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Deguchi, Yoshihiro*; Muranaka, Ryota*; Kamimoto, Takahiro*; Takagi, Taku*; Kikuchi, Shin; Kurihara, Akikazu
Applied Thermal Engineering, 114, p.1319 - 1324, 2017/03
Times Cited Count:2 Percentile:13.03(Thermodynamics)The purpose of this study aims to clarify the gas phase sodium-water reaction path and reaction products quantitatively. The counter-flow diffusion experiment device was employed to analyze the reaction path and reaction products using laser diagnostics. The main product of sodium-water reaction was determined to be NaOH and the sodium oxide was not notably measured compared with NaOH.
Inukai, Munehiro*; Horike, Satoshi*; Itakura, Tomoya*; Shinozaki, Ryota*; Ogiwara, Naoki*; Umeyama, Daiki*; Nagarker, S.*; Nishiyama, Yusuke*; Malon, M.*; Hayashi, Akari*; et al.
Journal of the American Chemical Society, 138(27), p.8505 - 8511, 2016/07
Times Cited Count:130 Percentile:95.54(Chemistry, Multidisciplinary)Deguchi, Yoshihiro*; Muranaka, Ryota*; Kamimoto, Takahiro*; Takagi, Taku*; Kikuchi, Shin; Kurihara, Akikazu
Proceedings of 3rd International Workshop on Heat Transfer Advances for Energy Conservation and Pollution Control (IWHT 2015) (CD-ROM), 6 Pages, 2015/10
The purpose of this study aims to clarify the gas phase sodium-water reaction path and reaction products quantitatively. The counter-flow diffusion experiment device was employed to analyze the reaction path and reaction products using laser diagnostics. The main product of sodium-water reaction was determined to be NaOH and the sodium oxide was not notably measured compared with NaOH.
Nishikino, Masaharu; Kawachi, Tetsuya; Hasegawa, Noboru; Ishino, Masahiko; Minami, Yasuo*; Suemoto, Toru*; Onishi, Naofumi*; Ito, Atsushi*; Sato, Katsutoshi*; Faenov, A.*; et al.
X-Ray Lasers and Coherent X-Ray Sources; Development and Applications XI (Proceedings of SPIE, Vol.9589), p.958902_1 - 958902_7, 2015/09
Inogamov, N. A.*; Zhakhovsky, V. V.*; Hasegawa, Noboru; Nishikino, Masaharu; Yamagiwa, Mitsuru; Ishino, Masahiko; Agranat, M. B.*; Ashitkov, S. I.*; Faenov, A. Y.*; Khokhlov, V. A.*; et al.
Applied Physics B, 119(3), p.413 - 419, 2015/06
Times Cited Count:6 Percentile:34.58(Optics)Deguchi, Yoshihiro*; Takata, Takashi*; Yamaguchi, Akira*; Kikuchi, Shin; Ohshima, Hiroyuki
Mechanical Engineering Journal (Internet), 2(1), p.14-00029_1 - 14-00029_11, 2015/02
In a sodium-cooled fast reactor (SFR), liquid sodium is used as a heat transfer fluid because of its excellent heat transport capability. On the other hand, it has strong chemical reactivity with water vapor. One of the design basis accidents of the SFR is the water leakage into the liquid sodium flow by a breach of heat transfer tubes. This process ends up damages on the heat transport equipment in the SFR. Therefore, the study on sodium-water chemical reactions is of paramount importance for security reasons. This study aims to clarify the sodium-water reaction mechanisms using an elementary reaction analysis. From analytical results, the main reaction was Na + HO = NaOH + H at gas-phase reaction.
Nishikino, Masaharu; Hasegawa, Noboru; Tomita, Takuro*; Eyama, Tsuyoshi*; Kakimoto, Naoya*; Onishi, Naofumi*; Ito, Atsushi*; Baba, Motoyoshi*; Minami, Yasuo*; Kawachi, Tetsuya; et al.
Reza Gakkai Dai-471-Kai Kenkyukai Hokoku; Tanhacho Ryoshi Bimu Hassei To Sono Oyo, p.9 - 12, 2014/12
no abstracts in English
Baba, Motoyoshi*; Nishikino, Masaharu; Hasegawa, Noboru; Tomita, Takuro*; Minami, Yasuo*; Takei, Ryota*; Yamagiwa, Mitsuru; Kawachi, Tetsuya; Suemoto, Toru
Japanese Journal of Applied Physics, 53(8), p.080302_1 - 080302_4, 2014/08
Times Cited Count:7 Percentile:31.01(Physics, Applied)A grazing incidence reflection-type soft X-ay microscope, using a Fresnel zone plate and a soft X-ray laser with wavelength 13.9 nm and pulse width 7 ps, was developed. Submicron size groove structures made on a Pt film were clearly captured at a single shot exposure, with spatial resolution of about 360 nm. A wide field view of 100 m square was secured under the Kohler illumination. This microscope also had a large depth of focus of more than 100 m and was proven to have a sufficient performance for observing surface morphological changes.
