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Sm M
ssbauer and Sm L
-edge X-ray absorption spectroscopiesTsutsui, Satoshi; Higashinaka, Ryuji*; Nakamura, Raito*; Fujiwara, Kosuke*; Nakamura, Jin*; Kobayashi, Yoshio*; Ito, Takashi; Yoda, Yoshitaka*; Kato, Kazuo*; Nitta, Kiyofumi*; et al.
Hyperfine Interactions, 242(1), p.32_1 - 32_10, 2021/12
Times Cited Count：1 Percentile：84.11(Physics, Atomic, Molecular & Chemical)
Bh in the 
Cm(
Na,5
)Bh reaction and its decay propertiesHaba, Hiromitsu*; Fan, F.*; Kaji, Daiya*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Komori, Yukiko*; Kondo, Narumi*; Kudo, Hisaaki*; Morimoto, Koji*; Morita, Kosuke*; et al.
Physical Review C, 102(2), p.024625_1 - 024625_12, 2020/08
Times Cited Count：6 Percentile：58.52(Physics, Nuclear)Strasser, P.*; Abe, Mitsushi*; Aoki, Masaharu*; Choi, S.*; Fukao, Yoshinori*; Higashi, Yoshitaka*; Higuchi, Takashi*; Iinuma, Hiromi*; Ikedo, Yutaka*; Ishida, Katsuhiko*; et al.
EPJ Web of Conferences, 198, p.00003_1 - 00003_8, 2019/01
Times Cited Count：13 Percentile：98.93(Quantum Science & Technology)
U oxide and fluorideShigekawa, Yudai*; Kasamatsu, Yoshitaka*; Yasuda, Yuki*; Kaneko, Masashi; Watanabe, Masayuki; Shinohara, Atsushi*
Physical Review C, 98(1), p.014306_1 - 014306_5, 2018/07
Times Cited Count：4 Percentile：36.08(Physics, Nuclear)The nuclear half-life of U has been reported to vary depending on the chemical environment. In this study, both the half-life and the internal-conversion (IC) electron energy spectrum were measured for U with identical chemical environments for the first time. U oxide and fluoride samples were subjected to these measurements, and clear differences in the half-life and the energy spectrum between these samples were observed. The peaks in the energy spectra were identified with the relativistic density functional theory calculation, and the molecular orbital states of the U oxide and fluoride estimated from the energy spectra and the calculation qualitatively explained the difference in the half-lives between the samples.
Ueno, Yasuhiro*; Aoki, Masaharu*; Fukao, Yoshinori*; Higashi, Yoshitaka*; Higuchi, Takashi*; Iinuma, Hiromi*; Ikedo, Yutaka*; Ishida, Katsuhiko*; Ito, Takashi; Iwasaki, Masahiko*; et al.
Hyperfine Interactions, 238(1), p.14_1 - 14_6, 2017/11
Times Cited Count：3 Percentile：86.37(Physics, Atomic, Molecular & Chemical)
Sato, Wataru*; Komatsuda, Sayaka*; Osa, Akihiko; Sato, Tetsuya; Okubo, Yoshitaka*
Hyperfine Interactions, 237(1), p.113_1 - 113_6, 2016/12
Times Cited Count：2 Percentile：61.66(Physics, Atomic, Molecular & Chemical)The magnetic hyperfine field and electric field gradient at the
Cd(
Cd) and 
Cd(In) probe nuclei introduced in a perovskite manganese oxide 
(
250 K) were measured for the study of the local magnetism and structure by means of time-differential perturbed angular correlation spectroscopy. In the ferromagnetic phase at 77 K, a very slight supertransferred magnetic hyperfine field (SMHF) (
0.014 T) combined with a well-defined electric field gradient was observed at the nonmagnetic Cd nucleus on the La/Ca A site. This observation suggests that the large magnetic hyperfine field (
= 6.9 T) measured, in our previous work, at the 
Ce probe nucleus on the A site originates from the contribution of a 4
spin oriented by the SMHF from adjacent Mn ions.
Strasser, P.*; Aoki, Masaharu*; Fukao, Yoshinori*; Higashi, Yoshitaka*; Higuchi, Takashi*; Iinuma, Hiromi*; Ikedo, Yutaka*; Ishida, Katsuhiko*; Ito, Takashi; Iwasaki, Masahiko*; et al.
