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Shibata, Motoki*; Nakanishi, Yohei*; Abe, Jun*; Arima, Hiroshi*; Iwase, Hiroki*; Shibayama, Mitsuhiro*; Motokawa, Ryuhei; Kumada, Takayuki; Takata, Shinichi; Yamamoto, Katsuhiro*; et al.
Polymer Journal, 55(11), p.1165 - 1170, 2023/11
Times Cited Count：1 Percentile：51.7(Polymer Science)Shinto, Katsuhiro; Okoshi, Kiyonori; Shibata, Takanori*; Nammo, Kesao*; Kawai, Isao*; Ikegami, Kiyoshi*; Ueno, Akira
Proceedings of 20th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.928 - 931, 2023/11
J-PARC initiated the operation of the high-intensity rf-driven negative hydrogen (H
) ion source in 2014 autumn. The ion source produces the H beam with the beam current of 60 mA and the beam energy of 50 keV in order to inject the H beam into the 3 GeV RCS with the beam current of 50 mA and the beam energy of 400 MeV from the J-PARC linac. We have achieved the longest continuous operation time of 4001 hours in the previous (2021/2022) campaign. The 2022/2023 campaign was the first time that the continuous operation of the H ion source without any exchanges of the ion source until the end of the campaign was examined. We present the operation status of the J-PARC H ion source in this campaign as well as the status of the J-PARC-made internal antenna test.
Shinto, Katsuhiro; Shibata, Takanori*; Wada, Motoi*
Proceedings of 20th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.392 - 395, 2023/11
Negative hydrogen (H) ion sources which are used at high-intensity proton accelerator facilities such as J-PARC or neutral beam injection system for plasma heating in the fusion devices such as ITER produce plasmas by using RF sources driving with the frequency of 1-2 MHz. We have shown that the H beams extracted from the RF-driven H ion source with the frequency of several MHz have some fluctuations with the frequency of the fundamental and second harmonics. The reason is that the high plasma density is produced in the ion source with the low driving frequency. Therefore, we propose the driving RF frequency same as the RF sources with that of 324 MHz in the J-PARC linac, which is much higher than the ion plasma frequency, is used for producing the plasma to suppress the H beam fluctuations. As a first step, we performed a design of a matching circuit for the higher frequency driven H ion source. We present the background for decision of a new RF amplifier with much higher frequency and the design results.
Nakahara, Masaumi; Shibata, Atsuhiro
Journal of Nuclear Science and Technology, 60(7), p.849 - 858, 2023/07
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)To develop the acid split method which has highly nuclear proliferation resistance, influence of Pu content in dissolver solutions derived from irradiated fast reactor fuel on the Pu stripping was investigated in experiments and a calculation. The Pu content in the U/Pu and U products increased with increasing the Pu content in the dissolver solution. Moreover, the calculated results indicate that the Pu leakage into the U product is suppressed with the Pu stripping solution only at low temperature.
Takahatake, Yoko; Watanabe, So; Arai, Tsuyoshi*; Sato, Takahiro*; Shibata, Atsuhiro
Applied Radiation and Isotopes, 196, p.110783_1 - 110783_5, 2023/06
Times Cited Count：0 Percentile：0.01(Chemistry, Inorganic & Nuclear)Shimokita, Keisuke*; Yamamoto, Katsuhiro*; Miyata, Noboru*; Nakanishi, Yohei*; Shibata, Motoki*; Takenaka, Mikihito*; Yamada, Norifumi*; Seto, Hideki*; Aoki, Hiroyuki; Miyazaki, Tsukasa*
Soft Matter, 19(11), p.2082 - 2089, 2023/03
Times Cited Count：0 Percentile：0(Chemistry, Physical) ion sourceShinto, Katsuhiro; Shibata, Takanori*; Okoshi, Kiyonori; Nammo, Kesao*; Ikegami, Kiyoshi*; Oguri, Hidetomo
Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.675 - 679, 2023/01
In J-PARC, we have been conducting the test of a J-PARC-made internal antenna in order to establish the production method and understand the beam characteristics of the antenna. At this time, we investigated the outgas characteristics during the production of a high-density plasma by using the J-PARC-made antenna. It is confirmed that no remarkable impurities are emitted from the antenna by a residual gas analysis using a quadrupole mass analyzer installed downstream the ion source and a spectroscopic analysis of the plasma in the ion source. It is found that the emittances of the H beam extracted from the J-PARC radio-frequency H ion source by using the antenna was similar as those in case by using SNS antenna.
