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JAEA Reports

Stabilization treatment of nuclear fuel material contained with organic matter

Senzaki, Tatsuya; Arai, Yoichi; Yano, Kimihiko; Sato, Daisuke; Tada, Kohei; Ogi, Hiromichi*; Kawanobe, Takayuki*; Ono, Shimpei; Nakamura, Masahiro; Kitawaki, Shinichi; et al.

JAEA-Testing 2022-001, 28 Pages, 2022/05

JAEA-Testing-2022-001.pdf:2.33MB

In preparation for the decommissioning of Laboratory B of the Nuclear Fuel Cycle Engineering Laboratory, the nuclear fuel material that had been stored in the glove box for a long time was moved to the Chemical Processing Facility (CPF). This nuclear fuel material was stored with sealed by a polyvinyl chloride (PVC) bag in the storage. Since it was confirmed that the PVC bag swelled during storage, it seems that any gas was generated by radiolysis of the some components contained in the nuclear fuel material. In order to avoid breakage of the PVC bag and keep it safety for long time, we began the study on the stabilization treatment of the nuclear fuel material. First, in order to clarify the properties of nuclear fuel material, radioactivity analysis, component analysis, and thermal analysis were carried out. From the results of thermal analysis, the existence of organic matter was clarified. Then, ion exchange resin with similar thermal characteristics was selected and the thermal decomposition conditions were investigated. From the results of these analyzes and examinations, the conditions for thermal decomposition of the nuclear fuel material contained with organic matter was established. Performing a heat treatment of a small amount of nuclear fuel material in order to confirm the safety, after which the treatment amount was scaled up. It was confirmed by the weight change after the heat treatment that the nuclear fuel material contained with organic matter was completely decomposed.

Journal Articles

PSTEP: Project for solar-terrestrial environment prediction

Kusano, Kanya*; Ichimoto, Kiyoshi*; Ishii, Mamoru*; Miyoshi, Yoshizumi*; Yoden, Shigeo*; Akiyoshi, Hideharu*; Asai, Ayumi*; Ebihara, Yusuke*; Fujiwara, Hitoshi*; Goto, Tadanori*; et al.

Earth, Planets and Space (Internet), 73(1), p.159_1 - 159_29, 2021/12

 Times Cited Count:6 Percentile:51.19(Geosciences, Multidisciplinary)

The PSTEP is a nationwide research collaboration in Japan and was conducted from April 2015 to March 2020, supported by a Grant-in-Aid for Scientific Research on Innovative Areas from the Ministry of Education, Culture, Sports, Science and Technology of Japan. It has made a significant progress in space weather research and operational forecasts, publishing over 500 refereed journal papers and organizing four international symposiums, various workshops and seminars, and summer school for graduate students at Rikubetsu in 2017. This paper is a summary report of the PSTEP and describes the major research achievements it produced.

Journal Articles

Observation of longitudinal magnetic fluctuations at a first-order ferromagnetic quantum phase transition in UGe$$_2$$

Noma, Yuichiro*; Kotegawa, Hisashi*; Kubo, Tetsuro*; To, Hideki*; Harima, Hisatomo*; Haga, Yoshinori; Yamamoto, Etsuji; Onuki, Yoshichika*; Ito, Kohei*; Nakamura, Ai*; et al.

Journal of the Physical Society of Japan, 90(7), p.073707_1 - 073707_5, 2021/07

 Times Cited Count:0 Percentile:0(Physics, Multidisciplinary)

Journal Articles

Thermally altered subsurface material of asteroid (162173) Ryugu

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.

Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03

 Times Cited Count:43 Percentile:96.93(Astronomy & Astrophysics)

Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 $$^{circ}$$C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 $$^{circ}$$C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.

Journal Articles

The Surface composition of asteroid 162173 Ryugu from Hayabusa2 near-infrared spectroscopy

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Arai, Takehiko*; Nakauchi, Yusuke*; Nakamura, Tomoki*; Matsuoka, Moe*; et al.

