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Journal Articles

Development of MA separation process with TEHDGA/SiO$$_{2}$$-P for an advanced reprocessing

Horiuchi, Yusuke; Watanabe, So; Sano, Yuichi; Takeuchi, Masayuki; Kida, Fukuka*; Arai, Tsuyoshi*

Journal of Radioanalytical and Nuclear Chemistry, 330(1), p.237 - 244, 2021/10

Applicability of tetra2-ehylhexyl diglycolamide (TEHDGA) impregnated adsorbent for minor actinide (MA) recovery from high level liquid waste (HLLW) in extraction chromatography technology was investigated through batch-wise adsorption and column separation experiments. Distribution ratio of representative fission product elements were obtained by the batch-wise experiments, and TEHDGA adsorbent was shown to be preferable to TODGA adsorbent for decontamination of several species. All Ln(III) supplied into the TEHDGA adsorbent packed column was properly eluted from the column, and the applicability of the adsorbent was successfully showed by this study.

Journal Articles

$$^{129}$$I/$$^{127}$$I and $$Delta$$$$^{14}$$C records in a modern coral from Rowley Shoals off northwestern Australia reflect the 20th-century human nuclear activities and ocean/atmosphere circulations

Mitsuguchi, Takehiro; Okabe, Nobuaki*; Yokoyama, Yusuke*; Yoneda, Minoru*; Shibata, Yasuyuki*; Fujita, Natsuko; Watanabe, Takahiro; Kokubu, Yoko

Journal of Environmental Radioactivity, 235-236, p.106593_1 - 106593_10, 2021/09

 Times Cited Count:0 Percentile:0(Environmental Sciences)

For a contribution to developing the usage of iodine-129 ($$^{129}$$I) as a tracer of deep-seated fluid, $$^{129}$$I/$$^{127}$$I and $$Delta$$$$^{14}$$C were measured for annual bands (AD 1931-1991) of a modern coral collected from Northwestern Australia; the measurements were performed using the JAEA-AMS-TONO-5MV for $$^{129}$$I/$$^{127}$$I and an AMS facility of the University of Tokyo for $$Delta$$$$^{14}$$C. Results indicate that both $$^{129}$$I/$$^{127}$$I and $$Delta$$$$^{14}$$C distinctly increase from 1950s. The $$Delta$$$$^{14}$$C increase can be ascribed to atmospheric nuclear tests, while the $$^{129}$$I/$$^{127}$$I increase is due to nuclear-fuel reprocessing as well as atmospheric nuclear tests. These results are in good agreement with previous studies, indicating that the $$^{129}$$I/$$^{127}$$I measurement by JAEA-AMS-TONO-5MV has been further developed.

Journal Articles

Kinetic study on eutectic reaction between boron carbide and stainless steel by differential thermal analysis

Kikuchi, Shin; Nakamura, Kinya*; Yamano, Hidemasa

Mechanical Engineering Journal (Internet), 8(4), p.20-00542_1 - 20-00542_13, 2021/08

In a postulated severe accidental condition of sodium-cooled fast reactor (SFR), eutectic melting between boron carbide (B$$_{4}$$C) and stainless steel (SS) may take place. Thus, kinetic behavior of B$$_{4}$$C-SS eutectic melting is one of the important phenomena to be considered when evaluating the core disruptive accidents in SFR. In this study, for the first step to obtain the fundamental information on kinetic feature of B$$_{4}$$C-SS eutectic melting, the thermal analysis using the pellet type samples of B$$_{4}$$C and Type 316L SS as different experimental technique was performed. The differential thermal analysis endothermic peaks for the B$$_{4}$$C-SS eutectic melting appeared from 1483K to 1534K and systematically shifted to higher temperatures when increasing heating rate. Based on this kinetic feature, apparent activation energy and pre-exponential factor for the B$$_{4}$$C-SS eutectic melting were determined by Kissinger method. It was found that the kinetic parameters obtained by thermal analysis were comparable to the literature values.

