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Osawa, Takahito
Kenkyu Kaihatsu Reda, 20(8), p.7 - 11, 2023/11
This review outlines technical methodologies for automating labor-intensive experiments, especially wet separation experiments.
Matsuoka, Moe*; Kagawa, Eiichi*; Amano, Kana*; Nakamura, Tomoki*; Tatsumi, Eri*; Osawa, Takahito; 51 of others*
Communications Earth & Environment (Internet), 4, p.335_1 - 335_12, 2023/09
Times Cited Count：3 Percentile：79.18(Environmental Sciences)Visible and near-infrared (Vis-NIR) spectra of returned samples from Cb-type asteroid (162173) Ryugu exhibit very low reflectance values and absorptions that are generally consistent with observations from the Hayabusa2 ONC-T and NIRS3 instruments. A notable difference is that a metal-OH absorption at 2.72 misrometer is more than twice as deep in laboratory sample spectra compared with those of Ryugu's surface. Based on the laboratory experiments to investigate the range of spectral variation by physical properties and space weathering, we conclude that the spectral differences between returned samples and asteroid surface are best explained by a combination of (1) porosity, (2) particle size, and (3) degree of space weathering effects, with the latter being the most effective. Those effects can explain spectral variations between Cb-type asteroids, suggesting that these asteroids consist of the same CI-chondrite material with different physical properties and weathering degrees. Extremely homogeneous Vis-NIR spectra of the entire Ryugu surface in comparison with the heterogeneous spectra of a near-Earth S-type asteroid (25143) Itokawa indicate that the space weathering has been processing more rapidly on Cb-type asteroids compared with S-type asteroids. Because the major component of Cb-type asteroids are porous hydrous silicates that have lower melting temperature and lower material strength than anhydrous silicates, the surface of Cb-type asteroids are more susceptible to the alteration by impacts of interplanetary dust particles.
Chiu, I.-H. ; Terada, Kentaro*; Osawa, Takahito; Park, C.*; Takeshita, Soshi*; Miyake, Yasuhiro*; Ninomiya, Kazuhiko*
Meteoritics & Planetary Science, 58(9), p.1333 - 1344, 2023/09
Times Cited Count：0 Percentile：0.01(Geochemistry & Geophysics)Osawa, Takahito
Shiki, 59, p.4 - 7, 2023/06
Elemental analysis using negative muons has made remarkable progress as a result of the research and development for the application of muons to the analysis of samples brought back to earth by the Hayabusa-2. This paper describes the analysis of Ryugu samples at J-PARC, from the development of the instrument to the analysis results.
Osawa, Takahito
Keisoku Gijutsu, 51(6), p.21 - 26, 2023/05
Decompression filtration is a common operation in wet chemistry, and the method using a filtration bell is often used. The author has been developing a fully automated system for wet separation operations, and has developed an automatic decompression filtration device exclusively for robots. In addition, the specifications of this device were changed so that it can be operated by human operators, and it was commercialized.
Osawa, Takahito; Nagasawa, Shunsaku*; Ninomiya, Kazuhiko*; Takahashi, Tadayuki*; Nakamura, Tomoki*; Wada, Taiga*; Taniguchi, Akihiro*; Umegaki, Izumi*; Kubo, Kenya*; Terada, Kentaro*; et al.
ACS Earth and Space Chemistry (Internet), 7(4), p.699 - 711, 2023/04
Times Cited Count：4 Percentile：93.95(Chemistry, Multidisciplinary)The concentrations of carbon and other major elements in asteroid samples provide very important information on the birth of life on the Earth and the solar-system evolution. Elemental analysis using muonic X-rays is one of the best analytical methods to determine the elemental composition of solid materials, and notably, is the only method to determine the concentration of light elements in bulk samples in a non-destructive manner. We developed a new analysis system using muonic X-rays to measure the concentrations of carbon and other major elements in precious and expectedly tiny samples recovered from the asteroid Ryugu by spacecraft Hayabusa2. Here we report the development process of the system in 4 stages and their system configurations, The analysis system is composed of a stainless-steel analysis chamber, an acrylic glove box for manipulating asteroid samples in a clean environment, and Ge semiconductor detectors arranged to surround the analysis chamber. The performance of the analysis system, including the background level, which is crucial for the measurement, was greatly improved from the first stage to the later ones. Our feasibility study showed that the latest model of our muonic X-ray analysis system is capable of determining the carbon concentration in Hayabusa2's sample model with an uncertainty of less than 10 percent in a 6-day measurement.
Osawa, Takahito
Hoshaka Bunseki, (34), p.34 - 50, 2023/04
This paper describes the nomenclature, principles, advantages and disadvantages of prompt gamma-ray analysis, the configuration of the PGA installed in JRR-3, what kind of analysis can be performed with the PGA, and how to use the PGA, respectively.
