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Journal Articles

The Hydrogen-bond network in sodium chloride tridecahydrate; Analogy with ice VI

Yamashita, Keishiro*; Nakayama, Kazuya*; Komatsu, Kazuki*; Ohara, Takashi; Munakata, Koji*; Hattori, Takanori; Sano, Asami; Kagi, Hiroyuki*

Acta Crystallographica Section B; Structural Science, Crystal Engineering and Materials (Internet), 79(5), p.414 - 426, 2023/10

 Times Cited Count:0 Percentile:0.02(Chemistry, Multidisciplinary)

The structure of a recently-found hyperhydrated form of sodium chloride, NaCl$$cdot$$ 13H(D)$$_{2}$$O, has been determined by ${it in situ}$ single-crystal neutron diffraction at 1.7 GPa and 298 K. It has large hydrogen-bond networks and some water molecules have distorted bonding features such as bifurcated hydrogen bonds and five-coordinated water molecules. The hydrogen-bond network has similarities to ice VI in terms of network topology and disordered hydrogen bonds. Assuming the equivalence of network components connected by pseudo symmetries, the overall network structure of this hydrate can be expressed by breaking it down into smaller structural units which correspond to the ice VI network structure. This hydrogen-bond network contains orientational disorder of water molecules in contrast to the known salt hydrates. Here, we present an example for further insights into a hydrogen-bond network containing ionic species.

Journal Articles

External exposure assessment in the Fukushima accident area for governmental policy planning in Japan, 2; Matters to be attended for assessments of external exposure

Yoshimura, Kazuya; Sanada, Yukihisa; Sato, Rina; Nakayama, Mariko*; Tsubokura, Masaharu*

Journal of Radiation Research (Internet), 64(2), p.203 - 209, 2023/03

 Times Cited Count:1 Percentile:0.01(Biology)

After the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident, individual exposure doses to residents have been assessed by many municipalities, governments and research institutes. Various methods including measurements with personal dosimeters and simulations have been used for this evaluation depending on purposes, but the information of assessments and methods has not been systematically organized. A comprehensive review of the knowledge and experiences of individual exposure doses assessments accumulated so far and understanding the characteristics of the assessment methods will be very useful for radiation protection and risk communication, following to governmental policy planning. We reviewed the efforts made by the Japanese government and research institutes to assess radiation doses to residents after the FDNPS accident in Part1. On the other hand, each method of assessing individual exposure doses includes uncertainties and points to be considered for the appropriate assessment. These knowledge and experiences are important for the assessment implementation and applying the assessment results to the governmental policy planning, and are summarized in Part2 of this article.

JAEA Reports

Individual exposure dose assessment of residents for lifting of evacuation orders (Contract research)

Sato, Rina; Sanada, Yukihisa; Yoshimura, Kazuya; Nakayama, Mariko*

JAEA-Review 2022-055, 42 Pages, 2023/01

JAEA-Review-2022-055.pdf:1.31MB

The evacuation order zones established after the accident at the Tokyo Electric Power Company's Fukushima Daiichi Nuclear Power Station have been reorganized according to the decrease in ambient dose equivalent rates and the decontamination progress. It has been decided to decontaminate the difficult-to-return zones and lift the evacuation order depending on the evacuee's intention of returning to the areas over the course of the 2020s. In order to consider the future of individual exposure dose assessment for residents for lifting of the evacuation orders, the methods and characteristics of the assessment that have been conducted after the accident using personal dosimeter measurements and simulations were systematically reviewed. This report summarized the results of the review.

Journal Articles

External exposure assessment in the Fukushima accident area for governmental policy planning in Japan, 1; Methodologies for personal dosimetry applied after the accident

Sanada, Yukihisa; Yoshimura, Kazuya; Sato, Rina; Nakayama, Mariko*; Tsubokura, Masaharu*

Journal of Radiation Research (Internet), 64(1), p.2 - 10, 2023/01

 Times Cited Count:0 Percentile:0.06(Biology)

The evacuation orderareas established due to the accident at the Tokyo Electric Power Company Holdings' (TEPCO) Fukushima Daiichi Nuclear Power Plant (FDNPP) have been reorganized according to the decrease in ambient dose rates and the decontamination progress. The Japanese government decided to decontaminate the difficult-to-return areas and lift the evacuation order by 2030. This radiation protection strategy can be optimized by examining emergency exposure situations to date and the existing exposure after the accident. This article reviews the methods that can determine the individual radiation doses of residents who should return to their homes when the evacuation order is lifted in the specific reconstruction reproduction base area and the difficult-to-return areas outside this base area and summarizes the points to be considered when implementing these methods. In Part 1 of this article, we review the efforts made by the Japanese government and research institutes to assess radiation doses to residents after the FDNPP accident.

