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Journal Articles

Development of an iron(II) complex exhibiting thermal- and photoinduced double proton-transfer-coupled spin transition in a short hydrogen bond

Nakanishi, Takumi*; Hori, Yuta*; Shigeta, Yasuteru*; Sato, Hiroyasu*; Kiyanagi, Ryoji; Munakata, Koji*; Ohara, Takashi; Okazawa, Atsushi*; Shimada, Rintaro*; Sakamoto, Akira*; et al.

Journal of the American Chemical Society, 145(35), p.19177 - 19181, 2023/08

 Times Cited Count:1 Percentile:0(Chemistry, Multidisciplinary)

Journal Articles

Factors regulating the concentration of particulate iodine in coastal seawater

Sato, Yuhi*; Otosaka, Shigeyoshi*; Suzuki, Takashi; Nakanishi, Takahiro

Limnology and Oceanography, 68(7), p.1580 - 1594, 2023/07

 Times Cited Count:2 Percentile:79.14(Limnology)

To investigate the factors regulating the concentration of particulate iodine (PI) in seawater, it was measured in two Pacific coastal areas adjacent to Japan in two seasons along with parameters such as particulate organic carbon (POC) and nitrogen (PON), dissolved iodine (DI), and phytoplankton pigments. The dataset was divided in three groups namely, lower (Group A), average (Group B), and higher (Group C) atomic ratios of PI to POC (I/C). The three groups were characterized by phytoplanktonic physiological states as highly productive, steady, and senescent states, respectively. Based on the finding that PI production is associated with the phytoplankton physiological state, the seasonal and regional differences in PI concentration and I/C in the observation areas were consistently explained. Finally, we suggest that the phytoplanktonic physiological state is one of the vital factors regulating the PI concentration in seawater.

Journal Articles

Observation of proton-transfer-coupled spin transition by single-crystal neutron-diffraction measurement

Nakanishi, Takumi*; Hori, Yuta*; Shigeta, Yasuteru*; Sato, Hiroyasu*; Wu, S.-Q.*; Kiyanagi, Ryoji; Munakata, Koji*; Ohara, Takashi; Sato, Osamu*

Physical Chemistry Chemical Physics, 25(17), p.12394 - 12400, 2023/05

 Times Cited Count:1 Percentile:50.66(Chemistry, Physical)

Journal Articles

Distribution and settling behavior of americium-241 in the tropical East Pacific

Kinoshita, Norikazu*; Nagaoka, Mika; Nakanishi, Takashi*

Science of the Total Environment, 753, p.142087_1 - 142087_10, 2021/01

 Times Cited Count:4 Percentile:26.95(Environmental Sciences)

The distribution of the anthropogenic radionuclide americium-241 ($$^{241}$$Am), a decay product of $$^{241}$$Pu discharged from atmospheric tests of nuclear weapons, was investigated to resolve its horizontal and vertical migration in the Tropical East Pacific. We analyzed $$^{241}$$Am concentrations in seawater samples collected in 2003. On comparing the $$^{241}$$Am concentrations with the previously determined concentrations of $$^{239+240}$$Pu in the same samples, the vertical profiles of $$^{241}$$Am were found to be similar to those of $$^{239+240}$$Pu. At some stations, the maximum concentration of $$^{241}$$Am occurred 100-200 m deeper than that of $$^{239+240}$$Pu. The $$^{241}$$Am/$$^{239+240}$$Pu ratios in the North Pacific and South Pacific were comparable to one another, and were typical of the ratio for the Pacific. The $$^{241}$$Am distribution was influenced by the water mass at depths below 400 m. The $$^{241}$$Am data support the view there is a current flowing at depths of 400-3000 m from the North Pacific through the equator to the South Pacific. In addition, the $$^{241}$$Am vertical profile was explained by using a box model that considers the decay of $$^{241}$$Pu and adsorption and scavenging by suspended particles. The different depths for the maximum concentrations of $$^{241}$$Am and $$^{239+240}$$Pu observed at some stations were well explained by the model and by the distribution of CaCO$$_{3}$$ particles. The residence time of $$^{241}$$Am in the Pacific was also estimated by using the model.

