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Journal Articles

Nested antiferromagnetic spin fluctuations and non-Fermi-liquid behavior in electron-doped CeCo$$_{1-x}$$Ni$$_{x}$$In$$_5$$

Sakai, Hironori; Tokunaga, Yo; Kambe, Shinsaku; Zhu, J.-X.*; Ronning, F.*; Thompson, J. D.*; Kotegawa, Hisashi*; To, Hideki*; Suzuki, Kohei*; Oshima, Yoshiki*; et al.

Physical Review B, 106(23), p.235152_1 - 235152_8, 2022/12

 Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)

We investigate the electronic state of Ni-substituted CeCo$$_{1-x}$$Ni$$_x$$In$$_5$$ by nuclear quadrupole and magnetic resonance (NQR/NMR) techniques. The heavy fermion superconductivity below $$T_{rm c} = 2.3$$ K for $$x = 0$$ is suppressed by Ni substitutions, and $$T_{rm c}$$ reaches zero for $$x = 0.25$$. The $$^{115}$$In NQR spectra for $$x = 0.125$$ and 0.25 can be explained by simulating the electrical field gradient that is calculated for a virtual supercell with density functional theory. The spin-lattice relaxation rate $$1/T_1$$ indicates that Ni substitution weakens antiferromagnetic correlations that are not localized near the substituent but instead are uniform in space. The temperature ($$T$$) dependence of $$(T_1T)^{-1}$$ for $$x = 0.25$$ shows a maximum around $$T_{rm g} = 2$$ K and $$(T_1T)^{-1}$$ decreases toward almost zero when temperature is further reduced as if a gap might be opening in the magnetic excitation spectrum; however, the magnetic specific heat and the static magnetic susceptibility evolve smoothly through $$T_{rm g}$$ with a $$-ln T$$ dependence. The peculiar T dependence of $$(T_1T)^{-1}$$ and non-Fermi-liquid specific heat and susceptibility can be interpreted in a unified way by assuming nested antiferromagnetic spin fluctuations in a quasi-two-dimensional electronic system.

Journal Articles

Nanoscale heterogeneity induced by nonmagnetic Zn dopants in the quantum critical metal CeCoIn$$_5$$; $$^{115}$$In NQR/NMR and $$^{59}$$Co NMR study

Sakai, Hironori; Tokunaga, Yo; Kambe, Shinsaku; Zhu, J.-X.*; Ronning, F.*; Thompson, J. D.*; Ramakrishna, S. K.*; Reyes, A. P.*; Suzuki, Kohei*; Oshima, Yoshiki*; et al.

Physical Review B, 104(8), p.085106_1 - 085106_12, 2021/08

 Times Cited Count:3 Percentile:27.71(Materials Science, Multidisciplinary)

Antiferromagnetism in a prototypical quantum critical metal CeCoIn$$_5$$ is known to be induced by slight substitutions of non-magnetic Zn atoms for In. In nominally 7% Zn substituted CeCoIn$$_5$$, an antiferromagnetic (AFM) state coexists with heavy fermion superconductivity. Heterogeneity of the electronic states is investigated in Zn doped CeCoIn$$_5$$ by means of nuclear quadrupole and magnetic resonances (NQR and NMR). Site-dependent NQR relaxation rates $$1/T_1$$ indicate that the AFM state is locally nucleated around Zn substituents in the matrix of a heavy fermion state, and percolates through the bulk at the AFM transition temperature $$T_{rm N}$$. At lower temperatures, an anisotropic superconducting (SC) gap below the SC transition temperature $$T_{rm c}$$, and the SC state permeates through the AFM regions via a SC proximity effect. Applying an external magnetic field induces a spin-flop transition near 5 T, reducing the volume of the AFM regions. Consequently, a short ranged inhomogeneous AFM state survives and coexists with a paramagnetic Fermi liquid state at high fields.

Journal Articles

Spin polarized neutron scattering study on metal-insulator crossover in uranium dichalcogenide $$beta$$-US$$_{2}$$

Metoki, Naoto; Sakai, Hironori; Suzuki, Michito; Yamamoto, Etsuji; Haga, Yoshinori; Matsuda, Tatsuma; Ikeda, Shugo*

JPS Conference Proceedings (Internet), 3, p.013011_1 - 013011_6, 2014/06

Uranium chalcogenides are highly interesting because of the variety of the physical properties from 5$$f$$-based metal and Mott-Hibbard insulator. Especially dichalcogenide family exhibits a metal-insulator crossover depending on the chalcogenide elements, or under magnetic field and pressure. In this talk we present a recent result of our neutron scattering study on uranium dichalcogenide, which demonstrates that the metal-insulator crossover is related to the change of 5$$f$$ character from localized to itinerant. The electronic structure related to this phenomenon is discussed based on the band calculation.

