JAEA-Review 2019-046, 36 Pages, 2020/03
Toward the revision of JENDL-4.0, we conducted a literature survey on how to compute the cross section of thermal neutrons scattered by a liquid. This report summarizes the computational methods for evaluating thermal neutron cross sections with molecular dynamics simulations. The cross section can be expressed with a function called as scattering law. For light and heavy water, the scattering law data instead of the cross sections have been provided in nuclear databases. In this report we review the formulations of the scattering laws. The scattering laws can be derived from both the intermediate scattering function and the space-time correlation function. Features of the derived scattering laws are briefly explained. It is shown that the scattering law data can be evaluated using a molecular dynamics simulation of the liquid that is the target of thermal neutrons.
Matsuda, Norihiro; Konno, Chikara; Ikehara, Tadashi; Okumura, Keisuke; Suyama, Kenya*
JAEA-Data/Code 2020-003, 33 Pages, 2020/03
Data handling modules for the radioactivity calculation code, ORIGEN-S, are developed for the reliable evaluations of radioactivity inventory. By using these modules, an activation cross-section data library for the ORIGEN-S code is updated easily and effectively based on a facility-specific neutron spectrum and multi-group neutron activation cross-section library for decommissioning of nuclear facilities, MAXS2015. In order to guarantee the reliability of the radioactivity calculations, functions of data verification in a visual way and numerical comparison between before and after the data processing are also prepared.
Shibata, Hiroki; Saito, Hiroaki; Hayashi, Hirokazu; Takano, Masahide
JAEA-Data/Code 2019-023, 138 Pages, 2020/03
Transmutation of minor actinides in the form of nitride fuel by the accelerator driven system has been developed to reduce the radiotoxicity and volume in the radioactive wastes. Nitride fuel behavior under irradiation condition is necessary for its design and development. Nitride fuel performance analysis module based on light water reactor fuel performance code, FEMAXI-7, was developed by introducing fundamental properties of nitride pellet, 9Cr-1Mo ferrite cladding, and Pi-Bi coolant. As a result of test analysis with this module, we have understood that the nitride fuel shows excellent behavior under irradiation due to its high thermal conductivity. We found that, however, it may be a main concern that fuel cladding integrity is maintained during irradiation in which pellet-cladding mechanical interaction is increased by He gas release, low creep rate of nitride pellet at low temperatures, and high creep rate of cladding above 873 K.
Matsuya, Yusuke; Nakano, Toshiaki*; Kai, Takeshi; Shikazono, Naoya*; Akamatsu, Ken*; Yoshii, Yuji*; Sato, Tatsuhiko
International Journal of Molecular Sciences (Internet), 21(5), p.1701_1 - 1701_13, 2020/03
Among various DNA damage induced after irradiation, clustered damage composed of at least two vicinal lesions within from 10 to 20 base pairs is recognized as fatal damage to human tissue. Such clustered damage yields have been evaluated by means of computational approaches; however, the simulation validity has not been sufficiently made yet. Meanwhile, the experimental technique to detect clustered DNA damage has been evolved in the recent decades, so both approaches with simulation and experiment get used to be available for investigating clustered damage recently. In this study, we have developed a simple model for estimating clustered damage yield based on the spatial density of ionization and electronic excitation events obtained by the PHITS code, and compared the computational results to the experimental clustered damage coupled with base damage (BD) measured by gel electrophoresis and atomic force microscopy. The computational results agreed well with experimental fractions of clustered damage of strand breaks (SB) and BD, when the yield ratio of BD/SSB is assumed to be 1.3. From the comparison of complex DNA double-strand break coupled with BDs between simulation and experimental data, it was suggested that aggregation degree of the events along electron track reflects the complexity of DNA damage. The resent simulation enables to quantify the type of clustered damage which cannot be measured in in vitro experiment, which succeeded in interpreting the experimental detection efficiency for clustered BD.
Terada, Hiroaki; Nagai, Haruyasu; Tsuzuki, Katsunori; Furuno, Akiko; Kadowaki, Masanao; Kakefuda, Toyokazu*
Journal of Environmental Radioactivity, 213, p.106104_1 - 106104_13, 2020/03
In order to assess the radiological dose to the public resulting from the Fukushima Daiichi Nuclear Power Station accident in Japan, the spatial and temporal distribution of radioactive materials in the environment is necessary to be reconstructed by computer simulations with the atmospheric transport, dispersion and deposition model (ATDM) and source term of radioactive materials discharged into the atmosphere is essential. In this study, we carried out refinement of the source term and improvement of ATDM simulation by using an optimization method based on Bayesian inference with various measurements (air concentration, surface deposition, and fallout). We also constructed the spatiotemporal distribution of some major radionuclides in the air and on the surface (optimized dispersion database) by using the optimized release rates and ATDM simulations which is used for the comprehensive dose assessment by coupling with the behavioral pattern of evacuees from the accident.
