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JAEA Reports

Technical note for the cavitation damage inspection for interior surface of the mercury target vessel, 2; Damage depth measurement for cavitation erosion

Naoe, Takashi; Wakui, Takashi; Kinoshita, Hidetaka; Kogawa, Hiroyuki; Teshigawara, Makoto; Haga, Katsuhiro

JAEA-Technology 2023-022, 81 Pages, 2024/01

JAEA-Technology-2023-022.pdf:9.87MB

In the liquid mercury target system for the pulsed spallation neutron source of Materials and Life Science Experimental Facility (MLF) in the Japan Proton Accelerator Research Complex (J-PARC), pressure waves that is generated by the high-energy proton beam injection simultaneously with the spallation reaction, resulting severe cavitation erosion damage on the interior surface of the mercury target vessel. Because the bubble of pressure wave-induced cavitation collapsing near the interior surface of the mercury target vessel with applying the large amplitude of localized impact on the surface. Since the wall thickness of the beam entrance portion of the target vessel is designed to be 3 mm to reduce thermal stress due to the internal heating, the erosion damage has the possibility to cause the vessel fatigue failure and mercury leakage originated from erosion pits during operation. To reduce the erosion damage by cavitation, a technique of gas microbubble injection into the mercury for pressure wave mitigation, and double-walled structure of the beam window of the target vessel has been applied. A specimen was cut from the beam window of the used mercury target vessel in order to investigate the effect of the damage mitigation technologies on the vessel, and to reflect the consideration of operation condition for the next target. We have observed cavitation damage on interior surface of the used mercury target vessel by cutting out the disk shape specimens. Damage morphology and depth of damaged surface were evaluated and correlation between the damage depth and operational condition was examined. The result showed that the erosion damage by cavitation is extremely reduced by injecting gas microbubbles and the damage not formed inside narrow channel of the double-walled structure for relatively high-power operated target vessels.

Journal Articles

Cavitation damage prediction in mercury target for pulsed spallation neutron source using Monte Carlo simulation

Wakui, Takashi; Takagishi, Yoichi*; Futakawa, Masatoshi

Materials, 16(17), p.5830_1 - 5830_16, 2023/09

 Times Cited Count:0 Percentile:0(Chemistry, Physical)

Cavitation damage on the mercury target vessel is induced by proton beam injection in mercury. The prediction method of the cavitation damage using Monte Carlo simulations was proposed taking into account of the uncertainties of the position of cavitation bubbles and impact pressure distributions. The distribution of impact pressure attributed to individual cavitation bubble collapsing was assumed to be the Gaussian distribution, and the probability distribution of the maximum value of impact pressures was assumed to be three kinds of distributions; the delta function, the Gaussian and Weibull distributions. Two parameters were estimated using Bayesian optimization by comparing the distribution of the cavitation damage obtained from experiment with that of accumulated plastic strain obtained from the simulation. It was found that the results obtained using the Weibull distribution reproduced the actual cavitation erosion phenomenon better than the other results.

Journal Articles

Cavitation damage prediction in mercury target for pulsed spallation neutron sources by Monte Carlo simulation

Wakui, Takashi; Takagishi, Yoichi*; Futakawa, Masatoshi; Tanabe, Makoto*

Jikken Rikigaku, 23(2), p.168 - 174, 2023/06

Cavitation damage on the inner surface of the mercury target for the spallation neutron source occurs by proton bombarding in mercury. The prediction method of the cavitation damage using Monte Carlo simulations was suggested taking variability of the bubble core position and impact pressure distribution into account. The impact pressure distribution was estimated using the inverse analysis with Bayesian optimization was conducted with comparison between cavitation damage distribution obtained from experiment and the cumulative plastic strain distribution obtained from simulation. The average value and spread of maximum impact pressure estimated assuming the Gaussian distribution were 3.1 GPa and 1.2 $$mu$$m, respectively. Simulation results reproduced experimental results and it can be said that this evaluation method is useful.

