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JAEA Reports

Waste acceptance criteria for waste packages destined for near surface disposal containing radioactive waste from research, industrial and medical facilities

Nakata, Hisakazu; Sakai, Akihiro; Okada, Shota; Izumo, Sari; Tsuji, Tomoyuki; Kurosawa, Ryohei; Amazawa, Hiroya

JAEA-Technology 2016-001, 112 Pages, 2016/03

JAEA-Technology-2016-001.pdf:16.71MB

The waste packages must meet the technical requirements that radioactive waste shall be solidified in a container by a method determined by the Nuclear Regulation Authority to prevent from radiation hazards. JAEA has been preparing operating procedure manual on quality control for radioactive waste disposal in order to promote the manufacturing the waste package. This report presents that simulant waste packages were produced by placing wastes in a 200 liter drum, which was then filled with mortar of a novel mix proportion, followed by curing in a controlled manner. Determination of the presence of harmful voidage and raw waste immobility were performed by direct measurement and visual inspection of a vertical cross section of the waste packages respectively.

JAEA Reports

Study on engineering technologies in the Mizunami Underground Research Laboratory (FY 2014); Development of recovery and mitigation technology on excavation damage (Contract research)

Fukaya, Masaaki*; Hata, Koji*; Akiyoshi, Kenji*; Sato, Shin*; Takeda, Nobufumi*; Miura, Norihiko*; Uyama, Masao*; Kaneda, Tsutomu*; Ueda, Tadashi*; Hara, Akira*; et al.

JAEA-Technology 2016-002, 195 Pages, 2016/03

JAEA-Technology-2016-002.pdf:46.3MB
JAEA-Technology-2016-002-appendix(CD-ROM).zip:16.11MB

The researches on examination of the plug applied to the future reflood test was conducted as a part of (5) development of technologies for restoration and/on reduction of the excavation damage relating to the engineering technology in the MIU (2014), specifically focused on (1) plug examination (e.g. functions, structure and material) and the quality control methods and (2) analytical evaluation of rock mass behavior around the plug through the reflood test. As the result, specifications of the plug were determined. These specifications should be able to meet requirements for the safety structure and surrounding rock mass against predicted maximum water pressure, temperature stress and seismic force, and for controlling the groundwater inflow, ensuring the access into the reflood gallery and the penetration performance of measurement cable. Also preliminary knowledge regarding the rock mass behavior around the plug after flooding the reflood gallery by installed plug was obtained.

JAEA Reports

Improvement and development of geochemical monitoring system for groundwater installed in the 350 m gallery of the Horonobe Underground Research Laboratory

Mezawa, Tetsuya; Miyakawa, Kazuya; Sasamoto, Hiroshi; Soga, Koichi*

JAEA-Technology 2016-003, 25 Pages, 2016/05

JAEA-Technology-2016-003.pdf:2.91MB

Development of the monitoring technique for hydro-geochemical conditions of groundwater in low permeable sedimentary rocks with high content of dissolved gases in the underground facility is one of key issues in the Underground Research Laboratory (URL) project in order to obtain the reliable geochemical data. Development of the monitoring system for the groundwater geochemistry was conducted previously at the 140m gallery in the Horonobe URL. Thereafter, improvement and development of the monitoring system have been performed at the 350m gallery as the course of development technology to monitor the hydro-geochemical conditions during the URL construction. In this report, the results including the improvement and development of the monitoring system for the groundwater geochemistry at the 350m gallery and the several examples of data acquisition are presented.

JAEA Reports

Decontamination test of gravel; Establishment of effective decontamination methods about paving gravel and ballast

Kato, Mitsugu; Tanabe, Tsutomu; Umezawa, Katsuhiro; Wada, Takao

JAEA-Technology 2016-004, 129 Pages, 2016/03

JAEA-Technology-2016-004.pdf:20.42MB

After the Fukushima-Daiichi Nuclear Power Station accident, widespread contamination by radioactive materials occurred. Thus, decontamination work have been developed because of reducing air dose rate. Of this, in order to examine decontamination effect about gravel which cover sites of houses, communal facilities and cemeteries, and about ballast laid on a track, JAEA examined a decontamination test by physical plural methods. The objective of this testing is to establish rational and high effective decontamination methods to decontaminate each different gravel of materials and the shape, using the equipment which have possibility of the decontamination effect by trituration or blast. From the test results, applicability of the decontamination method depending on a characteristic of the gravel and the decontamination effect (reduction rate) are confirmed. There are various characteristics with the thing said to be gravel. It is confirmed that one decontamination method cannot be applied to all types of gravel. Furthermore, it is confirmed that there is great variability among individual polluted condition in the gravel gathered from the same place. Therefore, it is important to measure the degree of pollution so that a measurement error becomes as little as possible. For example, to measure plural points of the measurement side and keeping the height of measurement constant.

JAEA Reports

Study on small-sized tailless beam formation using multipole magnetic field (Joint research)

Yokota, Wataru; Yuri, Yosuke; Watanabe, Shinichi*; Oshiro, Yukimitsu*; Kubono, Shigeru*

JAEA-Technology 2016-005, 21 Pages, 2016/03

JAEA-Technology-2016-005.pdf:2.24MB

The Center of Nuclear Science (CNS) of Tokyo University conducts the research on nuclear physics using CNS Radio-Isotope Beam Separator (CRIB) installed at the RIKEN AVF cyclotron. Takasaki Advanced Radiation Research Institute, JAEA has an AVF cyclotron of similar scale and is developing a technology to form a large-area uniform beam by an octupole magnetic field for the research on materials science. They carried out an R&D to increase the cyclotron beam intensity at a target under joint research. The nonlinear beam optics was designed to form a usual cyclotron beam having a large transverse tail into a small-sized tailless distribution so that the beam passes the gas target orifice (6 mm in diameter) of CRIB without a loss. As a result of particle tracking simulations based on the measured beam emittance, it has been found that an octupole magnetic field is effective in tail-folding and a 10-mm-diameter beam can be formed with two octupole magnets added in the present beam line. It has been also found that additional magnets need to be installed and the beam emittance should be reduced for the objective beam size of 6 mm. Moreover, the objective may be attained if the beam path length and configuration of the magnetic lens system are freely chosen.

