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Journal Articles

Pressure studies on the antiferromagnetic Kondo semiconductor Ce(Ru $_{1-x}$ Rh)Al $_{10}$ (x = 0,0.1)

Tanida, Hiroshi*; Kitagawa, Kentaro*; Tateiwa, Naoyuki; Sera, Masafumi*; Nishioka, Takashi*

Physical Review B, 96(23), p.235131_1 - 235131_7, 2017/12

https://doi.org/10.1103/PhysRevB.96.235131

Times Cited Count：1 Percentile：5.94(Materials Science, Multidisciplinary)

We have done high pressure experiments on Ce(Ru $_{1-x}$ Rh)Al $_{10}$ (x = 0 and 0.1) to study pressure-induced phase transitions from the antiferromagnetic to paramagnetic state at . Experimental data of the electrical resistivity suggest that the - hybridization gap could be not necessary to form the unusual AFM order. The pressure effects on the magnetic susceptibility is also studied. We discuss a difference in the pressure response of the magnetic susceptibility based the electronic state between x = 0 and 0.1.

Journal Articles

Influence of electron doping on magnetic order in CeRuAl $_{10}$

Kobayashi, Riki*; Kaneko, Koji; Saito, Kotaro*; Mignot, J.-M.*; Andr, G.*; Robert, J.*; Wakimoto, Shuichi; Matsuda, Masaaki*; Chi, S.*; Haga, Yoshinori; et al.

Journal of the Physical Society of Japan, 83(10), p.104707_1 - 104707_5, 2014/10

https://doi.org/10.7566/JPSJ.83.104707

Times Cited Count：17 Percentile：68.53(Physics, Multidisciplinary)

Journal Articles

Large ferroquadrupole moment induced in the octupole-ordered Ce $_{0.7}$ La $_{0.3}$ B revealed by high-resolution X-ray diffraction

Inami, Toshiya; Michimura, Shinji*; Hayashi, Yuya*; Matsumura, Takeshi*; Sera, Masafumi*; Iga, Fumitoshi*

Physical Review B, 90(4), p.041108_1 - 041108_5, 2014/07

https://doi.org/10.1103/PhysRevB.90.041108

Times Cited Count：9 Percentile：38.87(Materials Science, Multidisciplinary)

We carried out a high-resolution X-ray diffraction experiment on Ce $_{0.7}$ La $_{0.3}$ B. This compound exhibits antiferro-octupole order (AFO) below = 1.4 K, and it is theoretically suggested that ferroquadrupole moments and a resultant rhombohedral deformation are induced in the AFO phase. We observe the splitting of Bragg reflections below and find that the unit cell is rhombohedral with the elongated [111] axis. We also precisely evaluate the magnitude of the induced quadrupole moments from the obtained shear strain and find that the quadrupole moments are not reduced in the AFO phase.

Journal Articles

Multipole order and fluctuation in Ce $_{0.7}$ La $_{0.3}$ B studied by resonant X-ray diffraction

Matsumura, Takeshi*; Michimura, Shinji*; Inami, Toshiya; Otsubo, Toru*; Tanida, Hiroshi*; Iga, Fumitoshi*; Sera, Masafumi*

JPS Conference Proceedings (Internet), 3, p.014008_1 - 014008_6, 2014/06

https://doi.org/10.7566/JPSCP.3.014008

We study the $T_{beta}$ -type antiferro-octupole (AFO) ordered state of Ce $_{0.7}$ La $_{0.3}$ B below 1.5 K by resonant X-ray diffraction in magnetic fields. Multipole moments induced by the field in the AFO phase are identified. In a mean-field model for the $T_{beta}$ AFO order within the quartet crystal-field ground state, the $O_{22}$ and $O_{20}$ antiferroquadrupoles (AFQ) are expected as mostly induced AFQ. However, in contrast to this expectation, the main induced moment is found to be the $O_{xy}$ -type AFQ.