Hyperfine Interactions, 237(1), p.124_1 - 124_9, 2016/12
Times Cited Count：7 Percentile：90.97(Physics, Atomic, Molecular & Chemical)
Ni synchrotron radiation-based M
ssbauer spectroscopy of nickel-based nanoparticles with hexagonal structureMasuda, Ryo*; Kobayashi, Yasuhiro*; Kitao, Shinji*; Kurokuzu, Masayuki*; Saito, Makina*; Yoda, Yoshitaka*; Mitsui, Takaya; Hosoi, Kohei*; Kobayashi, Hirokazu*; Kitagawa, Hiroshi*; et al.
Scientific Reports (Internet), 6, p.20861_1 - 20861_8, 2016/02
Times Cited Count：9 Percentile：40.51(Multidisciplinary Sciences)ssbauer spectroscopyMibu, Ko*; Mitsui, Takaya; Tanaka, Masaaki*; Masuda, Ryo*; Kitao, Shinji*; Kobayashi, Yasuhiro*; Yoda, Yoshitaka*; Seto, Makoto*
Journal of Applied Physics, 117(17), p.17E126_1 - 17E126_4, 2015/05
Times Cited Count：2 Percentile：9.08(Physics, Applied)
Te synchrotron-radiation-based Mssbauer spectroscopyKurokuzu, Masayuki*; Kitao, Shinji*; Kobayashi, Yasuhiro*; Saito, Makina*; Masuda, Ryo*; Mitsui, Takaya; Yoda, Yoshitaka*; Seto, Makoto*
Hyperfine Interactions, 226(1), p.687 - 691, 2014/04
Times Cited Count：3 Percentile：69.7(Physics, Atomic, Molecular & Chemical)Te synchrotron-radiation-based Mssbauer spectroscopy of Fe
Te and FeTe
SeKurokuzu, Masayuki*; Kitao, Shinji*; Kobayashi, Yasuhiro*; Saito, Makina*; Masuda, Ryo*; Mitsui, Takaya; Yoda, Yoshitaka*; Seto, Makoto*
Journal of the Physical Society of Japan, 83(4), p.044708_1 - 044708_4, 2014/04
Times Cited Count：3 Percentile：20.34(Physics, Multidisciplinary)ssbauer spectra of 
Yb measured with internal conversion electronsMasuda, Ryo*; Kobayashi, Yasuhiro*; Kitao, Shinji*; Kurokuzu, Masayuki*; Saito, Makina*; Yoda, Yoshitaka*; Mitsui, Takaya; Iga, Fumitoshi*; Seto, Makoto
Applied Physics Letters, 104(8), p.082411_1 - 082411_5, 2014/02
Times Cited Count：21 Percentile：65.02(Physics, Applied)A detection system for synchrotron-radiation (SR)-based Mssbauer spectroscopy was developed to enhance the nuclear resonant scattering counting rate and thus increase the available nuclides. In the system, a windowless avalanche photodiode (APD) detector was combined with a vacuum cryostat to detect the internal conversion (IC) electrons and fluorescent X-rays accompanied by nuclear de-excitation. As a feasibility study, the SR-based Mssbauer spectrum using the 76.5 keV level of Yb was observed without Yb enrichment of the samples. The counting rate was five times higher than that of our previous system, and the spectrum was obtained within 10 h. This result shows that nuclear resonance events can be more efficiently detected by counting IC electrons for nuclides with high IC coefficients. Furthermore, the windowless detection system enables us to place the sample closer to the APD elements and is advantageous for nuclear resonant inelastic scattering measurements. Therefore, this detection system can not only increase the number of nuclides accessible in SR-based Mssbauer spectroscopy but also allows the nuclear resonant inelastic scattering measurements of small single crystals or enzymes with dilute probe nuclides that are difficult to measure with the previous detection system.
Hamada, Kazuya; Nunoya, Yoshihiko; Isono, Takaaki; Takahashi, Yoshikazu; Kawano, Katsumi; Saito, Toru; Oshikiri, Masayuki; Uno, Yasuhiro; Koizumi, Norikiyo; Nakajima, Hideo; et al.