Journal Articles

Emergent antiferromagnetism out of the "hidden-order" state in URu$$_2$$Si$$_2$$; High magnetic field nuclear magnetic resonance to 40 T

Sakai, Hironori; Urbano, R. R.*; Tokunaga, Yo; Kambe, Shinsaku; Suzuki, Michito; Kuhns, P. L.*; Reyes, A. P.*; Tobash, P. H.*; Ronning, F.*; Bauer, E. D.*; et al.

Physical Review Letters, 112(23), p.236401_1 - 236401_5, 2014/06

 Times Cited Count:7 Percentile:49.06(Physics, Multidisciplinary)

Very high field $$^{29}$$Si-NMR measurements using a fully $$^{29}$$Si-enriched URu$$_2$$Si$$_2$$ single crystal were carried out in order to microscopically investigate the "hidden order" (HO) state and adjacent magnetic phases in the high field limit. At the lowest measured temperature of 0.4 K, a clear anomaly reflecting a Fermi surface instability near 22 T inside the HO state is detected by the $$^{29}$$Si shift, $$^{29}K_c$$. Moreover, a strong enhancement of $$^{29}K_c$$ develops near a critical field $$H_{rm c}simeq 35.6$$ T, and the $$^{29}$$Si-NMR signal disappears suddenly at $$H_{rm c}$$, indicating the total suppression of the HO state. Nevertheless, a weak and shifted $$^{29}$$Si-NMR signal reappears for fields higher than $$H_{rm c}$$ at 4.2 K, providing evidence for a magnetic structure within the magnetic phase caused by the Ising-type anisotropy of the uranium ordered moments.

Journal Articles

Hexavalent chromium reduction by an actinobacterium ${it Flexivirga alba}$ ST13$$^{rm T}$$ in the family ${it Dermacoccaceae}$

Sugiyama, Tomoyasu*; Sugito, Hironori*; Mamiya, Ko*; Suzuki, Yoshinori*; Ando, Katsuhiko*; Onuki, Toshihiko

Journal of Bioscience and Bioengineering, 113(3), p.367 - 371, 2012/03

 Times Cited Count:28 Percentile:67.71(Biotechnology & Applied Microbiology)

An isolated strain ${it Flexivirga alba}$ ST13$$^{rm T}$$ was examined for the reducing activity of hexavalent chromium (Cr(VI)). XANES analysis of the precipitate shows the presence of Cr(OH)$$_{3}$$, indicating the bacterial reduction of Cr(VI) to trivalent chromium (Cr(III)). The bacterial Cr(VI) reduction was more efficient in minimal medium supplemented with molasses than with glucose. These results strongly suggest that the isolate ${it F.alba}$ ST13$$^{rm T}$$ is a novel actinobacterium with Cr(VI) reducing activity that is stimulated by molasses.

Journal Articles

NMR determination of noncollinear antiferromagnetic structure in TbCoGa$$_5$$

Tokunaga, Yo; Saito, Yo*; Sakai, Hironori; Kambe, Shinsaku; Sanada, Naoyuki*; Watanuki, Ryuta*; Suzuki, Kazuya*; Kawasaki, Yu*; Kishimoto, Yutaka*

Physical Review B, 84(21), p.214403_1 - 214403_7, 2011/12

 Times Cited Count:8 Percentile:36.17(Materials Science, Multidisciplinary)

We report NMR studies of TbCoGa$$_5$$, which has the tetragonal HoCoGa$$_5$$ structure and exhibits two antiferromagnetic (AF) transitions at $$T_{rm N1}$$=36.2 K and $$T_{rm N2}$$=5.4 K. From a symmetry analysis of internal magnetic fields at orthorhombic Ga sites, we have successfully determined the magnetic structures in the AF-I ($$T_{rm N2}<T<T_{rm N1}$$) and AF-II ($$T<T_{rm N2}$$) phases. The AF-I phase is a collinear AF order with a propagation vector $$q=[1/2, 0, 1/2]$$ and ordered moments parallel to the [001] direction. In the AF-II phase, on the other hand, we found a non-collinear AF structure described by double propagation vectors $$q_1=[1/2, 0, 1/2]$$ and $$q_{2}=[0, 1/2, 1/2]$$, where the moments tilt away from the [001] direction toward [100], keeping a constant value along the [001] direction. In the context of these results we discuss the possible presence of magnetic frustration in this system.