JAEA Reports

Light ion microbeam analysis / processing system and its improvement

Koka, Masashi; Ishii, Yasuyuki; Yamada, Naoto; Okubo, Takeru; Kada, Wataru*; Kitamura, Akane; Iwata, Yoshihiro*; Kamiya, Tomihiro; Sato, Takahiro

JAEA-Technology 2016-006, 41 Pages, 2016/03

JAEA-Technology-2016-006.pdf:14.03MB

A MeV-class light ion microbeam system has been developed for micro-analysis and micro-fabrication with high spatial resolution at 3-MV single-ended accelerator in Takasaki Ion Accelerators for Advanced Radiation Application of Takasaki Advanced Radiation Research Institute, Sector of Nuclear Science Research, Japan Atomic Energy Agency. This report describes the technical improvements for the main apparatus (the accelerator, beam-transport lines, and microbeam system), and auxiliary equipments/ parts for ion beam applications such as Particle Induced X-ray/Gamma-ray Emission (PIXE/PIGE) analysis, 3-D element distribution analysis using PIXE-Computed Tomography(CT), Ion Beam-Induced Luminescence (IBIL) analysis, and Proton Beam Writing with the microbeam scanning, with functional outline of these apparatus and equipments/parts.

JAEA Reports

The Second periodic safety review report of Tokai Reprocessing Plant

Shirai, Nobutoshi; Miura, Yasushi; Tachibana, Ikuya; Omori, Satoru; Wake, Junichi; Fukuda, Kazuhito; Nakano, Takafumi; Nagasato, Yoshihiko

JAEA-Technology 2016-007, 951 Pages, 2016/07

JAEA-Technology-2016-007-01.pdf:11.93MB
JAEA-Technology-2016-007-02.pdf:4.7MB

The periodic safety review of TRP is to confirm the safety activities and get effective additional measures the facility safety and its reliability. We implemented 4 items; for (1) evaluation of safety activity implementation, we confirmed we are adequately expanding its safety activities by the necessary documents and schemes. For (2) evaluation of status of safety activities reflecting the latest technical knowledges, we confirmed we reflect latest knowledges for improvement of safety and reliability. For (3) technical evaluation about aging degradation, we can keep the safety of the facilities important to safety and the sea discharge line, under assumption of the present maintenance, because of "focuses for aging degradation". For (4) planning measures about a 10-years-plan that the operator shall implement to keep the facility condition, by the technical evaluation, we found no additional safety plans into maintenance strategies.

JAEA Reports

Inspection and repair techniques in the reactor vessel of the experimental fast reactor Joyo; Replacement of upper core structure

Ito, Hiromichi*; Ota, Katsu; Kawahara, Hirotaka; Kobayashi, Tetsuhiko; Takamatsu, Misao; Nagai, Akinori

JAEA-Technology 2016-008, 87 Pages, 2016/05

JAEA-Technology-2016-008.pdf:18.11MB

In the experimental fast reactor Joyo, as a part of the restoration work of a partial dysfunction of fuel handling, the replacement of the upper core structure (UCS) was started from March 2014, and was completed in December 2014. In the jack-up test, the UCS was jacked-up to 1000 mm without significant sodium shearing resistance and interference. In the replacement of the UCS, a procedure was prepared with the use of wire-jack equipment assuming the interference. As a result, with the procedure and wire-jack were effectively functioned, the work was successfully completed.

JAEA Reports

Replacement of the glove box panel in the nuclear fuel reprocessing facility

Yamamoto, Masahiko; Shirozu, Hidetomo; Mori, Eito; Surugaya, Naoki

JAEA-Technology 2016-009, 58 Pages, 2016/05

JAEA-Technology-2016-009.pdf:3.95MB

The panels of glove box installed at Tokai Reprocessing Plant have been deteriorated and transparencies have been decreased due to the long-term use. Therefore, the panels have been replaced from the view point of preventive maintenance. In the new regulation formulated since the Fukushima Daiichi Nuclear Power Plant accident, it is demanded that the glove box consists of incombustible or inflammable materials. In this replacement, new panels have been manufactured with polycarbonate which satisfied the UL94 V-0 incombustible class. The inside of glove box has been contaminated with radioactive materials. Thus, the contamination and operator's exposure have been investigated. Then radiation protection equipment have been selected. Also, it is necessary to maintain the glove box enclosure during the replacement. The replacement has been conducted by covering the opening parts with vinyl sheets. The enclosure function has been verified by the inspection of the new panels and glove box.

JAEA Reports

Study of HTGR contribution to Japan's CO$$_{2}$$ emission reduction goal in 2050

Kamiji, Yu; Suzuki, Koichi*; Yan, X.

JAEA-Technology 2016-010, 24 Pages, 2016/07

JAEA-Technology-2016-010.pdf:1.05MB

Japanese government has set the goal of reducing CO$$_{2}$$ emission by 26% in 2030 below the 2013 level, in longer term, by 80% below the 1990 level. To achieve the goals, various measures should be taken. The GTHTR300, a commercial High Temperature Gas-cooled Reactor (HTGR) design being developed by JAEA offers spectrum of heat applications by using its high temperature heat up to 950$$^{circ}$$C. The potential contribution of CO$$_{2}$$ emission reduction by HTGR is estimated considering domestic and overseas deployment of the GTHTR300. The best estimate for domestic CO$$_{2}$$ reduction is 2.07$$times$$10$$^{8}$$ ton- CO$$_{2}$$/yr and that from oversea is 2.25$$times$$10$$^{8}$$ ton- CO$$_{2}$$/yr. The sum of these is about 47% of 9.13$$times$$10$$^{8}$$ ton- CO$$_{2}$$/yr which is CO$$_{2}$$ reduction target in 2050, for which deployment of 52 plants in Japan and 113 plants abroad, with each plant containing four 600 MWt reactor units, is required.

