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Journal Articles

Preliminary study of the criticality monitoring method based on the simulation for the activity ratio of short half-life noble-gas fission products from fuel debris

Riyana, E. S.; Okumura, Keisuke; Sakamoto, Masahiro; Matsumura, Taichi; Terashima, Kenichi; Kanno, Ikuo

Journal of Nuclear Science and Technology, 8 Pages, 2024/00

 Times Cited Count:0 Percentile:0.18(Nuclear Science & Technology)

Journal Articles

Alloy design and characterization of a recrystallized FeCrAl-ODS cladding for accident-tolerant BWR fuels; An Overview of research activity in Japan

Ukai, Shigeharu; Sakamoto, Kan*; Otsuka, Satoshi; Yamashita, Shinichiro; Kimura, Akihiko*

Journal of Nuclear Materials, 583, p.154508_1 - 154508_24, 2023/09

 Times Cited Count:5 Percentile:94.3(Materials Science, Multidisciplinary)

Journal Articles

Development of an iron(II) complex exhibiting thermal- and photoinduced double proton-transfer-coupled spin transition in a short hydrogen bond

Nakanishi, Takumi*; Hori, Yuta*; Shigeta, Yasuteru*; Sato, Hiroyasu*; Kiyanagi, Ryoji; Munakata, Koji*; Ohara, Takashi; Okazawa, Atsushi*; Shimada, Rintaro*; Sakamoto, Akira*; et al.

Journal of the American Chemical Society, 145(35), p.19177 - 19181, 2023/08

 Times Cited Count:0 Percentile:0(Chemistry, Multidisciplinary)

Journal Articles

Modelling heterogeneous hydration behaviour of bentonite by a FracMan-Thames coupling method for the Bentonite Rock Interaction Experiment (BRIE) at $"{A}$sp$"{o}$ HRL

Sawada, Atsushi; Sakamoto, Kazuhiko*; Watahiki, Takanori*; Imai, Hisashi*

SKB P-17-06, 154 Pages, 2023/08

Journal Articles

Thinning behavior of solid boron carbide immersed in molten stainless steel for core disruptive accident of sodium-cooled fast reactor

Emura, Yuki; Takai, Toshihide; Kikuchi, Shin; Kamiyama, Kenji; Yamano, Hidemasa; Yokoyama, Hiroki*; Sakamoto, Kan*

Journal of Nuclear Science and Technology, 10 Pages, 2023/00

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

Journal Articles

${it Operando}$ structure observation of pyroelectric ceramics during power generation cycle

Kawasaki, Takuro; Fukuda, Tatsuo; Yamanaka, Satoru*; Sakamoto, Tomokazu*; Murayama, Ichiro*; Kato, Takanori*; Baba, Masaaki*; Hashimoto, Hideki*; Harjo, S.; Aizawa, Kazuya; et al.

Journal of Applied Physics, 131(13), p.134103_1 - 134103_7, 2022/04

 Times Cited Count:1 Percentile:17.38(Physics, Applied)

Journal Articles

Study on eutectic melting behavior of control rod materials in core disruptive accidents of sodium-cooled fast reactors, 2; Kinetic study on eutectic reaction process between stainless steel with low boron carbide concentration and stainless steel

Kikuchi, Shin; Takai, Toshihide; Yamano, Hidemasa; Sakamoto, Kan*

Proceedings of 28th International Conference on Nuclear Engineering (ICONE 28) (Internet), 9 Pages, 2021/08

In a postulated severe accidental condition of sodium-cooled fast reactor (SFR), eutectic melting between boron carbide (B$$_{4}$$C) and stainless steel (SS) may occur. Thus, behavior of B$$_{4}$$C-SS eutectic melting is one of the phenomena to evaluate the core disruptive accidents in SFR. In this study, the reaction experiments using SS crucibles and the pellets of SS with low B$$_{4}$$C concentration as samples were performed to simulate the state of the reaction interface in which the eutectic reaction and interdiffusion of B$$_{4}$$C-SS have progressed to a certain extent. It was revealed that the rate constants of eutectic reaction between SS and SS with low B$$_{4}$$C concentration are smaller than that of B$$_{4}$$C-SS eutectic reaction at high temperatures.

