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Journal Articles

Laser heating induced spatial homogenization of phase separated Na$$_{2}$$O-B$$_{2}$$O$$_{3}$$-SiO$$_{2}$$ glass plate with bearing NiO for heat center and structural probe

Tomita, Kana*; Kishi, Tetsuo*; Matsumura, Daiju; Yano, Tetsuji*

Journal of Non-Crystalline Solids, 597, p.121891_1 - 121891_10, 2022/12

 Times Cited Count:1 Percentile:14.66(Materials Science, Ceramics)

Journal Articles

Odd-parity autoionizing levels of uranium observed by two-color two-step photoionization optogalvanic spectroscopy

Miyabe, Masabumi; Satou, Yukihiko; Wakaida, Ikuo; Terabayashi, Ryohei*; Sonnenschein, V.*; Tomita, Hideki*; Zhao, Y.*; Sakamoto, Tetsuo*

Journal of Physics B; Atomic, Molecular and Optical Physics, 54(14), p.145003_1 - 145003_8, 2021/07

 Times Cited Count:0 Percentile:0.01(Optics)

Two-color two-step photoionization optogalvanic spectroscopy was performed using high-repetition-rate titanium sapphire lasers and a uranium hollow cathode lamp to find the two-step resonance ionization schemes of uranium. Many ionization transitions were observed by exciting uranium atoms in a ground state into five, even parity, excited levels with the first-step laser and by scanning the second-step laser wavelengths. By blocking the first-step laser, single-color, two-photon ionization transitions were also identified. From these results, we have found more than 50 odd-parity autoionizing levels of uranium in the energy, ranging from the ionization potential (49958.4 cm$$^{-1}$$) to 51150 cm$$^{-1}$$. The determined energy levels are within 1 cm$$^{-1}$$ of previously reported values.

Journal Articles

Measurement of niobium reaction rate for material surveillance tests in fast reactors

Ito, Chikara; Maeda, Shigetaka; Inoue, Toshihiko; Tomita, Hideki*; Iguchi, Tetsuo*

Radiation Protection, 40(6), p.491 - 495, 2020/11

A highly accurate and precise technique for measurement of the $$^{93}$$Nb(n,n')$$^{93m}$$Nb reaction rate was established for the material surveillance tests, etc. in fast reactors. The self-absorption effect on the measurement of the characteristic X-rays emitted by $$^{93m}$$Nb was decreased by the solution and evaporation to dryness of niobium dosimeter. A highly precise count of the number of $$^{93}$$Nb atoms was obtained by measuring the niobium solution concentration using inductively coupled plasma mass spectrometry. X-rays of $$^{93m}$$Nb were measured accurately by means of comparing the X-ray intensity of irradiated niobium solution with that of the solution in which stable $$^{93}$$Nb was added. The difference between both intensities indicates the effect of $$^{182}$$Ta, which is generated from an impurity tantalum, and the intensity of X-rays from $$^{93m}$$Nb was evaluated. Measurement error of the $$^{93}$$Nb(n,n')$$^{93m}$$Nb reaction rate was reduced to be less than 4%, which was equivalent to the other reaction rate errors of dosimeters used for Joyo dosimetry. In addition, an advanced technique using Resonance Ionization Mass Spectrometry was proposed for the precise measurement of $$^{93m}$$Nb yield, and $$^{93m}$$Nb will be resonance-ionized selectively by discriminating the hyperfine splitting of the atomic energy levels between $$^{93}$$Nb and $$^{93m}$$Nb at high resolution.

Journal Articles

An Experimental setup for creating and imaging $$^{4}$$He$$_{2}$$$$^{ast}$$ excimer cluster tracers in superfluid helium-4 via neutron-$$^{3}$$He absorption reaction

Sonnenschein, V.*; Tsuji, Yoshiyuki*; Kokuryu, Shoma*; Kubo, Wataru*; Suzuki, So*; Tomita, Hideki*; Kiyanagi, Yoshiaki*; Iguchi, Tetsuo*; Matsushita, Taku*; Wada, Nobuo*; et al.