JAEA Reports

Long-term immersion experiments of low alkaline cementitious materials

Seno, Yasuhiro*; Noguchi, Akira*; Nakayama, Masashi; Sugita, Yutaka; Suto, Shunkichi; Tanai, Kenji; Fujita, Tomoo; Sato, Haruo*

JAEA-Technology 2016-011, 20 Pages, 2016/07

JAEA-Technology-2016-011.pdf:7.56MB

Cementitious materials are expected to be used for the construction of an underground repository for the geological disposal of radioactive wastes. Ordinary Portland Cement(OPC) would conventionally be used in the fields of civil engineering and architecture, however, OPC has the potential to generate a highly alkaline plume (pH$$>$$12.5), which will likely degrade the performance of other barriers in the repository such as the bentonite buffer and/or host rock. Low alkaline cementitious materials are therefore being developed that will mitigate the generation of a highly alkaline plume. JAEA has developed a High-volume Fly ash Silica fume Cement (HFSC) as a candidate low alkaline cementitious material. The workability of the HFSC shotcrete was confirmed by conducting In-situ full scale construction tests in the Horonobe underground research laboratory. This report summarizes the results of immersion tests to assess the long-term pH behavior of hardened HFSC cement pastes made with mix designs that are expected to be able to be used in the construction of an underground repository in Japan.

JAEA Reports

Solvent extraction and release behavior of ruthenium and europium in fire accident conditions in reprocessing plants (Contract research)

Amano, Yuki; Watanabe, Koji; Masaki, Tomoo; Tashiro, Shinsuke; Abe, Hitoshi

JAEA-Technology 2016-012, 21 Pages, 2016/06

JAEA-Technology-2016-012.pdf:1.81MB

To contribute to safety evaluation of fire accident in fuel reprocessing plants, solvent extraction behavior of ruthenium, which could form volatile species, was investigated. Distribution ratios of ruthenium at fire accident conditions were obtained by extraction experiments with several solvent composition at different temperature as parameters. In order to investigate release behavior of ruthenium and europium at fire accident, release ratios of ruthenium and europium were also obtained by solvent combustion experiments.

JAEA Reports

Study on radionuclide analysis of rubble and plants for decommissioning of Fukushima Daiichi Nuclear Power Station

Seki, Kotaro; Sasaki, Takayuki*; Akimoto, Yuji*; Tokunaga, Takahito; Tanaka, Kiwamu; Haraga, Tomoko; Ueno, Takashi; Ishimori, Kenichiro; Hoshi, Akiko; Kameo, Yutaka

JAEA-Technology 2016-013, 37 Pages, 2016/07

JAEA-Technology-2016-013.pdf:2.09MB

In this study, based on the simple and rapid analytical method established from the wastes from research facilities, we created analytical schemes which is applicable to rubble and plants collected at Fukushima Daiichi, then transported to Nuclear Science Research Institute of JAEA. We examined the applicability, and confirmed quantifiability of radioactivity concentration with high recovery rate without being affected by fission products such as $$^{90}$$Sr and $$^{137}$$Cs.

JAEA Reports

Selection of design basis event for modular high temperature gas-cooled reactor

Sato, Hiroyuki; Nakagawa, Shigeaki; Ohashi, Hirofumi

JAEA-Technology 2016-014, 64 Pages, 2016/06

JAEA-Technology-2016-014.pdf:4.21MB

In this study, we investigate a deterministic approach to select design basis events utilizing information obtained from probabilistic approach. In addition, selections of design basis events are conducted for commercial HTGR designed by JAEA. As a result, an approach for selecting design basis event considering multiple failures of safety systems is established which has not been considered as design basis in the safety guideline for existing nuclear facility. Furthermore, selection of design basis events for commercial HTGR has completed.

JAEA Reports

Enhancement of control rod drive mechanism seating position detector for JRR-3

Ouchi, Satoshi; Kurumada, Osamu; Kamiishi, Eigo; Sato, Masayuki; Ikekame, Yoshinori; Wada, Shigeru

JAEA-Technology 2016-015, 42 Pages, 2016/06

JAEA-Technology-2016-015.pdf:3.53MB

The purpose of the control rod drive mechanism seating position detector for JRR-3 is one of a method for confirming the shutdown condition of the reactor. The detector has been utilizing more than 25 years with maintenance regularly. However, it is occurred some trouble recently. Moreover, the detector has already been end of manufacture, and even in the successor detector, it unsuitable for the control rod drive mechanism of JRR-3 was confirmed. Therefore, it was necessary to select the adequate detector to the control rod drive mechanism of JRR-3. Accordingly, we built a test device with the aim of verify several detectors for integrity and function. At the time of the test for performance confirmation, it was occurred unexpected problems. Nevertheless, we devise improvement of the problems and took measures. Thus we were able to collect adequate detector for JRR-3 and replace to enhanced detector. This paper reports the Enhanced of Control rod drive mechanism seat position detector.

JAEA Reports

HTTR thermal load fluctuation test (non-nuclear heating test); Confirmation of HTGR system response against temperature transient

Honda, Yuki; Tochio, Daisuke; Nakagawa, Shigeaki; Sekita, Kenji; Homma, Fumitaka; Sawahata, Hiroaki; Sato, Hiroyuki; Sakaba, Nariaki; Takada, Shoji

JAEA-Technology 2016-016, 16 Pages, 2016/08

JAEA-Technology-2016-016.pdf:2.84MB

A system analysis code is validated with the thermal-load fluctuation absorption test with nun-nuclear heating by using the High Temperature Engineering test Reactor (HTTR) to clarify the High Temperature Gas-cooled Reactor (HTGR) system response against temperature transient. The thermal-load fluctuation absorption test consists on the thermal load fluctuation tests (non-nuclear heating) and heat application system abnormal simulating test (non-nuclear heating). The HTGR reactor response against temperature transient is clarified in the thermal load fluctuation test (non-nuclear heating). The Intermediate Heat Exchanger (IHX) reactor response against temperature transient is clarified in the heat application system abnormal simulating test (non-nuclear heating). With the two HTTR non-nuclear heating test, HTGR system response against temperature transient is obtained.

