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Journal Articles

Performance comparison of monoamides on U recovery by temperature swing extraction using Ce

Iwamoto, Toshihiro; Saito, Madoka*; Takahatake, Yoko; Watanabe, So; Watanabe, Masayuki; Naruse, Atsuki*; Tsukahara, Takehiko*

Mechanical Engineering Journal (Internet), 11(2), p.23-00444_1 - 23-00444_7, 2024/04

JAEA Reports

Annual report for research on geosphere stability for long-term isolation of radioactive waste in fiscal year 2022

Niwa, Masakazu; Shimada, Koji; Sueoka, Shigeru; Ishihara, Takanori; Ogawa, Hiroki; Hakoiwa, Hiroaki; Watanabe, Tsuyoshi; Nishiyama, Nariaki; Yokoyama, Tatsunori; Ogata, Manabu; et al.

JAEA-Research 2023-005, 78 Pages, 2023/10

JAEA-Research-2023-005.pdf:6.51MB

This annual report documents the progress of research and development (R&D) in the 1st fiscal year of the Japan Atomic Energy Agency 4th Medium- and Long-term Plan (fiscal years 2022-2028) to provide the scientific base for assessing geosphere stability for long-term isolation of high-level radioactive waste. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. The current status of R&D activities with previous scientific and technological progress is summarized.

Journal Articles

Evaluation of the remaining spent extraction solvent in vermiculite after leaching tests via PIXE analysis

Arai, Yoichi; Watanabe, So; Hasegawa, Kenta; Okamura, Nobuo; Watanabe, Masayuki; Takeda, Keisuke*; Fukumoto, Hiroki*; Ago, Tomohiro*; Hagura, Naoto*; Tsukahara, Takehiko*

Nuclear Instruments and Methods in Physics Research B, 542, p.206 - 213, 2023/09

 Times Cited Count:1 Percentile:63.33(Instruments & Instrumentation)

Journal Articles

Treatment of U contaminated waste generated from nuclear fuel fabrication process, 1; Ce(IV) recovery by temperature swing extraction with monoamides

Iwamoto, Toshihiro; Saito, Madoka*; Takahatake, Yoko; Watanabe, So; Watanabe, Masayuki; Naruse, Atsuki*; Tsukahara, Takehiko*

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 4 Pages, 2023/05

Applicability of temperature swing extraction technology employing monoamides was examined for uranium contaminated waste treatment procedure. Separation experiments on simulated target solution with three kinds of monoamides with different structure showed that Ce(IV) in the solution was selectively recovered by the temperature swing extraction operation. Based on the experiments, an appropriate monoamide for the procedure was selected.

JAEA Reports

A GIS-based approach for geomorphological analysis of volcanic edifices to estimate latent magma plumbing system (Contract research)

Nishiyama, Nariaki; Goto, Akira*; Tsukahara, Yuzuko; Kawamura, Makoto; Umeda, Koji*; Niwa, Masakazu

JAEA-Testing 2022-003, 51 Pages, 2022/09

JAEA-Testing-2022-003.pdf:5.24MB
JAEA-Testing-2022-003-appendix(CD-ROM).zip:1.12MB

Advancement of the evaluation technology of the magma activity range is essential as one of the technical issues related to volcanic and igneous activities in the evaluation of the long-term stability of the geological environment in the geological disposal of high-level radioactive waste. As an effective method, topographical analysis of volcanic edifices is expected to be used to determine the distribution area of dikes. In recent years, the development of computer-based topographic analysis technology has made it possible to simply perform a large volume of work that would otherwise be difficult due to the manual handling. This report describes an analysis method for the shape of contour lines that forms volcanic edifices using GIS software.

JAEA Reports

Research plan on geosphere stability for long-term isolation of radioactive waste (Scientific program for fiscal year 2022)

Sasao, Eiji; Ishimaru, Tsuneari; Niwa, Masakazu; Shimada, Akiomi; Shimada, Koji; Watanabe, Takahiro; Sueoka, Shigeru; Yokoyama, Tatsunori; Fujita, Natsuko; Ogita, Yasuhiro; et al.

