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Yang, Q.*; Yang, X.*; Wang, Y.*; Fei, Y.*; Li, F.*; Zheng, H.*; Li, K.*; Han, Y.*; Hattori, Takanori; Zhu, P.*; et al.
Nature Communications (Internet), 15, p.7778_1 - 7778_9, 2024/09
Luminescent materials that simultaneously embody bright singlet and triplet excitons hold great potential in optoelectronics, signage, and information encryption. However, achieving high-performance white-light emission is severely hampered by their inherent unbalanced contribution of fluorescence and phosphorescence. Herein, we address this challenge by pressure treatment engineering via hydrogen bonding cooperativity effect to realize the mixture of n-- transitions, where the triplet state emission was boosted from 7% to 40% in isophthalic acid (IPA). A superior white-light emission based on hybrid fluorescence and phosphorescence was harvested in pressure-treated IPA, and the photoluminescence quantum yield was increased to 75% from the initial 19% (blue-light emission). In-situ high-pressure IR spectra, X ray diffraction, and neutron diffraction reveal continuous strengthening of the hydrogen bonds with the increase of pressure. Furthermore, this enhanced hydrogen bond is retained down to the ambient conditions after pressure treatment, awarding the targeted IPA efficient intersystem crossing for balanced singlet/triplet excitons population and resulting in efficient white-light emission. This work not only proposes a route for brightening triplet states in organic small molecule, but also regulates the ratio of singlet and triplet excitons to construct high-performance white-light emission.
Hu, Q.*; Wang, Q. M.*; Zhang, T.*; Zhao, C.*; Iltaf, K. H.*; Liu, S. Q.*; Fukatsu, Yuta
Energy Reports (Internet), 9, p.3661 - 3682, 2023/12
Times Cited Count:4 Percentile:78.27(Energy & Fuels)Yuan, X.*; Hu, Q.*; Lin, X.*; Zhao, C.*; Wang, Q.*; Tachi, Yukio; Fukatsu, Yuta; Hamamoto, Shoichiro*; Siitari-Kauppi, M.*; Li, X.*
Journal of Hydrology, 618, p.129172_1 - 129172_15, 2023/03
Times Cited Count:0 Percentile:0.00(Engineering, Civil)Sheng, J.*; Wang, L.*; Candini, A.*; Jiang, W.*; Huang, L.*; Xi, B.*; Zhao, J.*; Ge, H.*; Zhao, N.*; Fu, Y.*; et al.
Proceedings of the National Academy of Sciences of the United States of America, 119(51), p.e2211193119_1 - e2211193119_9, 2022/12
Times Cited Count:4 Percentile:63.40(Multidisciplinary Sciences)Wang, Q.*; Hu, Q.*; Zhao, C.*; Yang, X.*; Zhang, T.*; Ilavsky, J.*; Kuzmenko, I.*; Ma, B.*; Tachi, Yukio
International Journal of Coal Geology, 261, p.104093_1 - 104093_15, 2022/09
Times Cited Count:5 Percentile:63.89(Energy & Fuels)Sheng, Q.*; Kaneko, Tatsuya*; Yamakawa, Kohtaro*; Guguchia, Z.*; Gong, Z.*; Zhao, G.*; Dai, G.*; Jin, C.*; Guo, S.*; Fu, L.*; et al.
