Water fraction dependence of the aggregation behavior of hydrophobic fluorescent solutes in water-tetrahydrofuran

Tsuji, Hayato*; Nakahata, Masaki*; Hishida, Mafumi*; Seto, Hideki*; Motokawa, Ryuhei; Inoue, Takeru*; Egawa, Yasunobu*

Journal of Physical Chemistry Letters (Internet), 14(49), p.11235 - 11241, 2023/12

https://doi.org/10.1021/acs.jpclett.3c02882

Radiocesium-bearing microparticles cause a large variation in Cs activity concentration in the aquatic insect (Tricoptera: Stenopsychidae) in the Ota River, Fukushima, Japan

Ishii, Yumiko*; Miura, Hikaru*; Jo, J.*; Tsuji, Hideki*; Saito, Rie; Koarai, Kazuma; Hagiwara, Hiroki; Urushidate, Tadayuki*; Nishikiori, Tatsuhiro*; Wada, Toshihiro*; et al.

PLOS ONE (Internet), 17(5), p.e0268629_1 - e0268629_17, 2022/05

https://doi.org/10.1371/journal.pone.0268629

We investigated the variability in Cs activity concentration in individual aquatic insects in detritivorous caddisfly () and carnivorous dobsonfly () larvae from the Ota River, Fukushima. Caddisfly larvae showed sporadically higher radioactivity, whereas no such outliers were observed in dobsonfly larvae. Autoradiography and scanning electron microscopy analyses confirmed that these caddisfly larvae samples contained radiocesium-bearing microparticles (CsMPs), which are insoluble Cs-bearing silicate glass particles. CsMPs were also found in potential food sources of caddisfly larvae, such as periphyton and drifting particulate organic matter, indicating that larvae may ingest CsMPs along with food particles of similar size. Although CsMPs distribution and uptake by organisms in freshwater ecosystems is relatively unknown, our study demonstrates that CsMPs can be taken up by aquatic insects.

Dynamics of Cs in water and phyto- and zooplankton in a reservoir affected by the Fukushima Daiichi Nuclear Power Plant Accident

Tsuji, Hideki*; Nakagawa, Megumi*; Iijima, Kazuki; Funaki, Hironori; Yoshimura, Kazuya; Sakuma, Kazuyuki; Hayashi, Seiji*

Global Environmental Research (Internet), 24(2), p.115 - 127, 2021/06

Lake water, phytoplankton and zooplankton were sampled by a total of 12 quarterly surveys from August 2014 to May 2017 at a dam lake in the Fukushima nuclear disaster area, and variations of dissolved form of Cs and planktonic Cs were observed. Seasonal variations in dissolved Cs concentration with high in summer and low in winter were observed in the upstream, midstream and downstream areas of the lake, but no seasonal or site specific differences in planktonic Cs concentrations and dominant species were found. The amount of planktonic form of Cs in the water was less than 1.4% of the total Cs in the lake water, therefore the effect of plankton on the dynamics of Cs in the lake was minimal.

An Experimental setup for creating and imaging He excimer cluster tracers in superfluid helium-4 via neutron-He absorption reaction

Sonnenschein, V.*; Tsuji, Yoshiyuki*; Kokuryu, Shoma*; Kubo, Wataru*; Suzuki, So*; Tomita, Hideki*; Kiyanagi, Yoshiaki*; Iguchi, Tetsuo*; Matsushita, Taku*; Wada, Nobuo*; et al.

Review of Scientific Instruments, 91(3), p.033318_1 - 033318_12, 2020/03

https://doi.org/10.1063/1.5130919

Repeatability and reproducibility of measurements of low dissolved radiocesium concentrations in freshwater using different pre-concentration methods

Kurihara, Momo*; Yasutaka, Tetsuo*; Aono, Tatsuo*; Ashikawa, Nobuo*; Ebina, Hiroyuki*; Iijima, Takeshi*; Ishimaru, Kei*; Kanai, Ramon*; Karube, Jinichi*; Konnai, Yae*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 322(2), p.477 - 485, 2019/11

https://doi.org/10.1007/s10967-019-06696-2

We assessed the repeatability and reproducibility of methods for determining low dissolved radiocesium concentrations in freshwater in Fukushima. Twenty-one laboratories pre-concentrated three of 10 L samples by five different pre-concentration methods (prussian-blue-impregnated filter cartridges, coprecipitation with ammonium phosphomolybdate, evaporation, solid-phase extraction disks, and ion-exchange resin columns), and activity of radiocesium was measured. The z-scores for all of the Cs results were within 2, indicating that the methods were accurate. The relative standard deviations (RSDs) indicating the variability in the results from different laboratories were larger than the RSDs indicating the variability in the results from each separate laboratory.