JAEA Reports

Inspection and repair techniques in the reactor vessel of the experimental fast reactor Joyo; Observation technical development in a reactor vessel of the fast reactor, 3

Okuda, Eiji; Sasaki, Jun; Suzuki, Nobuhiro; Takamatsu, Misao; Nagai, Akinori

JAEA-Technology 2016-017, 20 Pages, 2016/07

JAEA-Technology-2016-017.pdf:5.75MB

In-Vessel Observation (IVO) techniques for Sodium Cooled Fast Reactors (SFRs) in service are important for confirming their safety and integrity. Since IVO equipment for an SFR has to be designed to tolerate the severe conditions (high temperature, high radiation dose and limited access route), fiberscopes used to be used in previous IVO for SFRs. However, in order to attain an IVO with higher quality and resolution, IVO using a radiation resistant camera was conducted in the fast experimental reactor Joyo and obtained some results. The demonstration results provided valuable insights for use in further improving and verifying IVO techniques in SFRs.

JAEA Reports

Calculation of the dose equivalent rate based on the unit concentration of contaminated soil in a flexible container

Sugaya, Toshikatsu; Abe, Daichi; Takebe, Shinichi; Nakatani, Takayoshi; Sakai, Akihiro

JAEA-Technology 2016-018, 20 Pages, 2016/09

JAEA-Technology-2016-018.pdf:2.41MB

Decontamination to the pollution which occurred with an accident of a nuclear power plant with Tohoku-district Pacific offing earthquake has been performed. The contaminated soil which occurred in decontamination stores it in the flexible container back, and is the kept situation. To presume concentration of radioactivity of contents from the dose of the flexible container, the 1cm dose equivalent rate per the unit concentration of radioactivity was calculated with QAD-CGGP2R.

JAEA Reports

Design study for impermeable function of trench disposal facility for very low level waste generated from research, industrial and medical facilities (Joint research)

Sakai, Akihiro; Kurosawa, Ryohei*; Nakata, Hisakazu; Okada, Shota; Izumo, Sari; Sato, Makoto*; Kitamura, Yoichi*; Honda, Yasutake*; Takaoka, Katsuki*; Amazawa, Hiroya

JAEA-Technology 2016-019, 134 Pages, 2016/10

JAEA-Technology-2016-019.pdf:8.25MB

Japan Atomic Energy Agency has been developing to design trench disposal facility with impermeable layers in order to dispose of miscellaneous waste. Geomembrane liners have a function that prevent seepage of leachant and collect the leachant. However, the geomembrane liners do not necessarily provide the expected performance due to damage generated when heavy equipment contacts with the liner. Therefore, we studied the impermeable layers having high performance of preventing seepage of leachant including radioactivity taking into account characteristics of low permeable materials and effect of multiple layer structure. As results, we have evaluated that the composite layers composed by a drainage layer, geomembrane liners and a low permeable layer are most effective structure to prevent seepage of leachant. Taking into account disposal of waste including cesium, we also considered zeolite containing sheets for adsorption of cesium were installed in the impermeable layers.

JAEA Reports

Current status of a decommissioning project in the Enrichment Engineering Facility; Results in the second-half of the fiscal year of 2014

Matsumoto, Takashi; Takahashi, Nobuo; Hayashibara, Kenichi; Ishimori, Yuu; Mita, Yutaka; Kakiya, Hideyoshi

JAEA-Technology 2016-020, 80 Pages, 2016/11

JAEA-Technology-2016-020.pdf:17.8MB

The Enrichment Engineering Facility of the Ningyo-toge Environmental Engineering Center was constructed in order to establish the technological basis of plant engineering for uranium enrichment in Japan. Uranium enrichment tests, using natural and reprocessed uranium, were carried out from 1979 to 1989 with two types of centrifuges in the facility. According to the decommissioning plan of the facility, UF$$_{6}$$ handling equipment and supplemental equipment in these plants are intended to be dismantled by 2019 in order to make vacant spaces for future projects use, for example, inventory investigation, precipitation treatment, etc. This report shows the current state of the decommissioning project in the second-half of the fiscal year of 2014.

JAEA Reports

Optimization of the magnetic field environment in the polarization analysis system of BL22 "RADEN" at J-PARC/MLF (Contract research)

Hiroi, Kosuke; Shinohara, Takenao; Hayashida, Hirotoshi*; Su, Y. H.; Kai, Tetsuya; Oikawa, Kenichi

JAEA-Technology 2016-021, 14 Pages, 2016/10

JAEA-Technology-2016-021.pdf:16.4MB

Energy resolved neutron imaging techniques have been developed at BL22 "RADEN" installed in the Materials and Life Science Experimental Facility (MLF) of J-PARC. A polarized neutron imaging technique attracts much attention as a magnetic imaging method that enables to obtain a quantitative magnetic field distribution in an industrial product under driving state. At RADEN, a polarization analysis apparatus for polarized neutron imaging experiments has been prepared, but its performance was not fully achieved due to imperfectness of the field connection between devices. To improve the performance of polarization analysis system at RADEN, we performed magnetic field simulation of this system, and optimized the magnetic field environment by evaluating the magnetic field connection. After the optimization, we rearranged devices of the system, and confirmed that uniform polarization distribution could be obtained within 4$$times$$4 cm$$^{2}$$ field of view.