Review of Scientific Instruments, 91(3), p.033318_1 - 033318_12, 2020/03

 Times Cited Count:0 Percentile:0(Instruments & Instrumentation)

Journal Articles

Repeatability and reproducibility of measurements of low dissolved radiocesium concentrations in freshwater using different pre-concentration methods

Kurihara, Momo*; Yasutaka, Tetsuo*; Aono, Tatsuo*; Ashikawa, Nobuo*; Ebina, Hiroyuki*; Iijima, Takeshi*; Ishimaru, Kei*; Kanai, Ramon*; Karube, Jinichi*; Konnai, Yae*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 322(2), p.477 - 485, 2019/11

 Times Cited Count:2 Percentile:21.58(Chemistry, Analytical)

We assessed the repeatability and reproducibility of methods for determining low dissolved radiocesium concentrations in freshwater in Fukushima. Twenty-one laboratories pre-concentrated three of 10 L samples by five different pre-concentration methods (prussian-blue-impregnated filter cartridges, coprecipitation with ammonium phosphomolybdate, evaporation, solid-phase extraction disks, and ion-exchange resin columns), and activity of radiocesium was measured. The z-scores for all of the $$^{137}$$Cs results were within $$pm$$2, indicating that the methods were accurate. The relative standard deviations (RSDs) indicating the variability in the results from different laboratories were larger than the RSDs indicating the variability in the results from each separate laboratory.

Journal Articles

Generation of $$^{4}$$He$$_2^{*}$$ clusters via neutron-$$^{3}$$He absorption reaction toward visualization of full velocity field in quantum turbulence

Matsushita, Taku*; Sonnenschein, V.*; Guo, W.*; Hayashida, Hirotoshi*; Hiroi, Kosuke; Hirota, Katsuya*; Iguchi, Tetsuo*; Ito, Daisuke*; Kitaguchi, Masaaki*; Kiyanagi, Yoshiaki*; et al.

Journal of Low Temperature Physics, 196(1-2), p.275 - 282, 2019/07

 Times Cited Count:1 Percentile:4.76(Physics, Applied)

Journal Articles

Isotope-selective microscale imaging of radioactive Cs without isobaric interferences using sputtered neutral mass spectrometry with two-step resonant ionization employing newly-developed Ti:Sapphire lasers

Sakamoto, Tetsuo*; Morita, Masato*; Kanenari, Keita*; Tomita, Hideki*; Sonnenschein, V.*; Saito, Kosuke*; Ohashi, Masaya*; Kato, Kotaro*; Iguchi, Tetsuo*; Kawai, Toshihide*; et al.

Analytical Sciences, 34(11), p.1265 - 1270, 2018/11

 Times Cited Count:8 Percentile:31.98(Chemistry, Analytical)

Journal Articles

A Study on fast digital discrimination of neutron and $$gamma$$-ray for improvement neutron emission profile measurement

Uchida, Yuki*; Takada, Eiji*; Fujisaki, Akihiro*; Isobe, Mitsutaka*; Ogawa, Kunihiro*; Shinohara, Koji; Tomita, Hideki*; Kawarabayashi, Jun*; Iguchi, Tetsuo*

Review of Scientific Instruments, 85(11), p.11E118_1 - 11E118_4, 2014/11

 Times Cited Count:9 Percentile:40.01(Instruments & Instrumentation)

Journal Articles

Fast neutron detection under intense $$gamma$$-ray fields with novel nuclear emulsion technique

Ishihara, Kohei*; Takagi, Keisuke*; Minato, Haruna*; Kawarabayashi, Jun*; Tomita, Hideki*; Maeda, Shigetaka; Naka, Tatsuhiro*; Morishima, Kunihiro*; Nakano, Toshiyuki*; Nakamura, Mitsuhiro*; et al.