JAEA Reports

Technical note for the cavitation damage inspection for interior surface of the mercury target vessel, 1; Development of specimen cutting machine for remote handling

Naoe, Takashi; Kinoshita, Hidetaka; Wakui, Takashi; Kogawa, Hiroyuki; Haga, Katsuhiro

JAEA-Technology 2022-018, 43 Pages, 2022/08

JAEA-Technology-2022-018.pdf:7.84MB

In the liquid mercury target system for the pulsed spallation neutron source of Materials and Life science experimental Facility (MLF) at the Japan in the Japan Proton Accelerator Research Complex (J-PARC), cavitation that is generated by the high-energy proton beam-induced pressure waves, resulting severe erosion damage on the interior surface of the mercury target vessel. The erosion damage is increased with increasing the proton beam power, and has the possibility to cause the leakage of mercury by the penetrated damage and/or the fatigue failure originated from erosion pits during operation. To achieve the long term stable operation under high-power proton beam, the mitigation technologies for cavitation erosion consisting of surface modification on the vessel interior surface, helium gas microbubble injection, double-walled beam window structure has been applied. The damage on interior surface of the vessel is never observed during the beam operation. Therefore, after the target operation term ends, we have cut out specimen from the target nose of the target vessel to inspect damaged surface in detail for verification of the cavitation damage mitigation technologies and lifetime estimation. We have developed the techniques of specimen cutting out by remote handling under high-radiation environment. Cutting method was gradually updated based on experience in actual cutting for the used target vessel. In this report, techniques of specimen cutting out for the beam entrance portion of the target vessel in high-radiation environment and overview of the results of specimen cutting from actual target vessels are described.

Journal Articles

Material properties evaluation on radiation shielding lead glasses irradiated by pulsed laser

Wakui, Takashi; Yamasaki, Kazuhiko*; Futakawa, Masatoshi

Advanced Experimental Mechanics, 7, p.103 - 109, 2022/08

As part of the development of technique to cut and reduce the volume of highly radioactive components in the closed space, pulsed Nd:YAG laser was irradiated to radiation shielding glasses with the different lead content in the different irradiation condition; power and number of irradiation. The large black irradiated area with concave shape and cracks around it occurred with an increase of the lead content, power and number of irradiation. General mechanical properties in unirradiated and irradiated area were investigated to investigate the influence of mechanical properties on the irradiation damage. The thermal impact fracture toughness calculated based on the estimated mechanical properties decreased with increasing the lead content. The micro hardness in black irradiated area was 10% smaller than that in the unirradiated area. The change of the mechanical property due to the laser irradiation was confirmed.

Journal Articles

Effect of pulsed laser irradiation on the micro-plastic behavior of radiation shielding lead glasses

Wakui, Takashi; Yamasaki, Kazuhiko*; Futakawa, Masatoshi

Jikken Rikigaku, 22(2), p.96 - 104, 2022/06

Pulsed laser irradiation and indentation tests on radiation shielding glasses and a lead-free glass were carried out. The size of irradiation damage of the glass with high lead content was larger than that with low content. The micro plastic behavior of glasses was quantitatively determined using the inverse analyses based on indentation results. Flow stress decreased with an increase of lead content and that in irradiated area was lower than that in unirradiated area. On the other hand, plastic flow resistance increased with an increase of the lead content and that in irradiated area was higher than that in unirradiated area. Fracture energy and critical size of plastic zone around tip of crack in unirradiated and irradiated areas were calculated based on experimental results including constants evaluated using the inverse analysis. These values decreased with an increase of the lead content and these values in irradiated area were lower than that in unirradiated area.