Journal Articles

Distribution and fate of $$^{129}$$I in the seabed sediment off Fukushima

Otosaka, Shigeyoshi; Sato, Yuhi*; Suzuki, Takashi; Kuwabara, Jun; Nakanishi, Takahiro

Journal of Environmental Radioactivity, 192, p.208 - 218, 2018/12

AA2017-0744.pdf:1.17MB

 Times Cited Count:15 Percentile:47.7(Environmental Sciences)

From August 2011 to October 2013, the concentration of iodine-129 ($$^{129}$$I) in the seabed sediment collected from 26 stations located within 160 km from the Fukushima Daiichi Nuclear Power Plant was estimated. The concentrations of $$^{129}$$I in seabed sediment off Fukushima in 2011 ranged between 0.02 and 0.45 mBq/kg. Although iodine is a biophilic element, the accident-derived radioiodine negligibly affects the benthic ecosystem. Until October 2013, a slightly increased activity of $$^{129}$$I in the surface sediment in the shelf-edge region (bottom depth: 200-400 m) was observed. The increase of the $$^{129}$$I concentrations in the shelf-edge sediments was affected by the (1) transport of $$^{129}$$I-bound particles from the land through rivers and (2) re-deposition of $$^{129}$$I desorbed from the contaminated coastal sediment to the shelf-edge sediments, which were considered to be dominant processes.

Journal Articles

Study on current US views on bilateral civilian nuclear cooperation agreements

Tazaki, Makiko; Tamai, Hiroshi; Shimizu, Ryo; Kimura, Takashi; Kitade, Yuta; Nakanishi, Hiroaki; Suda, Kazunori

Nihon Kaku Busshitsu Kanri Gakkai Dai-39-Kai Nenji Taikai Rombunshu (Internet), 7 Pages, 2018/11

no abstracts in English

Journal Articles

A Study on the tendencies on the member states from which Broader Conclusion (BC) has been drawn and on those from which BC has not been drawn yet by the International Atomic Energy Agency; Extracting possible requirements for drawing the BC

Nakanishi, Hiroaki; Kimura, Takashi; Shimizu, Ryo; Kitade, Yuta; Tazaki, Makiko; Tamai, Hiroshi; Suda, Kazunori

Nihon Kaku Busshitsu Kanri Gakkai Dai-39-Kai Nenji Taikai Rombunshu (Internet), 9 Pages, 2018/11

To extract the possible requirements for the Broader Conclusion (BC) drawn by the IAEA in the Member States, this study is to conduct the comparative analysis of the tendencies on the Member States from which the BC has been drawn and those from which the BC has not been drawn yet.

Journal Articles

Summary of research result of State Level Concept (SLC)

Kimura, Takashi; Tazaki, Makiko; Kitade, Yuta; Shimizu, Ryo; Tamai, Hiroshi; Nakanishi, Hiroaki; Suda, Kazunori

Nihon Kaku Busshitsu Kanri Gakkai Dai-39-Kai Nenji Taikai Rombunshu (Internet), 5 Pages, 2018/11

This is the summary of research result of State Level Concept (SLC) which has been developed and conducted by the IAEA and a major purpose of the research reported here is to promote the nuclear operator's understandings for the importance of Broder Conclusion drawn continuously by the IAEA under SLC.

Journal Articles

Study on elements of establishing the regional safeguards

Kitade, Yuta; Tamai, Hiroshi; Tazaki, Makiko; Shimizu, Ryo; Kimura, Takashi; Nakanishi, Hiroaki; Suda, Kazunori

Nihon Kaku Busshitsu Kanri Gakkai Dai-39-Kai Nenji Taikai Rombunshu (Internet), 9 Pages, 2018/11

Regional Safeguards is considered as one of the measures for strengthening IAEA safeguards and its concept is recognized at NPT Review Conference and also NSG Guidelines amended in 2011. This Study examines the elements for the proper establishment of Regional Safeguards.

