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JAEA Reports

Utilization of gamma ray irradiation at the WASTEF Facility

Sano, Naruto; Yamashita, Naoki; Watanabe, Masaya; Tsukada, Manabu*; Hoshino, Kazutoyo*; Hirai, Koki; Ikegami, Yuta*; Tashiro, Shinsuke; Yoshida, Ryoichiro; Hatakeyama, Yuichi; et al.

JAEA-Technology 2023-029, 36 Pages, 2024/03

JAEA-Technology-2023-029.pdf:2.47MB

At the Waste Safety Testing Facility (WASTEF), the gamma ray irradiation device "Gamma Cell 220" was relocated from the 4th research building of the Nuclear Science Research Institute in FY2019, and the use of gamma ray irradiation has begun. Initially, Fuel Cycle Safety Research Group, Fuel Cycle Safety Research Division, Nuclear Safety Research Center, Sector of Nuclear Safety Research and Emergency Preparedness, the owner of this device, conducted the tests as the main user, but since 2022, other users, including those outside the organization, have started using it. The gamma ray irradiation device "Gamma Cell 220" is manufactured by Nordion International Inc. in Canada. Since it was purchased in 1989, the built-in 60Co radiation source has been updated once, and safety research related to nuclear fuel cycles, etc. It is still used for this purpose to this day. This report summarizes the equipment overview of the gamma ray irradiation device "Gamma Cell 220", its permits and licenses at WASTEF, usage status, maintenance and inspection, and future prospects.

Journal Articles

Neutron production in the interaction of 200-MeV deuterons with Li, Be, C, Al, Cu, Nb, In, Ta, and Au

Watanabe, Yukinobu*; Sadamatsu, Hiroki*; Araki, Shohei; Nakano, Keita; Kawase, Shoichiro*; Kin, Tadahiro*; Iwamoto, Yosuke; Satoh, Daiki; Hagiwara, Masayuki*; Yashima, Hiroshi*; et al.

EPJ Web of Conferences, 284, p.01041_1 - 01041_4, 2023/05

 Times Cited Count:0 Percentile:0.21(Nuclear Science & Technology)

Intensive fast neutron sources using deuteron accelerators have been proposed for the study of medical RI production, radiation damage for fusion reactor materials, nuclear transmutation of radioactive waste, and so on. Neutron production data from various materials bombarded by deuterons are required for the design of such neutron sources. In the present work, we have conducted a systematic measurement of double-differential neutron production cross sections (DDXs) for a wide atomic number range of targets (Li, Be, C, Al, Cu, Nb, In, Ta, and Au) at an incident energy of 200 MeV in the Research Center for Nuclear Physics (RCNP), Osaka University. A deuteron beam accelerated to 200 MeV was transported to the neutron experimental hall and focused on a thin target foil. Emitted neutrons from the target were detected by two different-size EJ301 liquid organic scintillators located at two distances of 7 m and 20 m, respectively. The neutron DDXs were measured at six angles from 0$$^{circ}$$ to 25$$^{circ}$$). The neutron energy was determined by a conventional time-of-flight (TOF) method. The measured DDXs were compared with theoretical model calculations by the DEUteron-induced Reaction Analysis Code System (DEURACS) and PHITS. The result indicated that the DEURACS calculation provides better agreement with the measured DDXs than the PHITS calculation.

Journal Articles

Free-surface flow simulations with floating objects using lattice Boltzmann method

Watanabe, Seiya*; Kawahara, Jun*; Aoki, Takayuki*; Sugihara, Kenta; Takase, Shinsuke*; Moriguchi, Shuji*; Hashimoto, Hirotada*

Engineering Applications of Computational Fluid Mechanics, 17(1), p.2211143_1 - 2211143_23, 2023/00

 Times Cited Count:1 Percentile:61.52(Engineering, Multidisciplinary)

In tsunami inundations or slope disasters of heavy rain, a lot of floating debris or driftwood logs are included in the flows. The damage to structures from solid body impacts is more severe than the damage from the water pressure. In order to study free-surface flows that include floating debris, developing a high-accurate simulation code of free-surface flows with high performance for large-scale computations is desired. We propose the single-phase free-surface flow model based on the cumulant lattice Boltzmann method coupled with a particle-based rigid body simulation. The discrete element method calculates the contact interaction between solids. An octree-based AMR (Adaptive Mesh Refinement) method is introduced to improve computational accuracy and time-to-solution. High-resolution grids are assigned near the free surfaces and solid boundaries. We conducted two kinds of tsunami flow experiments in the 15 and 70 m water tanks at Hachinohe Institute of Technology and Kobe University to validate the accuracy of the proposed model. The simulation results have shown good agreement with the experiments for the drifting speed, the number of trapped wood pieces, and the stacked angles.