Journal Articles

${it Operando}$ structure observation of pyroelectric ceramics during power generation cycle

Kawasaki, Takuro; Fukuda, Tatsuo; Yamanaka, Satoru*; Sakamoto, Tomokazu*; Murayama, Ichiro*; Kato, Takanori*; Baba, Masaaki*; Hashimoto, Hideki*; Harjo, S.; Aizawa, Kazuya; et al.

Journal of Applied Physics, 131(13), p.134103_1 - 134103_7, 2022/04

 Times Cited Count:1 Percentile:15.88(Physics, Applied)

JAEA Reports

Synthesis report on the R&D for the Horonobe Underground Research Laboratory; Project carried out during fiscal years 2015-2019

Nakayama, Masashi; Saiga, Atsushi; Kimura, Shun; Mochizuki, Akihito; Aoyagi, Kazuhei; Ono, Hirokazu; Miyakawa, Kazuya; Takeda, Masaki; Hayano, Akira; Matsuoka, Toshiyuki; et al.

JAEA-Research 2019-013, 276 Pages, 2020/03

JAEA-Research-2019-013.pdf:18.72MB

The Horonobe Underground Research Laboratory (URL) Project is being pursued by the Japan Atomic Energy Agency (JAEA) to enhance the reliability of relevant disposal technologies for geological disposal of High-level Radioactive Waste through investigations of the deep geological environment within the host sedimentary rock at Horonobe Town in Hokkaido, north Japan. The investigations will be conducted in three phases, namely "Phase 1: Surface based investigations", "Phase 2: Construction phase" (investigations during construction of the underground facilities) and "Phase 3: Operation phase" (research in the underground facilities). According to the research plan described in the 3rd Mid- and Long- term Plan of JAEA, "Near-field performance study", "Demonstration of repository design option", and "Verification of crustal-movement buffering capacity of sedimentary rocks" are important issues of the Horonobe URL Project, and schedule of future research and backfill plans of the project will be decided by the end of 2019 Fiscal Year. The present report summarizes the research and development activities of these 3 important issues carried out during 3rd Medium to Long-term Research Phase.

Journal Articles

Pyroelectric power generation from the waste heat of automotive exhaust gas

Kim, J.*; Yamanaka, Satoru*; Murayama, Ichiro*; Kato, Takanori*; Sakamoto, Tomokazu*; Kawasaki, Takuro; Fukuda, Tatsuo; Sekino, Toru*; Nakayama, Tadachika*; Takeda, Masatoshi*; et al.

Sustainable Energy & Fuels (Internet), 4(3), p.1143 - 1149, 2020/03

 Times Cited Count:16 Percentile:63.91(Chemistry, Physical)

Journal Articles

Enhancement of element production by incomplete fusion reaction with weakly bound deuteron

Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.

Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07

 Times Cited Count:8 Percentile:55.71(Physics, Multidisciplinary)

Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for $$^{107}$$Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.

JAEA Reports

Horonobe Underground Research Laboratory Project; Synthesis of Phase II (Construction Phase) investigations to a depth of 350m

Sato, Toshinori; Sasamoto, Hiroshi; Ishii, Eiichi; Matsuoka, Toshiyuki; Hayano, Akira; Miyakawa, Kazuya; Fujita, Tomoo*; Tanai, Kenji; Nakayama, Masashi; Takeda, Masaki; et al.

