Assessment of hydrogen embrittlement behavior in Al-Zn-Mg alloy through multi-modal 3D image-based simulation

Fujihara, Hiro*; Toda, Hiroyuki*; Ebihara, Kenichi; Kobayashi, Masakazu*; Mayama, Tsuyoshi*; Hirayama, Kyosuke*; Shimizu, Kazuyuki*; Takeuchi, Akihisa*; Uesugi, Masayuki*

International Journal of Plasticity, 174, p.103897_1 - 103897_22, 2024/03

https://doi.org/10.1016/j.ijplas.2024.103897

Hydrogen(H) embrittlement in high-strength aluminum(Al) alloys is a crucial problem. H accumulation at the interface of precipitates in Al alloy is considered to cause embrittlement. However, there is no quantitative knowledge regarding the interaction between H distribution and stress field near cracks. In this study, using a multi-modal three-dimensional image-based simulation combining the crystal plasticity finite element method and H diffusion analysis, we tried to capture the stress distribution near the crack, its influence on the H distribution, and the probability of crack initiation in the experimental condition. As a result, it was found that grain boundary cracks transition to quasi-cleavage cracks in the region where the cohesive energy of the semi-coherent interface of MgZn precipitates decreases due to H accumulation near the tip. We believe the present simulation method successfully bridges nanoscale delamination and macroscale brittle fracture.

Results of environmental impact investigations as part of environmental monitoring investigation in backfilling of shafts and tunnels of Mizunami Underground Research Laboratory (2022)

Takeuchi, Ryuji; Nishio, Kazuhisa*; Kokubu, Yoko

JAEA-Data/Code 2023-013, 74 Pages, 2024/01

JAEA-Data-Code-2023-013.pdf:4.2MB

The Tono Geoscience Center of Japan Atomic Energy Agency (JAEA) has been conducting the environmental monitoring investigation to confirm the environmental impacts associated with the backfilling of shafts and tunnels at the Mizunami Underground Research Laboratory (MIU). This report summarizes the results of the environmental impact investigations conducted as part of the environmental monitoring investigation around the MIU Site in FY2022, which include groundwater level measurement in wells, river flow rate measurement, water analysis of Hazama river, noise and vibration surveys, and soil survey.

Effect of dissolved oxygen concentration on dynamic strain aging and stress corrosion cracking of SUS304 stainless steel under high temperature pressurized water

Hirota, Noriaki; Nakano, Hiroko; Fujita, Yoshitaka; Takeuchi, Tomoaki; Tsuchiya, Kunihiko; Demura, Masahiko*; Kobayashi, Yoshinao*

The IV International Scientific Forum "Nuclear Science and Technologies"; AIP Conference Proceedings 3020, p.030007_1 - 030007_6, 2024/01

https://doi.org/10.1063/5.0192888

Dynamic strain aging (DSA) and intergranular stress corrosion cracking (intragranular SCC) occur in high temperature pressurized water simulating a boiling water reactor environment due to changes in dissolved oxygen (DO) content, respectively. In order to clearly understand the difference between these phenomena, the mechanism of their occurrence was summarized. As a result, it was found that DSA due to intragranular cracking occurred in SUS304 stainless steel at low DO 1 ppb, while DSA was suppressed at DO 100 to 8500 ppb due to the formation of oxide films on the surface. On the other hand, when DO was increased to 20000 ppb, the film was peeled from the matrix, O element diffused to the grain boundary of the matrix, resulting in intergranular SCC. These results are indicated that the optimum DO concentration must be adjusted to suppress crack initiation due to DSA and intergranular SCC.

Estimation of future caesium-137 flux through river using climate change scenarios

Irisawa, Ayumi*; Sakuma, Kazuyuki; Takeuchi, Yukio*; Taniguchi, Keisuke*; Onda, Yuichi*

KEK Proceedings 2023-2, p.29 - 33, 2023/11

no abstracts in English

Ion beam induced luminescence analysis of europium complexes in styrene-divinylbenzene copolymer-coated spherical silica by proton and argon ion beams irradiation

Nakahara, Masaumi; Watanabe, So; Takeuchi, Masayuki; Yuyama, Takahiro*; Ishizaka, Tomohisa*; Ishii, Yasuyuki*; Yamagata, Ryohei*; Yamada, Naoto*; Koka, Masashi*; Kada, Wataru*; et al.

Nuclear Instruments and Methods in Physics Research B, 542, p.144 - 150, 2023/09

https://doi.org/10.1016/j.nimb.2023.06.012

The structures of Eu complexes in the adsorbents prepared with various extractants were evaluated by ion beam induced luminescence analysis in an extraction chromatography for minor actinides recovery. The luminescence of Eu was measured with a proton beam obtained from the single-ended accelerator and an argon ion beam obtained from the azimuthally varying field cyclotron in Takasaki Ion Accelerators for Advanced Radiation Application in National Institutes for Quantum Science and Technology. In this study, it was confirmed that the spectral shape of Eu complexes in the adsorbents varied depending on the kinds of extractants, and the correlation between the change in the spectra and the structures of Eu complexes was investigated.