Kwon, Saerom*; Konno, Chikara; Ota, Masayuki*; Kasugai, Atsushi*
Journal of Nuclear Science and Technology, 57(3-4), p.344 - 351, 2020/03
We found out that there was a questionable iron DPA value just above 20 MeV neutron energy in neutronics analyses of A-FNS using FENDL-3.1d. Our detailed investigation on the iron data in FENDL-3.1d figured out that residual nucleus production yield data of Fe just above 20 MeV had a problem, which caused a sharp spike just above 20 MeV in the DPA cross section of Fe. Thus we modified the yield data of Fe and verified that the questionable DPA value disappeared using the modified data. We also examined DPA cross sections of other nuclei in FENDL-3.1d. It was found out that DPA cross sections of more than 70% of nuclei in FENDL-3.1d have similar problems as that of Fe.
Tateno, Haruka; Sato, Takumi; Tsubata, Yasuhiro; Hayashi, Hirokazu
Journal of Nuclear Science and Technology, 57(3-4), p.224 - 235, 2020/03
Fuel cycle technology for the transmutation of long-lived minor actinides (MAs) using an accelerator-driven system has been developed using the double-strata fuel cycle concept. A mononitride solid solution of MAs and Pu diluted with ZrN is a prime fuel candidate for the accelerator-driven transmutation of MAs. Pyro-reprocessing is suitable for recycling the residual MAs in irradiated nitride fuel with high radiation doses and decay heat. Spent nitride fuel is anodically dissolved, and the actinides are recovered simultaneously into a liquid cadmium cathode via molten salt electrorefining. The process should be designed to achieve the target recovery yield of MAs and the acceptable impurity level of rare earths in the recovered material. We evaluated the material balance during the pyro-reprocessing of spent nitride fuel to gain important insight on the design process. We examined the effects of changing processing conditions on material flow and quantity of waste.
Kawamura, Hideyuki; Kamidaira, Yuki; Kobayashi, Takuya
Journal of Nuclear Science and Technology, 57(3-4), p.472 - 485, 2020/03
The Japan Atomic Energy Agency developed a Short-Term Emergency Assessment system of the Marine Environmental Radioactivity (STEAMER) to predict the oceanic dispersion of radionuclides in the ocean around Japan. The purpose of this study is to validate the predictability of STEAMER using oceanographic forecast and reanalysis data, which were saved for past several years. Results of oceanic dispersion simulations that are driven by oceanographic reanalysis data are assumed to be true solutions. Oceanic dispersion simulations are conducted for Cs-137 released hypothetically from the Fukushima Daiichi Nuclear Power Plant. The predictability of STEAMER is quantitatively examined for the length of the forecast period. Ensemble forecast simulations are also conducted to successfully improve the predictability of STEAMER.
Iwamoto, Hiroki; Meigo, Shinichiro
Journal of Nuclear Science and Technology, 57(3-4), p.276 - 290, 2020/03
This paper presents an approach to uncertainty estimation of spallation particle multiplicity of lead (Pb), primarily focusing on proton-induced spallation neutron multiplicity () and its propagation to a neutron energy spectrum. The uncertainty is estimated from experimental proton-induced neutron-production double-differential cross sections (DDXs) and model calculations with the Particle and Heavy Ion Transport code System (PHITS). Uncertainties in multiplicities for , , and reactions are then inferred from the estimated uncertainty and the PHITS calculation. Using these uncertainties, uncertainty in a neutron energy spectrum produced from a thick Pb target bombarded with 500 MeV proton beams, measured in a previous experiment, is quantified by a random sampling technique, and propagation to the neutron energy spectrum is examined. Relatively large uncertainty intervals (UIs) were observed outside the lower limit of the measurement range, which is prominent in the backward directions. Our findings suggest that a reliable assessment of spallation neutron energy spectra requires systematic DDX experiments for detector angles and incident energies below 100 MeV as well as neutron energy spectrum measurements at lower energies below 1.4 MeV with an accuracy below the quantified UIs.
