JAEA
  • help
  • PC | SP
  • JP | EN
          
Refine your search：     
Report No.
 - 
Clear All
Search Results: Records 1-5 displayed on this page of 5
  • 1

Presentation/Publication Type

Initialising ...

Refine

Journal/Book Title

Initialising ...

Meeting title

Initialising ...

First Author

Initialising ...

Keyword

Initialising ...

Language

Initialising ...

Publication Year

Initialising ...

Held year of conference

Initialising ...

Save select records

Journal Articles

$$^{33}$$S nuclear magnetic resonance spectra of uranium disulfide $$beta$$-US$$_2$$

Sakai, Hironori; Tokunaga, Yo; Haga, Yoshinori; Kambe, Shinsaku; Ramakrishna, S. K.*; Reyes, A. P.*; Rosa, P. F. S.*; Ronning, F.*; Thompson, J. D.*; Fisk, Z.*; et al.

JPS Conference Proceedings (Internet), 30, p.011169_1 - 011169_6, 2020/03

https://doi.org/10.7566/JPSCP.30.011169

Uranium disulfide $$beta$$-US$$_2$$ showing a semimetal-to-semiconductor crossover has been investigated by the nuclear magnetic resonance (NMR) technique for $$^{33}$$S nuclei with the nuclear spin of $$I=3/2$$. Since the natural concentration 0.76% of NMR active $$^{33}$$S nuclei is too dilute, the isotopic enrichment to $$sim$$50% has been carried out for the single crystal growth. The $$^{33}$$S NMR spectra have been successfully obtained using a single crystal of $$beta$$-US$$_2$$ with external fields along the crystallographic $$c$$ axis. The S sites assignments have been made based on these NMR spectra.

Journal Articles

Polar rotor scattering as atomic-level origin of low mobility and thermal conductivity of perovskite CH$$_{3}$$NH$$_{3}$$PbI$$_{3}$$

Li, B.; Kawakita, Yukinobu; Liu, Y.*; Wang, M.*; Matsuura, Masato*; Shibata, Kaoru; Kawamura, Seiko; Yamada, Takeshi*; Lin, S.*; Nakajima, Kenji; et al.

Nature Communications (Internet), 8, p.16086_1 - 16086_9, 2017/06

https://doi.org/10.1038/ncomms16086
 Times Cited Count：84 Percentile：90.11(Multidisciplinary Sciences)

Journal Articles

Multi-intruder structures in $$^{34}$$P

Bender, P. C.*; Tabor, S. L.*; Tripathi, V.*; Hoffman, C. R.*; Hamilton, L.*; Volya, A.*; Clark, R. M.*; Fallon, P.*; Macchiavelli, A. O.*; Paschalis, S.*; et al.

Physical Review C, 85(4), p.044305_1 - 044305_10, 2012/04

https://doi.org/10.1103/PhysRevC.85.044305
 Times Cited Count：12 Percentile：54.89(Physics, Nuclear)

The available experimental information on $$^{34}$$P has been greatly increased through the analysis of $$gamma$$ decays in coincidence with protons from the interaction of an $$^{18}$$O beam at 24 MeV with an $$^{18}$$O target. Light charged particles from the reaction were detected with Microball, and multiple $$gamma$$ ray coincidences with Gammasphere. Many newly observed $$gamma$$ transitions have been identified and placed in the level scheme. Additionally, for most states, spins have been assigned based on measured $$gamma$$ ray angular distributions while parities were inferred from lifetimes determined through Doppler-broadened line-shape analysis. Most of the states observed have been interpreted in terms of shell-model calculations using the WBP-a and SDPF-NR interactions having one particle in the 0$$f$$$$_{7/2}$$ or 1$$p$$$$_{3/2}$$ orbital. The two calculations agree almost equally well with the data resulting in root-mean-square differences of about 200 keV. However, two of a few high-lying states may be associated with stretched $$pi$$$$f$$$$_{7/2}$$ $$otimes$$ $$nu$$$$f$$$$_{7/2}$$ states, but the calculations over-predict their energies by 2-3 MeV. Furthermore, a newly observed long-lived 7919-keV state is established for which no explanation is available at present.

Oral presentation

$$^{33}$$S NMR study in $$beta$$-US$$_2$$

Sakai, Hironori; Tokunaga, Yo; Kambe, Shinsaku; Ramakrishna, S. K.*; Reyes, A. P.*; Rosa, P. F. S.*; Ronning, F.*; Thompson, J. D.*; Bauer, E. D.*

no journal, , 

Uranium disulfide $$beta$$-US$$_2$$ is a paramagnetic semiconductor with a narrow band gap of 90 K at low temperatures, whereas above 80 K it is a semimetal with an extremely low density of carriers. Another characteristic feature in $$beta$$-US$$_2$$ is the strong response of the electrical resistivity to magnetic field. The magnetoresistance is similar to that of colossal magnetoresistance materials but very anisotropic. In order to clarify the microscopic spin dynamics in $$beta$$-US$$_2$$, nuclear magnetic resonance experiments have been performed. Since the natural concentration of $$^{33}$$S nuclei ($$I=frac{3}{2}$$) is only 0.76%, isotopic enrichment to 50% has been carried out. In the presentation, we would like to discuss about the microscopic magnetism in $$beta$$-US$$_2$$ to show the NMR results under high fields.

Oral presentation

$$^{33}$$S-NMR study in $$beta$$-US$$_2$$

Sakai, Hironori; Hattori, Taisuke; Higa, Nonoka; Tokunaga, Yo; Tateiwa, Naoyuki; Yamamoto, Etsuji; Haga, Yoshinori; Kambe, Shinsaku; Reyes, A. P.*; Bauer, E. D.*; et al.

no journal, , 

$$beta$$-US$$_2$$ is a paramagnetic narrow-gap semiconductor with the energy band gap of 90 K. A characteristic feature of $$beta$$-US$$_2$$ is the strong response of the electrical resistivity to magnetic field. On the other hand, ferromagnetism is easily induced by pressure of about 1 GPa. Consequently, it is considered to be close to a ferromagnetic instability. To elucidate microscopically this very sensitive electronic states to external fields, $$^{33}$$S-NMR study has been performed. We will show our recent $$^{33}$$S-NMR results and discuss the electronic states.

5 (Records 1-5 displayed on this page)
  • 1