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Journal Articles

Oxygen reduction activity and interfacial structures of La$$_{0.8}$$Sr$$_{0.2}$$CoO$$_{3}$$ at initial electrochemical process in an alkaline solution

Matsuzaki, Akira*; Hirayama, Masaaki*; Oguchi, Shoya*; Komo, Mamoru*; Ikezawa, Atsunori*; Suzuki, Kota*; Tamura, Kazuhisa; Arai, Hajime*; Kanno, Ryoji*

Electrochemistry (Internet), 90(10), p.107001_1 - 107001_8, 2022/10

 Times Cited Count:0 Percentile:0.01(Electrochemistry)

Oxygen reduction and evolution reactions (ORR and OER) of perovskite-type La$$_{0.8}$$Sr$$_{0.2}$$CoO$$_{3}$$ were characterized using two-dimensional model electrodes with different reaction planes. Synthesized by pulsed laser deposition, these thin and flat electrodes can reveal the reaction plane dependence of the ORR activity. From steady-state polarization measurements in KOH (aq.), the ORR activity was the highest on the (001) film during the first ORR/OER cycle, and it decreased significantly during the second cycle. In-situ synchrotron X-ray diffraction clarified crystal structure changes in the bulk and surface regions of La$$_{0.8}$$Sr$$_{0.2}$$CoO$$_{3}$$, and these changes are associated with forming oxygen defects during the initial electrochemical process. Furthermore, the La$$_{0.8}$$Sr$$_{0.2}$$CoO$$_{3}$$ surface partially decomposed upon reacting. Therefore, the interfacial structures formed in the electrochemical reaction field is important for enhancing ORR and OER activities.

Journal Articles

$$omega N$$ scattering length from $$omega$$ photoproduction on the proton near the reaction threshold

Ishikawa, Takatsugu*; Fujimura, Hisako*; Fukasawa, Hiroshi*; Hashimoto, Ryo*; He, Q.*; Honda, Yuki*; Hosaka, Atsushi; Iwata, Takahiro*; Kaida, Shun*; Kasagi, Jirota*; et al.

Physical Review C, 101(5), p.052201_1 - 052201_6, 2020/05

Journal Articles

Synthesis of new perovskite-type oxyfluorides, BaInO$$_{2}$$F and comparison of the structure among perovskite-type oxyfluorides

Katsumata, Tetsuhiro*; Suzuki, Ryo*; Sato, Naoto*; Suzuki, Shumpei*; Nakashima, Mamoru*; Inaguma, Yoshiyuki*; Mori, Daisuke*; Aimi, Akihisa*; Yoneda, Yasuhiro

Journal of Solid State Chemistry, 279, p.120919_1 - 120919_8, 2019/11

 Times Cited Count:7 Percentile:48.4(Chemistry, Inorganic & Nuclear)

Journal Articles

High-resolution crystal structure of copper amine oxidase from ${it Arthrobacter globiformis}$; Assignment of bound diatomic molecules as O$$_{2}$$

Murakawa, Takeshi*; Hayashi, Hideyuki*; Sunami, Tomoko; Kurihara, Kazuo; Tamada, Taro; Kuroki, Ryota; Suzuki, Mamoru*; Tanizawa, Katsuyuki*; Okajima, Toshihide*

Acta Crystallographica Section D, 69(12), p.2483 - 2494, 2013/12

 Times Cited Count:13 Percentile:68.93(Biochemical Research Methods)

The crystal structure of a Cu amine oxidase from ${it Arthrobacter globiformis}$ was determined at 1.08 ${AA}$ resolution with the use of low-molecular-weight polyethylene glycol (LMW PEG; average molecular weight $$sim$$200) as a cryoprotectant. The final crystallographic $$R$$-factor and $$R$$$$_{rm free}$$ value are 13.0% and 15.0%, respectively. Several molecules of LMW PEG were found to occupy cavities in the protein interior including the active site, which resulted in the marked reduction of the overall ${it B}$ factor and consequently led to a sub-atomic resolution structure for a relatively large protein with a monomer molecular weight of $$sim$$70,000. About 40% of all the presumed hydrogen atoms were observed as clear electron densities in the $$F$$$$_{rm o}$$ - $$F$$$$_{rm c}$$ difference map. Multiple minor conformers were also identified for many residues. Anisotropic displacement fluctuations were evaluated in the active site that contains a post-translationally derived quinone cofactor and a Cu atom. Furthermore, diatomic molecules, most likely molecular oxygen, are bound to the protein, one of which is located in the region that has been previously proposed as an entry route for the substrate dioxygen from the central cavity of the dimer interface to the active site.