Journal Articles

Calculation of deuteron-induced reaction cross-sections for nuclear transmutation of long-lived fission products

Nakayama, Shinsuke; Furutachi, Naoya; Iwamoto, Osamu; Watanabe, Yukinobu*

NEA/NSC/R(2020)4 (Internet), p.345 - 349, 2022/10

Long-lived fission products (LLFPs) generated in nuclear reactors are strongly desired to be converted to stable or short-lived nuclides. Recently, it has been considered to transmute LLFPs by spallation reactions with high energy particles, and some experimental studies revealed that spallation reaction cross-sections induced by deuteron are larger than proton-induced ones. These results suggest the possibility that nuclear transmutation of LLFPs using deuteron beams is more efficient than one using proton beams. On the other hand, we have been developing a code system dedicated for deuteron-induced reactions, called DEURACS. DEURACS has been originally developed to contribute to the design of deuteron accelerator neutron sources. In the present study, we apply DEURACS to calculation of deuteron-induced spallation reactions on LLFPs. Through comparison with measured data, the applicability of DEURACS will be discussed.

Journal Articles

Clogging properties of HEPA filter induced by loading of soot from burned glove-box panel materials

Tashiro, Shinsuke; Ono, Takuya; Amano, Yuki; Yoshida, Ryoichiro; Watanabe, Koji*; Abe, Hitoshi

Nuclear Technology, 208(10), p.1553 - 1561, 2022/10

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

To contribute to the confinement safety evaluation of the radioactive materials in the Glove box (GB) fire accident, combustion tests with the Polymethyl methacrylate (PMMA) and the Polycarbonate (PC) as typical panel materials for the GB have been conducted with a relatively large scale apparatus. As the important data for evaluating confinement safety, the release ratio and the particle size distribution of the soot generated from the burned materials were obtained. Furthermore, the rise of the differential pressure ($$Delta$$P) of the high efficiency particle air (HEPA) filter by the soot loading was also investigated. As results, the release ratio of the soot from the PC was about seven times as large as the PMMA. In addition, it was found that the behavior of the rise of the $$Delta$$P with soot loading could be represented uniformly regardless of kinds of combustion materials by considering effect of the loading volume of the soot particle in the relatively low loading region.

Journal Articles

Theoretical study of deuteron-induced reactions in the nuclear data field

Nakayama, Shinsuke; Iwamoto, Osamu; Watanabe, Yukinobu*; Ogata, Kazuyuki*

Few-Body Systems, 63(1), p.4_1 - 4_6, 2022/03

 Times Cited Count:0 Percentile:0(Physics, Multidisciplinary)

Intensive neutron sources using deuteron accelerators have been proposed for not only science and engineering fields but also medical applications. For the engineering design of such facilities, accurate and comprehensive nuclear data of deuteron-induced reactions are indispensable. However, it is difficult to meet the requirement by employing experimental data alone. Thus, theoretical model calculations play a key role in completing the necessary nuclear data by interpolation and extrapolation of experimental data. Under the above situations, we have been developing a code system dedicated for deuteron-induced reactions, called DEURACS. In the present work, calculations using DEURACS are compared with available experimental data and validation of the present modelling in DEURACS is discussed. Moreover, the importance of consideration of the breakup processes for accurate prediction of deuteron-induced reactions is also presented.

Journal Articles

PSTEP: Project for solar-terrestrial environment prediction

Kusano, Kanya*; Ichimoto, Kiyoshi*; Ishii, Mamoru*; Miyoshi, Yoshizumi*; Yoden, Shigeo*; Akiyoshi, Hideharu*; Asai, Ayumi*; Ebihara, Yusuke*; Fujiwara, Hitoshi*; Goto, Tadanori*; et al.

Earth, Planets and Space (Internet), 73(1), p.159_1 - 159_29, 2021/12

 Times Cited Count:6 Percentile:51.19(Geosciences, Multidisciplinary)

The PSTEP is a nationwide research collaboration in Japan and was conducted from April 2015 to March 2020, supported by a Grant-in-Aid for Scientific Research on Innovative Areas from the Ministry of Education, Culture, Sports, Science and Technology of Japan. It has made a significant progress in space weather research and operational forecasts, publishing over 500 refereed journal papers and organizing four international symposiums, various workshops and seminars, and summer school for graduate students at Rikubetsu in 2017. This paper is a summary report of the PSTEP and describes the major research achievements it produced.