Tomita, Takuro*; Nishikino, Masaharu; Hasegawa, Noboru; Minami, Yasuo*; Takei, Ryota*; Baba, Motoyoshi*; Eyama, Tsuyoshi*; Takayoshi, Shodai*; Kaihori, Takeshi*; Morita, Toshimasa; et al.
Journal of Laser Micro/Nanoengineering, 9(2), p.137 - 142, 2014/06
Times Cited Count:5 Percentile:29.68(Nanoscience & Nanotechnology)Femtosecond laser ablation processes on platinum, gold, and tungsten were observed by the single shot pump and probe reflective imaging using a soft X-ray laser probe. To avoid the timing error due to the jitter, we adopted a posteriori correction technique by simultaneous measurement of timing between the pump and probe pulses for every single shot, using a soft X-ray streak camera. A clear difference was found in the temporal behavior of the dynamical response of the soft X-ray reflectivity depending on the irradiated laser fluence in these three materials. On the other hand, the narrow dark rings were found in Pt and W, while an additional bright ring was found outside the dark disk in Au. Our result gives the experimental data comparable with various numerical simulations.
Hayashi, Hiroaki*; Shibata, Michihiro*; Asai, Masato; Osa, Akihiko; Sato, Tetsuya; Koizumi, Mitsuo; Kimura, Atsushi; Oshima, Masumi*
Nuclear Instruments and Methods in Physics Research A, 747, p.41 - 51, 2014/05
Times Cited Count:10 Percentile:61.24(Instruments & Instrumentation)To measure -decay energy of short-lived fission products with good accuracy and high efficiency, we have developed a new total absorption clover detector and demonstrated its performance. Using a large-volume clover-type Ge detector having a through-hole in its center, we could measure total absorption spectra of + rays with extremely high efficiency and high energy resolution, and could determine values with 30 keV accuracy. Using this detector, we have determined the values of Eu and Gd for the first time, and of Eu and Gd with better accuracies. In addition, we have observed a new isomeric state in Gd, and determined its half-life and excitation energy.
Deki, Manato*; Oka, Tomoki*; Takayoshi, Shodai*; Naoi, Yoshiki*; Makino, Takahiro; Oshima, Takeshi; Tomita, Takuro*
Materials Science Forum, 778-780, p.661 - 664, 2014/02
Times Cited Count:2 Percentile:72.87no abstracts in English
Deki, Manato*; Makino, Takahiro; Kojima, Kazutoshi*; Tomita, Takuro*; Oshima, Takeshi
Materials Science Forum, 778-780, p.440 - 443, 2014/02
Times Cited Count:2 Percentile:82.41no abstracts in English
Nishikino, Masaharu; Baba, Motoyoshi*; Suemoto, Toru; Hasegawa, Noboru; Ishino, Masahiko; Kaihori, Takeshi; Kawachi, Tetsuya; Yamagiwa, Mitsuru
X-Ray Lasers 2012; Springer Proceedings in Physics, Vol.147, p.199 - 202, 2014/00
Times Cited Count:0 Percentile:0The dynamical processes of the laser-induced surface modifications such as laser ablation come to attract much attention for the micro processing by the ultra-short laser pulse. It is difficult to observe these phenomena directly, because they are non-repetitive, unrepeatable, and occur very rapidly (pico-second) in a very small (micron) area. In order to observe the detailed laser-ablation process, we have developed the proto-type reflected soft X-ray microscopy using the Fresnel zone plate. The experimental setup and spatial resolution of the X-ray microscopy will be presented.
Tamura, Kenta*; Deguchi, Yoshihiro*; Muranaka, Ryota*; Kusano, Koji*; Takata, Takashi*; Kikuchi, Shin; Kurihara, Akikazu
Proceedings of 24th International Symposium on Transport Phenomena (ISTP-24) (USB Flash Drive), 5 Pages, 2013/11
The purpose of this study aims to clarify the gas phase sodium-water reaction path and reaction products. The counter-flow diffusion experiment device is in the form of introducing the argon-based water vapor from the top of depressurized reaction chamber to the liquid sodium pool. Na, Na, HO, and reaction products in the counter-flow sodium-water reaction field were measured using laser diagnostics. The temperature controlled device was also improved to reduce the condensation of Na in the reaction zone for the better measurement performance. The main product in the sodium-water reaction was determined to be NaOH from the experimental results and its reaction path was discussed using Na-HO elementary reaction analysis.
Deguchi, Yoshihiro*; Tamura, Kenta*; Muranaka, Ryota*; Kusano, Koji*; Kikuchi, Shin; Kurihara, Akikazu
Reza Kenkyu, 41(11), p.927 - 931, 2013/11
In a sodium-cooled fast reactor (SFR), liquid sodium is used as a heat transfer fluid because of its excellent heat transport capability. On the other hand, it has strong chemical reactivity with water vapor. One of the design basis accidents of the SFR is the water leakage into the liquid sodium flow by a breach of heat transfer tubes. Therefore the study on sodium-water chemical reactions is of paramount importance for security reasons. This study aims to clarify the sodium-water reaction mechanisms using laser diagnostics. The measurement results show that the sodium-water reaction proceeds mainly by the reaction Na + HO = NaOH + H and the main product is NaOH from this reaction.
