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Journal Articles

Role of retained austenite in low alloy steel at low temperature monitored by neutron diffraction

Yamashita, Takayuki; Morooka, Satoshi; Harjo, S.; Kawasaki, Takuro; Koga, Norimitsu*; Umezawa, Osamu*

Scripta Materialia, 177, p.6 - 10, 2020/03

 Times Cited Count:0

Journal Articles

Solution neutron scattering

Sugiyama, Masaaki*; Inoue, Rintaro*; Nakagawa, Hiroshi; Saio, Tomohide*

Hamon, 30(1), p.16 - 25, 2020/02

Neutron has distinct features as a scattering probe to analyze structure and dynamics of biological macromolecules. The theme of this review is to try to describe how we did/do utilize them. And "How we should utilize them more effectively in the trend of integrative structural biology?" with solution scattering.

Journal Articles

What should we learn from the back numbers of HAMON ?

Takeda, Masayasu

Hamon, 30(1), p.7 - 8, 2020/02

Safety review of JRR-3 under the New Regulatory Requirements was completed on 7th November 2018. Neutron beam will come back in early 2021 after reinforcement works of the roof of the reactor building, the peripheral structures like a stack, a cooling tower, and the experimental hall. The future of neutron sciences using the research reactor strongly depends on how many impacted researches using JRR-3 are achieved after restarting JRR-3. At this stage, we can learn a lot of things from the back numbers of HAMON.

Journal Articles

Pseudo-triplet 5$$f$$ electron state in the heavy fermion superconductor NpPd$$_5$$Al$$_2$$

Metoki, Naoto; Aoki, Dai*; Griveau, J.-C.*; Otsuki, Junya*

Journal of the Physical Society of Japan, 89(2), p.024707_1 - 024707_6, 2020/02

The pseudo triplet ground state in the heavy-fermion superconductor NpPd$$_5$$Al$$_2$$ was concluded. The magnetic susceptibility $$chi$$ can be reproduced by the singlet ground state $$Gamma_{t1}$$ with the main component of $$|0rangle$$ and the first excited doublet $$Gamma_{t5}$$ dominated by $$|pm1rangle$$ at $$Delta E=49$$,K. The magnetization curve can be explained from the effective local hamiltonian for pseudo spin $$J$$=1 with $$DJ_z^2$$($$D=Delta E$$) equivalent to the quadrupole operator $$O_{20}$$. The specific heat can be described with the Kondo model normalized to give the entropy R$$ln3$$, corresponding to the pseudo triplet state. The derived Kondo temperature $$T_{rm K}=55$$,K comparable to the level splitting $$Delta E=49$$,K indicates the contribution of the excited doublet $$Gamma_{t5}$$ to the possible multi-channel Kondo effect.

Journal Articles

Weak-coupling mean-field theory of magnetic properties of NiGa$$_{2}$$S$$_{4}$$

Nomura, Takuji*; Yamamoto, Yuji*; Yoshii, Kenji

Journal of the Physical Society of Japan, 89(2), p.024704_1 - 024704_10, 2020/02

We report a mean-field theoretical study of a triangular magnet NiGa$$_{2}$$S$$_{4}$$. Using the localized Wannier functions obtained from a band calculation, the most stable magnetic state was found to be spiral with the incommensurate structure, consistent with the result from neutron diffraction. The Ni-site Coulomb interaction was not strong (U about 2 eV). The spin value at the Ni site was also not so large about 1.1 mb. These results mean that the hybridization between Ni and S may play an important role. The dynamical spin correlation function was found to in accord with the results from neutron scattering.

Journal Articles

$$f$$-electron states of heavy-fermion superconductor NpPd$$_5$$Al$$_2$$ and rare-earth- and actinide-based isostructural compounds

Metoki, Naoto

Journal of the Physical Society of Japan, 89(2), p.025001_1 - 025001_2, 2020/02

Good correspondence of the $$LS$$ and $$j$$-$$j$$ coupling scheme can be realized in the $$f$$-electron states of the heavy-fermion superconductor NpPd$$_5$$Al$$_2$$ and the isostructural family. The rare-earth and actinide elements are under a common strong uniaxial point charge potential with tetragonal point symmetry $$D_{4h}$$. The systematic development of the $$f$$-electron states can be understood in the $$LS$$ coupling scheme of $$^nf$$ configuration (the number of $$f$$ electrons $$nleq6$$). We can find the corresponding states in $$j$$-$$j$$ coupling scheme with three $$f$$-orbitals $$Gamma_7^{rm; i}, Gamma_7^{rm; ii}$$, and $$Gamma_6$$ determined from CePd$$_5$$Al$$_2$$ with $$^1f$$ configuration.

