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Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; et al.
Radiation Protection Dosimetry, 199(14), p.1620 - 1625, 2023/09
Times Cited Count：0 Percentile：0.01(Environmental Sciences)We have been conducting dose assessments for Japanese macaques captured in Fukushima to reveal radiobiological effects on the low-dose expose animals. To accurately determine the external exposure dose, it is desirable to examine the analysis of the CO
radical intensity. We examined ESR spectra of teeth of 10 macaques captured in Fukushima by two spectrum-decomposition algorithms.
Sanada, Yukihisa; Abe, Tomohisa; Sasaki, Miyuki; Kanno, Marina*; Yamada, Tsutomu*; Nakasone, Takamasa*; Miyazaki, Nobuyuki*; Oshikiri, Keisuke*; Watabe, Hiroshi*
Journal of Nuclear Science and Technology, 10 Pages, 2023/00
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)The "treated water" from which the main radioactive materials were removed contains tritium, and stakeholders in Japan have been debating how to treat it. The amount of treated water stored in the facility has reached its limit, and the Japanese government has decided that the treatment method will be to discharge the water into the ocean by FY 2023 (FY: Fiscal Year). The present research developed a simple and practical tritium monitor for the Fukushima Daiichi Nuclear Power Station (FDNPS) tritiated water release. A simple and practical tritium monitor was developed for FDNPS tritiated water release based on thin plastic scintillator sheets. The developed devices were calibrated using standard tritium solutions and a method for calculating the minimum detectable activity. Fifteen 0.25 mm-thick scintillators can be placed in the 0.26 L flow cell where the sample water is fed, yielding an active surface area of 3,200 mm
. The efficiency of tritiated water with full water is 0.000035 cps Bq
. The minimum detectable activity under simple shielding conditions was 7,800 Bq L (Measurement time was 3,600 s).
Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; et al.
KEK Proceedings 2022-2, p.120 - 125, 2022/11
We investigate the effect of sample's anisotropy and measurement condition to obtain the higher reproducibility for the shape of the ESR spectrum and the intensity of CO radical.
Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; Osaka, Ken*; Sasaki, Keiichi*; et al.
Journal of Radiation Research (Internet), 63(4), p.609 - 614, 2022/07
Times Cited Count：1 Percentile：27.14(Biology)Electron spin resonance (ESR) dosimetry is one of the most powerful tools for radiation dose reconstruction. The detection limit of this technique using human teeth is reported to be 56 mGy or 67 mGy; however, the absorbed dose of Fukushima residents after the Fukushima Daiichi Nuclear Power Plant (FNPP) accident was estimated to be lower than this detection limit. Our aim is to assess the absorbed radiation dose of children in Fukushima Prefecture after the accident; therefore, it is important to estimate the detection limit for their teeth. The detection limit for enamel of deciduous teeth of Japanese children separated by the mechanical method is estimated to be 115.0 mGy. The density separation method can effectively separate enamel from third molars of Japanese people. As we have collected thousands of teeth from children in Fukushima, the present technique may be useful to examine their external absorbed dose after the FNPP accident.
Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.
KEK Proceedings 2021-2, p.91 - 96, 2021/12
We examined whether the ESR dose estimation method could be applied to wild Japanese macaque. In this work, we investigated the enamel preparation protocol and the analytical method of the ESR spectra.
Sr in cattle bone and tooth samples by inductively coupled plasma mass spectrometryKoarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Yanagisawa, Kayo*; Terashima, Motoki; Fujiwara, Kenso; Kino, Yasushi*; Oka, Toshitaka; Takahashi, Atsushi*; Suzuki, Toshihiko*; et al.
Journal of Analytical Atomic Spectrometry, 36(8), p.1678 - 1682, 2021/08
Times Cited Count：5 Percentile：55.72(Chemistry, Analytical)Rapid analysis of Sr in bone and tooth samples of cattle were achieved by an inductively coupled plasma mass spectrometry (ICP-MS) coupled with mass shift and solid phase extraction techniques. Limit of detection (LOD) in the ICP-MS measurement of 0.1 g samples was lower than that of the radioactivity measurement. Analytical time of the ICP-MS method was reduced from 20 days to 11 hours, compared with the radiometric method. Therefore, the ICP-MS method can be rapid and useful procedure of Sr in small bone and tooth samples derived from terrestrial animals.
Nishimura, Shoichiro*; Torii, Hiroyuki*; Fukao, Yoshinori*; Ito, Takashi; Iwasaki, Masahiko*; Kanda, Sotaro*; Kawagoe, Kiyotomo*; Kawall, D.*; Kawamura, Naritoshi*; Kurosawa, Noriyuki*; et al.