Journal Articles

Orientation dependence of yield strength in a new single crystal-like FeCrAl oxide dispersion strengthened alloy

Aghamiri, S. M. S.*; Sugawara, Naoya*; Ukai, Shigeharu; Ono, Naoko*; Sakamoto, Kan*; Yamashita, Shinichiro

Materials Characterization, 176, p.111043_1 - 111043_6, 2021/06

Advanced oxidation-resistant FeCrAl ODS alloys were developed via the control of composition-processing conditions for the accident tolerant fuel (ATF) cladding. For the first time, a single-crystal like recrystallized FeCrAl ODS alloy was achieved with a unique crystallographic texture of 110-plane and 211-direction and a high number density of fine nanoscale oxide particles. Evaluation of yield strengths at different temperatures showed higher values in transverse (T) direction than longitudinal (L) direction. The crystal orientation dependence of the yield strength up to 800$$^{circ}$$C was attributed to lower value of Schmid factor in transverse direction. Accordingly, the critical resolved shear stress of this practical class of advanced materials was calculated in various temperatures.

Journal Articles

Kinetic study on eutectic melting process between boron carbide and stainless steel in sodium-cooled fast reactor

Kikuchi, Shin; Sakamoto, Kan*; Takai, Toshihide; Yamano, Hidemasa

Nihon Kikai Gakkai 2020-Nendo Nenji Taikai Koen Rombunshu (Internet), 4 Pages, 2020/09

In a postulated severe accidental condition of sodium-cooled fast reactor (SFR), eutectic melting between boron carbide (B$$_{4}$$C) as control rod element and stainless steel (SS) as control rod cladding or related structure may occur. Thus, behavior of B$$_{4}$$C-SS eutectic melting is one of the phenomena to evaluate the core disruptive accidents in SFR. In order to clarify the kinetic feature of B$$_{4}$$C-SS eutectic melting process in the interface, the thinning test for SS crucibles using the pellets of B$$_{4}$$C or SS with low B$$_{4}$$C concentration were performed to obtain the rate constant with dependence of B$$_{4}$$C concentration against SS. It was found that the rate constants of eutectic melting between SS and SS low B$$_{4}$$C concentration were smaller than that of B$$_{4}$$C-SS in the high temperature range. Besides, the rate constant of eutectic melting between SS and B$$_{4}$$C containing SS became small when decreasing the B$$_{4}$$C concentration against SS.

Journal Articles

Pyroelectric power generation from the waste heat of automotive exhaust gas

Kim, J.*; Yamanaka, Satoru*; Murayama, Ichiro*; Kato, Takanori*; Sakamoto, Tomokazu*; Kawasaki, Takuro; Fukuda, Tatsuo; Sekino, Toru*; Nakayama, Tadachika*; Takeda, Masatoshi*; et al.

Sustainable Energy & Fuels (Internet), 4(3), p.1143 - 1149, 2020/03

 Times Cited Count:16 Percentile:64.8(Chemistry, Physical)

Journal Articles

Microstructure and texture evolution and ring-tensile properties of recrystallized FeCrAl ODS cladding tubes

Aghamiri, S. M. S.*; Sowa, Takashi*; Ukai, Shigeharu*; Ono, Naoko*; Sakamoto, Kan*; Yamashita, Shinichiro

Materials Science & Engineering A, 771, p.138636_1 - 138636_12, 2020/01

 Times Cited Count:32 Percentile:90.98(Nanoscience & Nanotechnology)