Shibata, Takanori*; Ishida, Masaki*; Nammo, Kesao*; Ikegami, Kiyoshi*; Okoshi, Kiyonori; Shinto, Katsuhiro; Oguri, Hidetomo
Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.863 - 867, 2023/01
Continuous operation duration of the J-PARC Radio Frequency (RF) ion source has been extended step by step these years for the goal to supply stable beam during the entire period of J-PARC user operation (around 7 months) each year. A 3651 hours (5 months) continuous ion source operation has been achieved from Nov. 2020 to Apr. 2021. As the lifetime of the ion source is mainly limited by failure on the RF antenna coil, detailed evaluation of the antenna surface condition is required to ensure the feasibility of the further extension of the operation time. In the present study, dimension measurements and SEM/EDS analyses were applied to understand the surface discoloration of the RF antenna. The discoloration after the long-term continuous operation is due to deposition of injected cesium (for H surface production process) and of stainless used steel (Fe, Cr, Ni) from the ion source components sputtered by plasma. The results show that the enamel coating of the RF antenna has not worn out in the long-term continuous operation for several months and, hence, extension of the ion source continuous operation duration can be extended.
Shimokita, Keisuke*; Yamamoto, Katsuhiro*; Miyata, Noboru*; Arima-Osonoi, Hiroshi*; Nakanishi, Yohei*; Takenaka, Mikihito*; Shibata, Motoki*; Yamada, Norifumi*; Seto, Hideki*; Aoki, Hiroyuki; et al.
Langmuir, 38(41), p.12457 - 12465, 2022/10
Times Cited Count：0 Percentile：0(Chemistry, Multidisciplinary)Nakahara, Masaumi; Watanabe, So; Aihara, Haruka; Takahatake, Yoko; Arai, Yoichi; Ogi, Hiromichi*; Nakamura, Masahiro; Shibata, Atsuhiro; Nomura, Kazunori
Proceedings of International Conference on Nuclear Fuel Cycle; Sustainable Energy Beyond the Pandemic (GLOBAL 2022) (Internet), 4 Pages, 2022/07
Various radioactive wastes have been generated from Chemical Processing Facility for basic research on advanced reactor fuel reprocessing, radioactive waste disposal, and nuclear fuel cycle technology. Many types of reagents have been used for the experiments, and some troublesome materials were produced in the course of experiments. The radioactive liquid wastes were treated for stable and safe storage using decomposition, solvent extraction, precipitation, and solidification methods. In this study, current status of harmless treatment for the radioactive liquid wastes would be reported.
Senzaki, Tatsuya; Arai, Yoichi; Yano, Kimihiko; Sato, Daisuke; Tada, Kohei; Ogi, Hiromichi*; Kawanobe, Takayuki*; Ono, Shimpei; Nakamura, Masahiro; Kitawaki, Shinichi; et al.