JAEA Reports

Calculation by PHITS code for recoil tritium release rate from beryllium under neutron irradiation (Joint research)

Ishitsuka, Etsuo; Kenzhina, I. E.*; Okumura, Keisuke; Takemoto, Noriyuki; Chikhray, Y.*

JAEA-Technology 2016-022, 35 Pages, 2016/10

JAEA-Technology-2016-022.pdf:3.73MB

As a part of study on the mechanism of tritium release to the primary coolant in research and testing reactors, the calculation methods by PHITS code is studied to evaluate the recoil tritium release rate from beryllium core components. Calculations using neutron and triton sources were compared, and it is clear that the tritium release rates in both cases show similar values. However, the calculation speed for the triton source cases is two orders faster than that for the neutron source case. It is also clear that the calculation up to history number per unit volume of 2$$times$$10$$^{4}$$ (cm$$^{-3}$$) is necessary to determine the recoil tritium release rate of two effective digits precision. Furthermore, the relationship between the beryllium shape and recoil tritium release rate using the triton sources was studied. Recoil tritium release rate showed linear relation to the surface area per volume of beryllium, and the recoil tritium release rate showed about half of the conventional equation value.

JAEA Reports

Waste acceptance criteria for waste packages destined for near surface disposal containing radioactive waste from research, industrial and medical facilities

Okada, Shota; Izumo, Sari; Nakata, Hisakazu; Tsuji, Tomoyuki; Sakai, Akihiro; Amazawa, Hiroya

JAEA-Technology 2016-023, 129 Pages, 2016/11

JAEA-Technology-2016-023.pdf:8.95MB

Waste packages must meet the technical requirements. This is because JAEA has been preparing an operating procedure manual for quality control of radioactive waste disposal to be applied to the processing of the waste packages. Raw wastes generated by JAEA are segregated and stored by a method specified in the manual. The composition of raw wastes was characterized on the basis of records of the segregation process. Simulated waste packages were produced by placing the waste materials in a 200 liter drum, which was then filled with mortar, followed by curing in a controlled manner. The static load test was conducted to measure deformation and strain performance of the simulated waste package. Compression apparatuses which can imitate loading conditions in pit-type and trench-type facility that are planned by JAEA were used. Based on the test result, waste packages produced in accordance with the manual met the technical requirement under the condition.

JAEA Reports

Pretreatment works for disposal of radioactive wastes produced by research activities, 1

Ishihara, Keisuke; Yokota, Akira; Kanazawa, Shingo; Iketani, Shotaro; Sudo, Tomoyuki; Myodo, Masato; Irie, Hirobumi; Kato, Mitsugu; Iseda, Hirokatsu; Kishimoto, Katsumi; et al.

JAEA-Technology 2016-024, 108 Pages, 2016/12

JAEA-Technology-2016-024.pdf:29.74MB

Radioactive isotope, nuclear fuel material and radiation generators are utilized in research institutes, universities, hospitals, private enterprises, etc. As a result, various low-level radioactive wastes (hereinafter referred to as non-nuclear radioactive wastes) are produced. Disposal site for non-nuclear radioactive wastes have not been settled yet and those wastes are stored in storage facilities of each operator for a long period. The Advanced Volume Reduction Facilities (AVRF) are built to produce waste packages so that they satisfy requirements for shallow underground disposal. In the AVRF, low-level beta-gamma solid radioactive wastes produced in the Nuclear Science Research Institute are mainly treated. To produce waste packages meeting requirements for disposal safely and efficiently, it is necessary to cut large radioactive wastes into pieces of suitable size and segregate those depending on their types of material. This report summarizes activities of pretreatment to dispose of non-nuclear radioactive wastes in the AVRF.

JAEA Reports

Stabilization of MOX dissolving solution at STACY

Kobayashi, Fuyumi; Sumiya, Masato; Kida, Takashi; Kokusen, Junya; Uchida, Shoji; Kaminaga, Jota; Oki, Keiichi; Fukaya, Hiroyuki; Sono, Hiroki

JAEA-Technology 2016-025, 42 Pages, 2016/11

JAEA-Technology-2016-025.pdf:17.88MB

A preliminary test on MOX fuel dissolution for the STACY critical experiments had been conducted in 2000 through 2003 at Nuclear Science Research Institute of JAEA. Accordingly, the uranyl / plutonium nitrate solution should be reconverted into oxide powder to store the fuel for a long period. For this storage, the moisture content in the oxide powder should be controlled from the viewpoint of criticality safety. The stabilization of uranium / plutonium solution was carried out under a precipitation process using ammonia or oxalic acid solution, and a calcination process using a sintering furnace. As a result of the stabilization operation, recovery rate was 95.6% for uranium and 95.0% for plutonium. Further, the recovered oxide powder was calcined again in nitrogen atmosphere and sealed immediately with a plastic bag to keep its moisture content low and to prevent from reabsorbing atmospheric moisture.

JAEA Reports

Report on analytical activities in potentially hazardous materials mitigation measures at the Plutonium Conversion Development Facility; 2014.4 $$sim$$ 2015.12

Horigome, Kazushi; Suzuki, Hisanori; Suzuki, Yoshimasa; Ishibashi, Atsushi; Taguchi, Shigeo; Inada, Satoshi; Kuno, Takehiko; Surugaya, Naoki

JAEA-Technology 2016-026, 21 Pages, 2016/12

JAEA-Technology-2016-026.pdf:1.14MB

In order to mitigate potential hazards of storage plutonium in solution such as hydrogen generation, conversion of plutonium solution into MOX powder has been carried out since 2014 in the Plutonium Conversion Development Facility. With respect to the samples taken from the conversion process, about 3500 items of plutonium/uranium solutions and MOX powders have been analyzed for the operation control in the related analytical laboratories at the Tokai Reprocessing Plant. This paper describes the reports on analytical activities and related maintenance works in the analytical laboratories conducted from April 2014 to December 2015.