Journal Articles

Vertical and lateral transport of particulate radiocesium off Fukushima

Otosaka, Shigeyoshi; Nakanishi, Takahiro; Suzuki, Takashi; Sato, Yuhi; Narita, Hisashi*

Environmental Science & Technology, 48(21), p.12595 - 12602, 2014/11

 Times Cited Count:25 Percentile:58.4(Engineering, Environmental)

From August 2011 to July 2013, a sediment trap was deployed at 100 km east of the Fukushima Daiichi Nuclear Power Plant and sinking particles were collected. Sinking flux of $$^{137}$$Cs decreased over time with seasonal fluctuation. The $$^{137}$$Cs fluxes were mainly affected by two principal modes. One was a rapid sinking of radiocesium-bound particles (moderate mode). This mode was dominant especially in the early post-accident stage, and was presumed to establish the distribution of radiocesium in the offshore seabed. Another was the secondary transport of particles attributed to turbulence near the seabed and was observed in winter (turbulence mode). Although the latter process would not drastically change the distribution of sedimentary radiocesium, attention should be paid as this key process redistributing the accident-derived radiocesium may cumulatively affect the long-term distribution.

Journal Articles

The Project for grouting development for high level radioactive waste repository, 3; Study of allowable seepage water quantity by permiability test though contact face of buffer material blocks

Sekine, Ichiro*; Yamada, Tsutomu*; Sekiguchi, Takashi*; Fujita, Tomoo; Nakanishi, Tatsuro

Doboku Gakkai Heisei-23-Nendo Zenkoku Taikai Dai-66-Kai Nenji Gakujutsu Koenkai Koen Gaiyoshu (DVD-ROM), p.69 - 70, 2011/09

no abstracts in English

Journal Articles

Basic vacuum test of 500-kV photocathode DC gun components at KEK

Yamamoto, Masahiro*; Uchiyama, Takashi*; Miyajima, Tsukasa*; Honda, Yosuke*; Sato, Kotaro*; Matsuba, Shunya*; Saito, Yoshio*; Kobayashi, Masanori*; Kurisu, Hiriki*; Hajima, Ryoichi; et al.

Proceedings of 7th Annual Meeting of Particle Accelerator Society of Japan (DVD-ROM), p.717 - 720, 2010/08

A 500-kV photocathode DC electron gun which can supply the beam of a low emittance and a high average current has been developed in collaboration with KEK, JAEA, Hiroshima Univ., Nagoya Univ. and Yamaguchi Univ. The vacuum of the gun chamber has to be lower Extreme High Vacuum for maintain cathode-life time. A titanium chamber and new material of ceramic were employed to reduce outgassing rate. The result of outgassing rate of the gun chamber is described in this report.

Journal Articles

Recent progress in the energy recovery linac project in Japan

Sakanaka, Shogo*; Akemoto, Mitsuo*; Aoto, Tomohiro*; Arakawa, Dai*; Asaoka, Seiji*; Enomoto, Atsushi*; Fukuda, Shigeki*; Furukawa, Kazuro*; Furuya, Takaaki*; Haga, Kaiichi*; et al.

Proceedings of 1st International Particle Accelerator Conference (IPAC '10) (Internet), p.2338 - 2340, 2010/05

Future synchrotron light source using a 5-GeV energy recovery linac (ERL) is under proposal by our Japanese collaboration team, and we are conducting R&D efforts for that. We are developing high-brightness DC photocathode guns, two types of cryomodules for both injector and main superconducting (SC) linacs, and 1.3 GHz high CW-power RF sources. We are also constructing the Compact ERL (cERL) for demonstrating the recirculation of low-emittance, high-current beams using above-mentioned critical technologies.

Journal Articles

Design of a 500kV electron gun for ERL light source at KEK

Yamamoto, Masahiro*; Honda, Yosuke*; Miyajima, Tsukasa*; Uchiyama, Takashi*; Kobayashi, Masanori*; Muto, Toshiya*; Matsuba, Shunya*; Sakanaka, Shogo*; Sato, Kotaro*; Saito, Yoshio*; et al.

