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Journal Articles

Status of LBE study and experimental plan at JAEA

Saito, Shigeru; Wan, T.*; Okubo, Nariaki; Obayashi, Hironari; Watanabe, Nao; Ohdaira, Naoya*; Kinoshita, Hidetaka; Yamaki, Kenichi*; Kita, Satoshi*; Yoshimoto, Hidemitsu*; et al.

JPS Conference Proceedings (Internet), 33, p.011041_1 - 011041_6, 2021/03

An Accelerator Driven System (ADS) for waste transmutation investigated in JAEA employs lead-bismuth eutectic (LBE) as a neutron production target material and coolant. The neutrons are to be produced via the spallation with 1.5 GeV proton beam injection. As materials irradiation data are important for ADS development, JAEA plans to construct an irradiation facility with LBE neutron production target in J-PARC. There are many technical issues on LBE for practical use. In JAEA, various R&Ds are being carried out. Concerning corrosion study, conditioning operation and functional tests of OLLOCHI started. Oxygen concentration control technology has also developing. In the large scale LBE loop experiment, the operation for steady state and transient experiments was performed by using IMMORTAL. In the area of instrument, development of ultrasonic flow meter and freeze seal valve are progressing as a key technology for the LBE loop system. Investigation of behavior of impurities in LBE, which is important for design of the irradiation facility, started. In this paper, the status of the LBE studies and experimental plan will be presented.

Journal Articles

Characterization of mechanical strain induced by lead-bismuth eutectic (LBE) freezing in stainless steel cup

Ohdaira, Naoya*; Saito, Shigeru

Heliyon (Internet), 6(2), p.e03429_1 - e03429_8, 2020/02

 Times Cited Count:4 Percentile:40.44(Multidisciplinary Sciences)

Lead-bismuth eutectic (LBE) is a candidate liquid metal coolant for a fast reactor, especially accelerator driven system (ADS). Freeze sealed valve is a candidate design to be possible to add passive safety to the reactor. On the other hand, since LBE is known that it causes expansion after its solidification, quantitative evaluation of the stress to the pipe produced by the LBE expansion should be considered. Many researchers produced related data for the expansion, however, evaluations of the strain by LBE expansion was barely reported. Therefore, the strain measurement using a stainless steel cup and the stress evaluation was performed together with visual observation using an optical microscopy. The results indicated keeping above room temperature (RT) was a significantly effective way to reduce the strain to the pipe.

Journal Articles

The Analytical study of inventories and physicochemical configuration of spallation products produced in Lead-Bismuth Eutectic of Accelerator Driven System

Miyahara, Shinya*; Ohdaira, Naoya*; Arita, Yuji*; Maekawa, Fujio; Matsuda, Hiroki; Sasa, Toshinobu; Meigo, Shinichiro

Nuclear Engineering and Design, 352, p.110192_1 - 110192_8, 2019/10

 Times Cited Count:4 Percentile:49.54(Nuclear Science & Technology)

Lead-Bismuth Eutectic (LBE) is used as a spallation neutron target and coolant materials of Accelerator Driven System (ADS), and many kinds of elements are produced as spallation products. It is important to evaluate the release and transport behavior of the spallation products in the LBE. The inventories and the physicochemical composition of the spallation products produced in LBE have been investigated for an LBE loop in the ADS Target Test Facility (TEF-T) in J-PARC. The inventories of the spallation products in the LBE were estimated using the PHITS code. The physicochemical composition of the spallation products in the LBE was calculated using the Thermo-Calc code under the conditions of the operation temperatures of LBE from 350$$^{circ}$$C to 500$$^{circ}$$C and the oxygen concentrations in LBE from 10 ppb to 1 ppm. The calculation showed that the 5 elements of Rb, Tl, Tc, Os, Ir, Pt, Au and Hg were soluble in LBE under the all given conditions and any kinds of compound were not formed in LBE. It was suggested that the oxides of Ce, Sr, Zr and Y were stable as CeO$$_{2}$$, SrO, ZrO$$_{2}$$ and Y$$_{2}$$O$$_{3}$$ in the LBE.

