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Cs vertical distribution in forest soilsKoarashi, Jun; Atarashi-Andoh, Mariko; Nishimura, Shusaku
Ecotoxicology and Environmental Safety, 262, p.115177_1 - 115177_9, 2023/09
Times Cited Count：0 Percentile：0.01(Environmental Sciences)Predicting the fate of radiocesium (Cs) vertical distribution in Japanese forest soils is key to assessing the radioecological consequences of the Fukushima Daiichi Nuclear Power Plant accident. It is well documented that in mineral soil, the Cs behavior is mostly governed by interaction with clay minerals; however, observations have also been accumulated suggesting the role of soil organic matter (SOM) in enhancing the mobility of Cs. Here, we hypothesized that soil organic carbon (SOC) concentration profile determines the ultimate vertical distribution of Cs in Japanese forest soils. To test this hypothesis, we investigated the detailed vertical distributions of Cs in four Japanese forest soils with varying SOC concentration profiles roughly half a century after global fallout in the early 1960s. Results revealed that Cs retention ratios in each of 2-cm thick soil layers were negatively correlated with SOC concentrations of the layers, across all soils and depths. This demonstrates that the long-term fate of Cs vertical distribution is predictable as a function of SOC concentration for Japanese forest soils.
Nakada, Akira; Kanai, Katsuta; Seya, Natsumi; Nishimura, Shusaku; Futagawa, Kazuo; Nemoto, Masashi; Tobita, Keiji; Yamada, Ryohei*; Uchiyama, Rei; Yamashita, Daichi; et al.
JAEA-Review 2022-078, 164 Pages, 2023/03
JAEA-Review-2022-078.pdf:2.64MB
Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2021 to March 2022. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.
Oishi, Kazuki*; Igarashi, Daisuke*; Tatara, Ryoichi*; Kawamura, Yukihiko*; Hiroi, Kosuke; Suzuki, Junichi*; Umegaki, Izumi*; Nishimura, Shoichiro*; Koda, Akihiro*; Komaba, Shinichi*; et al.
Journal of Physics; Conference Series, 2462, p.012048_1 - 012048_5, 2023/03
Times Cited Count：0 Percentile：0.2(Physics, Applied)Nakada, Akira; Nakano, Masanao; Kanai, Katsuta; Seya, Natsumi; Nishimura, Shusaku; Nemoto, Masashi; Tobita, Keiji; Futagawa, Kazuo; Yamada, Ryohei; Uchiyama, Rei; et al.
JAEA-Review 2021-062, 163 Pages, 2022/02
JAEA-Review-2021-062.pdf:2.87MB
Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2020 to March 2021. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.
Atarashi-Andoh, Mariko; Koarashi, Jun; Tsuzuki, Katsunori; Takeuchi, Erina; Nishimura, Shusaku; Muto, Kotomi*; Matsunaga, Takeshi*
Journal of Environmental Radioactivity, 238-239, p.106725_1 - 106725_8, 2021/11
Times Cited Count：1 Percentile：6.09(Environmental Sciences)To understand the spatial variation in soil Cs inventory in complex mountainous topography, a whole-area investigation of Cs deposition in a broad-leaved forest catchment of a mountain stream was conducted using grid sampling. Across the catchment, organic and surface mineral soil layers were collected at 42 locations in 2013 and 6 locations in 2015. Cs deposition on the forest floor exhibited high spatial heterogeneity and altitude-dependent distribution over the catchment. The Cs retention ratio in the organic layer ranged from 6% to 82% in 2013. The Cs retention ratios had positive correlations with the material inventory in the organic layer and the elevation. The Cs retention ratios in the organic layer were less than 20% in 2015, even at the locations where the retention ratio was higher than 55% in 2013. Although there was spatial variation in the migration speed, Cs migration from the organic layer to mineral soil was almost completed within 4 y of the deposition.