Science, 364(6437), p.272 - 275, 2019/04

 Times Cited Count:259 Percentile:99.73(Multidisciplinary Sciences)

The near-Earth asteroid 162173 Ryugu, the target of Hayabusa2 sample return mission, is believed to be a primitive carbonaceous object. The Near Infrared Spectrometer (NIRS3) on Hayabusa2 acquired reflectance spectra of Ryugu's surface to provide direct measurements of the surface composition and geological context for the returned samples. A weak, narrow absorption feature centered at 2.72 micron was detected across the entire observed surface, indicating that hydroxyl (OH)-bearing minerals are ubiquitous there. The intensity of the OH feature and low albedo are similar to thermally- and/or shock-metamorphosed carbonaceous chondrite meteorites. There are few variations in the OH-band position, consistent with Ryugu being a compositionally homogeneous rubble-pile object generated from impact fragments of an undifferentiated aqueously altered parent body.

Journal Articles

Anisotropic magnetic fluctuations in ferromagnetic superconductor UGe$$_2$$; $$^{73}$$Ge-NQR study at ambient pressure

Noma, Yuichiro*; Kotegawa, Hisashi*; Kubo, Tetsuro*; To, Hideki*; Harima, Hisatomo*; Haga, Yoshinori; Yamamoto, Etsuji; Onuki, Yoshichika*; Ito, Kohei*; Haller, E. E.*; et al.

Journal of the Physical Society of Japan, 87(3), p.033704_1 - 033704_5, 2018/03

 Times Cited Count:4 Percentile:35.9(Physics, Multidisciplinary)

Journal Articles

An Evaluation method of reflectance spectra to be obtained by Hayabusa2 Near-Infrared Spectrometer (NIRS3) based on laboratory measurements of carbonaceous chondrites

Matsuoka, Moe*; Nakamura, Tomoki*; Osawa, Takahito; Iwata, Takahiro*; Kitazato, Kohei*; Abe, Masanao*; Nakauchi, Yusuke*; Arai, Takehiko*; Komatsu, Mutsumi*; Hiroi, Takahiro*; et al.

Earth, Planets and Space (Internet), 69(1), p.120_1 - 120_12, 2017/12

AA2017-0327.pdf:1.53MB

 Times Cited Count:6 Percentile:21.84(Geosciences, Multidisciplinary)

We have conducted ground-based performance evaluation tests of the Near-Infrared Spectrometer (NIRS3) onboard Hayabusa2 spacecraft and established a method for evaluating its measured reflectance spectra. Reflectance spectra of nine powdered carbonaceous chondrite samples were measured by both NIRS3 and a FT-IR spectrometer. Since raw data obtained by NIRS3 had considerable spectral distortion caused by systematic offsets in sensitivity of individual pixels, we have established two methods for correcting the NIRS3 data by comparing them with the corresponding FT-IR data. In order to characterize the absorption bands in NIRS3 spectra, the depth of each band component D$$lambda$$ is defined for each wavelength $$lambda$$ ($$mu$$m). Reflectance spectra of asteroid Ryugu, the target asteroid of Hayabusa2, to be recorded by the NIRS3 are expected to reveal the characteristics of the surface materials by using the evaluation technique.

Journal Articles

NIRS3; The Near Infrared Spectrometer on Hayabusa2

Iwata, Takahiro*; Kitazato, Kohei*; Abe, Masanao*; Otake, Makiko*; Arai, Takehiko*; Arai, Tomoko*; Hirata, Naru*; Hiroi, Takahiro*; Honda, Chikatoshi*; Imae, Naoya*; et al.