Journal Articles

MeV- and sub-MeV-photon sources based on Compton backscattering at SPring-8 and KPSI-JAEA

Kawase, Keigo; Kando, Masaki; Hayakawa, Takehito; Daito, Izuru; Kondo, Shuji; Homma, Takayuki; Kameshima, Takashi; Kotaki, Hideyuki; Chen, L.*; Fukuda, Yuji; et al.

Nuclear Physics Review, 26(Suppl.), p.94 - 99, 2009/07

We constructed MeV- and sub-MeV-photon sources by means of Compton backscattering with a laser light and an electron beam at SPring-8 and KPSI-JAEA. MeV-photon source consists of a continuous-wave optically-pumped far infrared laser and an 8-GeV stored electron beam. Sub-MeV-photon source consists of a Nd:YAG pulse-laser and an 150-MeV electron beam accelerated by a microtron. Both source have been succeeded backscattered photon generation. In this talk, I will present characteristics and future prospects of these photon sources.

Journal Articles

Nano-particle materials prepared from a synthetic antigenic sequence of ${it plasmodium falciparum}$ enolase

Oku, Hiroyuki*; Yamada, Keiichi*; Kobayashi, Kyoko*; Katakai, Ryoichi*; Ashfaq, M.*; Hanaoka, Hirofumi*; Iida, Yasuhiko*; Endo, Keigo*; Hasegawa, Shin; Maekawa, Yasunari; et al.

Peptide Science 2008, p.439 - 442, 2009/03

Malaria is the major cause of mortality and morbidity in the tropical and subtropical regions in the world. Our previous studies have shown that a series of partial peptides of a Plasmodium falciparum enolase have antigenic reactivity against patients' sera. In this paper, we wish to report nano-encapsulation of a synthetic antigen into bioabsorbable polymer particles and their releasing studies in vitro and in vivo.

Journal Articles

MeV $$gamma$$-ray generation from backward Compton scattering at SPring-8

Kawase, Keigo; Arimoto, Yasushi*; Fujiwara, Mamoru; Okajima, Shigeki*; Shoji, Masazumi*; Suzuki, Shinsuke*; Tamura, Kazuhiro*; Yorita, Tetsuhiko*; Okuma, Haruo*

Nuclear Instruments and Methods in Physics Research A, 592(3), p.154 - 161, 2008/07

 Times Cited Count:20 Percentile:77.77(Instruments & Instrumentation)

A test experimental line at SPring-8 has been constructed for the generation of backward Compton scattered (BCS) $$gamma$$-ray by head-on collision between an 8 GeV electron beam and a far-infrared (FIR) laser. For the FIR laser, we use a continuous-wave methanol laser optically pumped by a carbon dioxide ($${rm CO}_{2}$$) laser. The FIR laser output power achieved is 1.6 W at maximum for 118.8 $$mu$$m lasing; this value is the highest in the case of this type of laser. As a result of the direct measurement, the generated BCS $$gamma$$-ray flux was found to be about $$10^{3}$$ photons/s. This value is consistent with the estimation calculated by taking into account the input laser power and the transmittance of the laser transport system.

Journal Articles

Overview of national centralized tokamak program; Mission, design and strategy to contribute ITER and DEMO

Ninomiya, Hiromasa; Akiba, Masato; Fujii, Tsuneyuki; Fujita, Takaaki; Fujiwara, Masami*; Hamamatsu, Kiyotaka; Hayashi, Nobuhiko; Hosogane, Nobuyuki; Ikeda, Yoshitaka; Inoue, Nobuyuki; et al.

Journal of the Korean Physical Society, 49, p.S428 - S432, 2006/12

To contribute DEMO and ITER, the design to modify the present JT-60U into superconducting coil machine, named National Centralized Tokamak (NCT), is being progressed under nationwide collaborations in Japan. Mission, design and strategy of this NCT program is summarized.

Journal Articles

Overview of the national centralized tokamak programme

Kikuchi, Mitsuru; Tamai, Hiroshi; Matsukawa, Makoto; Fujita, Takaaki; Takase, Yuichi*; Sakurai, Shinji; Kizu, Kaname; Tsuchiya, Katsuhiko; Kurita, Genichi; Morioka, Atsuhiko; et al.

Nuclear Fusion, 46(3), p.S29 - S38, 2006/03

 Times Cited Count:13 Percentile:41.84(Physics, Fluids & Plasmas)

The National Centralized Tokamak (NCT) facility program is a domestic research program for advanced tokamak research to succeed JT-60U incorporating Japanese university accomplishments. The mission of NCT is to establish high beta steady-state operation for DEMO and to contribute to ITER. The machine flexibility and mobility is pursued in aspect ratio and shape controllability, feedback control of resistive wall modes, wide current and pressure profile control capability for the demonstration of the high-b steady state.