Physical Review A, 104(2), p.L020801_1 - L020801_6, 2021/08
Times Cited Count：13 Percentile：83.13(Optics)Takahashi, Atsushi*; Chiba, Mirei*; Tanahara, Akira*; Aida, Jun*; Shimizu, Yoshinaka*; Suzuki, Toshihiko*; Murakami, Shinobu*; Koarai, Kazuma; Ono, Takumi*; Oka, Toshitaka; et al.
Scientific Reports (Internet), 11(1), p.10355_1 - 10355_11, 2021/05
Times Cited Count：6 Percentile：41.49(Multidisciplinary Sciences)Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Mitsuyasu, Yusuke*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; Osaka, Ken*; et al.
Radiation Measurements, 134, p.106315_1 - 106315_4, 2020/06
Times Cited Count：5 Percentile：53.85(Nuclear Science & Technology)The relationship between the CO
radical intensity and the absorbed dose (dose response curve) of tooth enamel of Japanese macaque was observed by electron spin resonance and the detection limit of our system was estimated to be 33.5 mGy, which is comparable to the detection limit for human molar teeth. Using the dose response curve, external exposure dose for seven wild Japanese macaques captured in Fukushima prefecture were examined. The results suggest that the external exposure dose for the wild Japanese macaques were ranged between 45 mGy to 300 mGy.
Strasser, P.*; Abe, Mitsushi*; Aoki, Masaharu*; Choi, S.*; Fukao, Yoshinori*; Higashi, Yoshitaka*; Higuchi, Takashi*; Iinuma, Hiromi*; Ikedo, Yutaka*; Ishida, Katsuhiko*; et al.
EPJ Web of Conferences, 198, p.00003_1 - 00003_8, 2019/01
Times Cited Count：13 Percentile：99.06(Quantum Science & Technology)Ueno, Yasuhiro*; Aoki, Masaharu*; Fukao, Yoshinori*; Higashi, Yoshitaka*; Higuchi, Takashi*; Iinuma, Hiromi*; Ikedo, Yutaka*; Ishida, Katsuhiko*; Ito, Takashi; Iwasaki, Masahiko*; et al.
Hyperfine Interactions, 238(1), p.14_1 - 14_6, 2017/11
Times Cited Count：3 Percentile：86.59(Physics, Atomic, Molecular & Chemical)Strasser, P.*; Aoki, Masaharu*; Fukao, Yoshinori*; Higashi, Yoshitaka*; Higuchi, Takashi*; Iinuma, Hiromi*; Ikedo, Yutaka*; Ishida, Katsuhiko*; Ito, Takashi; Iwasaki, Masahiko*; et al.
Hyperfine Interactions, 237(1), p.124_1 - 124_9, 2016/12
Times Cited Count：7 Percentile：90.97(Physics, Atomic, Molecular & Chemical)Sanada, Yukihisa; Munakata, Masahiro; Mori, Airi; Ishizaki, Azusa; Shimada, Kazumasa; Hirouchi, Jun; Nishizawa, Yukiyasu; Urabe, Yoshimi; Nakanishi, Chika*; Yamada, Tsutomu*; et al.
JAEA-Research 2016-016, 131 Pages, 2016/10
JAEA-Research-2016-016.pdf:20.59MB
By the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company (TEPCO), caused by the East Japan earthquake and the following tsunami occurred on March 11, 2011, a large amount of radioactive materials was released from the NPS. After the nuclear disaster, airborne radiation monitoring using manned helicopter was conducted around FDNPS. In addition, background dose rate monitoring was conducted around Sendai Nuclear Power Station. These results of the aerial radiation monitoring using the manned helicopter in the fiscal 2015 were summarized in the report.
Sasaki, Kenji*; Naito, Katsuaki*; Oki, Shigeo; Okubo, Tsutomu; Kotake, Shoji*
Progress in Nuclear Science and Technology (Internet), 4, p.94 - 98, 2014/04
This paper evaluates the amount of activation of the secondary sodium in Direct Heat Exchanger (DHX) by neutrons leaked from the core, the radioactivity density, and the dose rate around the secondary sodium pipes in Direct Reactor Auxiliary Cooling System (DRACS) and confirms that the requirements in radioactivity free areas are satisfied by improving the exactness of calculation model with Monte Carlo Methodology.