Experiences in dismantlement of gloveboxes for wet recovery and other use that are contaminated with nuclear fuel materials

Kitamura, Akihiro; Hirano, Hiroshi*; Yoshida, Masato; Takeuchi, Kentaro

Hoken Butsuri (Internet), 58(2), p.76 - 90, 2023/08

https://doi.org/10.5453/jhps.58.76

The alpha contaminated gloveboxes have been dismantled for over 20 years in Plutonium Fuel Fabrication Facility. The so called wet recovery equipment gloveboxes, which recover plutonium and uranium from scrap fuel by dissolving and extracting processes, were chosen as the priority gloveboxes to be dismantled. These gloveboxes and other gloveboxes in the same room were size reduced and removed up until 2022. Also, non-radioactive ancillary facility and non-radioactive giant glovebox were removed from 2007 to 2010 for ease of glovebox dismantling activities that follows and for making waste storage spaces. Several incidents were occurred and recidivism prevention measures were implemented on each occasion. In this report, glovebox dismantling activities we conducted in the past 20 years are reviewed and lessons we have learned are summarized.

Level structures of Ca cast doubt on a doubly magic Ca

Chen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; Tsunoda, Yusuke*; Otsuka, Takaharu*; Chazono, Yoshiki*; Hagen, G.*; Holt, J. D.*; et al.

Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08

https://doi.org/10.1016/j.physletb.2023.138025

Gamma decays were observed in Ca and Ca following quasi-free one-proton knockout reactions from Sc. For Ca, a ray transition was measured to be 1456(12) keV, while for Ca an indication for a transition was observed at 1115(34) keV. Both transitions were tentatively assigned as the decays. A shell-model calculation in a wide model space with a marginally modified effective nucleon-nucleon interaction depicts excellent agreement with experiment for level energies, two-neutron separation energies, and reaction cross sections, corroborating the formation of a new nuclear shell above the N = 34 shell. Its constituents, the and orbitals, are almost degenerate. This degeneracy precludes the possibility for a doubly magic Ca and potentially drives the dripline of Ca isotopes to Ca or even beyond.

Report of backfilling and restoration works in the Mizunami Underground Research Laboratory

Takeuchi, Ryuji; Mikake, Shinichiro; Ikeda, Koki; Nishio, Kazuhisa*; Kokubu, Yoko; Hanamuro, Takahiro

JAEA-Review 2023-007, 114 Pages, 2023/07

JAEA-Review-2023-007.pdf:12.02MB

Japan Atomic Energy Agency (JAEA) at Tono Geoscience Center has been conducting the Mizunami Underground Research Laboratory (MIU) Project to enhance the reliability of geological disposal technologies through investigations of the deep geological environment in the crystalline rock (granite) at Mizunami City, Gifu Prefecture, central Japan since fiscal year 1996. Backfilling and restoration works in the MIU site have been being conducted based on "the MIU Project from FY2020 onwards" which is defined the way forward of backfilling and restoration works and environmental monitoring investigations in the MIU site, since fiscal year 2020. This report summarizes the outline, process, and achievements of the construction and the safety patrol of the backfilling and restoration works in the MIU site performed from May 16, 2020 to January 16, 2022.

Fuel unloading work in decommissioning of the prototype fast breeder reactor Monju; First stage of Monju decommissioning project

Shiota, Yuki; Kudo, Junki; Tsuno, Hiromi; Takeuchi, Ryotaro; Ariyoshi, Hideo; Shiohama, Yasutaka; Hamano, Tomoharu; Takagi, Tsuyohiko; Nagaoki, Yoshihiro

JAEA-Technology 2023-002, 87 Pages, 2023/06

JAEA-Technology-2023-002.pdf:8.53MB

In the first stage of Monju decommissioning project, fuel unload work began to be carried out. There are two tasks in this work. One is Fuel Treatment and Storage work that gets rid of sodium on the fuel assemblies unloaded from Ex-Vessel fuel Storage Tank (EVST) and carries it in the storage pool, and the other is Fuel Unloading that the fuel assemblies in the reactor core is replaced with dummy fuels and stored in EVST. Fuel Treatment and Storage work and Fuel Unloading work are performed alternately, and 370 fuel assemblies in the core and 160 fuel assemblies in EVST are all carried to the storage pool. Monju had a large amount of sodium in the reactor vessel and EVST, and there was a residual risk of fuel failure due to the superposition of a large scale sodium fire. Therefore, in the first stage of the Monju decommissioning project, it was decided to take about 5.5 years to remove the residual risk by storing all the fuel rods in the fuel storage pool. There are few Fuel handling system of Sodium Fast Reactor in the world, so the driving record and experience are not enough. So, events that occur even if taken measure are assumed. The following three events apply to this; first, events that are difficult to prevent, events. Second, that are due to lack of experience, and final, events optimization of system is not enough. Plans were taken to suppress these events. This report summarizes the "Monju decommissioning project" work conducted so far in all four campaigns.

Proposition of confirmation items on the borehole sealing for the disposal of radioactive waste

Murakami, Hiroaki; Nishiyama, Nariaki; Takeuchi, Ryuji; Iwatsuki, Teruki

Oyo Chishitsu, 64(2), p.60 - 69, 2023/06

https://doi.org/10.5110/jjseg.64.60

In order to confirm the quality control items for borehole closure in radioactive waste disposal projects, in-situ borehole sealing tests using bentonite material were conducted. As a result, the closure performance was successfully demonstrated by comparing the data of water injection tests conducted before and after the installation of the closure material. However, the breakthrough was observed after closing, probably due to high differential pressure applied to the seal section. Thus, it is important to ascertain throughout the entire operation that the borehole is adequately closed. The placement and specifications of the closure material should be determined according to the hydrogeological structure in the borehole. The confirmation items to use bentonite for sealing material are identified to be: to consider swelling and density loss in the borehole; to place the planned depth using appropriate emplacement technique; to be placed without damage to seals when use some backfilling materials, considering effect of permeability on adjacent seals.