of additively manufactured Ti-6Al-4V alloys using X-ray diffraction line profile analysis

Yamanaka, Kenta*; Kuroda, Asumi*; Ito, Miyu*; Mori, Manami*; Bian, H.*; Shobu, Takahisa; Sato, Shigeo*; Chiba, Akihiko*

Additive Manufacturing, 37, p.101678_1 - 101678_12, 2021/01

 Times Cited Count:23 Percentile:86.72(Engineering, Manufacturing)

Journal Articles

Crystallographical and morphological changes in charge-ordering transition of RFe$$_{2}$$O$$_{4}$$ (R: Y, Lu) investigated by transmission electron microscopy

Horibe, Yoichi*; Mori, Shigeo*; Ikeda, Naoshi*; Yoshii, Kenji; Maeno, Hiroshi*; Murakami, Yasukazu*

Ferroelectrics, 584(1), p.20 - 30, 2021/00

 Times Cited Count:1 Percentile:7.92(Materials Science, Multidisciplinary)

Temperature dependence of charge-ordered crystal structures and domain structures in RFe$$_{2}$$O$$_{4}$$ (R: Y and Lu) was investigated by energy-filtered transmission electron microscopy, combined with conventional transmission electron microscopy. The presence of three-dimensional to two-dimensional charge ordering transition were observed in both RFe$$_{2}$$O$$_{4}$$ on heating. Furthermore, real-space images obtained with the energy-filtered transmission electron microscopy revealed that YRFe$$_{2}$$O$$_{4}$$ has less anisotropic nanometer-scale charge-ordered domains than LuRFe$$_{2}$$O$$_{4}$$. These findings in RFe$$_{2}$$O$$_{4}$$ indicate the importance of the interchange interactions between Fe-O bilayers in addition to those within bilayers in the structural phase transitions associated with charge ordering in this system.

JAEA Reports

Status of study of long-term assessment of transport of radioactive contaminants in the environment of Fukushima (FY2018) (Translated document)

Nagao, Fumiya; Niizato, Tadafumi; Sasaki, Yoshito; Ito, Satomi; Watanabe, Takayoshi; Dohi, Terumi; Nakanishi, Takahiro; Sakuma, Kazuyuki; Hagiwara, Hiroki; Funaki, Hironori; et al.

JAEA-Research 2020-007, 249 Pages, 2020/10

JAEA-Research-2020-007.pdf:15.83MB

The accident of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. occurred due to the Great East Japan Earthquake, Sanriku offshore earthquake, of 9.0 magnitude and the accompanying tsunami. As a result, large amount of radioactive materials was released into the environment. Under these circumstances, Japan Atomic Energy Agency (JAEA) has been conducting "Long-term Assessment of Transport of Radioactive Contaminants in the Environment of Fukushima" concerning radioactive materials released in environment, especially migration behavior of radioactive cesium since November 2012. This report is a summary of the research results that have been obtained in environmental dynamics research conducted by JAEA in Fukushima Prefecture.

Journal Articles

High-temperature short-range order in Mn$$_3$$RhSi

Yamauchi, Hiroki; Sari, D. P.*; Watanabe, Isao*; Yasui, Yukio*; Chang, L.-J.*; Kondo, Keietsu; Ito, Takashi; Ishikado, Motoyuki*; Hagihara, Masato*; Frontzek, M. D.*; et al.

Communications Materials (Internet), 1, p.43_1 - 43_6, 2020/07

High-temperature short-range order is discovered up to 720 K in Mn$$_3$$RhSi by complementary use of neutron scattering and muon spin relaxation measurements.

JAEA Reports

Status of study of long-term assessment of transport of radioactive contaminants in the environment of Fukushima (FY2018)

Nagao, Fumiya; Niizato, Tadafumi; Sasaki, Yoshito; Ito, Satomi; Watanabe, Takayoshi; Dohi, Terumi; Nakanishi, Takahiro; Sakuma, Kazuyuki; Hagiwara, Hiroki; Funaki, Hironori; et al.

JAEA-Research 2019-002, 235 Pages, 2019/08

JAEA-Research-2019-002.pdf:21.04MB

The accident of the Fukushima Daiichi Nuclear Power Station (hereinafter referred to 1F), Tokyo Electric Power Company Holdings, Inc. occurred due to the Great East Japan Earthquake, Sanriku offshore earthquake, of 9.0 magnitude and the accompanying tsunami. As a result, large amount of radioactive materials was released into the environment. Under these circumstances, JAEA has been conducting Long-term Environmental Dynamics Research concerning radioactive materials released in environment, especially migration behavior of radioactive cesium since November 2012. This report is a summary of the research results that have been obtained in environmental dynamics research conducted by JAEA in Fukushima Prefecture.