Physical Review Research (Internet), 4(3), p.033172_1 - 033172_14, 2022/09
Zhao, Q.*; Saito, Takeshi*; Miyakawa, Kazuya; Sasamoto, Hiroshi; Kobayashi, Taishi*; Sasaki, Takayuki*
Journal of Hazardous Materials, 428, p.128211_1 - 128211_10, 2022/04
Times Cited Count:5 Percentile:57.04(Engineering, Environmental)The influence of humic acid and its radiological degradation on the sorption of Cs and Eu by sedimentary rock was investigated to understand the sorption process of metal ions and humic substances. Aldrich humic acid (HA) solution was irradiated with different doses of gamma irradiation using a Co-60 gamma-ray source prior to the contact between the metal ions and the solid sorbent. The HA molecule decomposed to smaller molecules with a lower complexation affinity. Batch sorption experiments were performed to evaluate the effect of gamma-irradiated HA on the sorption of Cs and Eu ions. The addition of non-irradiated HA weakened the sorption of Eu because of the lower sorption of the neutral or negatively charged Eu-HA complexes compared with free Eu ions. The sorption of monovalent Cs ions was barely affected by the presence of HA and its gamma irradiation. The concentration ratio of HA complexed species and non-complexed species in the solid and liquid phases was evaluated by sequential filtration and chemical equilibrium calculations. The ratios supported the minimal contribution of HA to Cs sorption. However, the concentration ratio for Eu in the liquid phase was high, indicating that the complexing ability of HA to Eu was higher than that of HA to Cs ions. Therefore, the sorption of free Eu would predominate with the gamma irradiation dose applied to the HA solution under a radiation field near the HLW package.
Hao, Y. Q.*; Wo, H. L.*; Gu, Y. M.*; Zhang, X. W.*; Gu, Y. Q.*; Zheng, S. Y.*; Zhao, Y.*; Xu, G. Y.*; Lynn, J. W.*; Nakajima, Kenji; et al.
Science China; Physics, Mechanics & Astronomy, 64(3), p.237411_1 - 237411_6, 2021/03
Times Cited Count:6 Percentile:59.12(Physics, Multidisciplinary)Wang, Y.*; Jia, G.*; Cui, X.*; Zhao, X.*; Zhang, Q.*; Gu, L.*; Zheng, L.*; Li, L. H.*; Wu, Q.*; Singh, D. J.*; et al.
Chem, 7(2), p.436 - 449, 2021/02
Times Cited Count:199 Percentile:99.80(Chemistry, Multidisciplinary)Zhao, Q.*; Taruta, Yasuyoshi; Kobayashi, Shigeto*; Hashimoto, Takashi*
Chishiki Kyoso (Internet), 9, p.III 1_1 - III 1_9, 2019/06
no abstracts in English
Wo, H.*; Wang, Q.*; Shen, Y.*; Zhang, X.*; Hao, Y.*; Feng, Y.*; Shen, S.*; He, Z.*; Pan, B.*; Wang, W.*; et al.
Physical Review Letters, 122(21), p.217003_1 - 217003_5, 2019/05
Times Cited Count:5 Percentile:41.86(Physics, Multidisciplinary)Zhao, Q.*; Taruta, Yasuyoshi; Kobayashi, Shigeto*; Hashimoto, Takashi*
Chishiki Kyoso (Internet), 8, p.V 13_1 - V 13_2, 2018/08
no abstracts in English
Liu, X.-H.*; Oka, Makoto; Zhao, Q.*
Physics Letters B, 753, p.297 - 302, 2016/02
Times Cited Count:89 Percentile:98.56(Astronomy & Astrophysics)We investigate the anomalous triangle singularity (ATS) and its possible manifestations in various processes. We show that the ATS should have important impact on our understanding of the nature of some newly observed threshold states. Discussions on how to distinguish the ATS phenomena from genuine dynamic pole structures are presented.
Deng, Z.*; Zhao, K.*; Gu, B.; Han, W.*; Zhu, J. L.*; Wang, X. C.*; Li, X.*; Liu, Q. Q.*; Yu, R. C.*; Goko, Tatsuo*; et al.
Physical Review B, 88(8), p.081203_1 - 081203_5, 2013/08
Times Cited Count:74 Percentile:92.00(Materials Science, Multidisciplinary)Annadi, A.*; Zhang, Q.*; Renshaw Wang, X.*; Tuzla, N.*; Gopinadhan, K.*; L, W. M.*; Roy Barman, A.*; Liu, Z. Q.*; Srivastava, A.*; Saha, S.*; et al.
Nature Communications (Internet), 4, p.1838_1 - 1838_7, 2013/05
Times Cited Count:97 Percentile:94.64(Multidisciplinary Sciences)Pitcher, C. S.*; Andrew, P.*; Barnsley, R.*; Bertalot, L.*; Counsell, G. G.*; Encheva, A.*; Feder, R. E.*; Hatae, Takaki; Johnson, D. W.*; Kim, J.*; et al.