Journal Articles

Engineering design and control scenario for steady-state high-beta operation in national centralized tokamak

Tsuchiya, Katsuhiko; Akiba, Masato; Azechi, Hiroshi*; Fujii, Tsuneyuki; Fujita, Takaaki; Fujiwara, Masami*; Hamamatsu, Kiyotaka; Hashizume, Hidetoshi*; Hayashi, Nobuhiko; Horiike, Hiroshi*; et al.

Fusion Engineering and Design, 81(8-14), p.1599 - 1605, 2006/02

 Times Cited Count:1 Percentile:9.98(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Design study of national centralized tokamak facility for the demonstration of steady state high-$$beta$$ plasma operation

Tamai, Hiroshi; Akiba, Masato; Azechi, Hiroshi*; Fujita, Takaaki; Hamamatsu, Kiyotaka; Hashizume, Hidetoshi*; Hayashi, Nobuhiko; Horiike, Hiroshi*; Hosogane, Nobuyuki; Ichimura, Makoto*; et al.

Nuclear Fusion, 45(12), p.1676 - 1683, 2005/12

 Times Cited Count:15 Percentile:45.55(Physics, Fluids & Plasmas)

Design studies are shown on the National Centralized Tokamak facility. The machine design is carried out to investigate the capability for the flexibility in aspect ratio and shape controllability for the demonstration of the high-beta steady state operation with nation-wide collaboration, in parallel with ITER towards DEMO. Two designs are proposed and assessed with respect to the physics requirements such as confinement, stability, current drive, divertor, and energetic particle confinement. The operation range in the aspect ratio and the plasma shape is widely enhanced in consistent with the sufficient divertor pumping. Evaluations of the plasma performance towards the determination of machine design are presented.

JAEA Reports

Feasibility Study on Commercialization of Fast Breeder Reactor Cycle Systems Interim Report of Phase II; Technical Study Report for Reactor Plant Systems

Konomura, Mamoru; Ogawa, Takashi; Okano, Yasushi; Yamaguchi, Hiroyuki; Murakami, Tsutomu; Takaki, Naoyuki; Nishiguchi, Youhei; Sugino, Kazuteru; Naganuma, Masayuki; Hishida, Masahiko; et al.

JNC TN9400 2004-035, 2071 Pages, 2004/06

JNC-TN9400-2004-035.pdf:76.42MB

The attractive concepts for Sodium-, lead-bismuth-, helium- and water-cooled FBRs have been created through using typical plant features and employing advanced technologies. Efforts on evaluating technological prospects of feasibility have been paid for these concepts. Also, it was comfirmed if these concepts satisfy design requierments of capability and performance presumed in the feasibilty study on commertialization of Fast Breeder Reactor Systems. As results, it was concluded that the selection of sodium-cooled reactor was most rational for practical use of FBR technologies in 2015.

Journal Articles

Progress in physics and technology developments for the modification of JT-60

Tamai, Hiroshi; Matsukawa, Makoto; Kurita, Genichi; Hayashi, Nobuhiko; Urata, Kazuhiro*; Miura, Yushi; Kizu, Kaname; Tsuchiya, Katsuhiko; Morioka, Atsuhiko; Kudo, Yusuke; et al.

Plasma Science and Technology, 6(1), p.2141 - 2150, 2004/02

 Times Cited Count:2 Percentile:6.52(Physics, Fluids & Plasmas)

The dominant issue for the the modification program of JT-60 (JT-60SC) is to demonstrate the steady state reactor relevant plasma operation. Physics design on plasma parameters, operation scenarios, and the plasma control method are investigated for the achievement of high-$$beta$$. Engineering design and the R&D on the superconducting magnet coils, radiation shield, and vacuum vessel are performed. Recent progress in such physics and technology developments is presented.

Journal Articles

Noninductive current drive and steady-state operation in JT-60U

Ushigusa, Kenkichi; Ide, Shunsuke; Oikawa, Toshihiro; Suzuki, Takahiro; Kamada, Yutaka; Fujita, Takaaki; Ikeda, Yoshitaka; Naito, Osamu; Matsuoka, Mamoru*; Kondoh, Takashi; et al.

