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Journal Articles

Study on the free corrosion potential at an interface between an Al electrode and an acidic aqueous NaCl solution through density functional theory combined with the reference interaction site model

Kano, Koichi*; Hagiwara, Satoshi*; Igarashi, Takahiro; Otani, Minoru*

Electrochimica Acta, 377, p.138121_1 - 138121_10, 2021/05

AA2020-0599.pdf:0.95MB

 Times Cited Count:14 Percentile:70.49(Electrochemistry)

We investigated the free corrosion potential at an interface between an Al electrode and an aqueous NaCl solution under acidic conditions via density functional theory combined with the effective screening medium and reference interaction site model (ESM-RISM). The electrode potentials for the anodic and cathodic corrosion reactions were obtained from the grand potential profile as a function of the electron chemical potential at the interface. Thereafter, we determined the free corrosion potential using the Tafel extrapolation method. The results of the free corrosion potential were consistent with previous experimental data. By controlling the pH, we determined the pH dependence of the free corrosion potential, and the results agreed well with the experimental results. Our results indicated that the ESM-RISM method duly described the environmental effect of an acidic solution and precisely determined the free corrosion potential.

Journal Articles

Establishment of a Laboratory for $$gamma$$-ray Spectrometry of Environmental Samples Collected in Fukushima

Saegusa, Jun; Yoda, Tomoyuki; Maeda, Satoshi; Okazaki, Tsutomu; Otani, Shuichi; Yamaguchi, Toshio; Kurita, Yoshiyuki; Hasumi, Atsushi; Yonezawa, Chushiro*; Takeishi, Minoru

Proceedings of 14th International Congress of the International Radiation Protection Association (IRPA-14), Vol.3 (Internet), p.1078 - 1085, 2017/11

After the nuclear accident at the Fukushima Daiichi Nuclear Power Plant in March 2011, the Japan Atomic Energy Agency has newly set up a laboratory for radioactivity analysis in Fukushima. At the laboratory, radioactivity concentrations of environmental samples such as soil, water, dust filter, plant, etc., approximately 1,000 samples in a month, are measured with high-resolution $$gamma$$-ray spectrometry systems. The systems employ n-type HPGe detectors from Ortec. Since September 2012, characterization and upgrade of the systems have been performed aimed at enhancing reliability of analysis and convenience of customers. Resolving both systematic and technical issues, the laboratory has been accredited the ISO/IEC 17025 standard as a testing laboratory for radioactivity analysis.

JAEA Reports

Annual report on the effluent control of low level liquid waste in Nuclear Fuel Cycle Engineering Laboratories FY2008

Takeishi, Minoru; Matsuura, Kenichi; Watanabe, Hitoshi; Nakano, Masanao; Kono, Takahiko; Hiyama, Yoshinori; Fujii, Jun*; Kikuchi, Masaaki*; Sagawa, Fumiaki*; Otani, Kazunori*

JAEA-Review 2009-039, 131 Pages, 2009/12

JAEA-Review-2009-039.pdf:15.22MB

Based on the regulations (the safety regulation of Tokai reprocessing plant, the safety regulation of nuclear fuel material usage facilities, the radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear regulatory acts, and the local agreement concerning with safety and environment conservation around nuclear facilities, the water pollution control law, and byelaw of Ibaraki prefecture), this report describes the effluent control results of liquid waste discharged from the JAEA's Nuclear Fuel Cycle Engineering Laboratories in the fiscal year 2008, from 1st April 2008 to 31st March 2009. In this period, the concentrations and the quantities of the radioactive liquid waste discharged from the reprocessing plant, the plutonium fuel fabrication facilities, and the other facilities were much lower than the authorized limits of the above regulations.

JAEA Reports

Annual report on the effluent control of low level liquid waste in Nuclear Fuel Cycle Engineering Laboratories FY2007

Takeishi, Minoru; Matsuura, Kenichi; Watanabe, Hitoshi; Nakano, Masanao; Kono, Takahiko; Hiyama, Yoshinori; Fujii, Jun*; Kikuchi, Masaaki*; Sagawa, Fumiaki*; Otani, Kazunori*

JAEA-Review 2008-060, 131 Pages, 2008/12

JAEA-Review-2008-060.pdf:13.33MB

Based on the regulations (the safety regulation of Tokai reprocessing plant, the safety regulation of nuclear fuel material usage facilities, radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear regulatory acts, and the local agreement concerning with safety and environment conservation around nuclear facilities, the water pollution control law, and byelaw of Ibaraki prefecture), this report describes the effluent control results of liquid waste discharged from the JAEA's Nuclear Fuel Cycle Engineering Laboratories in the fiscal year 2007, from 1st April 2007 to 31st March 2008. In this period, the concentrations and the quantities of the radioactive materials discharged from the reprocessing plant, the plutonium fuel fabrication facilities, and the other facilities were much lower than the authorized limits of the above regulations.