Journal of Nuclear Materials, 415(Suppl.1), p.S1127 - S1132, 2011/08
Times Cited Count:0 Percentile:0.01(Materials Science, Multidisciplinary)Shi, W.-Q.*; Fu, H.-Y.*; Bounds, P. L.*; Muroya, Yusa*; Lin, M.; Katsumura, Yosuke*; Zhao, Y.-L.*; Chai, Z.-F.*
Radiation Research, 176(1), p.128 - 133, 2011/07
Times Cited Count:3 Percentile:17.09(Biology)3-Nitrotyrosine (3-NT) has been reported as an important biomarker of oxidative stress and potential source of reactive oxygen species (ROSs). In this work, the UV-visible absorption spectra of the transients formed by hydrated electron (e) reacting with 3-NT and its derivatives were investigated, the spectra showed many characteristics of aromatic nitro anion radical. The reaction rate constants of e reacting with 3-NT, N-acetyl-3-nitrotyrosine ethyl ester (NANTE) and nitrotyrosine-containing peptide Gly-nitroTyr-Gly at neutral pH were determined, respectively, which were almost two orders of magnitude higher than that of tyrosine and tyrosine-containing peptides. The pH-dependence of e decay rate constants in presence of 3-NT was also studied.
Son, N. T.*; Ivanov, I. G.*; Kuznetsov, A. Yu.*; Svensson, B. G.*; Zhao, Q. X.*; Willander, M.*; Morishita, Norio; Oshima, Takeshi; Ito, Hisayoshi; Isoya, Junichi*; et al.
Physica B; Condensed Matter, 401-402, p.507 - 510, 2007/12
Times Cited Count:3 Percentile:17.80(Physics, Condensed Matter)Defects in electron-irradiated (3, 6 MeV) ZnO substrates were investigated using optical detection of magnetic response (ODMR). The shallow donor and the Zn vacancy were detected. In addition, several ODMR centers with S= were also observed. Among these, LU3 and LU4 shows a behavior as recombination centers. After annealing at 400C, both LU3 and LU4 still remain in ZnO substrates.
Son, N. T.*; Ivanov, G.*; Kuznetsov, A.*; Svensson, B. G.*; Zhao, Q. X.*; Willander, M.*; Morishita, Norio; Oshima, Takeshi; Ito, Hisayoshi; Isoya, Junichi*; et al.
Journal of Applied Physics, 102(9), p.093504_1 - 093504_5, 2007/11
Times Cited Count:18 Percentile:56.58(Physics, Applied)Optical detection of magnetic resonance (ODMR) was performed to investigate defects in ZnO irradiated with 3 MeV electrons at room temperature. As a result, the Zn vacancy and some other centers were detected by ODMR. The Zn vacancy and two other centers whish are labeled as LU3 and LU4, were also commonly observed in different types of as-grown ZnO. Therefore, it can be concluded that the both LU3 and LU4 might be related to intrinsic defects, and they act as dominating recombination centers in irradiated and as-grown ZnO.
Fujisawa, Akihide*; Ido, Takeshi*; Shimizu, Akihiro*; Okamura, Shoichi*; Matsuoka, Keisuke*; Iguchi, Harukazu*; Hamada, Yasuji*; Nakano, Haruhisa*; Oshima, Shinsuke*; Ito, Kimitaka*; et al.
Nuclear Fusion, 47(10), p.S718 - S726, 2007/10
Times Cited Count:101 Percentile:95.26(Physics, Fluids & Plasmas)Present status of experiments on zonal flows is overviewed. Innovative use of modern diagnostics has revealed the existence of zonal flows, their spatio-temporal characteristics, their relationship with turbulence, and their effects on confinement. Particularly a number of observations have been accumulated on the oscillatory branch of the zonal flow, dubbed as geodesic acoustic modes suggesting necessity of theories to give their proper description. Several new methods have elucidated the zonal flow generation processes from the turbulence. Further investigation of relationship between the zonal flows and confinement is strongly encouraged as cross-device activity.