JAEA-Testing 2022-001, 28 Pages, 2022/05
JAEA-Testing-2022-001.pdf:2.33MB
In preparation for the decommissioning of Laboratory B of the Nuclear Fuel Cycle Engineering Laboratory, the nuclear fuel material that had been stored in the glove box for a long time was moved to the Chemical Processing Facility (CPF). This nuclear fuel material was stored with sealed by a polyvinyl chloride (PVC) bag in the storage. Since it was confirmed that the PVC bag swelled during storage, it seems that any gas was generated by radiolysis of the some components contained in the nuclear fuel material. In order to avoid breakage of the PVC bag and keep it safety for long time, we began the study on the stabilization treatment of the nuclear fuel material. First, in order to clarify the properties of nuclear fuel material, radioactivity analysis, component analysis, and thermal analysis were carried out. From the results of thermal analysis, the existence of organic matter was clarified. Then, ion exchange resin with similar thermal characteristics was selected and the thermal decomposition conditions were investigated. From the results of these analyzes and examinations, the conditions for thermal decomposition of the nuclear fuel material contained with organic matter was established. Performing a heat treatment of a small amount of nuclear fuel material in order to confirm the safety, after which the treatment amount was scaled up. It was confirmed by the weight change after the heat treatment that the nuclear fuel material contained with organic matter was completely decomposed.
Shibata, Takanori*; Okoshi, Kiyonori; Shinto, Katsuhiro; Nammo, Kesao*; Ikegami, Kiyoshi*; Oguri, Hidetomo
Journal of Physics; Conference Series, 2244, p.012041_1 - 012041_5, 2022/04
Times Cited Count：1 Percentile：0.32(Engineering, Electrical & Electronic)In the J-PARC user operation from Nov. 2020 - Apr. 2021, continuous operation of J-PARC Radio Frequency (RF) negative hydrogen ion (H) source up to 3,651 hours (5 months) has been achieved. The ion source was operated with the output H current of 60 mA, the duty factor (for plasma generation) 2% and the input RF power up to 30 kW. After the operation, phase space diagrams at the Radio Frequency Quadrupole (RFQ) entrance were measured by the emittance monitor at the ion source test stand (IS-TS) under the same operation condition as in the J-PARC Linac. Comparison of the phase spaces and the beam emittances between the ion sources in the present and the previous operations shows slight difference. From the direct observation of the antenna coil, no exhaustion or the decrease in the thickness of the enamel coating of the coil have been confirmed. The results indicate the possibility of the next goal of the long-run up to 7 months, which is the same as the full duration of the J-PARC user operation in 1 year.
Grambow, B.; Nitta, Ayako; Shibata, Atsuhiro; Koma, Yoshikazu; Utsunomiya, Satoshi*; Takami, Ryu*; Fueda, Kazuki*; Onuki, Toshihiko*; Jegou, C.*; Laffolley, H.*; et al.
Journal of Nuclear Science and Technology, 59(1), p.1 - 24, 2022/01
Times Cited Count：15 Percentile：71.66(Nuclear Science & Technology) beam extracted from an RF-driven high-intensity H ion sourceShinto, Katsuhiro; Shibata, Takanori*; Wada, Motoi*
Proceedings of 18th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.230 - 233, 2021/10
In most proton accelerator facilities such as J-PARC, SNS, CERN, a H ion source equipped with a 2-MHz rf driver for plasma generation produces H beams. We have reported H beam characteristics extracted from the J-PARC rf-driven high-intensity H ion source. We have been developing an emittance measurement apparatus equipped with a highly time-resolved data acquisition system in order to observe fluctuation of the beam emittance in association with the frequency of the rf driver. By using this apparatus, we found that the beam emittance is fluctuated with the frequency with the rf driver and higher harmonics. We will show some obtained results of the emittance fluctuation.
Shibata, Takanori*; Hirano, Koichiro; Hirane, Tatsuya*; Shinto, Katsuhiro; Hayashi, Naoki; Oguri, Hidetomo
Proceedings of 18th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.417 - 421, 2021/10
In J-PARC linac, the operation of an rf-driven high-intensity H ion source was initiated in 2014. For plasma ignition, the 2-MHz rf amplifier outputs the power of several tens kW. However the rf amplifier for the ion source and those for the accelerating cavities have not been synchronized. As a result, the wave hights in the beam waveforms were different in shot by shot. Therefore, we have developed an synchronization system between the rf system for the ion source and those for the cavity systems and succeeded the same wave hights in the waveforms.