Oxide dispersion strengthened (ODS) FeCrAl ferritic steels are being developed as potential accident tolerance fuel cladding materials for the light water reactors (LWRs) due to significant improvement in steam oxidation by alumina forming scale and good mechanical properties up to high temperatures. In this study, the microstructural characteristics and tensile properties of the two FeCrAl ODS cladding tubes with different extrusion temperatures of 1100$$^{circ}$$C and 1150$$^{circ}$$C were investigated during processing conditions. While the hot extruded sample showed micron sized elongated grains with strong $$alpha$$-fiber in $$<$$110$$>$$ texture, cold pilger rolling process change the microstructure to submicron/micron size grain structure along with texture evolution to both $$alpha$$-fiber ($$<$$110$$>$$ texture) and $$gamma$$-fiber ({111} texture) via crystalline rotations. Subsequently, final annealing resulted in evolution of microstructure to large grain recrystallized structure starting at recrystallization temperature of $$sim$$810-850$$^{circ}$$C. Two distinct texture development happened in recrystallized cladding tubes, i.e., only large elongated grains of (110) $$<$$211$$>$$ texture following extrusion temperature of 1100$$^{circ}$$C; and two texture components of (110) $$<$$211$$>$$ and {111} $$<$$112$$>$$ following higher extrusion temperature of 1150$$^{circ}$$C. The different texture development and retarding of recrystallization progress in 1100$$^{circ}$$C-extruded cladding tubes were attributed to higher distribution of oxide particles.

Journal Articles

Development of a structured overset Navier-Stokes solver with a moving grid and full multigrid method

Ohashi, Kunihide*; Hino, Takanori*; Kobayashi, Hiroshi*; Onodera, Naoyuki; Sakamoto, Nobuaki*

Journal of Marine Science and Technology, 24(3), p.884 - 901, 2019/09

 Times Cited Count:16 Percentile:76.61(Engineering, Marine)

An unsteady Reynolds averaged Navier-Stokes solver with a structured overset grid method has been developed. Velocity pressure coupling is achieved using an artificial compressibility approach, spatial discretization is based on a FVM. Body motions are considered using the grid deformation technique and grid velocities in the convective term. The full multigrid (FMG) method is applied to obtain fast convergence. The cell flag on a coarse grid level is determined using the cell flag on a fine grid level. In the coarse and fine grid level calculations at the FMG stage, the data are interpolated until the finest grid level is achieved at an overset update interval. Then, the data are updated based on the overset relations at the finest grid level and then transferred to a coarser grid level. The computations for flows around a hull form, including an unsteady simulation with regular waves, are demonstrated.

Journal Articles

Overview of accident-tolerant fuel R&D program in Japan

Yamashita, Shinichiro; Ioka, Ikuo; Nemoto, Yoshiyuki; Kawanishi, Tomohiro; Kurata, Masaki; Kaji, Yoshiyuki; Fukahori, Tokio; Nozawa, Takashi*; Sato, Daiki*; Murakami, Nozomu*; et al.

Proceedings of International Nuclear Fuel Cycle Conference / Light Water Reactor Fuel Performance Conference (Global/Top Fuel 2019) (USB Flash Drive), p.206 - 216, 2019/09

After the nuclear accident at Fukushima Daiichi Power Plant, research and development (R&D) program for establishing technical basis of accident-tolerant fuel (ATF) started from 2015 in Japan. Since then, both experimental and analytical studies necessary for designing a new light water reactor (LWR) core with ATF candidate materials are being conducted within the Japanese ATF R&D Consortium for implementing ATF to the existing LWRs, accompanying with various technological developments required. Until now, we have accumulated experimental data of the candidate materials by out-of-pile tests, developed fuel evaluation codes to apply to the ATF candidate materials, and evaluated fuel behavior simulating operational and accidental conditions by the developed codes. In this paper, the R&D progresses of the ATF candidate materials considered in Japan are reviewed based on the information available such as proceedings of international conference and academic papers, providing an overview of ATF program in Japan.