Proceedings of 6th Annual Meeting of Particle Accelerator Society of Japan (CD-ROM), p.860 - 862, 2009/08

A newly 500 kV electron gun (2nd - 500 kV gun) for an ERL light source is designed at KEK. A new concept and state of-the-art technologies of vacuum system, ceramic insulators, high voltage power supply, photocathode and preparation system will be employed. The details are described in this report.

Journal Articles

Partition coefficient of Ra in gypsum

Yoshida, Yasushi*; Nakazawa, Toshiyuki*; Yoshikawa, Hideki; Nakanishi, Takashi*

Journal of Radioanalytical and Nuclear Chemistry, 280(3), p.541 - 545, 2009/06

 Times Cited Count:12 Percentile:62.2(Chemistry, Analytical)

Coprecipitation experiment of Ra in gypsum was done with oversaturation method. Derived partition coefficient is,0.71$$pm$$0.53. Partition coefficient of Ra in gypsum was not reported. Comparing with that of Ra in barite and of Sr in gypsum, a value of partition coefficient in the present study is though to be reasonable.

Journal Articles

$$^{52}$$Fe translocation in barley as monitored by a Positron-Emitting Tracer Imaging System (PETIS); Evidence for the direct translocation of Fe from roots to young leaves via phloem

Tsukamoto, Takashi*; Nakanishi, Hiromi*; Uchida, Hiroshi*; Watanabe, Satoshi; Matsuhashi, Shimpei; Mori, Satoshi*; Nishizawa, Naoko*

Plant & Cell Physiology, 50(1), p.48 - 57, 2009/01

 Times Cited Count:88 Percentile:90.15(Plant Sciences)

Journal Articles

Deoxymugineic acid increases Zn translocation in Zn-deficient rice plants

Suzuki, Motofumi*; Tsukamoto, Takashi*; Inoue, Haruhiko*; Watanabe, Satoshi; Matsuhashi, Shimpei; Takahashi, Michiko*; Nakanishi, Hiromi*; Mori, Satoshi*; Nishizawa, Naoko*

Plant Molecular Biology, 66(6), p.609 - 617, 2008/04

 Times Cited Count:138 Percentile:95.23(Biochemistry & Molecular Biology)

Journal Articles

New system of nuclear education by network

Hasegawa, Makoto; Nakanishi, Takashi*; Fujii, Yasuhiko*; Odaka, Tomohiro*

Hosha Kagaku Nyusu, (17), p.29 - 35, 2008/03

no abstracts in English

Journal Articles

Partition coefficients of Ra and Ba in calcite

Yoshida, Yasushi*; Yoshikawa, Hideki; Nakanishi, Takashi*

Geochemical Journal, 42(3), p.295 - 304, 2008/00

 Times Cited Count:15 Percentile:37.62(Geochemistry & Geophysics)

Partition coefficients ($$D$$) of Ra and Ba in calcite were derived in an experiment of coprecipitation. Free Drift Method (FDM) was adopted. As a result of experiment, $$D$$ of Ra and Ba were 9.4e-3 and 4.7e-3, respectively. A saturation state is expected to be a low oversaturation in duration of experiment and according to an estimated saturation index, a composition of a final solution was close to equilibrium with calcite. The values of $$D$$$$_{rm Ra}$$ and $$D$$$$_{rm Ba}$$ showed the similar extent. It implies that difference of size of ionic radius does not affect incorporation behavior of Ra and Ba in calcite.

Journal Articles

Mutational reconstructed ferric chelate reductase confers enhanced tolerance in rice to iron deficiency in calcareous soil

Ishimaru, Yasuhiro*; Kim, S.*; Tsukamoto, Takashi*; Oki, Hiroyuki*; Kobayashi, Takanori*; Watanabe, Satoshi; Matsuhashi, Shimpei; Takahashi, Michiko*; Nakanishi, Hiromi*; Mori, Satoshi*; et al.

Proceedings of the National Academy of Sciences of the United States of America, 104(18), p.7373 - 7378, 2007/05

 Times Cited Count:131 Percentile:93.39(Multidisciplinary Sciences)

51 (Records 1-20 displayed on this page)