Applicability of for modelling dissolved Cs concentrations in Fukushima river water; Case study of the upstream Ota River

Sakuma, Kazuyuki; Tsuji, Hideki*; Hayashi, Seiji*; Funaki, Hironori; Malins, A.; Yoshimura, Kazuya; Kurikami, Hiroshi; Kitamura, Akihiro; Iijima, Kazuki; Hosomi, Masaaki*

Journal of Environmental Radioactivity, 184-185, p.53 - 62, 2018/04

https://doi.org/10.1016/j.jenvrad.2018.01.001

A study is presented on the applicability of the distribution coefficient () absorption/desorption model to simulate dissolved Cs concentrations in Fukushima river water. The simulation results were in good agreement with the observations on water and suspended sediment fluxes, and on particulate bound Cs concentrations under both ambient and high flow conditions. By contrast the measured concentrations of dissolved Cs in the river water were much harder to reproduce with the simulations. By tuning the values for large particles, it was possible to reproduce the mean dissolved Cs concentrations during base flow periods (observation: 0.32 Bq/L, simulation: 0.36 Bq/L). However neither the seasonal variability in the base flow dissolved Cs concentrations (0.14-0.53 Bq/L), nor the peaks in concentration that occurred during storms (0.18-0.88 Bq/L, mean: 0.55 Bq/L), could be reproduced with realistic simulation parameters.

Experimental Study on Gas Entrainment from Free-surface Generation Mechanism of Dimple-Eddy

Tsuji, Yoshiyuki*; Kamide, Hideki

JNC TY9400 2005-017, 54 Pages, 2005/03

JNC-TY9400-2005-017.pdf:4.22MB

Compact reactor vessel is designed to reduce construction cost of a fast reactor. In a compact reactor vessel flow velocity will increase and it causes gas entrainment at free surface. Thus, gas entrainment is one of significant issue of the reactor design. In this study we carried out a water experiment on the gas entrainment, especially the onset condition of a dimple vortex, which causes the gas entrainment in order to establish a guide line in a deisgn.This study is planned to carry in three years from 2003 to 2005. The year of 2004 corresponds to the second term. In this year, water experiment was carried out using a flow channel, vertical suction pipe, and an obstacle in order to see influences of obstacles on the gas entrainment and dimple vortex. Onset conditions of the gas entrainment due to the dimple vortex were obtained with experimental parameters of flow velocity in the channel, water level, and free surface wave or disturbance. It was shown that the onset of gas entrainment needed vertical vortex, e.g. in a wake of an obstacle, and disturbance of free surface block the onset of the dimple vortex and the gas entrainment.

Relativistic laser plasma from micron-sized argon clusters as a debris-free X-ray source for pulse X-ray diffraction

Fukuda, Yuji; Akahane, Yutaka; Aoyama, Makoto; Inoue, Norihiro*; Ueda, Hideki; Nakai, Yoshiki*; Tsuji, Koichi*; Yamakawa, Koichi; Hironaka, Yoichiro*; Kishimura, Hiroaki*; et al.

Applied Physics Letters, 85(21), p.5099 - 5101, 2004/11

https://doi.org/10.1063/1.1823589

We have demonstrated diffraction from Si(111) crystal using X-rays from highly ionized Ar ions produced by laser irradiation with an intensity of 610 W/cm and a pulse duration of 30 fs acting upon micron-sized Ar clusters. The measured total photon flux and line width in the He line (3.14 keV) were 410 photons/shot/4sr and 3.7 eV (FWHM), respectively, which is sufficient to utilize as a debris-free light source for time-resolved X-ray diffraction studies.

Program of in-pile IASCC testing under the simulated actual plant condition; Thermohydraulic design study of saturated temperature capsule for IASCC irradiation test

Ide, Hiroshi; Matsui, Yoshinori; Nagao, Yoshiharu; Komori, Yoshihiro; Itabashi, Yukio; Tsuji, Hirokazu; Tsukada, Takashi; Nagata, Nobuaki*; Dozaki, Koji*; Takiguchi, Hideki*

Proceedings of 11th International Conference on Nuclear Engineering (ICONE-11) (CD-ROM), 7 Pages, 2003/04

The advanced water chemistry controlled irradiation research device has been developed in JAERI to perform irradiation tests for research on IASCC. The irradiation device consists of the SATCAP (Saturated Temperature Capsule) inserted into the JMTR core and the water control unit installed out-of-core. Regarding the SATCAP, thermohydraulic design of the SATCAP was performed aiming at controlling the specimen temperature with high accuracy and increasing water flow velocity on the specimen surface to improve the controllability of water chemistry. As a result of irradiation test using the new type SATCAP, each specimen temperature and water chemistry were able to be controlled as designed.

Radiocesium behavior of water and plankton in Dam Lake in Fukushima Prefecture

Tsuji, Hideki*; Hayashi, Seiji*; Funaki, Hironori; Iijima, Kazuki

no journal, , 

no abstracts in English