Nishimura, Shoichiro*; Torii, Hiroyuki*; Fukao, Yoshinori*; Ito, Takashi; Iwasaki, Masahiko*; Kanda, Sotaro*; Kawagoe, Kiyotomo*; Kawall, D.*; Kawamura, Naritoshi*; Kurosawa, Noriyuki*; et al.
Physical Review A, 104(2), p.L020801_1 - L020801_6, 2021/08
Times Cited Count：13 Percentile：83.13(Optics)Nakano, Masanao; Fujii, Tomoko; Nemoto, Masashi; Tobita, Keiji; Seya, Natsumi; Nishimura, Shusaku; Hosomi, Kenji; Nagaoka, Mika; Yokoyama, Hiroya; Matsubara, Natsumi; et al.
JAEA-Review 2020-069, 163 Pages, 2021/02
JAEA-Review-2020-069.pdf:4.78MB
Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2019 to March 2020. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.
Oto, Tsutomu; Asano, Norikazu; Kawamata, Takanori; Yanai, Tomohiro; Nishimura, Arashi; Araki, Daisuke; Otsuka, Kaoru; Takabe, Yugo; Otsuka, Noriaki; Kojima, Keidai; et al.
JAEA-Review 2020-018, 66 Pages, 2020/11
JAEA-Review-2020-018.pdf:8.87MB
A collapse event of the cooling tower of secondary cooling system in the JMTR (Japan Materials Testing Reactor) was caused by the strong wind of Typhoon No.15 on September 9, 2019. The cause of the collapse of the cooling tower was investigated and analyzed. As the result, it was identified that four causes occurred in combination. Thus, the soundness of the cooling tower of Utility Cooling Loop (UCL cooling tower), which is a wooden cooling tower installed at the same period as the cooling tower of secondary cooling system, was investigated. The items of soundness survey are to grasp the operation conditions of the UCL cooling tower, to confirm the degradation of structural materials, the inspection items and inspection status of the UCL cooling tower, and to investigate the past meteorological data. As the results of soundness survey of the UCL cooling tower, the improvement of inspection items of the UCL cooling tower was carried out and the replacement and repair of the structural materials of the UCL cooling tower were planned for safe maintenance and management of this facility. And the renewal plan of new cooling tower was created to replace the existing UCL cooling tower. This report is summarized the soundness survey of the UCL cooling tower.
Nakano, Masanao; Hosomi, Kenji; Nishimura, Shusaku; Matsubara, Natsumi; Okura, Takehisa; Kuramochi, Akihiko; Kawasaki, Masatsugu; Takeuchi, Erina; Fujii, Yutaka*; Jinno, Tsukasa*; et al.
Hoken Butsuri (Internet), 55(2), p.102 - 109, 2020/06
After the Fukushima-Daiichi Nuclear Power Station (1F) Accident in March 2011, the increase was significantly observed in a part of the result of the environmental radiation monitoring in Ibaraki prefecture. "The review meeting of the environmental effect from 1F accident" was established to discuss technically the fluctuation of monitoring data. The review meeting collected the monitoring data from the four nuclear operators, and discussed a fluctuating trend, 
Cs/Cs activity ratio, and so on. In this report, the results of the dose rate and Cs in fallout, surface soil, flatfish and seabed sediment are introduced. Also the problem solving in the review meeting is introduced.
Koarashi, Jun; Atarashi-Andoh, Mariko; Nishimura, Shusaku; Muto, Kotomi*
Scientific Reports (Internet), 10(1), p.6614_1 - 6614_11, 2020/04
Times Cited Count：9 Percentile：34.78(Multidisciplinary Sciences)We conducted a pilot-scale decontamination study in a deciduous broadleaved forest in Fukushima. The entire forest, other than two untreated areas, was decontaminated by removing the litter layer approximately 3.3 years after the accident. For three years after decontamination, we quantified Cs contamination levels in the litter and topsoil layers and in the tree leaves, in the untreated and decontaminated areas. The decreased inventories of litter-associated Cs in the decontaminated areas were observed only in the first year after decontamination. Generally, no decontamination effects were observed on the Cs transfer in tree leaves. The primary reason for this was the rapid shift in the main reservoir of Cs from litter layers to the underlying mineral soil, which differs from the observations in post-Chernobyl studies of European forest ecosystems. The results suggest that litter-removal decontamination can only be successful if it is implemented more quickly for Japanese forest ecosystems.