JAEA-Review 2022-022, 29 Pages, 2022/09

JAEA-Review-2022-022.pdf:0.97MB

This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2022. The objectives and contents in fiscal year 2022 are described in detail based on the JAEA 4th Medium- and Long-term Plan (fiscal years 2022-2028). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques

Journal Articles

Design of microchannel suitable for packing with anion exchange resins; Uranium separation from seawater containing a large amount of cesium

Ouchi, Kazuki; Tsukahara, Takehiko*; Brandt, A.*; Muto, Yuki*; Nabatame, Nozomi*; Kitatsuji, Yoshihiro

Analytical Sciences, 37(12), p.1789 - 1794, 2021/12

 Times Cited Count:1 Percentile:6.06(Chemistry, Analytical)

We attempted to scale down a separation process of uranium (U) using the microchip column loaded with anion exchange resin to develop safety and waste-reducing separation technique. The ideal separation performance of U was obtained by the properly design of a microchannel. The concentration of U in seawater as a real-world sample could be quantified with the prepared microchip column. It indicates that the microchip column is sufficiently practical. Compared to separation of U with a general column, the column size was successfully scaled down to $$<$$ 1/5000.

Journal Articles

Determination of $$^{135}$$Cs/$$^{137}$$Cs isotopic ratio in soil collected near Fukushima Daiichi Nuclear Power Station through mass spectrometry

Shimada, Asako; Tsukahara, Takehiko*; Nomura, Masao*; Kim, M. S.*; Shimada, Taro; Takeda, Seiji; Yamaguchi, Tetsuji

Journal of Nuclear Science and Technology, 58(11), p.1184 - 1194, 2021/11

 Times Cited Count:5 Percentile:63.04(Nuclear Science & Technology)

Determining the completeness of nuclear reactor decommissioning is an important step in safely utilizing nuclear power. For example, $$^{137}$$Cs from the Fukushima Daiichi Nuclear Power Station (FDNPS) accident can be treated as background radioactivity, so determining the origin of $$^{137}$$Cs is essential. To accomplish this, measuring the $$^{135}$$Cs/$$^{137}$$Cs isotope ratio can be useful, so this study optimized a solvent extraction method, with calix[4]arene-bis(t-octylbenzo-crown-6) [BOBCalixC6] in 1-octanol, to purify radioactive Cs, radiocesium, from a solution of major environmental soil elements and mass spectrometry interference elements. This optimized method was applied to Cs purification in soil samples (40 g), and the final solutions contained a total of 10$$mu$$g/ml of the major soil elements and ng/ml concentrations at most of interfering elements. Soil samples collected near the FDNPS were then purified, and the $$^{135}$$Cs/$$^{137}$$Cs isotope ratios were measured, using both thermal ionization mass spectrometry (TIMS) and triple quadrupole induced coupled plasma mass spectrometry (ICP-QQQ). The results of each of these measurements were compared, and we found that Cs isotope ratios obtained by TIMS were more precise, by an order of magnitude, while the ICP-QQQ results possessed good abundance sensitivities. A slightly higher $$^{135}$$Cs/$$^{137}$$Cs ratio in the northwest area of the FDNPS was observed, while other areas exhibited similar values, all within the measurement error range, which indicated different origins of radiocesium. These results agreed with previously reported $$^{134}$$Cs/$$^{137}$$Cs activity distributions, suggesting that this ratio may be useful in identifying radiocesium origins for evaluating future nuclear reactor decommissions.

JAEA Reports

Annual report for research on geosphere stability for long-term isolation of radioactive waste in fiscal year 2020

Ishimaru, Tsuneari; Ogata, Nobuhisa; Kokubu, Yoko; Shimada, Koji; Niwa, Masakazu; Shimada, Akiomi; Watanabe, Takahiro; Sueoka, Shigeru; Yokoyama, Tatsunori; Fujita, Natsuko; et al.

JAEA-Research 2021-007, 65 Pages, 2021/10

JAEA-Research-2021-007.pdf:4.21MB

This annual report documents the progress of research and development (R&D) in the 6th fiscal year during the JAEA 3rd Mid- and Long-term Plan (fiscal years 2015-2021) to provide the scientific base for assessing geosphere stability for long-term isolation of the high-level radioactive waste. The planned framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. The current status of R&D activities with previous scientific and technological progress is summarized.

JAEA Reports

Research plan on geosphere stability for long-term isolation of radioactive waste (Scientific program for fiscal year 2021)

Ishimaru, Tsuneari; Kokubu, Yoko; Shimada, Koji; Shimada, Akiomi; Niwa, Masakazu; Watanabe, Takahiro; Sueoka, Shigeru; Yokoyama, Tatsunori; Fujita, Natsuko; Ogita, Yasuhiro; et al.

