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JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2022

Kokubun, Yuji; Nakada, Akira; Seya, Natsumi; Koike, Yuko; Nemoto, Masashi; Tobita, Keiji; Yamada, Ryohei*; Uchiyama, Rei; Yamashita, Daichi; Nagai, Shinji; et al.

JAEA-Review 2023-046, 164 Pages, 2024/03

JAEA-Review-2023-046.pdf:4.2MB

The Nuclear Fuel Cycle Engineering Laboratories conducts environmental radiation monitoring around the reprocessing plant in accordance with the "Safety Regulations for Reprocessing Plant of JAEA, Part IV: Environmental Monitoring". This report summarizes the results of environmental radiation monitoring conducted during the period from April 2022 to March 2023 and the results of dose calculations for the surrounding public due to the release of radioactive materials into the atmosphere and ocean. In the results of the above environmental radiation monitoring, many items were affected by radioactive materials emitted from the accident at the Fukushima Daiichi Nuclear Power Plant of Tokyo Electric Power Company, Incorporated (changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016), which occurred in March 2011. Also included as appendices are an overview of the environmental monitoring plan, an overview of measurement methods, measurement results and their changes over time, meteorological statistics results, radioactive waste release status, and an evaluation of the data which deviated of the normal range.

Journal Articles

Assessment of hydrogen embrittlement behavior in Al-Zn-Mg alloy through multi-modal 3D image-based simulation

Fujihara, Hiro*; Toda, Hiroyuki*; Ebihara, Kenichi; Kobayashi, Masakazu*; Mayama, Tsuyoshi*; Hirayama, Kyosuke*; Shimizu, Kazuyuki*; Takeuchi, Akihisa*; Uesugi, Masayuki*

International Journal of Plasticity, 174, p.103897_1 - 103897_22, 2024/03

 Times Cited Count:0

Hydrogen(H) embrittlement in high-strength aluminum(Al) alloys is a crucial problem. H accumulation at the interface of precipitates in Al alloy is considered to cause embrittlement. However, there is no quantitative knowledge regarding the interaction between H distribution and stress field near cracks. In this study, using a multi-modal three-dimensional image-based simulation combining the crystal plasticity finite element method and H diffusion analysis, we tried to capture the stress distribution near the crack, its influence on the H distribution, and the probability of crack initiation in the experimental condition. As a result, it was found that grain boundary cracks transition to quasi-cleavage cracks in the region where the cohesive energy of the semi-coherent interface of MgZn$$_2$$ precipitates decreases due to H accumulation near the tip. We believe the present simulation method successfully bridges nanoscale delamination and macroscale brittle fracture.

Journal Articles

Stress corrosion cracking induced by the combination of external and internal hydrogen in Al-Zn-Mg-Cu alloy

Tang, J.*; Wang, Y.*; Fujihara, Hiro*; Shimizu, Kazuyuki*; Hirayama, Kyosuke*; Ebihara, Kenichi; Takeuchi, Akihisa*; Uesugi, Masayuki*; Toda, Hiroyuki*

Scripta Materialia, 239, p.115804_1 - 115804_5, 2024/01

 Times Cited Count:0 Percentile:0(Nanoscience & Nanotechnology)

Stress corrosion cracking (SCC) behaviors induced by the combination of external and internal hydrogen (H) in an Al-Zn-Mg-Cu alloy were systematically investigated via in situ 3D characterization techniques. SCC of the Al-Zn-Mg-Cu alloy could initiate and propagate in the potential crack region where the H concentration exceeded a critical value, in which the nanoscopic H-induced decohesion of $$eta$$-MgZn$$_2$$ precipitates resulted in macroscopic cracking. External H that penetrated the alloy from the environment played a crucial role during the SCC of the Al-Zn-Mg-Cu alloy by generating gradient-distributed H-affected zones near the crack tips, which made Al alloys in water environment more sensitive to SCC. Additionally, the pre-existing internal H was driven toward the crack tips during plastic deformation. It was involved in the SCC and made contributions to both the cracks initiation and propagation.