Journal Articles

Tuning strain-induced $$gamma$$-to-$$varepsilon$$ martensitic transformation of biomedical Co-Cr-Mo alloys by introducing parent phase lattice defects

Mori, Manami*; Yamanaka, Kenta*; Sato, Shigeo*; Tsubaki, Shinki*; Sato, Kozue*; Kumagai, Masayoshi*; Imafuku, Muneyuki*; Shobu, Takahisa; Chiba, Akihiko*

Journal of the Mechanical Behavior of Biomedical Materials, 90, p.523 - 529, 2019/02

 Times Cited Count:19 Percentile:71.16(Engineering, Biomedical)

Journal Articles

Presence of $$varepsilon$$-martensite as an intermediate phase during the strain-induced transformation of SUS304 stainless steel

Hatano, Masaharu*; Kubota, Yoshiki*; Shobu, Takahisa; Mori, Shigeo*

Philosophical Magazine Letters, 96(6), p.220 - 227, 2016/06

 Times Cited Count:7 Percentile:35.46(Materials Science, Multidisciplinary)

We have investigated the formation process of $$alpha$$'-martensite from the $$gamma$$-phase induced by external strain using ${it in situ}$ synchrotron diffraction experiments, combined with Lorentz transmission electron microscopy (TEM) and high-resolution TEM observations. It is clearly demonstrated that $$varepsilon$$-martensite with hexagonal symmetry appears as an intermediate structure during the plastic deformation of SUS304 stainless steel. In addition to stacking faults and dislocations, interfaces between the twin structures presumably play a key role in the formation of $$varepsilon$$-martensite.

JAEA Reports

Measurement of hydrogen generating from radiolysis of highly active liquid waste and its quantitative evaluation

Yamamoto, Masahiko; Surugaya, Naoki; Mori, Eito; Taguchi, Shigeo; Sato, Soichi

JAEA-Research 2015-013, 27 Pages, 2015/10

JAEA-Research-2015-013.pdf:2.84MB

The H$$_{2}$$ concentration generating from Highly Active Liquid Waste (HALW) of Tokai Reprocessing Plant is measured in a closed experimental system. The experimental results show that H$$_{2}$$ concentration gradually increases at first and then approaches a steady-state due to the H$$_{2}$$ consumption reaction by Pd ions. The highest H$$_{2}$$ concentration is 1200 ppm (0.1%) when the solution temperature is at 23$$^{circ}$$C. It is found that H$$_{2}$$ generating from HALW is equilibrated one order of magnitude lower than the H$$_{2}$$ combustion lower limit. Moreover, a model based on H$$_{2}$$ generation from HALW by the radiolysis and H$$_{2}$$ consumption reaction by Pd ions is proposed and applied to evaluate H$$_{2}$$ concentration behavior in the gas phase. The calculated H$$_{2}$$ concentrations from proposed model agreed well with the experimental values. It is demonstrated that the behavior of H$$_{2}$$ generating from HALW can be evaluated quantitatively by applying the proposed model in this study.

Journal Articles

The Cause of corrosion occurred in a glove box filter casing and its repair technique

Mori, Eito; Yamamoto, Masahiko; Taguchi, Shigeo; Sato, Soichi; Kitao, Takahiko; Surugaya, Naoki

Nihon Hozen Gakkai Dai-11-Kai Gakujutsu Koenkai Yoshishu, p.132 - 138, 2014/07

The contamination of the radioactive material was observed on the filter casing surface of the glove box installed at the analytical laboratory in Tokai Reprocessing Plant. The cause of the contamination was investigated with visual inspection, penetrant testing and ultrasonic thickness measurement. It was found that a micro through-hole due to the corrosion of stainless-steel was generated in the glove box filter casing. The repair work of the filter casing was performed keeping the glove box negative pressure. The corrosion part of filter casing was replaced and newly fabricated casing was connected to the glove box with Tungsten Inert Gas welding method.