Journal Articles

The Impact of cement on argillaceous rocks in radioactive waste disposal systems; A Review focusing on key processes and remaining issues

Wilson, J.*; Bateman, K.; Tachi, Yukio

Applied Geochemistry, 130, p.104979_1 - 104979_19, 2021/07

 Times Cited Count:0 Percentile:0.65(Geochemistry & Geophysics)

The concept of deep geological disposal will include the multiple use of cement-based materials. In the case of argillaceous host rocks, the presence of hyperalkaline cement porefluid results in the destabilization of primary minerals in the argillite, resulting in the development of a zone of alteration at cement-rock interfaces. The process understanding gained from experimental, analogue, and modelling studies has been reviewed, and remaining areas of uncertainty identified. Although there is a reasonably good understanding of the mineral assemblages that are likely to occur due to cement-rock interactions, there are still some areas where a degree of uncertainty remains, in particular: the evolution of cement-argillite interfaces at T $$>$$ 25$$^{circ}$$C; the rates at which secondary minerals form; the extent of pore clogging due to secondary mineral precipitation; the implications of alteration for radionuclide transport.

Journal Articles

Evaluation report of Task 9B based on comparisons and analyses of modelling results for the $"A$sp$"o$ HRL LTDE-SD experiments

Soler, J. M.*; Meng, S.*; Moreno, L.*; Neretnieks, I.*; Liu, L.*; Kek$"a$l$"a$inen, P.*; Hokr, M.*; $v{R}$$'i$ha, J.*; Vete$v{s}$n$'i$k, A.*; Reimitz, D.*; et al.

SKB TR-20-17, 71 Pages, 2021/07

Task 9B of the SKB Task Force on Modelling of Groundwater Flow and Transport of Solutes in fractured rock focused on the modelling of experimental results from the LTDE-SD in situ tracer test performed at the $"A$sp$"o$ Hard Rock Laboratory in Sweden. Ten different modelling teams provided results for this exercise, using different concepts and codes. Three main types of modelling approaches were used: (1) analytical solutions to the transport-retention equations, (2) continuum-porous-medium numerical models, and (3) microstructure-based models accounting for small-scale heterogeneity (i.e. mineral grains and microfracture distributions). The modelling by the different teams allowed the comparison of many different model concepts, especially in terms of potential zonations of rock properties (porosity, diffusion, sorption), such as the presence of a disturbed zone at the rock and fracture surface, the potential effects of micro- and cm-scale fractures.

Journal Articles

Depositional age constraint on channel sediments in an incised meandering river using feldspar OSL dating: A case study in the Totsukawa River, Kii Mountains

Ogata, Manabu; Komatsu, Tetsuya; Nakanishi, Toshimichi

Dai Yonki Kenkyu, 60(2), p.27 - 41, 2021/06

no abstracts in English

Journal Articles

Effect of interlayer cations on montmorillonite swelling; Comparison between molecular dynamic simulations and experiments

Yotsuji, Kenji*; Tachi, Yukio; Sakuma, Hiroshi*; Kawamura, Katsuyuki*

Applied Clay Science, 204, p.106034_1 - 106034_13, 2021/04

 Times Cited Count:3 Percentile:94.49(Chemistry, Physical)

JAEA Reports

(U-Th)/He dating analysis at Tono Geoscience Center, Japan Atomic Energy Agency; Determination of He contents (Contract research)

Kanno, Mizuho; Sueoka, Shigeru; Fukuda, Shoma

JAEA-Testing 2020-010, 38 Pages, 2021/03

JAEA-Testing-2020-010.pdf:3.07MB

This report provides procedures of He measurement for (U-Th)/He dating at Tono Geoscience Center, Japan Atomic Energy Agency. (U-Th)/He method is a radiometric dating based on alpha decay of U and Th series isotopes, being utilized as a thermochronometer. (U-Th)/He thermochronometries on zircon and apatite are especially useful to estimate thermal history at low temperatures. The procedures are presented with the details, tips, and cautions because parts of the procedures can be carried out by beginners, including students and contractors. This report also includes some document formats helpful for conducting the procedures.

Journal Articles

Development of evaluation method for diffusion and filtration behavior of colloid in compacted bentonites using dendrimers

Endo, Takashi*; Tachi, Yukio; Ishidera, Takamitsu; Terashima, Motoki

Nihon Genshiryoku Gakkai Wabun Rombunshi, 20(1), p.9 - 22, 2021/03

Evaluation method of colloid diffusion and filtration in compacted bentonites was developed using dendrimers. Diffusion and filtration behavior of PAMAM dendrimers with the size of 5.7$$sim$$7.2nm was investigated by the through-diffusion experiment in bentonite compacted to 0.8 Mg/m$$^{3}$$ and saturated with 0.005$$sim$$0.5mol/L NaCl. Effective diffusivities (De) and filtration ratios (Rf) of dendrimers were determined from the breakthrough curves and the depth profiles in compacted bentonite, respectively. The De values of negatively charged dendrimer increased when porewater salinity increased and dendrimer size decreased as influenced by anion exclusion effect in negatively charged clay surfaces. The Rf values increased when porewater salinity decreased and dendrimer size increased, demonstrating significant fractions of dendrimer were filtered by narrow pores in complex pore networks. These trends consistent with the previous studies emphasize the validity of the evaluation method using dendrimer.