Space Science Reviews, 208(1-4), p.317 - 337, 2017/07

 Times Cited Count:54 Percentile:71.62(Astronomy & Astrophysics)

NIRS3: The Near Infrared Spectrometer is installed on the Hayabusa2 spacecraft to observe the target C-type asteroid 162173 Ryugu at near infrared wavelengths of 1.8 to 3.2 micrometer. It aims to obtain reflectance spectra in order to detect absorption bands of hydrated and hydroxide minerals in the 3 micrometer-band. We adopted a linear-image sensor with indium arsenide (InAs) photo diodes and a cooling system with a passive radiator to achieve an optics temperature of 188 K, which enables to retaining sufficient sensitivity and noise level in the 3 micrometer wavelength region. We conducted ground performance tests for the NIRS3 flight model (FM) to confirm its baseline specifications. The results imply that the properties such as the signal-to-noise ratio (SNR) conform to scientific requirements to determine the degree of aqueous alteration, such as CM or CI chondrite, and the stage of thermal metamorphism on the asteroid surface.

Journal Articles

Production of $$^{88}$$Nb and $$^{170}$$Ta for chemical studies of element 105, Db, using the GARIS gas-jet system

Huang, M.*; Haba, Hiromitsu*; Murakami, Masashi*; Asai, Masato; Kaji, Daiya*; Kanaya, Jumpei*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Kikutani, Yuki*; Komori, Yukiko*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 304(2), p.845 - 849, 2015/05

 Times Cited Count:3 Percentile:25.85(Chemistry, Analytical)

A technique to utilize radioisotopes of Nb and Ta was developed for chemical studies of element 105, Db, by coupling a gas-jet transport system to the RIKEN gas-filled recoil ion separator (GARIS). The short-lived $$^{88}$$Nb and $$^{170}$$Ta were produced with nuclear reactions using a $$^{19}$$F beam whose energy was the same as that to produce $$^{262}$$Db. Then, they were separated with GARIS and extracted to a chemistry laboratory with the gas-jet transport system. By changing only magnetic field of GARIS and inserting an energy degrader and a shutter for recoil ions, we could deliver the $$^{88}$$Nb and $$^{170}$$Ta to a chemistry device for $$^{262}$$Db without changing other experimental conditions.

Journal Articles

Solid-liquid extraction of Mo and W by Aliquat 336 from HCl solutions toward extraction chromatography experiments of Sg

Komori, Yukiko*; Yokokita, Takuya*; Kasamatsu, Yoshitaka*; Haba, Hiromitsu*; Toyoshima, Atsushi; Toyomura, Keigo*; Nakamura, Kohei*; Kanaya, Jumpei*; Huang, M.*; Kudo, Yuki*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 303(2), p.1385 - 1388, 2015/02

 Times Cited Count:2 Percentile:17.57(Chemistry, Analytical)

We studied solid-liquid extraction behavior of carrier-free Mo and W radiotracers onto an Aliquat 336-loaded resin from HCl solutions toward extraction chromatography experiments of element 106, seaborgium(Sg). Distribution coefficients ($${it K}$$$$_{d}$$) of Mo and W on the resin were determined as a function of HCl concentration by a batch method. On-line extraction chromatography of Mo and W was also carried out in 2-8 M HCl solutions with an automated rapid chemistry apparatus. The order of extraction probability from 2 to 8 M HCl was Mo$$>$$W, which reflected the order of the $${it K}$$$$_{d}$$ values in the batch experiment.

Journal Articles

Fast neutron detection under intense $$gamma$$-ray fields with novel nuclear emulsion technique

Ishihara, Kohei*; Takagi, Keisuke*; Minato, Haruna*; Kawarabayashi, Jun*; Tomita, Hideki*; Maeda, Shigetaka; Naka, Tatsuhiro*; Morishima, Kunihiro*; Nakano, Toshiyuki*; Nakamura, Mitsuhiro*; et al.

Radiation Measurements, 55, p.79 - 82, 2013/08

 Times Cited Count:1 Percentile:10.69(Nuclear Science & Technology)

In order to measure the neutron under a condition of high intensity of $$gamma$$-ray background, we made new nuclear emulsion based on non-sensitized OPERA emulsion which had small AgBr grain size (AgBr grain size of 60, 90 and 160 nm). The sensitivity of this new emulsion, which was a correlation between stopping power and grain density, was estimated experimentally by irradiating neutrons with several energies. We also simulated the response to $$gamma$$-ray induced electrons and compared with some experimental results by using $$^{60}$$Co $$gamma$$ source. The results showed that there might be a threshold energy deposited in one AgBr grain under which it was impossible to develop. We estimated efficiency to the $$gamma$$-ray and the neutron with this obtained response of the new emulsion.