Journal Articles

Development of the high-power spallation neutron target of J-PARC

Haga, Katsuhiro; Kogawa, Hiroyuki; Naoe, Takashi; Wakui, Takashi; Wakai, Eiichi; Futakawa, Masatoshi

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 13 Pages, 2022/03

The cross-flow type target was developed as the basic design of mercury target in J-PARC, and the design has been improved to realize the MW-class pulsed spallation neutron source. When the high-power and short-pulsed proton beam is injected into the mercury target, pressure waves are generated in mercury by rapid heat generation. The pressure waves induce the cavitation damages on the target vessel. Two countermeasures were adopted, namely, the injection of microbubbles into mercury and the double walled structure at the beam window. The bubble generator was installed in the target vessel to absorb the volume inflation of mercury and mitigate the pressure waves. Also, the double walled target vessel was designed to suppress the cavitation damage by the large velocity gradient of rapid mercury flow in the narrow channel of double wall. Finally, we could attain 1 MW beam operation with the duration time of 36.5 hours in 2020, and achieved the long term stable operation with 740 kW from April in 2021. This report shows the technical development of the high-power mercury target vessel in view of thermal hydraulics to attain 1 MW operation.

Journal Articles

Effect of gas microbubble injection and narrow channel structure on cavitation damage in mercury target vessel

Naoe, Takashi; Kinoshita, Hidetaka; Kogawa, Hiroyuki; Wakui, Takashi; Wakai, Eiichi; Haga, Katsuhiro; Takada, Hiroshi

Materials Science Forum, 1024, p.111 - 120, 2021/03

The mercury target vessel for the at the J-PARC neutron source is severely damaged by the cavitation caused by proton beam-induced pressure waves in mercury. To mitigate the cavitation damage, we adopted a double-walled structure with a narrow channel for the mercury at the beam window of the vessel. In addition, gas microbubbles were injected into the mercury to suppress the pressure waves. The front end of the vessel was cut out to inspect the effect of the damage mitigation technologies on the interior surface. The results showed that the double-walled target facing the mercury with gas microbubbles operating at 1812 MWh for an average power of 434 kW had equivalent damage to the single-walled target without microbubbles operating 1048 MWh for average power of 181 kW. The erosion depth due to cavitation in the narrow channel was clearly smaller than it was on the wall facing the bubbling mercury

Journal Articles

New design of high power mercury target vessel of J-PARC

Wakui, Takashi; Wakai, Eiichi; Kogawa, Hiroyuki; Naoe, Takashi; Hanano, Kohei*; Haga, Katsuhiro; Shimada, Tsubasa*; Kanomata, Kenichi*

Materials Science Forum, 1024, p.145 - 150, 2021/03

To realize a high beam power operation at the J-PARC, a mercury target vessel covered with water shroud was developed. In the first step, to realize an operation at 500 kW, the basic structure of the initial design was followed and the connection method between the mercury vessel and the water shroud was changed. Additionally, the operation at a beam power of 500 kW was realized in approximately eight months. In the second step, to realize the operation at 1 MW, the new structure in which only rear ends of vessels were connected was investigated. Cooling of the mercury vessel is used to reduce thermal stress and thick vessels of the water shroud are used to increase stiffness for the internal pressure; therefore, it was adopted. The stress in each vessel was lower than the allowable stress based on the pressure vessel code criteria prescribed in the Japan Industrial Standard, and confirmation was obtained that the operation with a beam power of 1 MW could be conducted.

Journal Articles

Pressure wave induced sound measurement for diagnosing the operation status of the J-PARC pulsed spallation neutron source

Naoe, Takashi; Kogawa, Hiroyuki; Wakui, Takashi; Teshigawara, Makoto; Haga, Katsuhiro; Futakawa, Masatoshi

Nuclear Instruments and Methods in Physics Research A, 982, p.164566_1 - 164566_6, 2020/12

 Times Cited Count:2 Percentile:25.94(Instruments & Instrumentation)

A liquid mercury target for the spallation neutron source is installed in the J-PARC. The liquid mercury is enclosed with the multi-walled stainless steel vessel. At the time of highly intense proton beams hits the target at a repetition rate of 25 Hz, pressure waves, that causes cavitation erosion, are generated owing the rapidly thermal expansion of mercury. We have installed the target diagnostic system consisting of a laser Doppler vibrometer (LDV) and a dynamic microphone to remotely investigate the structural integrity of the target under high-radiation environment. In this study, aiming to understand correlation between the acoustic vibration and the operation conditions such as the proton beam power and beam profile, proton beam induced acoustic vibration was measured by parametrically changing the target operation conditions. The result showed that the sound is well correlated with the operation conditions.