JAEA-Research 2016-025, 313 Pages, 2017/03

JAEA-Research-2016-025.pdf:45.1MB

The Horonobe Underground Research Laboratory (URL) Project is being pursued by the Japan Atomic Energy Agency (JAEA) to enhance the reliability of relevant disposal technologies through investigations of the deep geological environment within the host sedimentary formations at Horonobe, northern Hokkaido. This report summarizes the results of the Phase II investigations carried out from April 2005 to June 2014 to a depth of 350m. Integration of work from different disciplines into a "geosynthesis" ensures that the Phase II goals have been successfully achieved and identifies key issues that need to made to be addressed in the Phase II investigations Efforts are made to summarize as many lessons learnt from the Phase II investigations and other technical achievements as possible to form a "knowledge base" that will reinforce the technical basis for both implementation and the formulation of safety regulations.

JAEA Reports

Synthesized research report in the second mid-term research phase, Mizunami Underground Research Laboratory Project, Horonobe Underground Research Laboratory Project and Geo-stability Project (Translated document)

Hama, Katsuhiro; Sasao, Eiji; Iwatsuki, Teruki; Onoe, Hironori; Sato, Toshinori; Fujita, Tomoo; Sasamoto, Hiroshi; Matsuoka, Toshiyuki; Takeda, Masaki; Aoyagi, Kazuhei; et al.

JAEA-Review 2016-014, 274 Pages, 2016/08

JAEA-Review-2016-014.pdf:44.45MB

We synthesized the research results from the Mizunami/Horonobe Underground Research Laboratories (URLs) and geo-stability projects in the second midterm research phase. This report can be used as a technical basis for the Nuclear Waste Management Organization of Japan/Regulator at each decision point from siting to beginning of disposal (Principal Investigation to Detailed Investigation Phase).

Journal Articles

Spin pumping blocked by single-layer graphene

Haku, Satoshi*; Tashiro, Takaharu*; Nakayama, Hiroyasu*; Ieda, Junichi; Entani, Shiro; Sakai, Seiji; Ando, Kazuya*

Applied Physics Express, 8(7), p.073009_1 - 073009_3, 2015/07

 Times Cited Count:4 Percentile:18.5(Physics, Applied)

We found that the spin pumping in a Ni$$_{81}$$Fe$$_{19}$$/Pt bilayer is strongly suppressed by inserting single-layer graphene (SLG) at the interface. The spin pumping in the Ni$$_{81}$$Fe$$_{19}$$/Pt bilayer enhances the magnetization damping of the ferromagnetic layer, which is quantified from microwave frequency dependence of ferromagnetic resonance linewidth. We show that the enhancement of the magnetization damping due to the spin pumping disappears in a Ni$$_{81}$$Fe$$_{19}$$/SLG/Pt trilayer. This result indicates that the spin pumping is blocked by the atomic monolayer, demonstrating the crucial role of the interfacial short-range spin-exchange coupling in the spin pumping in metallic systems.

Journal Articles

Spin mixing conductance at a well-controlled platinum/yttrium iron garnet interface

Qiu, Z.*; Ando, Kazuya*; Uchida, Kenichi*; Kajiwara, Yosuke*; Takahashi, Ryo*; Nakayama, Hiroyasu*; An, Toshu*; Fujikawa, Yasunori*; Saito, Eiji

Applied Physics Letters, 103(9), p.092404_1 - 092404_4, 2013/08

 Times Cited Count:116 Percentile:95.79(Physics, Applied)

A platinum (Pt)/yttrium iron garnet (YIG) bilayer system with a well-controlled interface has been developed; spin mixing conductance at the Pt/YIG interface has been studied. A clear interface with good crystal perfection is experimentally demonstrated to be one of the important factors for an ultimate spin mixing conductance. The spin mixing conductance is obtained to be 1.3$$times$$10$$^{18}$$m$$^{-2}$$ at the well-controlled Pt/YIG interface, which is close to a theoretical prediction.

Journal Articles

Interface induced inverse spin Hall effect in bismuth/permalloy bilayer

Hou, D.*; Qiu, Z.*; Harii, Kazuya; Kajiwara, Yosuke*; Uchida, Kenichi*; Fujikawa, Yasunori*; Nakayama, Hiroyasu*; Yoshino, Tatsuro*; An, Toshu*; Ando, Kazuya*; et al.