JAEA-Review 2021-012, 48 Pages, 2021/08

JAEA-Review-2021-012.pdf:1.64MB

This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2021. The objectives and contents in fiscal year 2021 are described in detail based on the JAEA 3rd Medium- and Long-term Plan (fiscal years 2015-2021). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.

JAEA Reports

Research plan on geosphere stability for long-term isolation of radioactive waste (Scientific program for fiscal year 2020)

Ishimaru, Tsuneari; Ogata, Nobuhisa; Shimada, Koji; Kokubu, Yoko; Niwa, Masakazu; Asamori, Koichi; Watanabe, Takahiro; Sueoka, Shigeru; Komatsu, Tetsuya; Yokoyama, Tatsunori; et al.

JAEA-Review 2020-010, 46 Pages, 2020/07

JAEA-Review-2020-010.pdf:1.89MB

This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2020. The objectives and contents in fiscal year 2020 are described in detail based on the JAEA 3rd Medium- and Long-term Plan (fiscal years 2015-2021). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.

Journal Articles

No secondary waste recycle technology for rare metals using the hydrophilic extraction with phase transfer phenomena

Tsukahara, Takehiko*; Saga, Kaname*; Suzuki, Hideya*; Matsumura, Tatsuro

Kurin Tekunoroji, 29(12), p.4 - 7, 2019/12

no abstracts in English

Journal Articles

Direct temperature-swing extraction of rare-earth elements from acidic solution using the hydrophobic interactions of poly($$N$$-isopropylacrylamide) with diglycolamide-typed ligands

Saga, Kaname*; Suzuki, Hideya; Matsumura, Tatsuro; Tsukahara, Takehiko*

Analytical Sciences, 35(4), p.461 - 464, 2019/04

 Times Cited Count:3 Percentile:12.00(Chemistry, Analytical)

The phase transition-based gelification phenomenon of poly-$$N$$-isopropylacrylamide (PNIPAAm) in aqueous solutions has a great potential in developing new waste-free extraction processes of metal ions. By using hydrophobic diglycolamide-typed ligands in gelification extraction, a one-step complete extraction of all the RE ions from a nitric acid solution was successfully realized.

Journal Articles

Separation and recovery of raremetals using the hydrophiric extraction with phase transfer phenomena

Tsukahara, Takehiko*; Suzuki, Hideya*; Matsumura, Tatsuro; Saga, Kaname*

Bunri Gijutsu, 49(4), p.221 - 225, 2019/04

no abstracts in English

JAEA Reports

Research on engineering technology in the full-scale demonstration of EBS and operation technology for HLW disposal; Research report in 2012 (Joint research)

Nakatsuka, Noboru; Sato, Haruo; Tanai, Kenji; Nakayama, Masashi; Sawada, Sumiyuki*; Asano, Hidekazu*; Saito, Masahiko*; Yoshino, Osamu*; Tsukahara, Shigeki*; Hishioka, Sosuke*; et al.

JAEA-Research 2013-034, 70 Pages, 2014/01

JAEA-Research-2013-034.pdf:9.11MB

Japan Atomic Energy Agency (JAEA) and Radioactive Waste Management Funding and Research Center (RWMC) concluded the letter of cooperation agreement on the research and development of radioactive waste disposal in April, 2005, and have been carrying out the collaboration work based on the agreement. JAEA have been carrying out the Horonobe Underground Research Laboratory (URL) Project which is intended for a sedimentary rock in the Horonobe town, Hokkaido, since 2001. In the project, geoscientific research and research and development on geological disposal technology are being promoted. Meanwhile, the government (the Agency for Natural Resources and Energy, Ministry of Economy, Trade and Industry) has been promoting construction of equipments for the full-scale demonstration of engineered barrier system and operation technology for high-level radioactive waste (HLW) disposal since 2008, to enhance public's understanding to the geological disposal of HLW, e.g. using underground facility. RWMC received an order of the project in fiscal year 2012 (2011/2012) continuing since fiscal year 2008 (2008/2009). Since topics in this project are included in the Horonobe URL Project, JAEA carried out this project as collaboration work continuing in fiscal year 2008. This report summarizes the results of engineering technology carried out in this collaboration work in fiscal year 2012. In fiscal year 2012, part of the equipments for emplacement of buffer material was produced and visualization test for water penetration in buffer material were carried out.

JAEA Reports

Research on engineering technology in the full-scale demonstration of EBS and operation technology for HLW disposal; Research report in 2011 (Joint research)

Nakatsuka, Noboru; Sato, Haruo; Tanai, Kenji; Sugita, Yutaka; Nakayama, Masashi; Sawada, Sumiyuki*; Niinuma, Hiroaki*; Asano, Hidekazu*; Saito, Masahiko*; Yoshino, Osamu*; et al.