Journal Articles

Water leakage due to the welding defect and improvement to reach 1-MW beam operation in the mercury target of J-PARC

Kogawa, Hiroyuki; Wakui, Takashi; Naoe, Takashi; Haga, Katsuhiro; Takada, Hiroshi; Futakawa, Masatoshi

Journal of Nuclear Science and Technology, 57(5), p.487 - 494, 2020/05

 Times Cited Count:1 Percentile:12.16(Nuclear Science & Technology)

Neutron flux per pulse reached world record at neutron source in the J-PARC. In the J-PARC, mercury target system is used as a spallation neutron source. A target vessel has the multi-walled protection system that comprises a mercury vessel enclosed with a double-walled water shroud. This is to prevent the leakage of the mercury outside the mercury vessel. The multi-walled structure needed to be complicated with a lot of welding lines. However, during the operation, we faced an unscheduled shutdown due to water leakage to the intermediate layer between the mercury vessel and water shroud. An investigation on the cause of the leakage was carried out. It is deduced that the leakage path was formed due to the crack propagation from welding defects that is caused by the complicated multi-walled structure. The crack propagation is attributed to the repeated stress by pressure waves generated in the mercury target. Based on the investigation results, the design was improved to remove the welding line on the complicated structure and to realize the stable operation with 1 MW proton beam.

Journal Articles

How different is the core of $$^{25}$$F from $$^{24}$$O$$_{g.s.}$$ ?

Tang, T. L.*; Uesaka, Tomohiro*; Kawase, Shoichiro; Beaumel, D.*; Dozono, Masanori*; Fujii, Toshihiko*; Fukuda, Naoki*; Fukunaga, Taku*; Galindo-Uribarri, A.*; Hwang, S. H.*; et al.

Physical Review Letters, 124(21), p.212502_1 - 212502_6, 2020/05

 Times Cited Count:14 Percentile:74.18(Physics, Multidisciplinary)

The structure of a neutron-rich $$^{25}$$F nucleus is investigated by a quasifree ($$p,2p$$) knockout reaction. The sum of spectroscopic factors of $$pi 0d_{5/2}$$ orbital is found to be 1.0 $$pm$$ 0.3. The result shows that the $$^{24}$$O core of $$^{25}$$F nucleus significantly differs from a free $$^{24}$$O nucleus, and the core consists of $$sim$$35% $$^{24}$$O$$_{rm g.s.}$$, and $$sim$$65% excited $$^{24}$$O. The result shows that the $$^{24}$$O core of $$^{25}$$F nucleus significantly differs from a free $$^{24}$$O nucleus. The result may infer that the addition of the $$0d_{5/2}$$ proton considerably changes the neutron structure in $$^{25}$$F from that in $$^{24}$$O, which could be a possible mechanism responsible for the oxygen dripline anomaly.

Journal Articles

Mitigation of cavitation damage in J-PARC mercury target vessel

Naoe, Takashi; Kinoshita, Hidetaka; Kogawa, Hiroyuki; Wakui, Takashi; Wakai, Eiichi; Haga, Katsuhiro; Takada, Hiroshi

JPS Conference Proceedings (Internet), 28, p.081004_1 - 081004_6, 2020/02

The beam window of the mercury target vessel in J-PARC is severely damaged by the cavitation. The cavitation damage is a crucial factor to limit lifetime of the target because it increases with the beam power. Therefore, mitigating cavitation damage is an important issue to operate the target stably for long time at 1 MW. At J-PARC, to mitigate the cavitation damage: gas microbubbles are injected into mercury for suppressing pressure waves, and double-walled structure with a narrow channel of 2 mm in width to form high-speed mercury flow ($$sim$$4m/s) has been adopted. After operation, the beam window was cut to inspect the effect of the cavitation damage mitigation on inner wall. We optimized cutting conditions through the cold cutting tests, succeeding in cutting the target No.2 (without damage mitigation technologies) smoothly in 2017, and target No.8 with damage mitigation technologies. In the workshop, progress of cavitation damage observation for the target vessel will be presented.