Journal Articles

JENDL/DEU-2020; Deuteron nuclear data library for design studies of accelerator-based neutron sources

Nakayama, Shinsuke; Iwamoto, Osamu; Watanabe, Yukinobu*; Ogata, Kazuyuki*

Journal of Nuclear Science and Technology, 58(7), p.805 - 821, 2021/07

 Times Cited Count:20 Percentile:96.99(Nuclear Science & Technology)

Intensive fast neutron sources using deuteron accelerators have been proposed for various applications. To contribute to the design study of such neutron sources, a deuteron nuclear data library for $$^{6,7}$$Li, $$^{9}$$Be, and $$^{12,13}$$C up to 200 MeV, JENDL/DEU-2020 is developed. The evaluation of JENDL/DEU-2020 are performed by employing the code system DEURACS with particular attention to neutron production data. Toward the evaluation of JENDL/DEU-2020, some modifications are made to DEURACS. The validation of the library is performed though simulation with the Monte Carlo transport calculation codes. From the simulation, it is shown that the calculation results based on JENDL/DEU-2020 reproduce the measured neutron production data well in the incident energies up to 200 MeV. The new library is expected to make a large contribution to diverse design studies of deuteron accelerator neutron sources.

Journal Articles

Thermally altered subsurface material of asteroid (162173) Ryugu

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.

Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03

 Times Cited Count:43 Percentile:96.93(Astronomy & Astrophysics)

Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 $$^{circ}$$C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 $$^{circ}$$C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.

Journal Articles

Measurement of double-differential thick-target neutron yields of the C($$d,n$$) reaction at 12, 20, and 30 MeV

Patwary, M. K. A*; Kin, Tadahiro*; Aoki, Katsumi*; Yoshinami, Kosuke*; Yamaguchi, Masaya*; Watanabe, Yukinobu*; Tsukada, Kazuaki; Sato, Nozomi*; Asai, Masato; Sato, Tetsuya; et al.

Journal of Nuclear Science and Technology, 58(2), p.252 - 258, 2021/02

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

While designing deuteron accelerator neutron sources for radioisotopes production, nuclear data for light elements such as Li, Be, and C have been systematically measured in the deuteron energy range from a few MeV to around 50 MeV. Currently, the experimental data available on double-differential thick-target neutron yields (DDTTNYs) is insufficient, especially for deuteron energies between 18 and 33 MeV. In this study, we measured the DDTTNYs of ($$d,n$$) reactions on $$^{rm nat}$$C target for incident deuteron energies of 12, 20, and 30 MeV using the multiple-foils activation method to improve nuclear data insufficiency. We applied the GRAVEL code for the unfolding process to derive the DDTTNYs. The results were compared with the calculation by DEURACS. The present data were also used to confirm the systematics of the differential neutron yields at 0$$^{circ}$$ and total neutron yield per incident deuteron in the wide range of deuteron energy.

Journal Articles

Study of the Li($$d,xn$$) reaction for the development of accelerator-based neutron sources

Watanabe, Yukinobu*; Sadamatsu, Hiroki*; Araki, Shohei*; Nakano, Keita*; Kawase, Shoichiro*; Kin, Tadahiro*; Iwamoto, Yosuke; Satoh, Daiki; Hagiwara, Masayuki*; Yashima, Hiroshi*; et al.

EPJ Web of Conferences, 239, p.20012_1 - 20012_4, 2020/09

 Times Cited Count:2 Percentile:86.93(Nuclear Science & Technology)

Accelerator-based neutron sources induced by deuteron beams are attractive for study of nuclear transmutation of radioactive waste as well as radiation damage for fusion reactor materials. In the present work, we have carried out a Double Differential cross section (DDX) measurement for Li at 200 MeV in the Research Center for Nuclear Physics (RCNP), Osaka University. A deuteron beam accelerated to 200 MeV was transported to the neutron experimental hall and focused on a thin Li target. Emitted neutrons from the target were detected by two different-size EJ301 liquid organic scintillators located at two distances of 7 m and 20 m, respectively. The neutron DDXs were measured at six angles from 0$$^{circ}$$ to 25$$^{circ}$$). The neutron detection efficiencies of the detectors were calculated by SCINFUL-QMD code. We will present the results of the present DDX measurement and compare them with theoretical model calculations with DEURACS and PHITS.