Nakano, Masanao; Fujii, Tomoko; Nemoto, Masashi; Tobita, Keiji; Kono, Takahiko; Hosomi, Kenji; Nishimura, Shusaku; Matsubara, Natsumi; Maehara, Yushi; Narita, Ryosuke; et al.
JAEA-Review 2019-048, 165 Pages, 2020/03
JAEA-Review-2019-048.pdf:2.69MB
Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2018 to March 2019. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.
Nancekievill, M.*; Espinosa, J.*; Watson, S.*; Lennox, B.*; Jones, A.*; Joyce, M. J.*; Katakura, Junichi*; Okumura, Keisuke; Kamada, So*; Kato, Michio*; et al.
Sensors (Internet), 19(20), p.4602_1 - 4602_16, 2019/10
Times Cited Count：7 Percentile：38.52(Chemistry, Analytical)In order to contribute to fuel debris search at the Fukushima Daiichi Nuclear Power Station, we developed a system to search for submerged fuel debris by mounting a sonar on the remotely operated vehicle (ROV). The system can obtain 3D images of submerged fuel debris in real time by using the positioning system, depth sensor, and collected sonar data. As a demonstration test, a simulated fuel debris was installed at the bottom of the water tank facility at the Naraha Center for Remote Control Technology Development, and a 3D image was successfully obtained.
Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.
Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07
Times Cited Count：8 Percentile：56.2(Physics, Multidisciplinary)Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for 
Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.
Cs retention mechanism in surface soils during the early stage after the Fukushima nuclear accidentKoarashi, Jun; Nishimura, Shusaku; Atarashi-Andoh, Mariko; Muto, Kotomi; Matsunaga, Takeshi*
Scientific Reports (Internet), 9, p.7034_1 - 7034_10, 2019/05
Times Cited Count：32 Percentile：79.74(Multidisciplinary Sciences)The aim of the present study is to explore the retention mechanisms of Cs in the surface soil layers of terrestrial ecosystems affected by the Fukushima NPP accident, with a specific focus on the interactions between Cs, soil minerals, and organic matter. Soil samples were collected from field, orchard, and forest sites in July 2011, separated into three soil fractions with different mineral-organic interaction characteristics. The results show that 20-71% of the Cs was retained in association with relatively mineral-free, particulate organic matter-dominant fractions in the orchard and forest surface soil layers. Given the physicochemical and mineralogical properties and the Cs extractability of the soils, Cs incorporation into the complex structure of particulate organic matter is likely the main mechanism for Cs retention in the surface soil layers.
Nakano, Masanao; Fujita, Hiroki; Mizutani, Tomoko; Nemoto, Masashi; Tobita, Keiji; Kono, Takahiko; Hosomi, Kenji; Hokama, Tomonori; Nishimura, Tomohiro; Matsubara, Natsumi; et al.
JAEA-Review 2018-025, 171 Pages, 2019/02
JAEA-Review-2018-025.pdf:3.81MB
Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2016 to March 2017. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Electric Power Company Holdings, Inc. in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and were exceeded the normal range of fluctuation in the monitoring, were evaluated.
Strasser, P.*; Abe, Mitsushi*; Aoki, Masaharu*; Choi, S.*; Fukao, Yoshinori*; Higashi, Yoshitaka*; Higuchi, Takashi*; Iinuma, Hiromi*; Ikedo, Yutaka*; Ishida, Katsuhiko*; et al.