JAEA Reports

Preliminary tests on adsorption / desorption of alumina adsorbents

Suzuki, Yoshitaka; Ishida, Takuya*; Suzuki, Yumi*; Matsukura, Minoru*; Kurosaki, Fumio*; Nishikata, Kaori; Mimura, Hitoshi*; Tsuchiya, Kunihiko

JAEA-Technology 2016-027, 24 Pages, 2016/12

JAEA-Technology-2016-027.pdf:4.15MB

The research and development (R&D) on the production of $$^{99}$$Mo/$$^{99m}$$Tc by (n,$$gamma$$) method has been carried out in the Neutron Irradiation and Testing Reactor Center. The $$^{99}$$Mo production by (n,$$gamma$$) reaction is a simple and easy method, and it also is advantageous from viewpoints of nuclear proliferation resistance and waste management. However, it is difficult to produce the $$^{99m}$$Tc solution with high radioactive concentration because the specific radioactivity of $$^{99}$$Mo by this method is extremely low. Up to now, various Mo absorbents such as Polyzirconium Compound (PZC) and Polytitanium Compound (PTC) have been developed with high Mo adsorption efficiency. It is necessary for utilization to the generator of these absorbents to evaluate the effect of elements containing these absorbents and to assure the quality of $$^{99m}$$Tc solution. In this report, the status of R&D of the Mo adsorbents was investigated. The alumina as Mo adsorbent, which uses in medical $$^{99}$$Mo/$$^{99m}$$Tc generator, was focused and Mo adsorption/desorption properties of three kinds of alumina was evaluated by different properties such as crystal structure and specific surface.

JAEA Reports

Determination of metal impurities in MOX powder by direct current arc atomic emission spectroscopy; Application of standard addition method for direct analysis of powder sample

Furuse, Takahiro*; Taguchi, Shigeo; Kuno, Takehiko; Surugaya, Naoki

JAEA-Technology 2016-028, 19 Pages, 2016/12

JAEA-Technology-2016-028.pdf:1.79MB

Metal impurities in MOX powder obtained from uranium and plutonium recovered from reprocessing process of spent nuclear fuel are needed to be determined for its characterization. Direct current arc atomic emission spectroscopy (DCA-AES) is one of the useful methods for direct analysis of powder sample without dissolving the analyte into aqueous solution. However, the selection of standard material, which can overcome concerns such as matrix matching, is quite important to create adequate calibration curves for DCA-AES. In this study, we apply standard addition method using the certified U$$_{3}$$O$$_{8}$$ containing known amounts of metal impurities to avoid the matrix problems. The proposed method provides good results for determination of Fe, Cr and Ni at a significant quantity level contained in MOX samples.

JAEA Reports

Fabrication and test results of testing equipment for remote-handling of MA fuel, 3; Testing equipment for fuel loading

Tazawa, Yujiro; Nishihara, Kenji; Sugawara, Takanori; Tsujimoto, Kazufumi; Sasa, Toshinobu; Eguchi, Yuta; Kikuchi, Masashi*; Inoue, Akira*

JAEA-Technology 2016-029, 52 Pages, 2016/12

JAEA-Technology-2016-029.pdf:5.34MB

Transmutation Physics Experimental Facility (TEF-P) planned in the J-PARC project uses minor actinide (MA) fuels in the experiments. These MA fuels are highly-radioactive, so the fuel handling equipment in TEF-P is necessary to be designed as remote-handling system. This report summarizes fabrication and test results of the testing equipment for fuel loading that is one of components of the testing equipment for remote-handling of MA fuels. The testing equipment which had a remote-handling system for fuel loading was fabricated. And the test in combination with the mock-up core was performed. Through the test, it was confirmed to load/take the dummy fuel pin to/from the mock-up core without failure. It was shown that the concept design of the fuel loading equipment of TEF-P was reasonable.

JAEA Reports

Rapid heating rupture experiment using the high chromium steel tubes

Umeda, Ryota; Kurihara, Akikazu; Shimoyama, Kazuhito

JAEA-Technology 2016-030, 50 Pages, 2016/12

JAEA-Technology-2016-030.pdf:5.22MB

In case of tube failure of a steam generator in sodium-cooled fast reactors, the reaction jet with high temperature and high velocity under highly alkaline environment is formed by cited exothermic reaction (sodium-water reaction). When the high temperature reaction jet covers the adjacent tubes, the material strength of tube decreases in the high temperature condition, and the adjacent tube may be swollen and failed by inner pressure (overheating tube rupture). For evaluation of the overheating tube rupture, tube failure is judged by comparison the hoop stress loaded by inner pressure with stress strength standard defined as creep strength depending on tube temperature. Thus, it is important to confirm the validation of this failure criterion based on the findings obtained in the simulated experiment of overheating tube rupture. In this report, for consideration on the validation of the failure criteria and elucidation on the failure mode and strength characteristics of failure, the authors carried out the rapid heating rupture experiment for the thin single and double-walled 9Cr steel tubes at high temperature up to 1500 K by using TRUST-2 rig in the Japan Atomic Energy Agency.

JAEA Reports

History and current situation of mine water treatment in Ningyo-toge Uranium Mine

Nagayasu, Takaaki; Taki, Tomihiro; Fukushima, Shigeru

JAEA-Technology 2016-031, 53 Pages, 2017/02

JAEA-Technology-2016-031.pdf:4.42MB

The forerunner of JAEA, found a smelter in 1964 to do industrialization tests of hydrometallurgical extraction process from domestic uranium ore to uranium tetrafluoride, extracted at Ningyo-toge. Yotsugi Mill Tailings Pond was constructed for the purpose of depositing slag and other things generated due to the operation of the smelter. Furthermore supernatant water from the deposition field had been treated appropriately at wastewater treatment facilities, which has been provided in the downstream site of the pond. We have been utilizing the Yotsugi Mill Tailings Pond as a temporary storage field of mine water generated from the old mining gallery, mainly. After filing an abolition report of facilities of the smelter, with the completion of industrial trials of refinery in 1982. Ningyo-toge environmental engineering center has studied for processing uranium and radium, in wastewater, which must be reduced more safely by advancing these processing technical development. Supernatant water of The Pond is treated at the wastewater treatment facilities before discharging to Ikegogawa-river. And those collateralize the emission standards to discharge to the river set at the Center with continuing stable processing. This document summarized the history of the wastewater treatment, technical development for the water treatment, and the current situation of the water treatment.