Journal Articles

Identified charged hadron production in $$p + p$$ collisions at $$sqrt{s}$$ = 200 and 62.4 GeV

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Armendariz, R.*; et al.

Physical Review C, 83(6), p.064903_1 - 064903_29, 2011/06

 Times Cited Count:184 Percentile:99.44(Physics, Nuclear)

Transverse momentum distributions and yields for $$pi^{pm}, K^{pm}, p$$, and $$bar{p}$$ in $$p + p$$ collisions at $$sqrt{s}$$ = 200 and 62.4 GeV at midrapidity are measured by the PHENIX experiment at the RHIC. We present the inverse slope parameter, mean transverse momentum, and yield per unit rapidity at each energy, and compare them to other measurements at different $$sqrt{s}$$ collisions. We also present the scaling properties such as $$m_T$$ and $$x_T$$ scaling and discuss the mechanism of the particle production in $$p + p$$ collisions. The measured spectra are compared to next-to-leading order perturbative QCD calculations.

Journal Articles

Azimuthal correlations of electrons from heavy-flavor decay with hadrons in $$p+p$$ and Au+Au collisions at $$sqrt{s_{NN}}$$ = 200 GeV

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Aramaki, Y.*; et al.

Physical Review C, 83(4), p.044912_1 - 044912_16, 2011/04

 Times Cited Count:8 Percentile:49.7(Physics, Nuclear)

Measurements of electrons from the decay of open-heavy-flavor mesons have shown that the yields are suppressed in Au+Au collisions compared to expectations from binary-scaled $$p+p$$ collisions. Here we extend these studies to two particle correlations where one particle is an electron from the decay of a heavy flavor meson and the other is a charged hadron from either the decay of the heavy meson or from jet fragmentation. These measurements provide more detailed information about the interaction between heavy quarks and the quark-gluon matter. We find the away-side-jet shape and yield to be modified in Au+Au collisions compared to $$p+p$$ collisions.

Journal Articles

Intense femto-second laser-driven X-ray source coupled with multiple directional quantum beams for applications

Daido, Hiroyuki; Sagisaka, Akito; Ogura, Koichi; Orimo, Satoshi; Nishiuchi, Mamiko; Yogo, Akifumi; Mori, Michiaki; Li, Z.*; Kiriyama, Hiromitsu; Kanazawa, Shuhei; et al.

X-Ray Lasers 2006; Springer Proceedings in Physics, Vol.115, p.595 - 605, 2007/00

At present, using ultra-short high intensity lasers at APRC, JAEA Kansai photon research institute, we are developing laser driven multiple quantum beams such as protons, X-rays, electrons and THz waves. These beams are perfectly synchronized with each other. The pulse duration of each beam is lass than a pico-second. They have sharp directionality with high brightness. If we properly combined these, we have new pump-probe techniques for various applications.

JAEA Reports

Example of answers to the problems of the 36th examination for the chief engineer of nuclear fuel, 2004

Yachi, Shigeyasu; Nakamura, Jinichi; Amaya, Masaki; Nakajima, Kunihisa; Komuro, Yuichi; Nakajima, Katsuaki*; Kobayashi, Yasuhiko; Sato, Tadashi*; Suga, Shinichi*; Noguchi, Hiroshi; et al.

JAERI-Review 2004-020, 61 Pages, 2004/09

JAERI-Review-2004-020.pdf:1.85MB

This report provides an example of answers to the problems of the 36th Examination for the Chief Engineer of Nuclear Fuel. This examination was done as a national qualification in March 2004. Brief explanations or references are added to some answers.