Igarashi, Go*; Haga, Kazuko*; Yamada, Kazuo*; Aihara, Haruka; Shibata, Atsuhiro; Koma, Yoshikazu; Maruyama, Ippei*
Journal of Advanced Concrete Technology, 19(9), p.950 - 976, 2021/09
Times Cited Count：5 Percentile：39.74(Construction & Building Technology)Aihara, Haruka; Watanabe, So; Shibata, Atsuhiro; Mahardiani, L.*; Otomo, Ryoichi*; Kamiya, Yuichi*
Progress in Nuclear Energy, 139, p.103872_1 - 103872_9, 2021/09
Times Cited Count：2 Percentile：31.78(Nuclear Science & Technology)Shibata, Takanori*; Shinto, Katsuhiro; Wada, Motoi*; Oguri, Hidetomo; Ikegami, Kiyoshi*; Okoshi, Kiyonori; Nammo, Kesao*
AIP Conference Proceedings 2373, p.050002_1 - 050002_9, 2021/08
Oscillation of emittance and Twiss parameters in the negative ion beam from the J-PARC 2-MHz RF ion source is measured by applications of a double-slit emittance monitor located at the RFQ (Radio Frequency Quadrupole) entrance. The emittance monitor is equipped with a newly-developed 60 MS/s data acquisition system, so that beam current oscillation in a few MHz can be observed with enough time resolution. From the measurement, it is shown that the beam phase space consists of (1) a DC component in the beam core, (2) a 2-MHz oscillating component which takes place both in the beam core and the halo and (3) a doubled RF frequency (4 MHz) oscillation which slightly exists in the beam halo. The major component is the 2-MHz component, which resultantly decides the beam emittance oscillation frequency. A typical value of the beam emittance in the present experiment is 0.34 
mm-mrad, while the amplitude of the 2 MHz oscillation is around 0.04 mm-mrad. The results indicate that the high-frequency oscillation component occupying about ten-percent of the beam from the RF source travels a few meters passing through a magnetic lens focusing system.
Ogi, Hiromichi*; Arai, Yoichi; Aihara, Haruka; Watanabe, So; Shibata, Atsuhiro; Nomura, Kazunori
JAEA-Technology 2021-007, 27 Pages, 2021/06
JAEA-Technology-2021-007.pdf:2.43MB
Chemical Processing Facility (CPF) of Japan Atomic Energy Agency (JAEA) has been developing the fast reactor fuel reprocessing and vitrification technology. The various kinds of radioactive liquid wastes, which were generated by those experiments and analysis, stored in the hot cells and glove boxes of CPF. The treatment of radioactive liquid wastes were started since July 2015; however, treatment of several kinds of liquid wastes are revealed to be difficult due to contain the various hazardous chemicals. Therefore, in order to establish the new technology suitable for radioactive liquid waste treatment, several collaborative research programs with several universities and national research organizations were started. The combined project lead by JAEA was named to be STRAD (Systematic Treatments of Radioactive liquid wastes for Decommissioning) project. In this project, the process flow for treatment of several actual liquid wastes were established. In this report, treated method and progress of actual liquid wastes of CPF are summarized.
-P column by neutron resonance absorption imagingMiyazaki, Yasunori; Watanabe, So; Nakamura, Masahiro; Shibata, Atsuhiro; Nomura, Kazunori; Kai, Tetsuya; Parker, J. D.*
JPS Conference Proceedings (Internet), 33, p.011073_1 - 011073_7, 2021/03
Neutron resonance absorption imaging was adapted to observe the Eu band adsorbed in the CMPO/SiO-P column for minor actinide recovery by extraction chromatography. Several wet columns were prepared by either light water or heavy water and compared with the dry column to evaluate the neutron transmission. The neutron transmission spectra showed that 45% was transmitted through the dry column while 20% and 40% were transmitted through the wet columns of light water and heavy water, respectively. The results indicated that heavy water is more applicable than light water to observe the Eu adsorption band in the CMPO/SiO-P column.