JAEA Reports

Preliminary 3-dimensional analysis of groundwater flow in the surrounding environment of near surface disposal facility

Sakai, Akihiro; Kurosawa, Ryohei*; Totsuka, Masayoshi; Nakata, Hisakazu; Amazawa, Hiroya

JAEA-Technology 2016-032, 117 Pages, 2017/02

JAEA-Technology-2016-032.pdf:12.84MB

JAEA has been planning to implement near surface disposal of low level waste generated from research, medical, and industrial facilities. JAEA plans to carry out 3d analysis of groundwater flow in geological model around the disposal site because of development of migration assessment modeling of radioactivity materials in the site. In the safety demonstration test in JAEA, 3d analysis of groundwater flow was carried out on 1999. The analysis was calculated by using the code "3D-SEEP". But it is necessary to improve the conditions of the model in the analysis. Therefore, we improved the geological model which had been developed carried out 3d analysis of groundwater flow by using the current 3D-SEEP for the specified disposal site in the future. From the result, we expect that 3d analysis of groundwater flow in the environment around the specified near surface disposal site will be able to be sufficiently conducted by developing an appropriate model for the disposal site.

JAEA Reports

Shielding calculation by PHITS code during replacement works of startup neutron sources for HTTR operation

Shinohara, Masanori; Ishitsuka, Etsuo; Shimazaki, Yosuke; Sawahata, Hiroaki

JAEA-Technology 2016-033, 65 Pages, 2017/01

JAEA-Technology-2016-033.pdf:11.14MB

To reduce the neutron exposure dose for workers during the replacement works of the startup neutron sources of the High Temperature Engineering Test Reactor, calculations of the exposure dose in case of temporary neutron shielding at the bottom of fuels handling machine were carried out by the PHITS code. As a result, it is clear that the dose equivalent rate due to neutron radiation can be reduced to about an order of magnitude by setting a temporary neutron shielding at the bottom of shielding cask for the fuel handling machine. In the actual replacement works, by setting temporary neutron shielding, it was achieved that the cumulative equivalent dose of the workers was reduced to 0.3 man mSv which is less than half of cumulative equivalent dose for the previous replacement works; 0.7 man mSv.

JAEA Reports

Development of novel technique of negative C$$_{60}$$ ion production by electron attachment using cesium sputter ion source

Usui, Aya; Chiba, Atsuya; Yamada, Keisuke

JAEA-Technology 2016-034, 21 Pages, 2017/03

JAEA-Technology-2016-034.pdf:82.52MB

In the TIARA (Takasaki Ion Accelerators for Advanced Radiation Application), in order to propel the studies on the swift cluster ions, a novel technique was developed to increase the beam intensity of the fullerene ions which would have a considerably larger irradiation effect than any cluster ions. As a new method of negative ion production, the ionization mechanism by electron attachment was introduced as an alternative to the traditional method with the cesium sputtering to the existing cesium sputter type ion source (SNICS). In consequence, the intensity of the negative C$$_{60}$$ ion beam produced using an existing ion source with a novel technique was increased thousand times as high as those using the previous one for 12 hour operation. In this report, we describe the problems in the traditional ionization method and explain the production technique of the negative C$$_{60}$$ ions ionized via electron attachment process, which solves that only by the minor changes in SNICS.

JAEA Reports

Study on engineering technologies in the Mizunami Underground Research Laboratory (FY 2015); Development of recovery and mitigation technology on excavation damage (Contract research)

Fukaya, Masaaki*; Takeda, Nobufumi*; Miura, Norihiko*; Ishida, Tomoko*; Hata, Koji*; Uyama, Masao*; Sato, Shin*; Okuma, Fumiko*; Hayagane, Sayaka*; Matsui, Hiroya; et al.

JAEA-Technology 2016-035, 153 Pages, 2017/02

JAEA-Technology-2016-035.pdf:37.6MB

The researches on engineering technology in the Mizunami Underground Research Laboratory (MIU) project in FY2016, detailed investigations of the (mechanical) behaviors of the plug and the rock mass around the reflood tunnel through ongoing reflood test were performed as part of (5) development of technologies for restoration and/or reduction of the excavation damage. As the result, particularly for the temperature change of the plug, its analytical results agree fairly well agree with the measurement ones. This means cracks induced by temperature stress can be prevented by the cooling countermeasure works reviewed in designing stage. In addition, for the behaviors of the plug and the bedrock boundary after reflooding the reflood tunnel, comparison between the results obtained by coupled hydro-mechanical analysis (stress-fluid coupled analysis) with the ones by several measurements, concluded that the model established based on the analysis results is generally appropriated.

JAEA Reports

Technological study about a disposal measures of low-level radioactive waste including uranium and long-half-life radionuclides

Sugaya, Toshikatsu; Nakatani, Takayoshi; Sasaki, Toshihisa*; Nakamura, Yasuo*; Sakai, Akihiro; Sakamoto, Yoshiaki

JAEA-Technology 2016-036, 126 Pages, 2017/02

JAEA-Technology-2016-036.pdf:7.28MB

At the Radioactive Waste Management and Disposal Project Department Sector of Decommissioning and Radioactive Waste Management, we performed the technological study about the disposal measures of the low-level radioactive waste targeted for uranium-bearing waste and intermediate depth disposal-based waste occurring from the process of the nuclear fuel cycle.