Journal Articles

New design and fabrication technology applied in mercury target vessel #8 of J-PARC

Wakui, Takashi; Wakai, Eiichi; Kogawa, Hiroyuki; Naoe, Takashi; Hanano, Kohei; Haga, Katsuhiro; Takada, Hiroshi; Shimada, Tsubasa*; Kanomata, Kenichi*

JPS Conference Proceedings (Internet), 28, p.081002_1 - 081002_6, 2020/02

A mercury target vessel of J-PRAC is designed with a triple-walled structure consisting of the mercury vessel and a double-walled water shroud with internal and external vessels. During the beam operation at 500 kW in 2015, small water leakages from a water shroud of the mercury target vessel occurred twice. Design, fabrication and inspection processes were improved based on the lessons learned from the target failures. The total length of welding lines at the front of the mercury target vessel decreases drastically to approximately 55% by adopting monolithic structure cut out from a block of stainless steel by the wire-electrical discharge machining. Thorough testing of welds by radiographic testing and ultrasonic testing was conducted. The fabrication of the mercury target vessel #8 was finished on September 2017 and the beam operation using it started. Stable beam operation at 500 kW has been achieved and it could experience the maximum beam power of 1 MW during a beam test.

Journal Articles

Optimum temperature for HIP bonding invar alloy and stainless steel

Wakui, Takashi; Ishii, Hideaki*; Naoe, Takashi; Kogawa, Hiroyuki; Haga, Katsuhiro; Wakai, Eiichi; Takada, Hiroshi; Futakawa, Masatoshi

Materials Transactions, 60(6), p.1026 - 1033, 2019/06

 Times Cited Count:3 Percentile:17.96(Materials Science, Multidisciplinary)

The mercury target has large size as 1.3$$times$$1.3$$times$$2.5 m$$^{3}$$. In view of reducing the amount of wastes, we studied the structure so that the fore part could be separated. The flange is required to have high seal performance less than 1$$times$$10$$^{-6}$$ Pa m$$^{3}$$/s. Invar with low thermal expansion is a candidate. Due to its low stiffness, however, the flange may deform when it is fastened by bolts. Practically invar is reinforced with stainless steel where all interface between them has to be bonded completely with the HIP bonding. In this study, we made specimens at four temperatures and conducted tensile tests. The specimen bonded at 973 K had little diffusion layer, and so fractured at the interface. The tensile strength reduced with increasing the temperature, and the reduced amount was about 10% at 1473 K. The analyzed residual stresses near the interface increased by 50% at maximum. Then, we concluded that the optimum temperature was 1173 K.

Journal Articles

Ultrasonic inspection technique for weld part of mercury target vessel for spallation neutron source

Wakui, Takashi; Wakai, Eiichi; Naoe, Takashi; Kogawa, Hiroyuki; Haga, Katsuhiro; Takada, Hiroshi; Shintaku, Yohei*; Li, T.*; Kanomata, Kenichi*

Choompa Techno, 30(5), p.16 - 20, 2018/10

A mercury target vessel has been used for the spallation neutron source at J-PARC. It has a complicated multi-layered structure composed of a mercury target and a surrounding double-walled water shroud, which is assembled with thin plates (minimum thickness of 3 mm) by welding. Thus, welding inspection during the manufacturing process is important. We investigated the applicability of new ultrasonic inspections using specimens (thickness of 3 mm) with defects to improve the accuracy of welding inspection for the mercury target vessel. Immersion ultrasonic testing using a probe (frequency of 50 MHz) could detect a spherical defect with a diameter of 0.2 mm. The size was smaller than target value of 0.4 mm. The length of unwelded region estimated using the phased array ultrasonic testing corresponded with the actual length (0.8 - 1.5 mm).