Applied Physics Letters, 101(4), p.042403_1 - 042403_4, 2012/07

 Times Cited Count:76 Percentile:92.13(Physics, Applied)

Inverse spin Hall effect has been investigated in bismuth(Bi)/permalloy(Py) bilayer films by using the spin pumping at room temperature. From the ferromagnetic-resonance-spectrum linewidth data, Bi is proved to be a good spin sink in our structure. We measured inverse spin Hall voltage and conductance of the Bi/Py bilayer and found that the inverse spin Hall current, $$I_c$$, decreases with increasing the Bi thickness, which is in contrast to the former understanding in similar bilayer systems, e.g., Pt/Py. We constructed a model to explain the thickness dependence of $$I_c$$ quantitatively, in which spin transport modulation near Bi/Py interface is considered.

Journal Articles

Geometry dependence on inverse spin Hall effect induced by spin pumping in Ni$$_{81}$$Fe$$_{19}$$/Pt films

Nakayama, Hiroyasu*; Ando, Kazuya*; Harii, Kazuya; Yoshino, Tatsuro*; Takahashi, Ryo*; Kajiwara, Yosuke*; Uchida, Kenichi*; Fujikawa, Yasunori*; Saito, Eiji

Physical Review B, 85(14), p.144408_1 - 144408_7, 2012/04

 Times Cited Count:192 Percentile:97.97(Materials Science, Multidisciplinary)

Geometric effects on the inverse spin Hall effect (ISHE) induced by the spin pumping driven by the ferromagnetic resonance (FMR) have been investigated quantitatively. We measured the FMR spectra and the electromotive force induced by the ISHE with changing the size and the thickness in Ni$$_{81}$$Fe$$_{19}$$/Pt films. The intensity of generated charge currents due to the ISHE changes systematically with changing the film geometry. The experimental results show a clear difference between Ni$$_{81}$$Fe$$_{19}$$ and Pt thickness dependence of the ISHE induced by the spin pumping.

Journal Articles

Rational design of DNA sequence-specific zinc fingers

Kono, Hidetoshi; Imanishi, Miki*; Negi, Shigeru*; Tatsutani, Kazuya*; Sakaeda, Yui*; Hashimoto, Ayaka*; Nakayama, Chie*; Futaki, Shiro*; Sugiura, Yukio*

FEBS Letters, 586(6), p.918 - 923, 2012/03

 Times Cited Count:5 Percentile:14.67(Biochemistry & Molecular Biology)

Journal Articles

Inverse spin-Hall effect induced by spin pumping in metallic systems

Ando, Kazuya*; Takahashi, Saburo; Ieda, Junichi; Kajiwara, Yosuke*; Nakayama, Hiroyasu*; Yoshino, Tatsuro*; Harii, Kazuya*; Fujikawa, Yasunori*; Matsuo, Mamoru*; Maekawa, Sadamichi; et al.

Journal of Applied Physics, 109(10), p.103913_1 - 103913_11, 2011/05

 Times Cited Count:431 Percentile:99.5(Physics, Applied)

The inverse spin-Hall effect (ISHE) induced by the spin pumping has been investigated systematically in simple ferromagnetic/paramagnetic bilayer systems. The spin pumping driven by ferromagnetic resonance injects a spin current into the paramagnetic layer, which gives rise to an electromotive force transverse to the spin current using the ISHE in the paramagnetic layer. In a Ni$$_{81}$$Fe$$_{19}$$/Pt film, we found an electromotive force perpendicular to the applied magnetic field at the ferromagnetic resonance condition. The spectral shape of the electromotive force is well reproduced using a simple Lorentz function, indicating that the electromotive force is due entirely to the ISHE induced by the spin pumping; the extrinsic magnetogalvanic effects are eliminated in this measurement. The electromotive force varies systematically by changing the microwave power, magnetic-field angle, and film size, which are well reproduced by a calculation based on the Landau-Lifshitz-Gilbert equation combined with the models of the ISHE and spin pumping. The electromotive force was observed also in a Pt/Y$$_3$$Fe$$_4$$GaO$$_{12}$$ film, in which the metallic Ni$$_{81}$$Fe$$_{19}$$ layer is replaced by an insulating Y$$_3$$Fe$$_4$$GaO$$_{12}$$ layer, supporting that the spin-pumping-induced ISHE is responsible for the observed electromotive force.