Journal Articles

Applications of the energy-resolved neutron imaging system, RADEN

Kai, Tetsuya; Shinohara, Takenao; Matsumoto, Yoshihiro*

Kensa Gijutsu, 25(2), p.1 - 5, 2020/02

no abstracts in English

Journal Articles

Neutron transmission spectrum of liquid lead bismuth eutectic

Oba, Yojiro; Ito, Daisuke*; Saito, Yasushi*; Onodera, Yohei*; Parker, J. D.*; Shinohara, Takenao; Oikawa, Kenichi

Materials Research Proceedings, Vol.15, p.160 - 164, 2020/02

Lead Bismuth eutectic (LBE) is a promising candidate of the coolant for accelerator driven system (ADS) and fast breeder reactor. Neutron transmission imaging is a powerful technique to investigate the LBE in flow channel. However, previous studies have focused on the analysis of the neutron transmission spectra due to Bragg diffraction (Bragg edge transmission) from the solid phase of the LBE. If the neutron transmission spectra due to the diffraction from a liquid phase can be observed, it is useful to study the behavior of the molten LBE in the flow channel. Therefore, the energy-resolved neutron transmission imaging measurements of the molten LBE was carried out. The observed neutron transmission spectra can be explained by those calculated from the scattering profiles of the molten LBE. This indicates that the structure of the molten LBE can be characterized and mapped using the neutron transmission imaging.

Journal Articles

Ice I$$_{rm c}$$ without stacking disorder by evacuating hydrogen from hydrogen hydrate

Komatsu, Kazuki*; Machida, Shinichi*; Noritake, Fumiya*; Hattori, Takanori; Sano, Asami; Yamane, Ryo*; Yamashita, Keishiro*; Kagi, Hiroyuki*

Nature Communications (Internet), 11(1), p.464_1 - 464_5, 2020/02

Water freezes below 0$$^{circ}$$C at ambient pressure ordinarily to ice I$$_{rm h}$$, with hexagonal stacking sequence. Under certain conditions, ice with a cubic stacking sequence can also be formed, but ideal ice I$$_{rm c}$$ without stacking-disorder has never been formed until recently. Here we demonstrate a route to obtain ice I$$_{rm c}$$ without stacking-disorder by degassing hydrogen from the high-pressure form of hydrogen hydrate, C$$_{2}$$, which has a host framework isostructural with ice I$$_{rm c}$$. The stacking-disorder free ice I$$_{rm c}$$ is formed from C$$_{2}$$ via an intermediate amorphous or nano-crystalline form under decompression, unlike the direct transformations occurring in ice XVI from neon hydrate, or ice XVII from hydrogen hydrate. The obtained ice I$$_{rm c}$$ shows remarkable thermal stability, until the phase transition to ice I$$_{rm h}$$ at 250 K, originating from the lack of dislocations. This discovery of ideal ice I$$_{rm c}$$ will promote understanding of the role of stacking-disorder on the physical properties of ice as a counter end-member of ice I$$_{rm h}$$.

Journal Articles

Strong local moment antiferromagnetic spin fluctuations in V-doped LiFeAs

Xu, Z.*; Dai, G.*; Li, Y.*; Yin, Z.*; Rong, Y.*; Tian, L.*; Liu, P.*; Wang, H.*; Xing, L.*; Wei, Y.*; et al.

npj Quantum Materials (Internet), 5(1), p.11_1 - 11_7, 2020/02

Journal Articles

Anomalous small-angle X-ray scattering (ASAXS) study of irradiation-induced nanostructure change in Fe-ion beam irradiated oxide dispersion-strengthened (ODS) steel

Kumada, Takayuki; Oba, Yojiro; Motokawa, Ryuhei; Morooka, Satoshi; Tominaga, Aki; Tanida, Hajime; Shobu, Takahisa; Konno, Azusa; Owada, Kenji*; Ono, Naoko*; et al.