Nakamura, Shoji; Shibahara, Yuji*; Kimura, Atsushi; Iwamoto, Osamu; Uehara, Akihiro*; Fujii, Toshiyuki*
Journal of Nuclear Science and Technology, 57(3-4), p.388 - 400, 2020/03
The thermal-neutron capture cross-section () and resonance integral(I) were measured for the Cs(n,)Cs reaction by an activation method and mass spectrometry. We used Cs contained as an impurity in a normally available Cs standard solution. An isotope ratio of Cs and Cs in a standard Cs solution was measured by mass spectrometry to quantify Cs. The analyzed Cs samples were irradiated at the hydraulic conveyer of the research reactor in Institute for Integral Radiation and Nuclear Science, Kyoto University. Wires of Co/Al and Au/Al alloys were used as neutron monitors to measure thermal-neutron fluxes and epi-thermal Westcott's indices at an irradiation position. A gadolinium filter was used to measure the , and a value of 0.133 eV was taken as the cut-off energy. Gamma-ray spectroscopy was used to measure induced activities of Cs, Cs and monitor wires. On the basis of Westcott's convention, the and I values were derived as 8.570.25 barn, and 45.33.2 barn, respectively. The obtained in the present study agreed within the limits of uncertainties with the past reported value of 8.30.3 barn.
Tsutsui, Nao; Ban, Yasutoshi; Suzuki, Hideya*; Nakase, Masahiko*; Ito, Sayumi*; Inaba, Yusuke*; Matsumura, Tatsuro; Takeshita, Kenji*
Analytical Sciences, 36(2), p.241 - 246, 2020/02
To investigate the effective separation of actinides (Ans) from lanthanides (Lns), single-stage batch extraction experiments were performed with a novel extractant, tetradodecyl-1,10-phenanthroline-2,9-diamide (TDdPTDA) with various diluents such as 3-nitrobenzotrifluoride (F-3), nitrobenzene, and -dodecane for Am, Cm, and Lns. The extraction kinetics with TDdPTDA was rapid enough to perform the actual extraction flow sheet. The slopes of the distribution ratio versus TDdPTDA concentration and the distribution ratio versus nitric acid concentration were similar for F-3 and nitrobenzene systems but different from -dodecane system. These differences were attributed to the characteristics of the diluents. This study reveals high distribution ratios of Am ( ) and Cm ( ) for TDdPTDA, with the high separation factors (s) of Am from Lns enough for their separation.
Katata, Genki*; Grote, R.*; Mauder, M.*; Zeeman, M. J.*; Ota, Masakazu
Biogeosciences, 17(4), p.1071 - 1085, 2020/02
Mountain grassland productivity is limited by cold and long winters; thus, rising temperatures and changes in snow cover expected in the future may have large impacts on the grassland yields. To investigate this, we enhanced land surface model (SOLVEG) to account for snow, freeze-thaw events, and grass growth, and the model was applied to the managed grasslands affected by extremely warm winter. The model reproduced temporal variability of observed heat fluxes, soil temperatures and snow depth throughout the 3-year simulation period. High physiological activity during the extremely warm winter led to a CO uptake of 100 g-C m, which was, surprisingly, mainly allocated into the below-ground biomass and rarely used for plant growth during spring. This process, which is so far largely unaccounted for in global terrestrial biosphere models, may lead to carbon accumulation in the soil and/or heterotrophic respiration as a response to global warming.
Kumagai, Yuta; Jonsson, M.*
Dalton Transactions (Internet), 49(6), p.1907 - 1914, 2020/02
This study aims to reveal possible involvements of organic acids in the oxidative dissolution of UO. Using phthalic acid as a model compound, we have measured adsorption on UO and investigated effects on the reaction between HO and UO and on oxidative dissolution induced by -irradiation. Significant adsorption of phthalic acid was observed even at neutral pH. However, the reaction between HO and UO in phthalic acid solution induced oxidative dissolution of U(VI) similarly to aqueous bicarbonate solution. These results indicate that even though phthalic acid adsorbs on the UO surface, it is not involved in the interfacial reaction by HO. In contrast, the dissolution of U by irradiation was inhibited in aqueous phthalic acid solution, whereas HO generated by radiolysis was consumed by UO. The inhibition suggests that radical species derived from phthalic acid was involved in the redox reaction process of UO.
Minato, Futoshi; Tanimura, Yusuke*
European Physical Journal A, 56(2), p.45_1 - 45_18, 2020/02
For nuclei, three-body model of inert core can provide an understanding of pairing correlations in the ground state and spin-isospin excitations. However, residual core-nucleon interactions can impact the core nucleus significantly. The effect of core excitations thus has to be included for the detailed understanding of the ground state and the spin-isospin properties. We solve the three-body problem including core vibrational states to obtain the ground state as well as the spin-excitations. By including the effect of core excitation, (a) magnetic moment, (b) the enegy difference between the first and the excited states, (c) B(M1) and B(GT), are improved. It was also found that the root mean squares of distances between proton and neutron, and the center of mass of valence prton and neutron and core slightly increase.