Chiu, I.-H. ; Terada, Kentaro*; Osawa, Takahito; Park, C.*; Takeshita, Soshi*; Miyake, Yasuhiro*; Ninomiya, Kazuhiko*
Journal of Physics; Conference Series, 2462, p.012004_1 - 012004_6, 2023/03
Times Cited Count：0 Percentile：0.2(Physics, Applied)In the last decade, non-destructive elemental analysis using negative muon beams advanced significantly. This method can be used to determine the elemental composition of bulk materials without causing damage. In this study, we performed a negative muon irradiation experiment for a Northwest Africa 482 lunar meteorite (NWA482), which was installed in a stainless steel analysis chamber. The analysis chamber was filled with helium gas to suppress the background signals caused by air-scattering muons. The muonic X-rays from Al, Fe, Ca, Mg, Si, and O in the samples were detected using six high-purity germanium semiconductor detectors arranged around the analysis chamber. To correct the X-ray self-absorption effect of the samples, a Monte-Carlo simulation using Geant4 toolkit was used. Based on the quantitative analysis for muonic X-ray measurement with the correction application from the simulation, we successfully investigated the analytical sensitivity of each element in meteorites based on the NWA482 data.
Nakamura, Tomoki*; Osawa, Takahito; 219 of others*
Science, 379(6634), p.eabn8671_1 - eabn8671_14, 2023/02
Times Cited Count：98 Percentile：99.99(Multidisciplinary Sciences)Mineralogical, petrological, and physical properties of sixteen Ryugu particles measuring 1-8 mm indicate that they are most similar to CI chondrites. The presence of CO
-bearing water in pyrrhotite indicates that the original parent asteroid formed beyond the HO and CO snow lines in the solar nebula, where, based on Ryugu mineralogy, very limited amounts of high-temperature objects including small chondrules and Ca, Al-rich inclusions were present. Fluid-rock reactions occurred at low-temperature, high pH, and reducing conditions at water/rock mass ratios smaller than 1 and changed an olivine-pyroxene rich lithology, remaining as the least-altered fragments in Ryugu samples, into phyllosilicate-carbonate rich lithologies, the predominant material of Ryugu samples. The solar nebula might have been still present when magnetite crystallized from the fluid in Ryugu's parent body.
Kobayashi, Takane*; Onishi, Tsuyoshi*; Osawa, Takahito; Pratt, A.*; Tear, S.*; Shimoda, Susumu*; Baba, Hidetada*; Laitinen, M.*; Sajavaara, T.*
Small, 18(46), p.2204455_1 - 2204455_9, 2022/11
Times Cited Count：2 Percentile：34.67(Chemistry, Multidisciplinary)An all-solid-state battery is a secondary battery that is charged and discharged by the transport of lithium ions between positive and negative electrodes. To fully realize the significant benefits of this battery technology, for example, higher energy densities, faster charging times, safer operation, it will be essential to understand how lithium ions are transported and distributed in the battery during operation. However, as the third lightest element, methods for quantitatively analyzing lithium during operation of an all-solid-state device are limited such that real time tracking of lithium transport has not yet been demonstrated. Here, we report that the transport of lithium ions in an all-solid-state half-cell was quantitatively tracked in near real time by utilizing a thermal neutron-induced nuclear reaction, utilizing lithium-6 as a tracer, and utilizing a high-intensity thermal neutron source. Furthermore, it is also mentioned that the migration mechanism and migration region of lithium ions in the solid electrolyte used could be determined by tracking the transport of lithium ions. From these results, it can be said that the development of all-solid-state batteries has entered a phase where further advances could be carried out while understanding the transport of lithium ions in the batteries. As a result, the research and development of all-solid-state batteries would be further accelerated.
Barucci, M. A.*; Reess, J.-M.*; Bernardi, P.*; Doressoundiram, A.*; Fornasier, S.*; Le Du, M.*; Iwata, Takahiro*; Nakagawa, Hiromu*; Nakamura, Tomoki*; Andr
, Y.*; et al.
Earth, Planets and Space (Internet), 73(1), p.211_1 - 211_28, 2021/12
Times Cited Count：13 Percentile：80.63(Geosciences, Multidisciplinary)The MMX InfraRed Spectrometer (MIRS) is an imaging spectrometer on board of MMX JAXA mission. MIRS is built at LESIA-Paris Observatory in collaboration with four other French laboratories, collaboration and financial support of CNES and close collaboration with JAXA and MELCO. The instrument is designed to fully accomplish MMX's scientific and measurement objectives. MIRS will remotely provide near-infrared spectral maps of Phobos and Deimos containing compositional diagnostic spectral features that will be used to analyze the surface composition and to support the sampling site selection. MIRS will also study Mars atmosphere, in particular to spatial and temporal changes such as clouds, dust and water vapor.