Journal Articles

Effect of welding on gigacycle fatigue strength of austenitic stainless steels

Naoe, Takashi; Wakui, Takashi; Kogawa, Hiroyuki; Wakai, Eiichi; Haga, Katsuhiro; Takada, Hiroshi

Advanced Experimental Mechanics, 3, p.123 - 128, 2018/08

A mercury target vessel, composed of SUS316L, is used for the pulsed neutron source and is assembled via TIG welding. While in operation, the target vessel suffers ca. 10$$^9$$ loading cycles with a high strain rate of ca. 50 s$$^{-1}$$ because of the proton-beam-induced pressure waves in mercury. The gigacycle fatigue strength for solution annealed SUS316L stainless steels and its welded specimens were investigated through ultrasonic fatigue tests. The experimental results showed that an obvious fatigue limit was not observed at fewer than 10$$^9$$ cycles for the base metal. In the case of no weld defects observed via penetration tests, the fatigue strength of the removed-weld-bead specimen, in which the weld lines were arranged at the center of the specimen, appeared to be slightly higher than that of the base metal. By contrast, as-welded specimens with the weld bead intact showed apparent degradation of the fatigue strength owing to the stress concentration around the weld toe.

Journal Articles

Cavitation damage in double-walled mercury target vessel

Naoe, Takashi; Wakui, Takashi; Kinoshita, Hidetaka; Kogawa, Hiroyuki; Haga, Katsuhiro; Harada, Masahide; Takada, Hiroshi; Futakawa, Masatoshi

Journal of Nuclear Materials, 506, p.35 - 42, 2018/08

BB2016-1013.pdf:0.96MB

 Times Cited Count:6 Percentile:52.79(Materials Science, Multidisciplinary)

A mercury target vessel made of 316L SS is damaged due to the cavitation caused by the pressure waves in mercury. Cavitation damage reduces the structural integrity of the target front, called "beam window", being major factor to determine the lifetime of target vessel. Aiming at mitigating the cavitation damage by faster mercury flow in narrow channel, we employed a target vessel with a double-walled structure at the beam window along with a gas microbubbles injection. After operating the double-walled target vessel with a beam power of 300 to 500 kW, we cut out the beam window using an annular cutter to examine the damage inside it, and found that damages with maximum pit depth of approximately 25 $$mu$$m distributed in a belt on the specimen facing narrow channel. Furthermore, numerical simulation result showed that the distribution of negative pressure period from beam injection to 1 ms was correlated with the damage distribution in the narrow channel. It was suggested that the cavitation induced by relatively short negative pressure period contributed to the damage formation.

Journal Articles

Recent studies for structural integrity evaluation and defect inspection of J-PARC spallation neutron source target vessel

Wakui, Takashi; Wakai, Eiichi; Naoe, Takashi; Shintaku, Yohei*; Li, T.*; Murakami, Kazuya*; Kanomata, Kenichi*; Kogawa, Hiroyuki; Haga, Katsuhiro; Takada, Hiroshi; et al.

Journal of Nuclear Materials, 506, p.3 - 11, 2018/08

 Times Cited Count:3 Percentile:30.05(Materials Science, Multidisciplinary)

The mercury target vessel is designed as multi-walled structure with thin wall (min. 3 mm), and assembled by welding. In order to estimate the structural integrity of the vessel, it is important to measure the defects in welding accurately. For nondestructive tests of the welding, radiographic testing is applicable but it is difficult to detect for some defect shapes. Therefore it is effective to do ultrasonic testing together with it. Because ultrasonic methods prescribed in JIS inspect on the plate with more than 6 mm in thickness, these methods couldn't be applied as the inspection on the vessel with thin walls. In order to develop effective method, we carried out measurements using some testing method on samples with small defect whose size is specified. In the case of the latest phased array method, measured value agreed with actual size. It was found that this method was applicable to detect defects in the thin-walled structure for which accurate inspection was difficult so far.

Journal Articles

Off-gas processing system operations for mercury target vessel replacement at J-PARC

Kai, Tetsuya; Uchida, Toshitsugu; Kinoshita, Hidetaka; Seki, Masakazu; Oi, Motoki; Wakui, Takashi; Haga, Katsuhiro; Kasugai, Yoshimi; Takada, Hiroshi

Journal of Physics; Conference Series, 1021(1), p.012042_1 - 012042_4, 2018/06

 Times Cited Count:0 Percentile:0.11(Nuclear Science & Technology)

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