Journal Articles

Ultra-low-temperature thermochronology using optically stimulated luminescence (OSL)

Ogata, Manabu; Sueoka, Shigeru

Radioisotopes, 70(3), p.159 - 172, 2021/03

no abstracts in English

Journal Articles

Surface complexation of Ca and competitive sorption of divalent cations on montmorillonite under alkaline conditions

Sugiura, Yuki; Ishidera, Takamitsu; Tachi, Yukio

Applied Clay Science, 200, p.105910_1 - 105910_10, 2021/01

 Times Cited Count:0 Percentile:0.04(Chemistry, Physical)

Journal Articles

Dating of a fault zone distributed in the South Kyushu shear zone based on fission-track thermochronology and U-Pb dating

Sueoka, Shigeru; Shimada, Koji; Terusawa, Shuji*; Iwano, Hideki*; Danhara, Toru*; Ogita, Yasuhiro; Hirata, Takafumi*

Chishitsugaku Zasshi, 127(1), p.25 - 39, 2021/01

no abstracts in English

Journal Articles

Solidification depth and crystallization age of the Shiaidani Granodiorite; Constraints to the average denudation rate of the Hida Range, central Japan

Kawakami, Tetsuo*; Sueoka, Shigeru; Yokoyama, Tatsunori; Kagami, Saya; King, G. E.*; Herman, F.*; Tsukamoto, Sumiko*; Tagami, Takahiro*

Island Arc, 30(1), p.e12414_1 - e12414_11, 2021/01

 Times Cited Count:0 Percentile:0(Geosciences, Multidisciplinary)

Journal Articles

XAFS analysis of ruthenium in simulated iron phosphate radioactive waste glass

Okamoto, Yoshihiro; Kobayashi, Hidekazu; Shiwaku, Hideaki; Sasage, Kenichi; Hatakeyama, Kiyoshi*; Nagai, Takayuki

Journal of Non-Crystalline Solids, 551, p.120393_1 - 120393_8, 2021/01

 Times Cited Count:0 Percentile:0.02(Materials Science, Ceramics)

The chemical state of ruthenium in simulated iron phosphate radioactive waste glass was investigated by conventional X-ray absorption fine structure (XAFS) and imaging XAFS analyses. The EXAFS analysis suggested that ruthenium was contained as glass phase when content of the waste components was less than 10wt.% in 30 mol%Fe$$_{2}$$O$$_{3}$$-P$$_{2}$$O$$_{5}$$ base glass. In other samples, crystalline RuO$$_{2}$$ was predominant. According to the imaging XAFS analysis, RuO$$_{2}$$ particles in all samples had length smaller than 50$$mu$$m. Aggregations of RuO$$_{2}$$, which are found in nuclear waste borosilicate glass, were not seen in any of the iron phosphate glass samples.

Journal Articles

Electrochemical behavior of carbon steel with bentonite/sand in saline environment

Kitayama, Ayami; Taniguchi, Naoki; Mitsui, Seiichiro

Materials and Corrosion, 72(1-2), p.211 - 217, 2021/01

 Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)

Journal Articles

Pore distribution of compacted Ca-montmorillonite using NMR relaxometry and cryoporometry; Comparison with Na-montmorillonite

Okubo, Takahiro*; Yamazaki, Akio*; Fukatsu, Yuta; Tachi, Yukio

Microporous and Mesoporous Materials, 313, p.110841_1 - 110841_11, 2021/01

 Times Cited Count:1 Percentile:72.55(Chemistry, Applied)

Pore distributions in water-saturated Ca-montmorillonite were investigated using $$^{1}$$H NMR measurements under various dry densities (0.8 - 1.6 g/cm$$^{3}$$) and porewater salinity conditions (deionized water, 0.1 and 1 M CaCl$$_{2}$$), at the temperature range of 233 - 303 K. The volume fractions of the interlayer pore including two and three hydrated layers and the non-interlayer pore in compacted Ca-montmorillonite were quantified by NMR relaxometry including $$T1$$ and $$T1/T2$$ distribution analysis, and were compared with NMR cryoporometry and X-ray diffractometry. These analysis provided consistent pictures on the pore distributions in compacted Ca-montmorillonite, in contrast to Na-montmorillonite. The main factor affecting the pore distribution in compacted Ca- and Na-montmorillonite is the density, whereas the effect of porewater salinity is relatively smaller. The effect of interlayer cations is also relatively smaller at higher density, although the differences in the pore structures are significant at low density.