Ohdaira, Naoya*; Saito, Shigeru
Heliyon (Internet), 6(2), p.e03429_1 - e03429_8, 2020/02
Lead-bismuth eutectic (LBE) is a candidate liquid metal coolant for a fast reactor, especially accelerator driven system (ADS). Freeze sealed valve is a candidate design to be possible to add passive safety to the reactor. On the other hand, since LBE is known that it causes expansion after its solidification, quantitative evaluation of the stress to the pipe produced by the LBE expansion should be considered. Many researchers produced related data for the expansion, however, evaluations of the strain by LBE expansion was barely reported. Therefore, the strain measurement using a stainless steel cup and the stress evaluation was performed together with visual observation using an optical microscopy. The results indicated keeping above room temperature (RT) was a significantly effective way to reduce the strain to the pipe.
Iwamoto, Yosuke; Yoshida, Makoto*; Matsuda, Hiroki; Meigo, Shinichiro; Satoh, Daiki; Yashima, Hiroshi*; Yabuuchi, Atsushi*; Kinomura, Atsushi*; Shima, Tatsushi*
JPS Conference Proceedings (Internet), 28, p.061003_1 - 061003_5, 2020/02
To predict the lifetime of target materials in high-energy radiation environments at spallation neutron sources, radiation transport codes such as PHITS are used to calculate the displacements per atom (DPA) value. In this work, to validate calculated DPA values of tungsten, we implemented 0.25-mm-diameter wire sample of tungsten in a proton irradiation device with a Gifford-McMahon cryocooler and measured the defect-induced electrical resistivity changes related to the displacement cross section using 389-MeV protons at 10 K. In comparison with experimental data under 1.1 and 1.9 GeV proton irradiation, we found that damage rate of tungsten increases with proton energy due to increase the number of secondary particle s produced by nuclear reactions.
Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Yosuke; Yoshida, Makoto*; Hasegawa, Shoichi; Maekawa, Fujio; Iwamoto, Hiroki; Nakamoto, Tatsushi*; Ishida, Taku*; Makimura, Shunsuke*
JPS Conference Proceedings (Internet), 28, p.061004_1 - 061004_6, 2020/02
no abstracts in English
Saito, Shigeru; Okubo, Nariaki; Obayashi, Hironari; Wan, T.; Sugawara, Takanori; Sasa, Toshinobu; Maekawa, Fujio
JPS Conference Proceedings (Internet), 28, p.071003_1 - 071003_6, 2020/02
Japan Atomic Energy Agency (JAEA) proposes transmutation of minor actinides (MA) by accelerator-driven systems (ADS). The ADS designed by JAEA is a system composed by LBE (Lead-Bismuth Eutectic) spallation target and a subcritical core. In the ADS, a beam window (BW) is exposed in complex field of heavy irradiation by proton/neutron and corrosion by flowing LBE. To develop ADS structural materials, it is of critical importance to investigate materials used in such environment. Thus, JAEA plans to construct a proton irradiation facility at the J-PARC to prepare an irradiation database for candidate ADS structural materials and to investigate irradiation effects in flowing LBE environment. In this paper, giving a whole scope of the JAEA ADS development, some results of experimental measurements and the specific program for planed R&D will be presented.
Ishikawa, Norito; Taguchi, Tomitsugu*; Kitamura, Akane; Szenes, G.*; Toimil-Molares, M. E.*; Trautmann, C.*
Journal of Applied Physics, 127(5), p.055902_1 - 055902_7, 2020/02
Hillock formation is one of the important aspects of radiation-induced modification of solid material. To our knowledge this is first result showing that the hillock formation in ceramics is affected by the velocity effect. The present result include Se-dependences of hillock dimensions based on precise measurement using TEM (transmission electron microscopy). The paper should be published to make researchers aware that hillock size is actually comparable to ion-track size in wide Se range. In addition, the results include important insight about the hillock formation mechanism of ceramics irradiated with swift heavy ions.
Keikinzoku, 70(2), p.73 - 81, 2020/02
Elements strategy becomes important to investigate alternative materials of rare metals. I have dedicated to establish a new approach based on computational methods. In the present paper, I propose two approaches based on first-principles and theory of dislocations. These methods are introduced to magnesium alloys.