JAEA Reports

Annual report on the effluent control of low level liquid waste in Nuclear Fuel Cycle Engineering Laboratories FY2006

Takeishi, Minoru; Miyagawa, Naoto; Nakano, Masanao; Mizutani, Tomoko; Kono, Takahiko; Hiyama, Yoshinori*; Fujii, Jun*; Kikuchi, Masaaki*; Sagawa, Fumiaki*; Otani, Kazunori*

JAEA-Review 2007-041, 130 Pages, 2007/12

JAEA-Review-2007-041.pdf:25.46MB

Based on the regulations (the safety regulation of Tokai reprocessing plant, the safety regulation of nuclear fuel material usage facilities, radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear reguratory acts, and the local agreement concerning with security and environment conservation around nuclear facilities, the water pollution control law, and byelaw of Ibaraki prefecture), this report describes the effluent control results of low level liquid waste discharged from the JAEA's Nuclear Fuel Cycle Engineering Laboratories in the fiscal year 2006, from 1st April 2006 to 31st March 2007. In this period, the concentrations and the quantities of the discharged radioactive materials from the reprocessing plant, the plutonium fuel fabrication facilities, and the other facilities were much lower than the authorized limits of the above regulations.

JAEA Reports

Annual report on the effluent control of low level liquid waste in Nuclear Fuel Cycle Engineering Laboratories FY2005

Takeishi, Minoru; Miyagawa, Naoto; Uezu, Yasuhiro; Nakano, Masanao; Koarashi, Jun; Mizutani, Tomoko; Kono, Takahiko; Hiyama, Yoshinori*; Fujii, Yoshiyuki*; Kikuchi, Masaaki*; et al.

JAEA-Review 2006-024, 133 Pages, 2006/09

JAEA-Review-2006-024.pdf:6.69MB

Based on the regulations (the safety regulation of Tokai reprocessing plant, the safety regulation of nuclear fuel usage facilities, radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear reguratory acts, and the local agreement concerning with security and environment conservation around nuclear facilities, the water pollution control law, and byelaw of Ibaraki prefecture), this report describes the effluent control results of low level liquid waste discharged from the JAEA's Nuclear Fuel Cycle Engineering Laboratories in the fiscal year 2005, from 1st April 2005 to 31th March 2006. In this period, the concentrations and the quantities of the discharged radioactive materials from the reprocessing plant, the plutonium fuel fabrication facilities, and the other facilities were much lower than the authorized limits of the above regulations.

JAEA Reports

Stress and strain evaluation of the heat transfer tubes in the intermediate heat exchanger for the HTTR

Kunitomi, Kazuhiko; Shinozaki, Masayuki; ; Okubo, Minoru; Baba, Osamu; *; Otani, Akihito*

JAERI-M 92-147, 77 Pages, 1992/10

JAERI-M-92-147.pdf:1.77MB

no abstracts in English

Oral presentation

Multidimensional evaluation of FR cycle systems in the Phase-II of the feasibility study, 3; Methodology for weighting and results of the multidimensional evaluation

Kawasaki, Hirotsugu; Shiotani, Hiroki; Ono, Kiyoshi; Sonoyama, Minoru*; Suzuki, Atsushi*

no journal, , 

no abstracts in English

Oral presentation

Outline of Sasakino Analytical Laboratory, Fukushima Environmental Safety Center of JAEA

Saegusa, Jun; Yanagisawa, Kayo; Yamaguchi, Toshio; Manabe, Sachi; Yoda, Tomoyuki; Maeda, Satoshi; Utsumi, Azusa; Shibamichi, Masaru; Ejiri, Akira; Kurita, Yoshiyuki; et al.

no journal, , 

no abstracts in English

Oral presentation

Development of isothermal gas chromatography for volatility study of the seaborgium oxychloride

Otani, Ryo; Sato, Tetsuya; Aoki, Ryota*; Shirai, Kaori*; Suzuki, Hayato; Tsukada, Kazuaki; Asai, Masato; Ito, Yuta; Nagame, Yuichiro*; Sakama, Minoru*

no journal, , 

The adsorption enthalpy of the Sg dioxydichloride on a quartz surface ($$Delta H_{rm ads}$$(SgO$$_2$$Cl$$_2$$)) has been reported to be -98 kJ/mol. The result, however, is still ambiguous because the value was evaluated based on a few experimental points with large statistics errors. To obtain a reliable $$Delta H_{rm ads}$$(SgO$$_2$$Cl$$_2$$)) for a discussion of an influence of relativistic effects, a stable gas chemistry apparatus with good reproducibility is mandatory. In this study, we have conducted offline experiments of an isothermal gas chromatography) with short-lived Mo isotopes originated from a $$^{252}$$Cf fission source. We searched for experimental parameters for an on-line experiment. At the presentation, we will present the obtained optimum conditions for gas chromatographic separation of group-6 elements and determined $$Delta H_{rm ads}$$(MoO$$_2$$Cl$$_2$$)).

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