Journal of Nuclear Materials, 528, p.151890_1 - 151890_7, 2020/01

 Times Cited Count:0

We have developed an anomalous small-angle X-ray scattering (ASAXS) diffractometer in SPring-8 to investigate irradiation-induced nanostructural change in ion-beam irradiated stainless steel. A thermally-aged MA956 stainless steel sample displays power-law scattering that follows the Porod law at the magnitude of scattering vector, Q, below 0.5 nm$$^-1$$ and an overlapped shoulder around 0.7 nm$$^-1$$. After the ion-beam irradiation, the intensity of the shoulder remained unchanged, whereas that of the power-law scattering nearly doubled. This result indicates that none of the structural parameters of the Cr-rich nanoprecipitates, such as the number density, size, and interface roughness, were changed by the irradiation.

Journal Articles

Multi-step magnetic transitions in EuNiIn$$_4$$

Ikeda, Shugo*; Kaneko, Koji; Tanaka, Yuki*; Kawasaki, Takuro; Hanashima, Takayasu*; Munakata, Koji*; Nakao, Akiko*; Kiyanagi, Ryoji; Ohara, Takashi; Mochizuki, Kensei*; et al.

Journal of the Physical Society of Japan, 89(1), p.014707_1 - 014707_7, 2020/01

 Times Cited Count:0

Journal Articles

Various topological spin textures in a two-dimensional Heisenberg ferromagnet with dipole-dipole interactions

Yokota, Terufumi

Journal of the Physical Society of Japan, 89(1), p.014706_1 - 014706_6, 2020/01

Journal Articles

X-ray and neutron study on the structure of hydrous SiO$$_{2}$$ glass up to 10 GPa

Urakawa, Satoru*; Inoue, Toru*; Hattori, Takanori; Sano, Asami; Kohara, Shinji*; Wakabayashi, Daisuke*; Sato, Tomoko*; Funamori, Nobumasa*; Funakoshi, Kenichi*

Minerals (Internet), 10(1), p.84_1 - 84_13, 2020/01

The structure of hydrous amorphous SiO$$_{2}$$ is fundamental to investigate the effects of water on the physicochemical properties of oxide glasses and magma. The hydrous SiO$$_{2}$$ glass with 13 wt.% D$$_{2}$$O was synthesized under high-pressure and high-temperature conditions and its structure was investigated by small angle X-ray scattering, X-ray diffraction, and neutron diffraction experiments at pressures of up to 10 GPa and room temperature. This hydrous glass is separated into a SiO$$_{2}$$ rich major phase and a D$$_{2}$$O rich minor phase. Medium-range order of the hydrous glass shrinks compared to the anhydrous SiO$$_{2}$$ glass due to disruption of SiO$$_{4}$$ linkage by formation of Si-OD deuterioxyl, while the pressure response is similar. Most of D$$_{2}$$O molecules are in the small domains and hardly penetrate into SiO$$_{2}$$ major phase.

Journal Articles

Lattice dynamics in FeSe via inelastic X-ray scattering and first-principles calculations

Murai, Naoki; Fukuda, Tatsuo; Nakajima, Masamichi*; Kawamura, Mitsuaki*; Ishikawa, Daisuke*; Tajima, Setsuko*; Baron, A. Q. R.*

Physical Review B, 101(3), p.035126_1 - 035126_6, 2020/01

We report an inelastic X-ray scattering investigation of phonons in FeSe superconductor. Comparing the experimental phonon dispersion with density functional theory (DFT) calculations in the non-magnetic state, we found a significant disagreement between them. A better overall agreement was obtained by allowing for spin-polarization in DFT calculations, despite the absence of magnetic order in FeSe. This calculation gives a realistic approximation, at DFT level, of the disordered paramagnetic state of FeSe, in which strong spin fluctuations are present.