Journal Articles

Local structure around Ge atoms in IV-VI ferromagnetic semiconductor Ge$$_{0.6}$$Mn$$_{0.4}$$Te by X-ray fluorescence holography

Happo, Naohisa*; Tekehara, Yuki*; Fujiwara, Makoto*; Tanaka, Koichi*; Semba, Shinya*; Hosokawa, Shinya*; Hayashi, Koichi*; Hu, W.; Suzuki, Motohiro*; Asada, Hironori*

e-Journal of Surface Science and Nanotechnology (Internet), 9, p.247 - 250, 2011/06

Journal Articles

Local structure around Mn atoms in IV-VI ferromagnetic semiconductor Ge$$_{0.6}$$Mn$$_{0.4}$$Te investigated by X-ray fluorescence holography

Happo, Naohisa*; Tekehara, Yuki*; Fujiwara, Makoto*; Tanaka, Koichi*; Semba, Shinya*; Hosokawa, Shinya*; Hayashi, Koichi*; Hu, W.; Suzuki, Motohiro*; Asada, Hironori*

Japanese Journal of Applied Physics, 50(5), p.05FC11_1 - 05FC11_2, 2011/05

 Times Cited Count:5 Percentile:23.4(Physics, Applied)

Journal Articles

Investigation of irradiation conditions for recurrent breast cancer in JRR-4

Horiguchi, Hironori; Nakamura, Takemi; Kumada, Hiroaki*; Yanagie, Hironobu*; Suzuki, Minoru*; Sagawa, Hisashi

Proceedings of 14th International Congress on Neutron Capture Therapy (ICNCT-14) (CD-ROM), p.234 - 237, 2010/10

Recurrent breast cancer has been considered the application for boron neutron capture therapy using the JRR-4. The investigation of irradiation conditions for the recurrent breast cancer was performed by simulation with the JCDS. We performed the preliminary dosimetry of the model to verify the efficient irradiation conditions such as the neutron energy modes and multiple field technique. From the result, when the 30 Gy-Eq dose as minimum dose was delivered to the cancers, comparable dose distribution was delivered at the healthy tissues by both a one-port irradiation from anterior direction and a two-port irradiation from tangential direction. We revealed that the two-port irradiation was not valid to reduce the healthy tissues dose due to the isotopic scattering of neutrons in the body. We concluded that the optimal irradiation condition was the one-port irradiation with thermal neutron beam mode in terms of less healthy tissues dose and shorter irradiation time.

Journal Articles

La substitution effect and hyperfine-enhanced $$^{141}$$Pr nuclear spin dynamics in PrPb$$_3$$; $$^{139}$$La NMR study in Pr$$_{0.97}$$La$$_{0.03}$$Pb$$_3$$

Tokunaga, Yo; Sakai, Hironori; Chudo, Hiroyuki; Kambe, Shinsaku; Yasuoka, Hiroshi; Suzuki, Hiroyuki*; Walstedt, R. E.*; Homma, Yoshiya*; Aoki, Dai*; Shiokawa, Yoshinobu*

Physical Review B, 82(10), p.104401_1 - 104401_6, 2010/09

 Times Cited Count:5 Percentile:26.3(Materials Science, Multidisciplinary)

$$^{139}$$La NMR studies have been performed on PrPb$$_3$$ substituted with 3% La. The temperature dependence of the local magnetic susceptibility around La ions has been extracted from the $$^{139}$$La Knight shift. These data show that the non-magnetic $$Gamma_3$$ crystalline-electric-field (CEF) ground state (GS) is preserved even at the nearest neighboring Pr ions, although their CEF level scheme is slightly modified due to the La substitution. On the other hand, the temperature dependence of the nuclear spin-lattice relaxation rate $$1/T_1$$ is found to be well reproduced by assuming the same CEF level scheme over a wide temperature range. However, $$1/T_1$$ shows a strong upturn below 10 K, which is not expected from the non-magnetic CEF GS. We show that the low temperature anomaly can be quantitatively understood in terms of a cross-relaxation process between $$^{141}$$Pr and $$^{139}$$La nuclear spins.

Journal Articles

Formation of isotopically enriched silicon film from fluorosilane produced by isotopically selective infrared multiphoton dissociation

Oba, Hironori; Suzuki, Hiroshi*; Esaka, Fumitaka; Taguchi, Tomitsugu; Yamada, Yoichi; Yamamoto, Hiroyuki; Sasase, Masato*; Yokoyama, Atsushi

Journal of the Vacuum Society of Japan, 52(6), p.292 - 295, 2009/07

no abstracts in English

Journal Articles

Application of laser-accelerated protons to the demonstration of DNA double-strand breaks in human cancer cells

Yogo, Akifumi; Sato, Katsutoshi; Nishikino, Masaharu; Mori, Michiaki; Teshima, Teruki*; Numasaki, Hodaka*; Murakami, Masao*; Demizu, Yusuke*; Akagi, Takashi*; Nagayama, Shinichi*; et al.