Journal Articles

Recent progress of a code system DEURACS toward deuteron nuclear data evaluation

Nakayama, Shinsuke; Iwamoto, Osamu; Watanabe, Yukinobu*

EPJ Web of Conferences, 239, p.03014_1 - 03014_4, 2020/09

 Times Cited Count:2 Percentile:86.93(Nuclear Science & Technology)

Intensive neutron sources using deuteron accelerators have been proposed for various applications such as irradiation test for fusion reactor materials and production of radioisotopes for medical use. In addition, transmutation system using deuteron-induced spallation reactions has been recently proposed for LLFPs. Accurate and comprehensive deuteron nuclear data are indispensable in the design study of such facilities. Under the above situations, we have been developing a code system dedicated for deuteron-induced reactions, which is called DEURACS. In the present work, calculations using DEURACS are compared with available experimental data up to 200 MeV such as DDXs for emission of neutron or light charged particles. We also analyze isotopic production cross sections of residual nuclei. Validation of the present modelling in DEURACS is discussed through comparison with the experimental data.

Journal Articles

Spallation and fragmentation cross sections for 168 MeV/nucleon $$^{136}$$Xe ions on proton, deuteron, and carbon targets

Sun, X. H.*; Wang, H.*; Otsu, Hideaki*; Sakurai, Hiroyoshi*; Ahn, D. S.*; Aikawa, Masayuki*; Fukuda, Naoki*; Isobe, Tadaaki*; Kawakami, Shunsuke*; Koyama, Shumpei*; et al.

Physical Review C, 101(6), p.064623_1 - 064623_12, 2020/06

 Times Cited Count:5 Percentile:52.72(Physics, Nuclear)

The spallation and fragmentation reactions of $$^{136}$$Xe induced by proton, deuteron and carbon at 168 MeV/nucleon were studied at RIKEN Radioactive Isotope Beam Factory via the inverse kinematics technique. The cross sections of the lighter products are larger in the carbon-induced reactions due to the higher total kinetic energy of carbon. The energy dependence was investigated by comparing the newly obtained data with previous results obtained at higher reaction energies. The experimental data were compared with the results of SPACS, EPAX, PHITS and DEURACS calculations. These data serve as benchmarks for the model calculations.

Journal Articles

JENDL/ImPACT-2018; A New nuclear data library for innovative studies on transmutation of long-lived fission products

Kunieda, Satoshi; Furutachi, Naoya; Minato, Futoshi; Iwamoto, Nobuyuki; Iwamoto, Osamu; Nakayama, Shinsuke; Ebata, Shuichiro*; Yoshida, Toru*; Nishihara, Kenji; Watanabe, Yukinobu*; et al.

Journal of Nuclear Science and Technology, 56(12), p.1073 - 1091, 2019/12

 Times Cited Count:8 Percentile:66.68(Nuclear Science & Technology)

A new nuclear data library, JENDL/ImPACT-2018, is developed for an innovative study on the transmutation of long-lived fission products. Nuclear reaction cross- sections are newly evaluated for incident neutrons and protons up to 200 MeV for 163 nuclides including long-lived nuclei such as $$^{79}$$Se, $$^{93}$$Zr, $$^{107}$$Pd and $$^{135}$$Cs. Our challenge is an evaluation of cross-sections for a number of unstable nuclei over a wide energy range where the experimental data are very scarce. We estimated cross- sections based on a nuclear model code CCONE that incorporates an advanced knowledge on the nuclear structure theory and a model-parameterization based on a new experimental cross-sections measured by the inverse kinematics. Through comparisons with available experimental data on the stable isotopes, it is found that the present data give predictions of cross-sections better than those in the existing libraries.

Journal Articles

Consistent description of light composite particle emission in deuteron-induced reactions

Nakayama, Shinsuke; Iwamoto, Osamu; Watanabe, Yukinobu*

Physical Review C, 100(4), p.044603_1 - 044603_8, 2019/10

 Times Cited Count:7 Percentile:59.68(Physics, Nuclear)

The weakly-bound nature of the deuteron brings the complexity of deuteron-induced reactions compared to nucleon-induced ones, and is expected to affect various physical quantities observed in deuteron-induced reactions. Aiming to deep understanding and accurate prediction for the emission of light composite particle (LCP) in deuteron-induced reactions, we revise the computational system dedicated to deuteron-induced reactions, called DEURACS. The model by Iwamoto and Harada describing pre-equilibrium cluster emission which was successfully applied to LCP emission innucleon-induced reactions is integrated into the framework of DEURACS, in which the breakup processes of incident deuteron are explicitly taken into account. The phenomenological model by Kalbach is also adopted to estimate the contribution from the direct pickup process. Using the revised DEURACS, we analyze the $$(d,xt)$$, $$(d,xmathrm{^{3}He})$$, and $$(d,xalpha)$$ reactions in the target mass range $$27 leqslant A leqslant 90$$. Regardless of the targets, the calculation results successfully reproduced the experimental data for each reaction, simultaneously. These results demonstrates that the LCP emission from the pre-equilibrium and compound nucleus processes in deuteron-induced reactions,which occupies a large part of the total LCP emission,can be described by the same theoretical models as used in nucleon-induced reactions when the breakup processes of incident deuteron are properly considered.