Radiation Measurements, 55, p.79 - 82, 2013/08

 Times Cited Count:1 Percentile:10.69(Nuclear Science & Technology)

In order to measure the neutron under a condition of high intensity of $$gamma$$-ray background, we made new nuclear emulsion based on non-sensitized OPERA emulsion which had small AgBr grain size (AgBr grain size of 60, 90 and 160 nm). The sensitivity of this new emulsion, which was a correlation between stopping power and grain density, was estimated experimentally by irradiating neutrons with several energies. We also simulated the response to $$gamma$$-ray induced electrons and compared with some experimental results by using $$^{60}$$Co $$gamma$$ source. The results showed that there might be a threshold energy deposited in one AgBr grain under which it was impossible to develop. We estimated efficiency to the $$gamma$$-ray and the neutron with this obtained response of the new emulsion.

JAEA Reports

Inspection and repair techniques in the reactor vessel of the experimental fast reactor Joyo; Evaluation for the loose parts behavior in the reactor vessel

Kawahara, Hirotaka; Yamamoto, Masaya; Tomita, Etsuo; Takamatsu, Misao

JAEA-Technology 2012-030, 50 Pages, 2012/09

JAEA-Technology-2012-030.pdf:6.16MB
JAEA-Technology-2012-030-appendix(CD-ROM).zip:21.06MB

In the experimental fast reactor Joyo, in-vessel observation results showed that 6 pins which were connected between the handling head and the wrapper tube joint of the instrumented test subassembly (MARICO-2) were disconnected. Therefore, in order to confirm whether the disconnected 6 pins will influence reactor's safety or not, loose parts behavior in the reactor vessel was evaluated.

Journal Articles

In-vessel tritium

Ueda, Yoshio*; Oya, Kaoru*; Ashikawa, Naoko*; Ito, Atsushi*; Ono, Tadayoshi*; Kato, Daiji*; Kawashima, Hisato; Kawamura, Gakushi*; Kenmotsu, Takahiro*; Saito, Seiki*; et al.

Purazuma, Kaku Yugo Gakkai-Shi, 88(9), p.484 - 502, 2012/09

no abstracts in English

Journal Articles

Development of neutron measurement in intense $$gamma$$ field using new type of nuclear emulsion

Kawarabayashi, Jun*; Ishihara, Kohei*; Takagi, Keisuke*; Tomita, Hideki*; Iguchi, Tetsuo*; Naka, Tatsuhiro*; Morishima, Kunihiro*; Maeda, Shigetaka

Journal of ASTM International (Internet), 9(3), 5 Pages, 2012/03

In order to measure the neutron from a spent fuel assembly in fast breeder reactor precisely, we made new nuclear emulsion based on non-sensitized OPERA film with AgBr grain size of 60, 90 and 160 nm. The efficiency for $$^{252}$$Cf neutron of the new emulsion was calculated to be 0.7$$times$$10$$^{-4}$$ which energy ranged from 0.3 to 2 MeV that agrees with preliminary estimated value from experimental results. The sensitivity of the new emulsion was also estimated experimentally by irradiating 565 KeV and 14 MeV neutrons and found that the emulsion with the AgBr grain size of 60 nm showed the lowest sensitivity among these three emulsions but still had enough sensitivity for proton. Also, there was a suggestion from the experimental data that there was a threshold LET of 15 KeV/$$mu$$m for our new emulsion below which no silver cluster was developed. Further development of the response of nuclear emulsion with a few tens of nano-meter AgBr size is next step of this study.