Journal Articles

Evidence for hidden quadrupolar fluctuations behind the octupole order in Ce $_{0.7}$ La $_{0.3}$ B from resonant X-ray diffraction in magnetic fields

Matsumura, Takeshi*; Michimura, Shinji*; Inami, Toshiya; Otsubo, Toru*; Tanida, Hiroshi*; Iga, Fumitoshi*; Sera, Masafumi*

Physical Review B, 89(1), p.014422_1 - 014422_13, 2014/01

https://doi.org/10.1103/PhysRevB.89.014422

Times Cited Count：14 Percentile：52.23(Materials Science, Multidisciplinary)

The multipole ordered phase in Ce $_{0.7}$ La $_{0.3}$ B (phase IV) has been studied by resonant X-ray diffraction in magnetic fields. By utilizing diamond X-ray phase plates to rotate the incident linear polarization and a conventional crystal analyzer system, full linear polarization analysis has been performed to identify the order parameters. The analysis shows that the $Gamma_{rm 5g}$ quadrupoles are more induced by the field than the $Gamma_{rm 3g}$ quadrupoles in phase IV, in disagreement with mean-field calculations, in which the $Gamma_{rm 3g}$ quadrupole is the main induced moment. Hence, we consider that large fluctuations of the $Gamma_{rm 5g}$ quadrupole is hidden behind the primary ordering of the octupole.

Journal Articles

Be-NMR studies of the heavy-fermion superconductor UBe $_{13}$

To, Hideki*; Tsugawa, Norihiko*; Sera, Masafumi*; Haga, Yoshinori; Onuki, Yoshichika

Journal of Magnetism and Magnetic Materials, 310(2, Part1), p.706 - 708, 2007/03

Field-angle dependence of Be-NMR measurements has been carried out for a single crystal UBe $_{13}$ in the temperature range of 0.35-1.5 K. For the [001] direction, we observed that Be-NMR spectra consisted of 10 lines; one line comes from a Be(I) site located in the cubic symmetry, while nine lines come from Be(II) sites located in the lower symmetry. From the field angle dependence of the NMR spectra, we determined NQR parameters. In the superconducting state, we found that Be-NMR Knight shift for [001] direction does not change at all. This result is consistent with the spin triplet pairing state in UBe $_{13}$ .

Journal Articles

Hyperfine interactions in the heavy-fermion superconductor UBe $_{13}$ ; Be NMR studies

To, Hideki*; Tsugawa, Norihiko*; Sera, Masafumi*; Harima, Hisatomo*; Haga, Yoshinori; Onuki, Yoshichika

Journal of the Physical Society of Japan, 76(2), p.024705_1 - 024705_9, 2007/02

https://doi.org/10.1143/JPSJ.76.024705

Times Cited Count：15 Percentile：62.92(Physics, Multidisciplinary)

Be NMR measurements have been performed for a single crystal UBe $_{13}$ with $T_{rm c}$ = 0.86 K. For an applied field parallel to [001] direction, we have observed a well-split Be NMR line with the sharp line- width of 10 Oe, guaranteeing the high-quality of the single crystal from the microscopic viewpoint. We have also calculated the electric field gradient ( EFG) tensor at Be(II) site using the band-structure calculation based on an FLAPW-LDA method. The present results give direct evidence that the Be 2p orbital is responsible for conduction bands.

Oral presentation

Resonant X-ray diffraction study of multipole ordering in DyPdS

Michimura, Shinji; Inami, Toshiya; Otsubo, Toru*; Matsumura, Takeshi*; Tanida, Hiroshi*; Sera, Masafumi*; Matsuoka, Eiichi*; Watahiki, Masanori*; Tanigaki, Katsumi*; Onodera, Hideya*

no journal, ,

Oral presentation

Resonant X-ray diffraction study of Ce $_{0.7}$ La $_{0.3}$ B $_{6}$ in magnetic field

Michimura, Shinji; Inami, Toshiya; Otsubo, Toru*; Matsumura, Takeshi*; Tanida, Hiroshi*; Sera, Masafumi*; Iga, Fumitoshi*

no journal, ,

no abstracts in English

Oral presentation

Study of a multipole ordering in DyPdS by a resonant X-ray diffraction

Michimura, Shinji; Inami, Toshiya; Otsubo, Toru*; Matsumura, Takeshi*; Tanida, Hiroshi*; Sera, Masafumi*; Matsuoka, Eiichi*; Watahiki, Masanori*; Tanigaki, Katsumi*; Onodera, Hideya*

no journal, ,

no abstracts in English

Oral presentation

Effect of the Ru-site substitution on CeRuAl $_{10}$ , 3

Kobayashi, Riki; Kaneko, Koji; Wakimoto, Shuichi; Haga, Yoshinori; Matsuda, Tatsuma; Yamamoto, Etsuji; Robert, J.*; Mignot, J.-M.*; Andr, G.*; Matsuda, Masaaki*; et al.