Nishikino, Masaharu; Hasegawa, Noboru; Ishino, Masahiko; Yamagiwa, Mitsuru; Kawachi, Tetsuya; Minami, Yasuo*; Terakawa, Kota*; Takei, Ryota*; Baba, Motoyoshi*; Suemoto, Toru; et al.
JAEA-Conf 2013-001, p.16 - 19, 2013/09
The dynamics of the femtosecond laser ablation is still not clear at the early stage. Several studies on the time-resolved imaging of femtosecond laser ablation process have been performed on various materials. In this study, we have demonstrated a pump and probe imaging of the metal surface morphology during the femtosecond laser ablation by using the laser-driven plasma induced soft X-ray laser (SXRL) as a probe beam. The pumping laser used for ablation was a Ti:Sapphire laser system based on chirped pulse amplification. The pump beam had a Gaussian profile and the focal spot size on the metal surface was about 70 micron at FWHM. The dependence for the pump laser fluence of the ablation surface expansion and the surface condition (roughness and density gradient) were observed from the soft X-ray interferogram and reflective image, respectively.
Nishikino, Masaharu; Hasegawa, Noboru; Tomita, Takuro*; Minami, Yasuo*; Takei, Ryota*; Baba, Motoyoshi*; Eyama, Tsuyoshi*; Takayoshi, Shodai*; Kawachi, Tetsuya; Hatomi, Daiki*; et al.
Proceedings of SPIE, Vol.8849, p.88490E_1 - 88490E_6, 2013/09
Times Cited Count:2 Percentile:73.17We have developed the pump and probe interferometer and reflective imaging technique of the metal surfaces during the femtosecond laser ablation by using the laser-driven soft X-ray laser at the wavelength of 13.9 nm. The pumping laser used for ablation was a Ti: Sapphire laser pulse with the duration of 80 fs pulse at a central wavelength of 795 nm, and had a gaussian spatial profile. By using the X-ray imaging technique, the time resolved image of nano-scaled ablation dynamics of the platinum and the gold pumped by a femtosecond laser pulse was obtained.
Asai, Masato; Tsukada, Kazuaki; Sakama, Minoru*; Haba, Hiromitsu*; Ichikawa, Takatoshi*; Ishii, Yasuo; Toyoshima, Atsushi; Ishii, Tetsuro; Nishinaka, Ichiro; Nagame, Yuichiro; et al.
Physical Review C, 87(1), p.014332_1 - 014332_6, 2013/01
Times Cited Count:6 Percentile:43.85(Physics, Nuclear)The spin-parity and neutron configuration of the ground state of No have been identified through -decay spectroscopy. The No is the nucleus with the largest neutron number whose spin-parities and single-particle configurations have ever been identified. The neutron 9/2[615] configuration was assigned to the ground state of No as well as to the 231.4 keV level in Fm. This allowed us to establish energy spacings and order of the neutron single-particle orbitals in such heaviest nuclear region. The appearance of the 9/2[615] ground state at =157 implies that the order of the neutron orbitals between the =152 and 162 deformed shell gaps should change considerably with increasing neutron number.
Tomita, Takuro*; Yamamoto, Minoru*; Hasegawa, Noboru; Terakawa, Kota*; Minami, Yasuo*; Nishikino, Masaharu; Ishino, Masahiko; Kaihori, Takeshi*; Ochi, Yoshihiro; Kawachi, Tetsuya; et al.
Optics Express (Internet), 20(28), p.29329 - 29337, 2012/12
Times Cited Count:18 Percentile:65.08(Optics)Pump and probe reflective imaging using a soft X-ray laser probe was applied to the observation of the early stage of femtosecond laser ablation process on platinum. In strongly excited area, drastic and fast reflectivity drop was observed. In moderately excited area, the decay of the reflectivity is slower than that in the strongly excited area, and the reflectivity reaches its minimum at t = 160 ps. In weakly excited area, laser-induced reflectivity change was not observed. These results give the critical information about the femtosecond laser ablation.
Tomita, Takuro*; Hasegawa, Noboru; Nishikino, Masaharu; Kawachi, Tetsuya; Suemoto, Toru
Reza Kenkyu, 40(8), p.592 - 597, 2012/08
A single-shot soft X-ray laser pulse was used as a probe to investigate the early stage of the laser ablation process on platinum caused by the femtosecond near-infrared pump pulse. From time-resolved interferometry, we observed the dilation of the ablation front on a scale of 10 nm in the picosecond region. In the reflective imaging, we found three distinct types of dynamical responses, depending on the radial position in the pump beam spot. These characteristic behaviors correspond to different laser fluence and were attributed to different ablation schemes: spallation, homogeneous nucleation, and fragmentation/vaporization, which have been predicted from molecular dynamics simulation.