Oral presentation

The Analytical prediction of inventories and physicochemical composition of spallation products produced in Lead-Bismuth Eutectic of Accelerator Driven System

Miyahara, Shinya*; Arita, Yuji*; Ohdaira, Naoya*; Sasa, Toshinobu; Maekawa, Fujio; Matsuda, Hiroki

no journal, , 

Lead-Bismuth Eutectic (LBE) is used as a spallation neutron target and coolant materials of Accelerator Driven System (ADS), and many kinds of elements are produced as spallation products. It is important to evaluate the release and transport behavior of the spallation products in the LBE. The inventories and the physicochemical composition of the spallation products produced in LBE have been investigated for an LBE loop in the ADS Target Test Facility (TEF-T) in J-PARC. The inventories of the spallation products in the LBE were estimated using the PHITS code. The physicochemical composition of the spallation products in the LBE was calculated using the Thermo-Calc code under the conditions of the operation temperatures of LBE from 350$$^{circ}$$C to 500$$^{circ}$$C and the oxygen concentrations in LBE from 10 ppb to 1 ppm. The calculation showed that the 5 elements of Hg, Tl, Au, Os, Tc were soluble in LBE under the all given conditions and any kinds of compound were not formed in LBE. It was suggested that the oxides of Ce, Zr and Y were stable as CeO$$_{2}$$, ZrO$$_{2}$$ and Y$$_{2}$$O$$_{3}$$ in the LBE.

Oral presentation

Research on physicochemical composition of spallation products in lead-bismuth eutectic in ADS, 1; Estimation of inventories of spallation products

Maekawa, Fujio; Matsuda, Hiroki; Meigo, Shinichiro; Sasa, Toshinobu; Miyahara, Shinya*; Arita, Yuji*; Ohdaira, Naoya*

no journal, , 

To assess physicochemical composition of spallation products in Lead-Bismuth Eutectic (LBE) alloy which was to be used as a spallation neutron target and coolant materials of Accelerator Driven nuclear transmutation Systems (ADS), inventories of spallation products in an LBE loop of J-PARC ADS Target Test Facility (TEF-T) were evaluated.

Oral presentation

Research on physicochemical composition of spallation products in lead-bismuth eutectic in ADS, 2; Thermodynamic study of physicochemical composition of spallation products

Miyahara, Shinya*; Ohdaira, Naoya*; Arita, Yuji*; Sasa, Toshinobu; Maekawa, Fujio; Matsuda, Hiroki; Meigo, Shinichiro

no journal, , 

Representative spallation product elements in a lead-bismuth eutectic (LBE) loop in the ADS Target Test Facility (TEF-T) were selected. Chemical compounds of the elements and their concentrations which can be formed in the LBE were evaluated by one point equilibrium calculation by using the integrated thermodynamic calculation system Thermo-Calc.

Oral presentation

Stress minimization procedure for stainless steel tube produced by phase transition of solidified lead-bismuth eutectic

Ohdaira, Naoya; Saito, Shigeru; Wan, T.; Obayashi, Hironari; Sasa, Toshinobu

no journal, , 

J-PARC plans to install a lead-bismuth eutectic (LBE) spallation target to study the irradiation effects of structural materials in flowing LBE environment. A freeze seal valve is to be used for the LBE circulation system. LBE is known as a material which expands after solidification; hence the solidified LBE in freeze seal part will be deformed and tube in freeze seal part might be broken by the imposed stress consequently. To minimize the stress at freeze seal valve, deformation of stainless steel (SS) generated by LBE expansion in different cooling conditions were studied. It was found that annealing at a certain temperature for 24 hours is effective to reduce the stress.

Oral presentation

J-PARC LBE spallation target for ADS development

Sasa, Toshinobu; Saito, Shigeru; Obayashi, Hironari; Ariyoshi, Gen; Wan, T.*; Okubo, Nariaki; Ohdaira, Naoya*; Yamaki, Kenichi*; Kita, Satoshi*; Yoshimoto, Hidemitsu*

no journal, , 

Japan Atomic Energy Agency (JAEA) proposes to reduce the minor actinides by Partitioning and Transmutation Technology using Accelerator-driven system (ADS). To realize ADS, JAEA plans to locate Lead-Bismuth Eutectic alloy (LBE) spallation target in J-PARC. LBE spallation target will be used to solve technical issues for ADS design by preparing irradiation database. The 400 MeV - 250 kW proton beam can be used for ADS studies. The spallation target is optimized by thermal-hydraulic analysis and structural analysis to increase proton/neutron irradiation of ADS materials by sharply focused proton beam injection. The studies for elemental technologies such as a fully-remote target exchange procedure and freeze-sealed drain valve system are also performed and integrated into the design of LBE target. The latest design of the J-PARC LBE spallation target system will be presented.

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