Journal Articles

Routing study of above core structure with mock-up experiment for ASTRID

Takano, Kazuya; Sakamoto, Yoshihiko; Morohoshi, Kyoichi*; Okazaki, Hitoshi*; Gima, Hiromichi*; Teramae, Takuma*; Ikarimoto, Iwao*; Botte, F.*; Dirat, J.-F.*; Dechelette, F.*

Proceedings of 2019 International Congress on Advances in Nuclear Power Plants (ICAPP 2019) (Internet), 8 Pages, 2019/05

ASTRID has the objective to integrate innovative options in order to prepare the 4th generation reactors. In ASTRID, large number of tubes are installed above each fuel subassembly to monitor the core. These instrumentations such as thermocouples (TC) and Failed Fuel Detection and Location (FFDL) systems are integrated into Above Core Structure (ACS) with various sizes tubes. In the present study, the routing study for TC tubes and FFDL tubes was performed with 3D modeling and mock-up experiment of the ACS designed for ASTRID with 1500 MW thermal power in order to clarify the integration process and secure the design hypotheses. Although some problems on fabricability were found in the mock-up experiment, the possible solutions were proposed. The present study gives manufacturing feedback to design team and will contribute to increase the knowledge for ACS design and fabricability.

Journal Articles

Isotope-selective microscale imaging of radioactive Cs without isobaric interferences using sputtered neutral mass spectrometry with two-step resonant ionization employing newly-developed Ti:Sapphire lasers

Sakamoto, Tetsuo*; Morita, Masato*; Kanenari, Keita*; Tomita, Hideki*; Sonnenschein, V.*; Saito, Kosuke*; Ohashi, Masaya*; Kato, Kotaro*; Iguchi, Tetsuo*; Kawai, Toshihide*; et al.

Analytical Sciences, 34(11), p.1265 - 1270, 2018/11

 Times Cited Count:8 Percentile:31.98(Chemistry, Analytical)

Journal Articles

Simulation of fluidity, dispersion and mass transfer in an annular centrifugal contactor

Sano, Yuichi; Sakamoto, Atsushi; Takeuchi, Masayuki; Misumi, Ryuta*; Kunii, Kanako*; Todoroki, Kei*; Nishi, Kazuhiko*; Kaminoyama, Meguru*

Kagaku Kogaku Rombunshu, 44(6), p.335 - 340, 2018/11

Concerning an annular centrifugal contactor which has high throughput and separation performance, the effect of operational condition on fluidic and dispersion behavior, which are important to improve the contactor performance, was investigated by computational fluid dynamics (CFD) analysis based on the turbulence model, and the calculated results were validated by experimental data. The liquid phase in the annular zone was gradually divided into two regions vertically with increasing the rotor speed and decreasing the flowrate, and the liquid flow moved toward the center of the housing bottom was generated in the lower annular zone under any operational condition. The droplet size of the dispersed phase in the annular zone decreased with increasing the rotor speed and decreasing the flowrate. These calculation results showed a good agreement with experimental data. The CFD analysis considering mass transfer between aqueous and organic phases was also attempted, and it was confirmed that the change of extraction performance with the rotor speed showed the same tendency as the experimental result.

Journal Articles

Cation distribution and magnetic properties in ultrathin (Ni$$_{1-x}$$Co$$_{x}$$)Fe$$_{2}$$O$$_{4}$$ (x=0-1) layers on Si(111) studied by soft X-ray magnetic circular dichroism

Wakabayashi, Yuki*; Nonaka, Yosuke*; Takeda, Yukiharu; Sakamoto, Shoya*; Ikeda, Keisuke*; Chi, Z.*; Shibata, Goro*; Tanaka, Arata*; Saito, Yuji; Yamagami, Hiroshi; et al.

Physical Review Materials (Internet), 2(10), p.104416_1 - 104416_12, 2018/10

 Times Cited Count:10 Percentile:37.66(Materials Science, Multidisciplinary)

Journal Articles

High temperature oxidation test of simulated BWR fuel bundle in steam-starved conditions

Yamazaki, Saishun; Pshenichnikov, A.; Pham, V. H.; Nagae, Yuji; Kurata, Masaki; Tokushima, Kazuyuki*; Aomi, Masaki*; Sakamoto, Kan*

Proceedings of Annual Topical Meeting on Reactor Fuel Performance (TopFuel 2018) (Internet), 8 Pages, 2018/10