JAEA Reports

A Catalog showing distribution and features of lineaments and related landforms in an active shear zone with unclear fault displacement topography; An Example of an active left-lateral shear zone in southern Kyushu Island, southwest Japan (Contract research)

Goto, Akira; Sasaki, Akimichi*; Komatsu, Tetsuya; Miwa, Atsushi*; Terusawa, Shuji*; Kagohara, Kyoko*; Shimada, Koji

JAEA-Research 2020-013, 88 Pages, 2020/11

JAEA-Research-2020-013.pdf:22.86MB
JAEA-Research-2020-013-appendix(CD-ROM).zip:0.18MB

Improvement of the investigation techniques to identify active faults is important for the implementation of geological disposal projects from the viewpoint of avoiding locations where permeability increases due to fault displacement. Generally, the existence of active faults is confirmed by aerial photography interpretation of fault displacement topography, which is a topographical trace of fault movement, and on-site geological surveys. However, the investigation method for cases where the topographical traces are unclear is not sufficiently developed. Therefore, to improve existing topographical methods, this study deciphered lineaments up to the rank of poorly defined features, which are almost neglected in general active fault research. The investigation area is one of the geodetic strain concentration zone, called the southern Kyushu shear zone, where the seismogenic faults of the 1997 Kagoshima northwest earthquakes are concealed. We conducted aerial photography interpretation of 62 sheets of 1/25,000 topographic maps, and obtained 1,327 lineaments. Distribution density, direction and length of lineaments were also investigated with topographic and geologic information. As a result, it was clarified that the east-west lineaments in the south Kyushu shear zone predominate in the western part, and the lineaments are densely distributed in the aftershock distribution area of the Kagoshima northwest earthquake. Along with these results, we have compiled a catalog of typical 13 lineaments based on combinations of clarity, direction, length and geomorphic characters of lineaments.

Journal Articles

Simultaneous determination of zircon U-Pb age and titanium concentration using LA-ICP-MS for crystallization age and temperature

Yuguchi, Takashi*; Ishibashi, Kozue*; Sakata, Shuhei*; Yokoyama, Tatsunori; Ito, Daichi*; Ogita, Yasuhiro; Yagi, Koshi*; Ono, Takeshi*

Lithos, 372-373, p.105682_1 - 105682_9, 2020/11

 Times Cited Count:0 Percentile:0.02(Geochemistry & Geophysics)

Simultaneous determination of zircon U-Pb age and titanium concentration for a single analysis spot gives both the crystallization age and temperature. The crystallization age and temperature pairs in granitic zircons map the time-temperature ($$t-T$$) path of granitic magma before its solidification. In laser ablation inductively coupled plasma mass spectrometry (LA-ICP-MS) analysis, it is challenging to quantitatively analyse a low level of titanium concentration. This study employed two approaches using a Quadrupole mass spectrometer equipped with a collision/reaction cell (CRC). The methods were applied to zircon samples of the Kurobegawa granite (KRG), the Okueyama granite (OKG), the Toki granite (TKG), and the Tono plutonic complex (TPC) and provided U-Pb ages and titanium concentrations consistent with previous studies. The crystallization ages and temperatures collected from individual analysis spots of zircon samples in the KRG, OKG, TKG, and TPC are plotted in the $$t-T$$ diagrams and enable us to characterize the rapid cooling paths at thermal conditions of zircon crystallization at the sampling sites.

Journal Articles

Current status and prospects of FT and (U-Th)/He dating laboratory at Japan Atomic Energy Agency

Sueoka, Shigeru; Shimada, Koji; Kanno, Mizuho; Yokoyama, Tatsunori

Fisshion, Torakku Nyusureta, (33), p.15 - 18, 2020/10

no abstracts in English

Journal Articles

Estimation of the uplift/denudation history in Kitakami Mountains by thermochronology

Kajita, Yuya*; Fukuda, Shoma; Sueoka, Shigeru; Hasebe, Noriko*; Tamura, Akihiro*; Morishita, Tomoaki*; Kohn, B. P.*; Tagami, Takahiro*

Fisshion, Torakku Nyusureta, (33), p.28 - 30, 2020/10

no abstracts in English

707 (Records 1-20 displayed on this page)