no journal, ,

no abstracts in English

Oral presentation

Elucidation of high ordering temperature in CeRu $_{2}$ Al $_{10}$ using Rh substitution

Kobayashi, Riki; Kaneko, Koji; Wakimoto, Shuichi; Haga, Yoshinori; Matsuda, Tatsuma; Yamamoto, Etsuji; Robert, J.*; Mignot, J.-M.*; Andr, G.*; Matsuda, Masaaki*; et al.

no journal, ,

no abstracts in English

Oral presentation

Rhombohedral deformation of Ce $_{0.7}$ La $_{0.3}$ B observed by high-resolution X-ray diffraction

Inami, Toshiya; Michimura, Shinji*; Hayashi, Yuya*; Matsumura, Takeshi*; Sera, Masafumi*; Iga, Fumitoshi*

no journal, ,

no abstracts in English

Oral presentation

Rhombohedral deformation in the phase IV of Ce $_{0.7}$ La $_{0.3}$ B observed by high-resolution X-ray diffraction

Inami, Toshiya; Michimura, Shinji*; Hayashi, Yuya*; Matsumura, Takeshi*; Sera, Masafumi*; Iga, Fumitoshi*

no journal, ,

no abstracts in English

Oral presentation

High-resolution X-ray diffraction experiment on the octupole ordered phase in Ce $_{0.7}$ La $_{0.3}$ B

Inami, Toshiya; Michimura, Shinji*; Matsumura, Takeshi*; Hayashi, Yuya*; Sera, Masafumi*; Iga, Fumitoshi*

no journal, ,

We have carried out a high-resolution X-ray diffraction experiment at low temperatures and in magnetic fields on Ce $_{0.7}$ La $_{0.3}$ B that exhibits antiferrooctupole (AFO) order below =1.4K. Ferroquadrupole moments that accompany the AFO order and a resultant rhombohedral deformation of the cubic lattice were theoretically predicted and experimetanlly supported. However, the sign and magnitude of the rhombohedral deformation have not yet been determined. We observe the splitting of Bragg peaks below , which is consistent with a rhombohedral deformation of 4 $times10^{-5}$ elongated along the [111] axis. The response of rhombohedral domains to magnetic fields also well agrees with theoretical calculations. A particular outcome of this experiment is that the magnitude of the induced quadrupole moments is precisely evaluated from the obtained shear strain.

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Pressure studies on the antiferromagnetic Kondo semiconductor Ce(Ru $_{1-x}$ Rh)Al $_{10}$ (x = 0,0.1)

Influence of electron doping on magnetic order in CeRuAl $_{10}$

Large ferroquadrupole moment induced in the octupole-ordered Ce $_{0.7}$ La $_{0.3}$ B revealed by high-resolution X-ray diffraction

Multipole order and fluctuation in Ce $_{0.7}$ La $_{0.3}$ B studied by resonant X-ray diffraction

Evidence for hidden quadrupolar fluctuations behind the octupole order in Ce $_{0.7}$ La $_{0.3}$ B from resonant X-ray diffraction in magnetic fields

Be-NMR studies of the heavy-fermion superconductor UBe $_{13}$

Hyperfine interactions in the heavy-fermion superconductor UBe $_{13}$ ; Be NMR studies

Resonant X-ray diffraction study of multipole ordering in DyPdS

Resonant X-ray diffraction study of Ce $_{0.7}$ La $_{0.3}$ B $_{6}$ in magnetic field

Study of a multipole ordering in DyPdS by a resonant X-ray diffraction

Effect of the Ru-site substitution on CeRuAl $_{10}$ , 3

Elucidation of high ordering temperature in CeRu $_{2}$ Al $_{10}$ using Rh substitution

Rhombohedral deformation of Ce $_{0.7}$ La $_{0.3}$ B observed by high-resolution X-ray diffraction

Rhombohedral deformation in the phase IV of Ce $_{0.7}$ La $_{0.3}$ B observed by high-resolution X-ray diffraction

High-resolution X-ray diffraction experiment on the octupole ordered phase in Ce $_{0.7}$ La $_{0.3}$ B