It is predictively evaluated that degradation of fuel assembly proceeded in a certain steam-starved condition at the early stage of a SA at 1F unit 2 (BWR). As for PWR fuel assembly, effective steam flow rate was properly indicated by normalizing to a unit of g-H$$_{2}$$O/sec/rod which is used as an important parameter for evaluating fuel degradation progression. Due to the inhomogeneous configuration of BWR fuel assembly, the difference of Zry oxidation and hydrogen uptake between the inside and outside of the channel box cannot be properly evaluated by this normalization. Instead of g-H$$_{2}$$O/sec/rod, proper evaluation unit for BWR configuration is necessary. To accumulate Zry oxidation and hydrogen uptake data for steam-starved conditions, high temperature oxidation tests were performed using a simulated BWR fuel bundle sample. The use of equivalent diameter of the cross section of BWR fuel assembly was proposed for normalization of effective steam flow rate.

Journal Articles

Corrosion behaviour of FeCrAl-ODS steels in nitric acid solutions with several temperatures

Takahatake, Yoko; Ambai, Hiromu; Sano, Yuichi; Takeuchi, Masayuki; Koizumi, Kenji; Sakamoto, Kan*; Yamashita, Shinichiro

Proceedings of Annual Topical Meeting on Reactor Fuel Performance (TopFuel 2018) (Internet), 9 Pages, 2018/10

The corrosion behaviour of FeCrAl-ODS steels for the accident tolerant fuel cladding of LWRs were investigated in nitric acid solutions for the reprocessing process of spent fuels. The corrosion tests were carried out at 60$$^{circ}$$C, 80$$^{circ}$$C and the boiling point of the solutions, and the specimens were then analysed by XPS. The corrosion remarkably progressed at the boiling point, and the highest corrosion rate was 0.22 mm/y. In the oxide film, the atomic concentration of Fe was lower, than that in the base material, and those of Cr and Al were higher. The results show that the corrosion of FeCrAl-ODS steels in hot nitric acid solution is not severe because of the high corrosion resistance of the oxide film formed on the material; hence, the corrosion resistance of the new cladding materials in the dissolution process of spent fuel is acceptable for reprocessing operations.

Journal Articles

Flow behavior in annular centrifugal extractors with different vessel sizes

Misumi, Ryuta*; Todoroki, Kei*; Kunii, Kanako*; Nishi, Kazuhiko*; Kaminoyama, Meguru*; Sano, Yuichi; Sakamoto, Atsushi; Takeuchi, Masayuki

Kagaku Kogaku Rombunshu, 44(5), p.285 - 291, 2018/09

Annular centrifugal extractors have been anticipated for use as extractors in spent nuclear fuel recycling. The extraction rate and the liquid-liquid dispersion are related to the flow pattern in the vessel. However, no study has clarified flow patterns in vessels of various scales. For this study, flow pattern characteristics are quantified for extractors of two scales. An extractor has a mixing zone around the vessel bottom and a separation zone in the cylindrical rotor. For this experiment, distilled water was fed into the vessel. Flow behavior in the mixing zone was observed from a side view using a digital video camera at various rotor speeds and supply flow rates for extractors of two scales. In some cases, the liquid horizontal velocity vectors in the mixing zone were measured using particle image velocimetry. Results demonstrate that flow behaviors in the mixing zone in both scales of extractors are classifiable as three types, changing with operational conditions: Type A, Type B, and a Transition regime. For the Type A state, the mixing zone is fully filled with liquid from the vessel bottom up to the lower edge of the rotor. In the Type B state, the zone with existing liquid is vertically divisible into two regions. Lower rotor speeds and higher flow rates tend to produce Type A state flow behavior. The boundary operational condition between Type A and the Transition regime are correlated with the normalized supply flow rate and pumping capacity of the rotor, which is evaluated from liquid surface level in a rotor formed by centrifugal force. Furthermore, the fluid velocity in the mixing zone is roughly proportional to the rotor surface circumferential speed irrespective of the vessel scale.

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