Fusion Science and Technology (JT-60 Special Issue), 42(2-3), p.255 - 277, 2002/09

 Times Cited Count:8 Percentile:12.12(Nuclear Science & Technology)

Studies on non-inductive current drive and development of an integrated steady-state high performance operation in JT-60 are reviewed. Experiments on lower hybrid current drive in JT-60 haven shown a large non-inductive current up to 3.5MA, high current drive efficiency of 3.6x1019m-2A/W. Basic studies on LH waves in JT-60 have contributed to understand current drive physics. Significant progress in neutral beam current drive has been made in JT-60 by testing the performance of negative ion based NBI (N-NBI). The CD efficiency of ~1.5x1019m-2A /W, and N-NB driven current of ~1MA have been demonstrated in N-NBCD. Strongly localized driven current by electron cyclotron current drive was identified with a fundamental O-mode scheme. Efficiency of 0.5x1019m-2A/W and EC driven current of 0.2MA were achieved and suppression of neo-classical tearing mode was demonstrated. Based on these developments, two integrated steady-state operation scenarios were developed in JT-60, which are reversed magnetic shear (R/S) plasmas and high bp ELMy H-mode. In these operation regimes, discharges have been sustained near the steady-state current profile under full non-inductive current drive. High performance plasmas with a high nDotETio and at high normalized density were also produced under fully non-inductive condition in high bp ELMy H-mode and R/S mode.

Journal Articles

Development of a large D$$^{-}$$ ion source for the JT-60U negative-ion-based neutral beam injector

Okumura, Yoshikazu; Hanada, Masaya; Inoue, Takashi; Kuriyama, Masaaki; Maeno, Shuichi*; Matsuoka, Mamoru; Miyamoto, Kenji; Mizuno, Makoto; Ohara, Yoshihiro; Suzuki, Satoshi; et al.

Proceedings of 15th IEEE/NPSS Symposium on Fusion Engineering, p.466 - 469, 1993/00

no abstracts in English

JAEA Reports

Irradiation Test of Shielding Material for Fast Reactor JMTR-SH (I) (71M-84P)

Suzuki, Kazuhisa; Yamanouchi, Sadamu; Tani, Satoshi; Ichige, Akio; Naito, Takeshi; Harada, Mamoru; Ito, Masahiko; Osugi, Shoichi*; Shibata, Kenichi*

PNC TN951 76-05, 70 Pages, 1976/03

PNC-TN951-76-05.pdf:4.4MB

The serpentine concentrate in which two kinds of cement were used as a binder was irradiated in JMTR to the fast neutron fluence -1.7$$times$$$$^{19}$$ n/cm$$^{2}$$ (E$$>$$1Mev) and thermal neutron fluence -1.5$$times$$10$$^{20}$$ n/cm$$^{2}$$. Ave-rage irradiation temperature was estimated to be 200$$^{circ}C$$. Prior to the postirradiation examination, effect of thermal history was investigated in out-of-pile test. The integrity of specimens were kept after irradiation. From the results of thermal history examination and the post-irradiation examination, it was clearly noticed that the changes occuring in dimensions, weight and compressive strength were caused mainly by the thermal effect. The change in the Young's modulus seemed to be caused by the effect of both heating and neutron irradiation. It wasconcluded that the ordinary portland cement with the serpentine concrete is better than that of almina cement.

Oral presentation

Development of treatment for low radioactive effluent in Tokai Reprocessing Plant, 14; Study of Cs/Sr adsorption process by two linked column experiment

Takano, Masato; Ito, Yoshiyuki; Suzuki, Tatsuya*; Takimoto, Mayumi*; Matsukura, Minoru*; Mimura, Hitoshi*; Mori, Koichi*; Iwasaki, Mamoru*

no journal, , 

no abstracts in English

Patent

高周波加熱式焼却炉

鈴木 達也; 堂野前 寧; 原田 守

松本 武志*; 角田 俊也*; 佐藤 康士*

JP, 2010-005130  Patent licensing information  Patent publication (In Japanese)

【課題】廃棄物の高周波加熱を促進し、効率よく焼却処理を行えるようにし、しかも焼却筒の長寿命化を図ることができるようにする。また、廃棄物が破砕したプレス缶と可燃物の混合物であっても、高周波加熱による焼却処理の際にプレス缶同士の固着が生じず、そのため、再破砕などの後処理工程を要しないようにする。 【解決手段】高周波加熱装置10の内部に焼却器12が装着されており、該焼却器は、非磁性材料からなる焼却筒18と、該焼却筒を受ける焼却筒受け皿20と、前記焼却筒内に組み込まれている火格子22を備え、該火格子上に位置する廃棄物Wを高周波加熱により焼却し、火格子から落下する焼却灰を焼却筒受け皿で受ける構造であって、焼却筒内の火格子の下方に、強磁性の導電性材料からなり、落下する焼却灰を通過させる複数の空隙を備えた加熱促進体28が設置されている。

18 (Records 1-18 displayed on this page)
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