JAEA Reports

Example of answers to the problems of 31st to 35th examinations for the chief engineer of nuclear fuel, 1999 to 2003

Yachi, Shigeyasu; Sato, Tadashi; Suga, Shinichi*; Komuro, Yuichi; Uchida, Masaaki; Nakajima, Kunihisa; Nakamura, Jinichi; Amezawa, Hiroo; Omura, Hideaki*; Minato, Kazuo; et al.

JAERI-Review 2003-025, 162 Pages, 2003/09

JAERI-Review-2003-025.pdf:5.96MB

The report contains example of answers to the Problems of 31st(1999) to 35th(2003) Examinations for the Chief Engineer of Nuclear Fuel which were conducted as a national qualification examination. Brief explanations or references are given to some answers.

Oral presentation

Simultaneous generation of proton beam and terahertz radiation under intense ultrashort pulse-laser irradiation

Sagisaka, Akito; Daido, Hiroyuki; Pirozhkov, A. S.; Ogura, Koichi; Orimo, Satoshi; Mori, Michiaki; Yogo, Akifumi; Nakamura, Shu*; Iwashita, Yoshihisa*; Shirai, Toshiyuki*; et al.

no journal, , 

no abstracts in English

Oral presentation

Improvement of SiC-MOS devices with plasma nitridation and AlON/SiO$$_{2}$$ stacked dielectrics

Watanabe, Heiji*; Kagei, Yusuke*; Kosono, Kohei*; Kirino, Takashi*; Watanabe, Yu*; Mitani, Shuhei*; Nakano, Yuki*; Nakamura, Takashi*; Yoshigoe, Akitaka; Teraoka, Yuden; et al.

no journal, , 

SiC-MOSFET's are expected for normally-off-type high performance power devices. Electrical defects due to residual inpurities such as carbon are in the interface of thermally-oxidized SiC-MOS's so that channel mobility is degraded preferentially. Although upgrade of reliability of a gate insulator is necessary for practical use, insulator degradation mechanisms have not well known yet. We are studying high quality MOS interface made by plasma nitridation techniques, upgrade of reliability and insulation by a stuck structure of a high-k insulator (AlON) layer and an SiO$$_{2}$$ underlayer. Recent research results on those subjects are reported in this talk.

Oral presentation

Sensitivity control of nuclear emulsion using AgBr nano-grains

Ishihara, Kohei*; Takagi, Keisuke*; Kawarabayashi, Jun*; Tomita, Hideki*; Naka, Tatsuhiro*; Asada, Takashi*; Morishima, Kunihiro*; Nakamura, Mitsuhiro*; Kuge, Kenichi*; Maeda, Shigetaka; et al.

no journal, , 

The nuclear emulsion with AgBr nano-grains has been developed for neutron detection under high $$gamma$$-ray background. It has been demonstrated that the detection sensitivity of $$gamma$$-rays can be well suppressed compared to that of neutrons by adjusting the size of AgBr nano-grains to deposit the energy of the secondary electrons produced by $$gamma$$-rays below a certain threshold which can create Ag latent images.

Oral presentation

Temperature dependence of $$gamma$$-ray and neutron sensitivities of nuclear emulsion with AgBr nano-grains

Ishihara, Kohei*; Kawarabayashi, Jun*; Tomita, Hideki*; Naka, Tatsuhiro*; Asada, Takashi*; Morishima, Kunihiro*; Nakamura, Mitsuhiro*; Maeda, Shigetaka; Iguchi, Tetsuo*

no journal, , 

In order to establish a neutron spectrum measurement in high $$gamma$$ field such as spent nuclear fuel storage, advanced nuclear emulsion based on non-sensitized OPERA film with AgBr grain size of 60 nm has been developed. A nuclear emulsion has the feature of being easy to cause latent image degradation in the high temperature condition. In this study, the experiment estimated the temperature dependency of the sensitivity to the $$gamma$$ ray and neutron of a new nuclear emulsion. It is confirmed that the detection efficiency for a neutron and $$gamma$$ fell in more than 30 $$^{circ}$$C environment.

28 (Records 1-20 displayed on this page)