EPJ Web of Conferences, 198, p.00003_1 - 00003_8, 2019/01
Times Cited Count：13 Percentile：99.06(Quantum Science & Technology)Kamada, So*; Kato, Michio*; Nishimura, Kazuya*; Nancekievill, M.*; Watson, S.*; Lennox, B.*; Jones, A.*; Joyce, M. J.*; Okumura, Keisuke; Katakura, Junichi*
Progress in Nuclear Science and Technology (Internet), 6, p.199 - 202, 2019/01
As a technology development to investigate the distribution of submerged fuel debris in the primary containment vessel (PCV) of the Fukushima Daiichi Nuclear Power Station, we are conducting development experiments of sonar system to be mounted in a compact ROV. The experiments were conducted in two types of water tanks with different depths, simulating the PCV, using sonar with different sizes, ultrasonic frequencies, and beam scanning method, and simulated fuel debris. As a result, we characterized the shape discrimination performance of the simulated debris, and the noise due to multi-path in narrow closed space.
Nancekievill, M.*; Jones, A. R.*; Joyce, M. J.*; Lennox, B.*; Watson, S.*; Katakura, Junichi*; Okumura, Keisuke; Kamada, So*; Kato, Michio*; Nishimura, Kazuya*
IEEE Transactions on Nuclear Science, 65(9), p.2565 - 2572, 2018/09
Times Cited Count：25 Percentile：91.9(Engineering, Electrical & Electronic)In order to contribute to the development of technology to search fuel debris submerged in water inside the primary containment vessel of the Fukushima Daiichi Nuclear Power Station, we are developing a remotely operated vehicle (ROV) system equipped with a compact radiation detector and sonar. A cerium bromide (CeBr
) scintillator detector for dose rate monitoring and 
ray spectroscopy was integrated into ROV and experimentally validated with a Cs source, both in the conditions of laboratory and submerged. In addition, the ROV combined with the IMAGENEX 831L sonar could characterize the shape and size of a simulated fuel debris at the bottom of the water pool facility.
Koarashi, Jun; Nishimura, Shusaku; Atarashi-Andoh, Mariko; Matsunaga, Takeshi*; Sato, Tsutomu*; Nagao, Seiya*
Chemosphere, 205, p.147 - 155, 2018/08
Times Cited Count：19 Percentile：57.09(Environmental Sciences)There is little understanding of how soil aggregation can affect the mobility and bioavailability of Cs in soils. To explore this, soil samples were collected at seven sites under different land-use conditions in Fukushima and were separated into four aggregate-size fractions. The fractions were then analyzed for Cs content and extractability and mineral composition. In forest soils, aggregate formation was significant, and Cs was largely associated with large-sized aggregates. In contrast, there was less aggregation in agricultural field soils, and most of Cs was in the clay- and silt-sized fractions. Across all sites, the Cs extractability was higher in the large-sized aggregate fractions than in the clay-sized fractions. The results demonstrate that large-sized aggregates are a significant reservoir of potentially mobile and bioavailable Cs in organic-rich (forest and orchard) soils.
-ray pipe-monitoring capabilities for real-time process monitoring safeguards applications in reprocessing facilitiesRodriguez, D.; Tanigawa, Masafumi; Nishimura, Kazuaki; Mukai, Yasunobu; Nakamura, Hironobu; Kurita, Tsutomu; Takamine, Jun; Suzuki, Satoshi*; Sekine, Megumi; Rossi, F.; et al.
Journal of Nuclear Science and Technology, 55(7), p.792 - 804, 2018/07
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)Nuclear material in reprocessing facilities is safeguarded by random sample verification with additional continuous monitoring applied to solution masses and volume in important tanks to maintain continuity-of-knowledge of process operation. Measuring the unique rays of each solution as the material flows through pipes connecting all tanks and process apparatuses could potentially improve process monitoring by verifying the compositions in real time. We tested this ray pipe-monitoring method using plutonium-nitrate solution transferred between tanks at the PCDF-TRP. The rays were measured using a lanthanum-bromide detector with a list-mode data acquisition system to obtain both time and energy of -ray. The analysis and results of this measurement demonstrate an ability to determine isotopic composition, process timing, flow rate, and volume of solution flowing through pipes, introducing a viable capability for process monitoring safeguards verification.