IEEE Transactions on Applied Superconductivity, 22(3), p.4203404_1 - 4203404_4, 2012/06
Times Cited Count：17 Percentile：63.88(Engineering, Electrical & Electronic)Japan Atomic Energy Agency (JAEA) has the responsibility for procurement of all of the ITER central solenoid (CS) conductor lengths. The CS conductor is composed of 576 Nb
Sn superconducting strands and 288 Cu strands assembled together into a multistage cable and protected by a circle-in-square sheath tube (jacket) with the outer dimension of 49 mm. In preparation for CS conductor production, the following R&D activities have been performed; (1) Mechanical tests at 4 K have been performed for jacket candidate materials such as 316LN and JK2LB, (2) Welding test for filler selection, (3) Measurement of coefficient of sliding friction using a 100-m long dummy cable, (4) Deformation characteristics of the conductor cross section after compaction and spooling. As a result of these R&D, the CS conductor jacket manufacturing technologies have been confirmed to start the procurement of the CS conductor.
Hamada, Kazuya; Takahashi, Yoshikazu; Nabara, Yoshihiro; Kawano, Katsumi; Ebisawa, Noboru; Oshikiri, Masayuki; Tsutsumi, Fumiaki; Saito, Toru*; Nakajima, Hideo; Matsuda, Hidemitsu*; et al.
Teion Kogaku, 47(3), p.153 - 159, 2012/03
The Japan Atomic Energy Agency (JAEA) has the responsibility to procure 25% of the ITER Toroidal Field coil conductors as the Japanese Domestic Agency (JADA) in the ITER project. The TF conductor is a circular shaped, cable-in-conduit conductor, composed of a cable and a stainless steel conduit (jacket). The outer diameter and maximum length of the TF conductor are 43.7 mm and 760 m, respectively. JAEA has constructed newly conductor manufacturing facility. Prior to starting conductor, JAEA manufactured a 760-m long Cu dummy conductor as process qualification of dummy cable, the jacket sections and fabrication procedures, such as welding, cable insertion, compaction and spooling. Following qualification of all manufacturing processes, JAEA has started to fabricate superconducting conductors for the TF coils.
Hamada, Kazuya; Takahashi, Yoshikazu; Isono, Takaaki; Nunoya, Yoshihiko; Matsui, Kunihiro; Kawano, Katsumi; Oshikiri, Masayuki; Tsutsumi, Fumiaki; Koizumi, Norikiyo; Nakajima, Hideo; et al.
Fusion Engineering and Design, 86(6-8), p.1506 - 1510, 2011/10
Times Cited Count：12 Percentile：66.68(Nuclear Science & Technology)Japan Atomic Energy Agency has a responsibility for procurement of the ITER toroidal field coil conductors as Japanese Domestic Agency (JADA) of the ITER project. The TF conductor is a circular shaped cable-in-conduit conductor, which is composed of cable and stainless steel conduit (jacket). The outer diameter and wall thickness of jacket are 43.7mm and 2mm, respectively. The cable consists of 900 NbSn superconducting strands and 522 Cu strands. The length of TF conductor is 780m in maximum. Preparation of conductor fabrication was completed in December 2009. And then, to demonstrate a conductor manufacturing procedure, JADA fabricated 780m-long Cu dummy conductor as a process qualification. Finally, the 780m-long Cu dummy conductor has been successfully completed, ahead of other domestic agencies that are in charge of TF conductor procurement. Since all of manufacturing processes have been qualified, JADA started to fabricate superconducting conductors for TF coils.
Matsuoka, Takahiro*; Fujihisa, Hiroshi*; Hirao, Naohisa*; Oishi, Yasuo*; Mitsui, Takaya; Masuda, Ryo; Seto, Makoto*; Yoda, Yoshitaka*; Shimizu, Katsuya*; Machida, Akihiko; et al.
Physical Review Letters, 107(2), p.025501_1 - 025501_4, 2011/07
Times Cited Count：29 Percentile：77.56(Physics, Multidisciplinary)Europium-hydride EuH
exposed to high-pressure H conditions has been found to exhibit structural and valence changes, 
(
=2, divalent) 
63/
(=2, 7.2-8.7 GPa) 
4/
(
2, 8.7-9.7 GPa) 4/
(2, 9.7 GPa-, trivalent). Having trivalent character and distorted cubic fcc structure, the 4/ structure is the 
-phase which has been commonly observed for other rare-earth metal hydrides. Our study clearly demonstrates that EuH is no longer an "irregular" member of the rare earth metal hydrides.