JAEA Reports

Data acquisition of mass transport parameters

Iwasaki, Riyo*; Hama, Katsuhiro; Morikawa, Keita*; Hosoya, Shinichi*

JAEA-Technology 2016-037, 62 Pages, 2017/02

JAEA-Technology-2016-037.pdf:8.69MB

Mass transport study is mainly performed as part of Phase III in the Mizunami Underground Research Laboratory Project. In Phase III, the goal of mass transport study is to obtain a better understanding of mass transport phenomena in the geological environment as well as to develop technologies for measurement of the mass transport parameters, model construction, numerical analysis and validation of those technologies. This study was planned to understand the influence of the geological characteristics of fracture on the mass transport parameters.

JAEA Reports

Development of transportation container for neutron startup source of High Temperature Engineering Test Reactor (HTTR)

Shimazaki, Yosuke; Sawahata, Hiroaki; Yanagida, Yoshinori; Shinohara, Masanori; Kawamoto, Taiki; Takada, Shoji

JAEA-Technology 2016-038, 36 Pages, 2017/02

JAEA-Technology-2016-038.pdf:8.75MB

The High Temperature Engineering Test Reactor (HTTR) has three neutron startup sources (NSs) in the reactor core, each of which consists of $$^{252}$$Cf with 3.7GBq The NSs are exchanged at the interval of approximately 7 years. The NS holders including NSs are transported from the dealer's hot cell to the reactor facility of HTTR using a transportation container. The loading work of NS holders to the Control Rod guide blocks is subsequently carried out in the fuel handling machine maintenance pit of HTTR. Following technical issues were extracted from the experiences in the past two exchange works of NSs to develop a safety handling procedure; (1) The reduction and prevention of radiation exposure of workers. (2) The exclusion of falling of NS holder. Then, a new transportation container special to the NSs of HTTR was developed to solve the technical issues while keeping the cost as low as that for overhaul of conventional container and satisfying the regulation of A type transportation package.

JAEA Reports

Preliminary missions for the decommissioning of the laboratory building No.1 for the plutonium research program

Segawa, Yukari; Horita, Takuma; Kitatsuji, Yoshihiro; Kumagai, Yuta; Aoyagi, Noboru; Nakada, Masami; Otobe, Haruyoshi; Tamura, Yukito*; Okamoto, Hisato; Otomo, Takashi; et al.

JAEA-Technology 2016-039, 64 Pages, 2017/03

JAEA-Technology-2016-039.pdf:5.24MB

The laboratory building No.1 for the plutonium research program (Bldg. Pu1) was chosen as one of the facilities to decommission by Japan Atomic Energy Agency Reform in September, 2013. The research groups, users of Bldg. Pu1, were driven by necessity to remove used equipment and transport nuclear fuel to other facilities from Bldg. Pu1. Research Group for Radiochemistry proactively established the Used Equipment Removal Team for the smooth operation of the removal in April, 2015. The team classified six types of work into the nature of the operation, removal of used equipment, disposal of chemicals, stabilization of mercury, stabilization of nuclear fuel, transportation of nuclear fuel and radioisotope, and survey of contamination status inside the glove boxes. These works were completed in December, 2015. This report circumstantially shows six works process, with the exception of the approval of the changes on the usage of nuclear fuel in Bldg. Pu1 to help prospective decommission.

JAEA Reports

Neutronic characteristic of HTTR fuel compact with various packing models of coated fuel particle

Ho, H. Q.; Honda, Yuki; Goto, Minoru; Takada, Shoji

JAEA-Technology 2016-040, 16 Pages, 2017/03

JAEA-Technology-2016-040.pdf:2.89MB

To study the packing effects of the truncated coated fuel particle on the criticality for the High Temperature engineering Test Reactor (HTTR), four alternative models including the truncated uniform model, the non-truncated uniform model, the truncated random model and the non-truncated random model for the arrangement of CFP in fuel compact were used, and the neutronic and criticality calculation were performed by using Monte Carlo MCNP6 code with ENDF/B-VII.1 cross section library. The results showed that the infinite multiplication factors (k$$_{rm inf}$$) in the truncated models were lower than those of the non-truncated models regardless of the uniform or random arrangement, and the four factors in the four-factor-formula showed that the difference of k$$_{rm inf}$$ was mainly attributed to the resonance escape probability. The difference in resonance escape probability is caused by the increase of capture reactions in the resonance region as the influence of spatial-self-shielding-effect. It is because the equivalent kernel diameter of the CFP for the truncated model is smaller than that of the non-truncated model.

JAEA Reports

Fabrication techniques of the sample supporting jigs for Post Irradiation Examination with 3 dimension printer

Miyai, Hiromitsu; Suzuki, Miho; Kanazawa, Hiroyuki

JAEA-Technology 2016-041, 46 Pages, 2017/03

JAEA-Technology-2016-041.pdf:5.54MB

In the Reactor Fuel Examination Facility (RFEF) of Japan Atomic Energy Agency (JAEA), Post Irradiation Examinations (PIEs) have been carried out for a long time in order to verify the reliability and the safety of the nuclear fuels irradiated in nuclear power plants. Samples for the PIEs are small and have various shapes. In order to facilitate the handling of the samples using a manipulator, the several kinds of jigs have been used for PIEs at RFEF those jigs are usually manufactured by machining process. We tried to make the jigs, which is PLA resin, with 3D printer and instead of machining process for the reduction of the manufacturing time and the improvement of the dimensional accuracy of the jig this time. It became clear that the actual dimensions of the jigs manufactured with 3D printer were roughly smaller at the concave section and larger at the convex section compared with the dimensions of the plan. So it is necessary to make a plan for the jigs after consideration of the characteristic of the 3D printer. The jigs can be applied to SEM observation, because the deposition of carbon film onto the jigs was well. And the jigs can be used to for the metallography, because the jigs were applicable without any harmful effects on polishing and etching processes.

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