Journal Articles

Universality of the spin pumping in metallic bilayer films

Yoshino, Tatsuro*; Ando, Kazuya*; Harii, Kazuya*; Nakayama, Hiroyasu*; Kajiwara, Yosuke*; Saito, Eiji

Applied Physics Letters, 98(3), p.132503_1 - 132503_3, 2011/03

 Times Cited Count:33 Percentile:76.88(Physics, Applied)

We show a clear guideline for generating a large spin current using the spin pumping in metallic bilayer films. We measured spin currents generated by the spin pumping in Ni$$_{1-x}$$Fe$$_{x}$$/Pt bilayer films using the inverse spin-Hall effect (ISHE). The magnitude of the ISHE signals are well reproduced by a calculation based on the model of the spin pumping. The result shows that the amplitude of a spin current is universally determined by the product of the saturation magnetization, the additional damping constant, and the solid angle of the magnetization precession.

Journal Articles

Inverse spin-Hall effect induced by spin pumping in different size Ni$$_{81}$$Fe$$_{19}$$/Pt films

Nakayama, Hiroyasu*; Ando, Kazuya*; Harii, Kazuya*; Fujikawa, Yasunori*; Kajiwara, Yosuke*; Yoshino, Tatsuro*; Saito, Eiji

Journal of Physics; Conference Series, 266, p.012100_1 - 012100_4, 2011/01

 Times Cited Count:9 Percentile:95.67(Materials Science, Multidisciplinary)

The inverse spin-Hall effect, conversion of spin currents into electric voltage, has been investigated in Ni$$_{81}$$Fe$$_{19}$$/Pt bilayer films with different length and width. We measured the electric voltage generated by the inverse spin-Hall effect induced by the spin pumping at room temperature. The experimental results indicate that the electric voltage induced by the inverse spin-Hall effect is proportional to the length of Ni$$_{81}$$Fe$$_{19}$$/Pt bilayer films. In contrast, the electric voltage exhibits almost no variation by changing the width of the Ni$$_{81}$$Fe$$_{19}$$/Pt films. These results are consistent with the inverse spin-Hall effect model.

Journal Articles

Quantifying spin mixing conductance in $$F$$/Pt ($$F$$ = Ni, Fe, and Ni$$_{81}$$Fe$$_{19}$$) bilayer film

Yoshino, Tatsuro*; Ando, Kazuya*; Harii, Kazuya*; Nakayama, Hiroyasu*; Kajiwara, Yosuke*; Saito, Eiji

Journal of Physics; Conference Series, 266, p.012115_1 - 012115_4, 2011/01

 Times Cited Count:11 Percentile:97.44(Materials Science, Multidisciplinary)

The spin-mixing conductances in $$F$$/Pt ($$F$$ = Ni, Fe, and Ni$$_{81}$$Fe$$_{19}$$) bilayer films were quantified from the peak-to-peak linewidth of ferromagnetic resonance (FMR) spectra based on the model of the spin pumping. When the Pt layer is attached to the $$F$$ layer, we found the enhancement of the FMR linewidth due to the spin pumping. The experimental results show that the spin-mixing conductances in $$F$$/Pt ($$F$$ = Ni, Fe, and Ni$$_{81}$$Fe$$_{19}$$) bilayer films have the same order of magnitude, showing that spin injection efficiency in the spin pumping is almost identical in these films.

Journal Articles

Design and first experimental results of toroidal field ripple reduction using ferritic insertion in JFT-2M

Sato, Masayasu; Kawashima, Hisato; Miura, Yukitoshi; Tsuzuki, Kazuhiro; Kimura, Haruyuki; Uehara, Kazuya; Ogawa, Toshihide; Isei, Nobuaki; Tani, Takashi; Akiyama, Takashi*; et al.

Fusion Engineering and Design, 51-52(Part.B), p.1071 - 1076, 2000/11

 Times Cited Count:15 Percentile:68.6(Nuclear Science & Technology)

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