JAEA-Research 2013-027, 34 Pages, 2013/11

JAEA-Research-2013-027.pdf:5.84MB

Japan Atomic Energy Agency (JAEA) and Radioactive Waste Management Funding and Research Center (RWMC) concluded the letter of cooperation agreement on the research and development of radioactive waste disposal in April, 2005, and have been carrying out the collaboration work based on the agreement. JAEA have been carrying out the Horonobe Underground Research Laboratory (URL) Project which is intended for a sedimentary rock in the Horonobe town, Hokkaido, since 2001. In the project, geoscientific research and research and development on geological disposal technology are being promoted. Meanwhile, the government (the Agency for Natural Resources and Energy, Ministry of Economy, Trade and Industry) has been promoting construction of equipments for the full-scale demonstration of engineered barrier system and operation technology for high-level radioactive waste (HLW) disposal since 2008, to enhance public's understanding to the geological disposal of HLW, e.g. using underground facility. RWMC received an order of the project in fiscal year 2010 (2010/2011) continuing since fiscal year 2008 (2008/2009). Since topics in this project are included in the Horonobe URL Project, JAEA carried out this project as collaboration work continuing in fiscal year 2008. This report summarizes the results of engineering technology carried out in this collaboration work in fiscal year 2011. In fiscal year 2011, part of the equipments for emplacement of buffer material was produced and visualization test for water penetration in buffer material were carried out.

Journal Articles

Diagnostics system of JT-60U

Sugie, Tatsuo; Hatae, Takaki; Koide, Yoshihiko; Fujita, Takaaki; Kusama, Yoshinori; Nishitani, Takeo; Isayama, Akihiko; Sato, Masayasu; Shinohara, Koji; Asakura, Nobuyuki; et al.

Fusion Science and Technology (JT-60 Special Issue), 42(2-3), p.482 - 511, 2002/09

 Times Cited Count:6 Percentile:3.03(Nuclear Science & Technology)

The diagnostic system of JT-60U (JT-60upgrade) is composed of about 50 individual diagnostic devices. Recently, the detailed radial profile measurements of plasma parameters have been improved, so that the internal structure of plasmas has been explored. The understanding of plasma confinement has been enhanced by density and temperature fluctuation measurements using a mm-wave reflectometer and electron cyclotron emission measurements respectively. In addition, the real-time control experiments of electron density, neutron yield, radiated power and electron temperature gradient have been carried out successfully by corresponding diagnostic devices. These measurements and the real time control contribute to improving plasma performance. Diagnostic devices for next generation fusion devices such as a CO2 laser interferometer/polarimeter and a CO2 laser collective Thomson scattering system have been developed.

Journal Articles

Improvement of Thomson scattering system using SBS phase conjugation mirrors in JT-60U

Hatae, Takaki; Nakatsuka, Masahiro*; Yoshida, Hidetsugu*; Naito, Osamu; Kitamura, Shigeru; Sakuma, Takeshi*; Hamano, Takashi*; Tsukahara, Yoshimitsu

Proceedings of 29th European Physical Society Conference on Plasma Physics and Controlled Fusion, 4 Pages, 2002/00

no abstracts in English

Journal Articles

Giant monopole resonances in deformed nuclei

Ito, M.*; Sakaguchi, Harutaka*; Ishikawa, Takatsugu*; Kawabata, Takahiro*; Murakami, Tetsuya*; Takeda, H.*; Taki, T.*; Tsukahara, N.*; Uchida, Makoto*; Yasuda, Yusuke*; et al.

Nuclear Physics A, 687(1-2), p.52c - 57c, 2001/04

no abstracts in English

Journal Articles

Thin ice target for $$^{16}$$O (p,p') experiment

Kawabata, Takahiro*; Akimune, Hidetoshi*; Fujimura, Hisako*; Fujita, Hirohiko*; Fujita, Yoshitaka*; Fujiwara, Mamoru; Hara, Keigo*; Hatanaka, Kichiji*; Hosono, K.*; Ishikawa, Takatsugu*; et al.

Nuclear Instruments and Methods in Physics Research A, 459(1-2), p.171 - 176, 2001/02

 Times Cited Count:17 Percentile:74.75(Instruments & Instrumentation)

no abstracts in English

59 (Records 1-20 displayed on this page)