Journal Articles

Hydrogen embrittlement and its prevention in 7XXX aluminum alloys with high Zn concentrations

Shimizu, Kazuyuki*; Toda, Hiroyuki*; Fujihara, Hiro*; Yamaguchi, Masatake; Uesugi, Masayuki*; Takeuchi, Akihisa*; Nishijima, Masahiko*; Kamada, Yasuhiro*

Corrosion, 79(8), p.818 - 830, 2023/08

 Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)

7xxx aluminum alloys are representative high-strength aluminum alloys; however, mechanical property degradation due to hydrogen hinders further strengthening. We propose the dispersion of Mn-based second-phase particles as a novel technique for preventing 7xxx aluminum alloy hydrogen embrittlement. In this study, the deformation and fracture behaviors of high hydrogen 7xxx alloys containing 0.0% Mn and 0.6% Mn are observed in situ using synchrotron radiation X-ray tomography. The obtained macroscopic hydrogen embrittlement is quantitatively analyzed based on hydrogen partitioning in alloys. Adding 0.6% Mn, generating second-phase particles with high hydrogen trapping abilities, significantly suppresses hydrogen-induced quasicleavage fracture.

Journal Articles

A New X-ray fluorescence spectroscopy for extraterrestrial materials using muon beam

Terada, Kentaro*; Ninomiya, Kazuhiko*; Osawa, Takahito; Tachibana, Shogo*; Miyake, Yasuhiro*; Kubo, Kenya*; Kawamura, Naritoshi*; Higemoto, Wataru; Tsuchiyama, Akira*; Ebihara, Mitsuru*; et al.

Scientific Reports (Internet), 4, p.5072_1 - 5072_6, 2014/05

 Times Cited Count:45 Percentile:82.6(Multidisciplinary Sciences)

After the discovery of X-ray by Rontgen, mankind got a new eye to see through things. This fluoroscopy, so-called X-ray radiography that gives the density distribution of the inside of an object, has been applied to the vast research field such as natural/material/medical sciences, industry and technology. The recent development on the intense pulsed muon source at J-PARC MUSE (rate of 106 cps for 60 MeV/c) enabled us to pioneer a new frontier of analytical sciences. Here we report on a non-destructive elemental analysis by using muon capture. Controlling muon's momentum from 32.5 to 57.5 MeV/c. we successfully demonstrated a depth-profile analysis of light elements from several mm-thick layered materials, and non-destructive bulk analyses of meteorites containing organics. Now it is a beginning to utilize a new eye, muon radiography.

Journal Articles

Irradiation history of Itokawa regolith material deduced from noble gases in the Hayabusa samples

Nagao, Keisuke*; Okazaki, Ryuji*; Nakamura, Tomoki*; Miura, Yayoi*; Osawa, Takahito; Bajo, Kenichi*; Matsuda, Shintaro*; Ebihara, Mitsuru*; Ireland, T.*; Kitajima, Fumio*; et al.

Science, 333(6046), p.1128 - 1131, 2011/08

 Times Cited Count:130 Percentile:95.22(Multidisciplinary Sciences)

A steroid surface materials record regolith processes and a history of cosmic-ray irradiation. Noble gas isotopes in three rocky grains from Itokawa have been determined. High concentrations of solar He, Ne, and Ar, as high as those in lunar soils, are released at variable temperatures from each sample. The isotopic compositions are essentially identical to those of solar wind but distinguishable in He relative abundance. These noble gas characteristics can be explained by repeated implantation and preferential loss of solar He by removal of weathered He-rich rim on the grain surface through friction among regolith grains on Itokawa. Residence time of regolith materials on Itokawa is alculated to be shorter than 10 Myr, suggesting that regolith materials of small asteroids would escape easily to space.

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