Applied Physics Letters, 94(18), p.181502_1 - 181502_3, 2009/05

 Times Cited Count:110 Percentile:94.75(Physics, Applied)

Journal Articles

La-NMR study on a La dilute system of PrPb$$_3$$

Tokunaga, Yo; Suzuki, Hiroyuki*; Sakai, Hironori; Chudo, Hiroyuki; Kambe, Shinsaku; Yasuoka, Hiroshi; Homma, Yoshiya*; Aoki, Dai*; Shiokawa, Yoshinobu*

Journal of Physics; Conference Series, 150, p.042211_1 - 042211_4, 2009/00

 Times Cited Count:2 Percentile:74.15(Thermodynamics)

The first $$^{139}$$La-NMR measurement has been carried out on a La dilute system of PrPb$$_3$$. We have succeeded to detect $$^{139}$$La-NMR signal on a powder sample of Pr$$_{0.97}$$La$$_{0.03}$$Pb$$_3$$ and extracted the temperature dependence of the Knight shift $$^{139}K(T)$$ in a temperature range between 1.5 and 220 K. $$^{139}K(T)$$ has been found to maintain a linear relation with the bulk-susceptibility $$chi(T)^{rm bulk}$$ in wide temperature range, except for a small deviation in the temperature region below 6 K. The slopes of the $$^{139}K$$ vs $$chi^{rm bulk}$$ plots yield for the hyperfine coupling constants $$A_{rm hf}$$ the value 375 Oe/$$mu _B$$. From the NMR results, we discuss the effect of the La substitutions on microscopic magnetic properties of PrPb$$_3$$.

Journal Articles

Structural phase transition in the spin gap system YbAl$$_3$$C$$_3$$

Matsumura, Takeshi*; Inami, Toshiya; Kosaka, Masashi*; Kato, Yoshiaki*; Inukai, Takaki*; Ochiai, Akira*; Nakao, Hironori*; Murakami, Yoichi*; Katano, Susumu*; Suzuki, Hiroyuki*

Journal of the Physical Society of Japan, 77(10), p.103601_1 - 103601_4, 2008/10

 Times Cited Count:14 Percentile:62.95(Physics, Multidisciplinary)

Journal Articles

Gamow-Teller decay of the $$T=1$$ nucleus $$^{46}$$Cr

Onishi, Takeo*; Gelberg, A.*; Sakurai, Hiroyoshi*; Yoneda, Kenichiro*; Aoi, Nori*; Imai, Nobuaki*; Baba, Hidetada*; Von Brentano, P.*; Fukuda, Naoki*; Ichikawa, Yuichi*; et al.

Physical Review C, 72(2), p.024308_1 - 024308_7, 2005/08

 Times Cited Count:21 Percentile:77.65(Physics, Nuclear)

no abstracts in English

Journal Articles

Exchange of tritium implanted into oxide ceramics for protium by exposure to air vapors at room temperature

Morita, Kenji*; Suzuki, Hironori*; Soda, Kazuo*; Iwahara, Hiroiku*; Nakamura, Hirofumi; Hayashi, Takumi; Nishi, Masataka

Journal of Nuclear Materials, 307-311(2), p.1461 - 1465, 2002/12

 Times Cited Count:2 Percentile:17.03(Materials Science, Multidisciplinary)

no abstracts in English

Oral presentation

DMFC performance of crosslinked fluoropolymer electrolyte membranes

Yamaki, Tetsuya; Kawahito, Shimpei; Sawada, Shinichi; Asano, Masaharu; Ishiguro, Hironori*; Mohammad Ali, A.*; Nakagawa, Nobuyoshi*; Suzuki, Akihiro*; Terai, Takayuki*; Maekawa, Yasunari

no journal, , 

no abstracts in English

Oral presentation

DMFC performance of crosslinked-polytetrafluoroethylene electrolyte membranes

Yamaki, Tetsuya; Kawahito, Shimpei; Sawada, Shinichi; Asano, Masaharu; Ishiguro, Hironori*; Mohammad Ali, A.*; Nakagawa, Nobuyoshi*; Suzuki, Akihiro*; Terai, Takayuki*

no journal, , 

no abstracts in English

Oral presentation

Comparison between actual dose and calculated dose for verification of the adequacy of computation models for BNCT applied to lung tumor

Komeda, Masao; Horiguchi, Hironori; Yamamoto, Kazuyoshi; Kumada, Hiroaki; Suzuki, Minoru*

no journal, , 

no abstracts in English

Oral presentation

NMR study of quadrupole ordering and magnetic excitations in Pr$$_{1-x}$$La$$_x$$Pb$$_3$$

Tokunaga, Yo; Suzuki, Hiroyuki*; Sakai, Hironori; Kambe, Shinsaku; Chudo, Hiroyuki; Homma, Yoshiya*; Aoki, Dai*; Shiokawa, Yoshinobu*

no journal, , 

no abstracts in English

38 (Records 1-20 displayed on this page)