Oda, Chie; Honda, Akira; Takase, Hiroyasu*; Ozone, Kenji*; Sasaki, Ryoichi*; Yamaguchi, Kohei*; Sato, Tsutomu*
Nendo Kagaku, 51(2), p.34 - 49, 2013/02
Proposed TRU repository designs for geological disposal envisage the use of a bentonite buffer to limit the migration of radionuclides by impeding groundwater flow. Under highly alkaline conditions due to cementitious materials could cause a complex series of coupled changes in the porewater chemistry, mineralogy and, ultimately, the mass transport properties of the bentonite buffer. To elucidate the consequences of these coupled changes, reactive-transport model analyses have been conducted for eight bentonite alteration test cases using different combinations of secondary minerals that could form in the bentonite buffer. It was found that after 100,000 years the amount of dissolved bentonite was at a maximum when metastable secondary minerals precipitated. It was also found that the diffusion and hydraulic coefficients after 100,000 years in all test cases were on the same order of magnitude as the initial values.
Sakanaka, Shogo*; Akemoto, Mitsuo*; Aoto, Tomohiro*; Arakawa, Dai*; Asaoka, Seiji*; Enomoto, Atsushi*; Fukuda, Shigeki*; Furukawa, Kazuro*; Furuya, Takaaki*; Haga, Kaiichi*; et al.
Proceedings of 1st International Particle Accelerator Conference (IPAC '10) (Internet), p.2338 - 2340, 2010/05
Future synchrotron light source using a 5-GeV energy recovery linac (ERL) is under proposal by our Japanese collaboration team, and we are conducting R&D efforts for that. We are developing high-brightness DC photocathode guns, two types of cryomodules for both injector and main superconducting (SC) linacs, and 1.3 GHz high CW-power RF sources. We are also constructing the Compact ERL (cERL) for demonstrating the recirculation of low-emittance, high-current beams using above-mentioned critical technologies.
Sugo, Yumi; Sasaki, Yuji; Kimura, Takaumi; Sekine, Tsutomu*
Proceedings of International Conference on Advanced Nuclear Fuel Cycles and Systems (Global 2007) (CD-ROM), p.1870 - 1873, 2007/09
A tridentate diamide, 
-tetraoctyldiglycolamide (TODGA) is very useful for the recovery of actinide ions from spent nuclear fuel. Based on the mechanism of the radiolysis of TODGA in organic solution, an improvement of radiolytic stability of amidic extractants was attempted. The radiolytic degradation of TODGA was suppressed by the addition of appropriate compounds, due to reduction in the mole fraction of 
-dodecane. In addition, by using the solvents having low ionization potentials, TODGA could be protected from radiation. Because the charge transfer reaction in the primary process was inhibited. It was also confirmed that aromatic substituents in the molecule effectively improved the radiolytic stability.
Sugo, Yumi; Izumi, Yoshinobu*; Yoshida, Yoichi*; Nishijima, Shigehiro*; Sasaki, Yuji; Kimura, Takaumi; Sekine, Tsutomu*; Kudo, Hiroshi*
Radiation Physics and Chemistry, 76(5), p.794 - 800, 2007/05
Times Cited Count：78 Percentile：97.59(Chemistry, Physical)The radiolytic behavior of -tetraoctyldiglycolamide, 
-dimethyl--dioctyl-2-(3'-oxapentadecyl)malonamide, and 
-dioctylhexanamide in -dodecane was investigated by irradiation with 
-rays and electron pulses. The results showed -dodecane has a sensitization effect on the radiolysis of these amides, owing mainly to a charge transfer from radical cations of -dodecane to the amide molecules in the primary process observed in pulse radiolysis.
Sugo, Yumi; Sasaki, Yuji; Kimura, Takaumi; Sekine, Tsutomu*
Proceedings of 15th International Conference on Nuclear Engineering (ICONE-15) (CD-ROM), 5 Pages, 2007/04
no abstracts in English
Yokoo, Kenji; Horiguchi, Hironori; Yagi, Masahiro; Nagadomi, Hideki; Yamamoto, Kazuyoshi; Sasajima, Fumio; Oyama, Koji; Ishikuro, Yasuhiro; Sasaki, Tsutomu; Hirane, Nobuhiko; et al.
JAEA-Technology 2007-018, 104 Pages, 2007/03
JAEA-Technology-2007-018.pdf:5.92MB
Reactor operation training using JRR-4 (Japan Research Reactor No.4) was started in FY 1969, one of the curriculums of Nuclear Technology and Education Center (NuTEC). After that, the program was updated and carried out for reactor operation training, control rod calibration, and measurement of various kind of characteristics. JRR-4 has been contributed for nuclear engineer training that is over 1,700 trainees from bother domestic and foreign countries. JRR-4 can be used for experiment from zero power to 3500kW, and the trainees can make experience to operate the reactor from start up to shut down, not only zero-power experiments (critical approach, control rod calibration, reactivity measurement, etc.) but also other experiments under high power operation (xenon effect, temperature effects, reactor power calibration, etc.). This report is based on various kinds of guidance texts using for training, and collected for operation and experiments for reactor physics.