Osawa, Takahito
Hamon, 31(3), p.117 - 120, 2021/08
Muonic X-ray analysis is an elemental analysis method by detecting characteristic X-rays emitted from muonic atoms and has various advantages, for example, it can detect light elements such as carbon non-destructively. Our research group has been studying to apply this new analytical method to the sample of the asteroid Ryugu brought back by the asteroid explorer Hayabusa2. This paper outlines the research conducted at J-PARC muon facility so far and the preparation status of the experiment on Ryugu samples scheduled to be conducted from June to July 2021. To make this experiment successful, a device with a glove box has been developed that can analyze microsamples in a helium atmosphere, achieving very low background levels.
Okumura, Takuma*; Azuma, Toshiyuki*; Bennet, D. A.*; Caradonna, P.*; Chiu, I.-H.*; Doriese, W. B.*; Durkin, M. S.*; Fowler, J. W.*; Gard, J. D.*; Hashimoto, Tadashi; et al.
IEEE Transactions on Applied Superconductivity, 31(5), p.2101704_1 - 2101704_4, 2021/08
Times Cited Count：1 Percentile：11.15(Engineering, Electrical & Electronic)A superconducting transition-edge sensor (TES) microcalorimeter is an ideal X-ray detector for experiments at accelerator facilities because of good energy resolution and high efficiency. To study the performance of the TES detector with a high-intensity pulsed charged-particle beam, we measured X-ray spectra with a pulsed muon beam at the Japan Proton Accelerator Research Complex (J-PARC) in Japan. We found substantial temporal shifts of the X-ray energy correlated with the arrival time of the pulsed muon beam, which was reasonably explained by pulse pileup due to the incidence of energetic particles from the initial pulsed beam.
X raysOkumura, Takuma*; Azuma, Toshiyuki*; Bennet, D. A.*; Caradonna, P.*; Chiu, I. H.*; Doriese, W. B.*; Durkin, M. S.*; Fowler, J. W.*; Gard, J. D.*; Hashimoto, Tadashi; et al.
Physical Review Letters, 127(5), p.053001_1 - 053001_7, 2021/07
Times Cited Count：13 Percentile：79.44(Physics, Multidisciplinary)We observed electronic X rays emitted from muonic iron atoms using a superconducting transition-edge-type sensor microcalorimeter. The energy resolution of 5.2 eV in FWHM allowed us to observe the asymmetric broad profile of the electronic characteristic 
and 
X rays together with the hypersatellite X rays around 6 keV. This signature reflects the time-dependent screening of the nuclear charge by the negative muon and the 
-shell electrons, accompanied by electron side-feeding. Assisted by a simulation, this data clearly reveals the electronic - and -shell hole production and their temporal evolution during the muon cascade process.
Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.
Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03
Times Cited Count：43 Percentile：96.93(Astronomy & Astrophysics)Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 
C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.
Osawa, Takahito
Hamon, 31(1), p.7 - 8, 2021/02
Prompt Gamma-ray activation Analysis system (PGA) installed in JRR-3 is explained.
Maruoka, Teruyuki*; Nishio, Yoshiro*; Kogiso, Tetsu*; Suzuki, Katsuhiko*; Osawa, Takahito; Hatsukawa, Yuichi*; Terada, Yasuko*
GSA Bulletin, 132(9-10), p.2055 - 2066, 2020/09
Times Cited Count：2 Percentile：13.16(Geosciences, Multidisciplinary)Osawa, Takahito
Kodomo To Hatsuiku Hattatsu, 17(4), p.245 - 251, 2020/01
no abstracts in English
Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Arai, Takehiko*; Nakauchi, Yusuke*; Nakamura, Tomoki*; Matsuoka, Moe*; et al.
Science, 364(6437), p.272 - 275, 2019/04
Times Cited Count：259 Percentile：99.73(Multidisciplinary Sciences)The near-Earth asteroid 162173 Ryugu, the target of Hayabusa2 sample return mission, is believed to be a primitive carbonaceous object. The Near Infrared Spectrometer (NIRS3) on Hayabusa2 acquired reflectance spectra of Ryugu's surface to provide direct measurements of the surface composition and geological context for the returned samples. A weak, narrow absorption feature centered at 2.72 micron was detected across the entire observed surface, indicating that hydroxyl (OH)-bearing minerals are ubiquitous there. The intensity of the OH feature and low albedo are similar to thermally- and/or shock-metamorphosed carbonaceous chondrite meteorites. There are few variations in the OH-band position, consistent with Ryugu being a compositionally homogeneous rubble-pile object generated from impact fragments of an undifferentiated aqueously altered parent body.
-ray analysis for volcanic rocks by JRR-3 reactorOsawa, Takahito; Fukuoka, Takaaki*
Gekkan Chikyu, 40(5), p.302 - 309, 2018/05
Contents of boron, chlorine, hydrogen, and water in volcanic rocks provide important information of magma origin. Here we describe the measurement for boron in volcanic rocks using the automatic prompt -ray analysis system installed in Japan research reactor-3 (JRR-3) at Japan atomic Energy Agency.