Journal Articles

Current-induced enhancement of magnetic anisotropy in spin-charge-coupled multiferroic YbFe$$_{2}$$O$$_{4}$$

Yoshii, Kenji; Matsumura, Daiju; Saito, Hiroyuki; Kambe, Takashi*; Fukunaga, Mamoru*; Muraoka, Yuji*; Ikeda, Naoshi*; Mori, Shigeo*

Journal of the Physical Society of Japan, 83(6), p.063708_1 - 063708_4, 2014/06

 Times Cited Count:4 Percentile:34.67(Physics, Multidisciplinary)

We report the change of magnetic properties of multiferroic YbFe$$_{2}$$O$$_{4}$$, caused by cooling in the presence of an electrical current. The magnetization measured after the cooling becomes smaller by about 10-20% than that after cooling without a current. The current also affects the magnetic anisotropy below about 100 K; the magnetic coercivity is increased by about 10-20%. These phenomena may arise from a coexistence of ferromagnetic and antiferromagnetic domains, or a disturbance in the formation of charge-ordered domains. From the applied viewpoint, the enhancement of anisotropy by an electrical current offers a method for stabilizing magnetization other than the well-known method, i.e., exchange bias.

Journal Articles

Magnetic properties of R$$_{2}$$Fe$$_{3}$$O$$_{7}$$ (R=Yb and Lu)

Yoshii, Kenji; Ikeda, Naoshi*; Fukuyama, Ryota*; Nagata, Tomoko*; Kambe, Takashi*; Yoneda, Yasuhiro; Fukuda, Tatsuo; Mori, Shigeo*

Solid State Communications, 173, p.34 - 37, 2013/11

 Times Cited Count:4 Percentile:20.56(Physics, Condensed Matter)

We have investigated the magnetic properties of R$$_{2}$$Fe$$_{3}$$O$$_{7}$$ (R=Yb and Lu), which belongs to the homologous family of electronic ferroelectric RFe$$_{2}$$O$$_{4}$$. Magnetization measurements show ferrimagnetic ordering at the Neel temperature (T$$_{N}$$) of about 270 K, which is slightly higher than that of RFe$$_{2}$$O$$_{4}$$ (T$$_{N}$$ about 230-250 K). Observation of spin glass and exchange bias shows a coexistence of ferromagnetic and antiferromagneticinteractions, similarly to RFe$$_{2}$$O$$_{4}$$. This situation gives rise to a complex magnetic change and a broad peak of magnetic entropy change. Some characteristics, such as refrigeration temperatures higher than in RFe$$_{2}$$O$$_{4}$$, seem to offer a possibility of this system to applications.

Journal Articles

Magnetic properties of single crystalline YbFe$$_{2}$$O$$_{4}$$

Yoshii, Kenji; Mizumaki, Masaichiro*; Matsumoto, Keisuke*; Mori, Shigeo*; Endo, Naruki; Saito, Hiroyuki; Matsumura, Daiju; Kambe, Takashi*; Ikeda, Naoshi*

Journal of Physics; Conference Series, 428, p.012032_1 - 012032_5, 2013/04

 Times Cited Count:14 Percentile:96.93(Chemistry, Applied)

We have investigated a single crystal of multiferroic YbFe$$_{2}$$O$$_{4}$$. Its magnetic transition temperature was 250 K. The magnetization along the c-axis was much larger than that within the ab plane, indicating the Ising character of this system. The field-cooled magnetization became negative below 10 K. This was explained in terms of an antiparallel coupling between Yb and Fe moments. Magnetocaloric effects were also observed. The change of entropy was found to show a broad peak with a width of 100 K, which is favorable to application.

Journal Articles

Exchange bias in multiferroic $$R$$Fe$$_{2}$$O$$_{4}$$ ($$R$$=Y, Er, Tm, Yb, Lu and In)

Yoshii, Kenji; Ikeda, Naoshi*; Nishihata, Yasuo; Maeda, Daisuke*; Fukuyama, Ryota*; Nagata, Tomoko*; Kano, Jun*; Kambe, Takashi*; Horibe, Yoichi*; Mori, Shigeo*

Journal of the Physical Society of Japan, 81(3), p.033704_1 - 033704_4, 2012/03

 Times Cited Count:10 Percentile:55.37(Physics, Multidisciplinary)

Exchange bias (EB) behavior has been observed for multiferroic $$R$$Fe$$_{2}$$O$$_{4}$$ ($$R$$=Y, Er, Tm, Yb, Lu and In). The materials with the small $$R$$$$^{3+}$$ ions ($$R$$=Tm, Yb, Lu and In) exhibit large EB fields ($$_sim^{>}$$ 1 kOe) below $$sim$$100-150 K. This property is rooted in a magnetically glassy state, arising from the competition between ferro- and antiferromagnetic domain interactions. In addition, the exchange bias field tends to be more enhanced for smaller $$R$$$$^{3+}$$ ions. Hence, the EB is controlled by the substitution at the $$R$$-site in this series.

76 (Records 1-20 displayed on this page)