Journal Articles

Bacterium organizes hierarchical amorphous structure in microbial cellulose

Koizumi, Satoshi; Zhao, Y.; Tomita, Yoko*; Kondo, Tetsuo*; Iwase, Hiroki; Yamaguchi, Daisuke; Hashimoto, Takeji

European Physical Journal E, 26(1-2), p.137 - 142, 2008/05

 Times Cited Count:55 Percentile:86.02(Chemistry, Physical)

no abstracts in English

Oral presentation

Hierarchical structure of microbial cellulose determined by focusing ultra-small angle neutron scattering

Koizumi, Satoshi; Kondo, Tetsuo*; Tomita, Yoko*; Iwase, Hiroki; Yamaguchi, Daisuke; Hashimoto, Takeji

no journal, , 

no abstracts in English

Oral presentation

Applicability of multi-scattering time-of-flight neutron spectrometer to measure the fuel density ratio in experimental fusion reactor

Yukawa, Kyohei*; Asai, Keisuke*; Tomita, Hideki*; Iguchi, Tetsuo*; Iwai, Haruki*; Kawarabayashi, Jun*; Konno, Chikara

no journal, , 

We are developing a new neutron spectrometer to apply to the measurement of the D/T burning ratio in the ITER high-power operation region. This system is based on the conventional double crystal TOF method and consists of a water cell and several pairs of scintillators. A water cell is inserted before the first scintillator of the TOF system and acts as a radiator or neutron scattering material. Because DD neutrons have a larger cross section of elastic scattering with hydrogen than DT neutrons, the elastic scattering in the radiator enhances the relative ratio of DD/DT intensity by approximately three times before entering the TOF system. The enhancement of the relative intensity of DD neutrons makes the detection of DD neutrons easier. The feasibility of this method as a neutron spectrometer has been verified through a preliminary experiment using a DT neutron beam (20 mm$$phi$$) at the Fusion Neutronics Source, Japan Atomic Energy Agency, which includes a small amount of DD neutrons.

Oral presentation

Combined SANS, WANS and weighing studies of microbial cellulose; Elucidation of hierarchical structures in drying process

Zhao, Y.; Koizumi, Satoshi; Hashimoto, Takeji; Tomita, Yoko*; Kondo, Tetsuo*

no journal, , 

Oral presentation

Mechanism of water absorption in microbial cellulose; Hierarchical amorphous structure and capillarity

Koizumi, Satoshi; Tomita, Yoko*; Zhao, Y.; Iwase, Hiroki*; Yamaguchi, Daisuke; Kondo, Tetsuo*; Hashimoto, Takeji; Masui, Tomomi

no journal, , 

no abstracts in English

Oral presentation

Inspection and repair techniques in reactor vessel of sodium cooled fast reactor, 4-4; Safety evaluation for loose parts in reactor vessel

Kawahara, Hirotaka; Takamatsu, Misao; Yamamoto, Masaya; Tomita, Etsuo

no journal, , 

no abstracts in English

Oral presentation

Combined SANS, WANS, and weighing studies of microbial cellulose in drying process

Zhao, Y.; Koizumi, Satoshi; Hashimoto, Takeji; Tomita, Yoko*; Kondo, Tetsuo*

no journal, , 

Oral presentation

Development of 2.5 MeV neutron spectrometer toward deuterium plasma diagnostics in LHD

Tomita, Hideki*; Iwai, Haruki*; Iguchi, Tetsuo*; Kawarabayashi, Jun*; Isobe, Mitsutaka*; Konno, Chikara

no journal, , 

Neutron spectrometer based on coincident counting of associated particles has been developed for deuterium plasma diagnostics on Large Helical Device (LHD) at National Institute for Fusion Science. Efficient detection of 2.5 MeV neutron with high energy resolution would achievable by coincident detection of a scattered neutron and a recoiled proton associated to a elastic scattering of incident neutron in a plastic scintillator as a radiator. Calculated neutron spectra from deuterium plasma heated by neutral beam injection indicate that the energy resolution of less than 7% is required for the spectrometer to evaluate energetic deuterium confinement. By using a prototype of the proposed spectrometer, the energy resolution of 6.3% and the detection efficiency of 3.3$$times$$10$$^{-7}$$ counts/neutron were experimentally demonstrated for 2.5 MeV mono-energetic neutron, respectively.

33 (Records 1-20 displayed on this page)