Journal Articles

Enhancement of element production by incomplete fusion reaction with weakly bound deuteron

Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.

Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07

 Times Cited Count:8 Percentile:56.2(Physics, Multidisciplinary)

Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for $$^{107}$$Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.

Journal Articles

Role of breakup processes in deuteron-induced spallation reactions at 100-200 MeV/nucleon

Nakayama, Shinsuke; Furutachi, Naoya; Iwamoto, Osamu; Watanabe, Yukinobu*

Physical Review C, 98(4), p.044606_1 - 044606_8, 2018/10

 Times Cited Count:14 Percentile:75.94(Physics, Nuclear)

Use of deuteron-induced spallation reactions at intermediate energies has recently been proposed for transmutation of several long-lived fission products (LLFPs). In the design study of a transmutation system using a deuteron primary beam, accurate cross section data of deuteron-induced reactions on the LLFPs are indispensable. In the present study, production cross sections of residual nuclei in the deuteron-induced reactions on $$^{93}$$Zr and $$^{107}$$Pd at $$100-200$$ MeV/nucleon are analyzed using DEURACS, in which the breakup processes are explicitly taken into account. The calculated values reproduced the experimental data quantitatively well. From a component-by-component analysis, it was found that the components of nucleon absorption make the significant contributions to residual nuclei production. This result strongly indicates that consideration of the breakup processes is essentially important to predict production of residual nuclei in deuteron-induced reactions.

Journal Articles

Theoretical model analysis of $$(d,xn)$$ reactions on $$^7$$Li at 25, 40, and 102 MeV

Sadamatsu, Hiroki*; Nakayama, Shinsuke; Watanabe, Yukinobu*; Iwamoto, Osamu; Ogata, Kazuyuki*

JAEA-Conf 2017-001, p.135 - 140, 2018/01

In recent years, the demand for intense neutron sources has been increasing in various applications such as nuclear transmutation of high-level radioactive waste and medical radioisotopes production. Deuteron accelerator-based neutron sources are promised as one of the candidates. Therefore, we have developed a code system dedicated for the deuteron-induced reactions, called DEURACS. In the present work, we focus on deuteron-induced neutron production from $$^7$$Li target. The calculated double differential cross sections for $$(d,xn)$$ reactions at incident energies of 25, 40, and 102 MeV are compared with the measured ones, and the applicability of DEURACS is discussed.

Journal Articles

Theoretical model analysis of composite-particle emission from deuteron-induced reactions

Nakayama, Shinsuke; Iwamoto, Osamu; Watanabe, Yukinobu*

JAEA-Conf 2017-001, p.91 - 96, 2018/01

Toward evaluation of deuteron nuclear data, we have been developing a code system dedicated for the deuteron-induced reactions, called DEURACS. In the present work, we make an improvement in DEURACS and apply it to composite-particle emission from deuteron-induced reactions. The calculation using DEURACS reproduces the experimental double-differential cross sections of $$(d,xd)$$, $$(d,xt)$$, $$(d,x^3 {rm He})$$, and $$(d,xalpha)$$ reactions on $$^{27}$$Al and $$^{58}$$Ni at incident energy of 80 MeV quantitatively well. From the results of the analyses, it is shown that the treatment of inelastic scattering and pick-up reaction processes is important in the calculation of deuteron-induced composite-particle emission.

Journal Articles

Deuteron nuclear data for the design of accelerator-based neutron sources; Measurement, model analysis, evaluation, and application

Watanabe, Yukinobu*; Kin, Tadahiro*; Araki, Shohei*; Nakayama, Shinsuke; Iwamoto, Osamu

EPJ Web of Conferences, 146, p.03006_1 - 03006_6, 2017/09

 Times Cited Count:2 Percentile:78.04(Nuclear Science & Technology)

The design of $$(d,xn)$$ neutron sources requires comprehensive nuclear data of deuteron-induced reactions. Therefore, we have launched a research project on deuteron nuclear data, which is composed of measurements, theoretical model code development, cross section evaluation, and application to production of radioisotopes for medical use. Our goal is to develop a state-of-art deuteron nuclear data library up to 200 MeV necessary for the design of accelerator neutron sources with deuteron beam. The present status is reported in the presentation.

72 (Records 1-20 displayed on this page)