Journal Articles

Magnetic structures and quadratic magnetoelectric effect in LiNiPO$$_{4}$$ beyond 30 T

Fogh, E.*; Kihara, Takumi*; Toft-Petersen, R.*; Bartkowiak, M.*; Narumi, Yasuo*; Prokhnenko, O.*; Miyake, Atsushi*; Tokunaga, Masashi*; Oikawa, Kenichi; S${o}$rensen, M. K.*; et al.

Physical Review B, 101(2), p.024403_1 - 024403_12, 2020/01

Journal Articles

Structural and electrochemical features of (Li$$_{2}$$S)$$_{x}$$(SiS$$_{2}$$)$$_{100-x}$$ superionic glasses

Mori, Kazuhiro*; Iwase, Kenji*; Oba, Yojiro; Ikeda, Kazutaka*; Otomo, Toshiya*; Fukunaga, Toshiharu*

Solid State Ionics, 344, p.115141_1 - 115141_10, 2020/01

no abstracts in English

Journal Articles

Segmental motions of proteins under non-native states evaluated using quasielastic neutron scattering

Fujiwara, Satoru*; Matsuo, Tatsuhito*; Sugimoto, Yasunobu*; Shibata, Kaoru

Journal of Physical Chemistry Letters (Internet), 10(23), p.7505 - 7509, 2019/12

 Times Cited Count:0 Percentile:100(Chemistry, Physical)

Characterization of the dynamics of disordered polypeptide chains is required to elucidate the behavior of intrinsically disordered proteins and proteins under non-native states related to the folding process. Here we develop a method using quasielastic neutron scattering, combined with small-angle X-ray scattering and dynamic light scattering, to evaluate segmental motions of proteins as well as diffusion of the entire molecules and local side-chain motions. We apply this method to RNase A under the unfolded and molten-globule (MG) states. The diffusion coefficients arising from the segmental motions are evaluated and found to be different between the unfolded and MG states. The values obtained here are consistent with those obtained using the fluorescence-based techniques. These results demonstrate not only feasibility of this method but also usefulness to characterize the behavior of proteins under various disordered states.

Journal Articles

Development of low inductance circuit for radially symmetric circuit

Takayanagi, Tomohiro; Ueno, Tomoaki; Horino, Koki

Journal of Physics; Conference Series, 1350(1), p.012183_1 - 012183_7, 2019/12

As one of the advanced research and development for maintaining the stable operation of J-PARC RCS, we are developing semiconductor switch circuit for thyratron substitute adopted in kicker system. Radiation symmetric type circuits using semiconductors of SIC-MOSFETs are composed of circuits in which many semiconductor switches are multiplexed in parallel. Since the lengths of all parallel circuits are equal, the output waveform will not be distorted due to timing jitter or impedance. This circuit is useful for outputting the waveform of ultrafast short pulse. Therefore, we have developed a circuit that achieves further low inductance by making the power transmission circuit into a double circular ring structure equal to the coaxial shape. Compare the inductance value obtained from the structure and the output waveform. In addition, we compare the calculation and the measurement in the test and present the verification result of the developed circular ring structure.

Journal Articles

Simulations of beam loading compensation in a wideband accelerating cavity using a circuit simulator including a LLRF feedback control

Tamura, Fumihiko; Yamamoto, Masanobu; Sugiyama, Yasuyuki*; Yoshii, Masahito*; Omori, Chihiro*; Shimada, Taihei; Nomura, Masahiro; Hasegawa, Katsushi*; Hara, Keigo*; Furusawa, Masashi*

Journal of Physics; Conference Series, 1350(1), p.012189_1 - 012189_7, 2019/12

Magnetic alloy cavities are employed in the J-PARC RCS to generate high accelerating voltages. The cavity, which is driven by a vacuum tube amplifier, has a wideband frequency response and the beam loading in the cavity is multiharmonic. Therefore, the tube must generate a multiharmonic output current. An LTspice circuit model is developed to analyze the vacuum tube operation and the compensation of the multiharmonic beam loading. The model includes the cavity, tube amplifier, beam current, and LLRF feedback control. The feedback control consists of the I/Q demodulator including low pass filters, PI control, and I/Q modulator. In this presentation, we present the implementation of the LLRF functions in the LTspice simulations. The preliminary simulation results are also presented. The simulations fairly agree with the beam test results.

18724 (Records 1-20 displayed on this page)