Kamei, Gento; Honda, Akira; Mihara, Morihiro; Oda, Chie; Ichige, Satoru; Kurimoto, Yoshitaka; Hoshino, Seiichi; Akagi, Yosuke; Sato, Nobuyuki; Murakami, Hiroshi*; et al.
JAEA-Research 2011-002, 82 Pages, 2011/03
JAEA-Research-2011-002.pdf:5.64MB
Based on Japanese governmental policy and general scheme, research and development of geological disposal technology for TRU waste has been proceeding to improve reliability of the safety assessment of the co-locational disposal of TRU waste and of HLW, to expand the basement of generic safety assessment, and to develop the alternative technology to cope with the broad geologic environment of Japan. Japan Atomic Energy Agency is dealing with the assignments in the governmental generic scheme. We report here the progress of the studies at the end of H20 (2008) Japanese fiscal year, which are (1) evaluation of long-term mechanical stability in the near-field including development of a creep mode of rock and analyses of mechanical behavior of TRU waste repository, (2) performance assessment of the disposal system including data acquisition and preparation on radionuclides migration, cementitious material alteration, bentonite and hostrock alteration with alkaline solution and nitrate effect, and (3) alternative technology development including decomposition of nitrate.
ssbauer spectroscopySeto, Makoto; Masuda, Ryo; Higashitaniguchi, Satoshi*; Kitao, Shinji*; Kobayashi, Yasuhiro*; Inaba, Chika*; Mitsui, Takaya; Yoda, Yoshitaka*
Physical Review Letters, 102(21), p.217602_1 - 217602_4, 2009/05
Times Cited Count：57 Percentile：87.99(Physics, Multidisciplinary)We have developed a new method that yields Mssbauer absorption spectra using synchrotron radiation (SR); this method is applicable for almost all Mssbauer nuclides including those that cannot be measured by previous methods using radioisotope (RI) sources. The Mssbauer spectrum of the 68.752 keV excited state of 
Ge, which cannot be measured using a RI source, was measured using SR. Our results show that this method can be used to perform advanced Mssbauer spectroscopy measurements owing to the excellent features of SR.
Tsukada, Kazuaki; Haba, Hiromitsu*; Asai, Masato; Toyoshima, Atsushi; Akiyama, Kazuhiko*; Kasamatsu, Yoshitaka; Nishinaka, Ichiro; Ichikawa, Shinichi; Yasuda, Kenichiro; Miyamoto, Yutaka; et al.
Radiochimica Acta, 97(2), p.83 - 89, 2009/02
Times Cited Count：21 Percentile：77.63(Chemistry, Inorganic & Nuclear)Anion-exchange chromatography of element 105, dubnium (Db), produced in the Cm(
F, 5n)
Db reaction is investigated together with the homologues Nb and Ta, and the pseudo-homologue Pa in 13.9 M hydrofluoric acid (HF) solution. The distribution coefficient (K
) of Db on an anion-exchange resin is successfully determined by running cycles of the 1702 chromatographic column separations. The result clearly indicates that the adsorption of Db on the resin is significantly different from that of the homologues and that the adsorption of anionic fluoro complexes of these elements decreases in the sequence of Ta 
Nb Db 
Pa.
Fe Mssbauer radiationMasuda, Ryo; Mitsui, Takaya; Kitao, Shinji*; Higashitaniguchi, Satoshi*; Yoda, Yoshitaka*; Seto, Makoto
Japanese Journal of Applied Physics, 47(10), p.8087 - 8090, 2008/10
Times Cited Count：12 Percentile：44.53(Physics, Applied)A synchrotron-radiation-based neV-resolution spectrometer has been developed using single-line pure nuclear Bragg reflection. The developed optical system consists of two components: a FeBO single crystal near the N
el temperature for producing Fe Mssbauer radiation from synchrotron radiation, and a single-line Mssbauer absorber (Fe-enriched stainless steel foil) for analyzing the energy distribution. As a feasibility study, we have performed the measurement of the Mssbauer radiation diffracted by a Si crystal under ultrasound vibration with the optical system and have successfully observed the neV-range energy modulation due to the ultrasound vibration.
