Improvement of model for cesium chemisorption onto stainless steel in severe accident analysis code SAMPSON (Joint research)

Miwa, Shuhei; Karasawa, Hidetoshi; Nakajima, Kunihisa; Kino, Chiaki*; Suzuki, Eriko; Imoto, Jumpei

JAEA-Data/Code 2021-022, 32 Pages, 2023/01

JAEA-Data-Code-2021-022.pdf:1.41MB
JAEA-Data-Code-2021-022(errata).pdf:0.17MB

The improved model for cesium (Cs) chemisorption onto stainless steel (SS) in the fission product (FP) chemistry database named ECUME was incorporated into the severe accident (SA) analysis code SAMPSON for the more accurate estimation of Cs distribution within nuclear reactor vessels in the TEPCO's Fukushima Daiichi Nuclear Power Station (1F). The SAMPSON with the improved model was verified based on the analysis results reproducing the experimental results which were subjected to the modeling of Cs chemisorption behavior. Then, the experiment in the facility with the temperature gradient tube to simulate SA conditions such as temperature decrease and aerosol formation was analyzed to confirm availability of the improved model to the analysis of Cs chemisorption onto SS. The SAMPSON with the improved model successfully reproduced the experimental results, which indicates that the improved model and the analytical method such as setting a method of node-junction, models of aerosol formation and the calculation method of saturated CsOH vapor pressure can be applicable to the analysis of Cs chemisorption behavior. As the information on water-solubility of Cs deposits was also prerequisite to estimate the Cs distribution in the 1F because Cs can be transported through aqueous phase after the SA, the water-solubility of chemisorbed Cs compounds was investigated. The chemisorbed compounds on SS304 have been identified to CsFeO at 873 K to 973 K with higher water-solubility, CsFeSiO at 973 K to 1273 K and CsSiO at 1073 K to 1273 K with lower water-solubility. From these results, the water-solubility of chemisorbed Cs compounds can be estimated according to the SA analysis conditions such as temperature in the reactor and the CsOH concentration affecting the amount of chemisorbed Cs.

A Numerical simulation method for core internals behavior in severe accident conditions; Chemical reaction analyses in core structures by JUPITER

Yamashita, Susumu; Kino, Chiaki*; Yoshida, Hiroyuki

Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 7 Pages, 2020/08

https://doi.org/10.1115/ICONE2020-16817

In order to contribute the improvement of estimation accuracy for severe accident code such as SAMPSON, we have developed the chemical reaction model such as eutectic reaction and oxidation in micro scale, e.g., BC-SUS in the control rod blade and UO-Zry in fuel rods, and implemented them to the computational fluid dynamics code named JUPITER. And we try to develop the coupled analysis frame work using SAMPSON and JUPITER to decrease uncertainty due to micro scale phenomena which cannot be calculate by severe accident analysis codes. From the preliminary analysis in fuel rod heating analysis by JUPITER using SAMPSON output data, it was revealed that the implemented chemical reaction models work stably and obtain reasonable results.

Experimental study on U-Pu cocrystallization reprocessing process

Shibata, Atsuhiro; Oyama, Koichi; Yano, Kimihiko; Nomura, Kazunori; Koyama, Tomozo; Nakamura, Kazuhito; Kikuchi, Toshiaki*; Homma, Shunji*

Journal of Nuclear Science and Technology, 46(2), p.204 - 209, 2009/02

https://doi.org/10.3327/jnst.46.204

A new reprocessing system with 2-stage crystallization process has been developed. In the first stage of the system, U and Pu are recovered from dissolver solution by U-Pu co-crystallization. Laboratory scale experiments were carried out with U and Pu mixed solution and irradiated fuel dissolver solution to obtain fundamental data on U-Pu co-crystallization process. Pu co-crystallized with U, but crystallization yields of Pu were lower than those of U. FPs were separated from U and Pu by co-crystallization, and decontamination factors of Cs and Eu to U in crystal were over 100.

Design of small reduced-moderation water reactor

Okubo, Tsutomu; Iwamura, Takamichi; Takeda, Renzo*; Moriya, Kumiaki*; Yamauchi, Toyoaki*; Aritomi, Masanori*

Nihon Kikai Gakkai 2003-Nendo Nenji Taikai Koen Rombunshu, Vol.3, p.245 - 246, 2003/08

A design study on a 300MWe class small Reduced-Moderation Water Reactor (RMWR) has been performed, based on the experienced LWR technology. The core can be cooled by the natural circulation and can achieve a conversion ratio of 1.01, a negative void reactivity coefficient, a core average burn-up of 65 GWd/t and a cycle length of 25 months. The system has been simplified as much as possible by introducing the passive safety components, in order to reduce the construction cost per electric power output overcoming “the scale demerit" for a small reactor comparing with the large one. The results show a 1.35 times higher cost than for the ABWR case, but suggest the possible lower cost when the effects such as the mass production are taken into account.

Design of small Reduced-Moderation Water Reactor (RMWR) with natural circulation cooling

Okubo, Tsutomu; Suzuki, Motoe; Iwamura, Takamichi; Takeda, Renzo*; Moriya, Kumiaki*; Kanno, Minoru*

Proceedings of International Conference on the New Frontiers of Nuclear Technology; Reactor Physics, Safety and High-Performance Computing (PHYSOR 2002) (CD-ROM), 10 Pages, 2002/10

A small scale around 300 MWe reduced-moderation water reactor (RMWR) concept has been developed. For the core, a BWR type core concept with the tight-lattice fuel rod arrangement and the high void fraction is adopted to attain a high conversion ratio over 1.0. The negative void reactivity coefficients are also required, and the very flat short core concept is adopted to make the natural circulation cooling (NC) possible. The core burn-up of 60 GWd/t and the operation cycle of 24 months are also attained. For the system, simplification of the system with the passive safety features is a basic approach to overcome the scale demerit as well as the NC. For example, the HPCF system is replaced with the passive accumulator system resulting in the expensive emergency DGs reduction. The cost evaluation for concerned NSSS components gives about 20% reduction. Since MOX fuels in the RMWR contains Pu around 30 wt% and is irradiated to a high burn-up, the fuel safety evaluation has been performed and the acceptable results have been obtained from the thermal feasibility point of view.

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*; ; *; *

JNC TJ1420 2000-007, 241 Pages, 2000/03

JNC-TJ1420-2000-007.pdf:11.05MB

no abstracts in English

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Takeuchi, Shinji

JNC TJ7440 99-019, 334 Pages, 1999/04

JNC-TJ7440-99-019.pdf:17.5MB

no abstracts in English

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; Tsuchida, Toru*

PNC TJ1521 96-001, 141 Pages, 1996/02

PNC-TJ1521-96-001.pdf:5.31MB

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PNC TJ1521 94-001, 152 Pages, 1994/03

PNC-TJ1521-94-001.pdf:4.89MB

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PNC TJ1521 93-001, 138 Pages, 1993/02

PNC-TJ1521-93-001.pdf:4.11MB

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