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Journal Articles

Chemical composition of aerosols generated by heating prototypic fuel debris samples

Journeau, C.*; Delacroix, J.*; Gu$'e$var, C.*; Testud, V.*; Brackx, E.*; Porcheron, E.*; Bouland, A.*; Berlemont, R.*; Ikeda, Atsushi

Science Talks (Internet), 6, p.100215_1 - 100215_9, 2023/05

Oral presentation

Elemental analysis and radioactivity evaluation of aerosols generated during heating of simulated fuel debris in the URASOL project

Tsubota, Yoichi; Laffolley, H.; Porcheron, E.*; Journeau, C.*; Delacroix, J.*; Gu$'e$var, C.*; Brackx, E.*; Lallot, Y.*; Bouland, A.*

no journal, , 

In order to safely remove fuel debris from the Fukushima Daiichi Nuclear Power Station (1F), it is necessary to quantitatively evaluate radioactive airborne particulate generated by the cutting of nuclear fuel debris. We fabricated Uranium-bearing simulated fuel debris (SFD) with In/Ex-Vessel compositions and evaluated the physical and chemical properties of aerosols generated by heating the SFDs. Based on these results, we estimated the isotopic composition and radioactivity of aerosols produced when 1F-Unit2 fuel debris is laser cut, which is a typical example of a heating method. Plutonium, mainly $$^{238}$$Pu,$$^{241}$$Am, and $$^{244}$$Cm were found to be the alpha nuclide, and $$^{241}$$Pu, $$^{137}$$Cs-Ba, and $$^{90}$$Sr-Y were found to be the beta nuclide of interest.

Oral presentation

Chemical and microstructural analyses techniques for Fuel Debris simulants and airborne particles

Gu$'e$var, C.*; Faure, J.*; Testud, V.*; Roger, J.*; Domenger, R.*; Valette, R.*; Brackx, E.*; Bouyer, V.*; Journeau, C.*; Berlemont, R.*; et al.

no journal, , 

The URASOL and the DA projects, respectively led by JAEA and CRIEPI in collaboration with ONET/CEA/IRSN, were proposed to obtain basic data on aerosols generation and characteristics from prototypic FD-simulants containing depleted uranium oxide cut by thermal or mechanical processing tools. The whole process developed by ONET/CEA/IRSN allows the manufacturing of specific compositions and supplying corium samples for cutting, the realization of cutting tests and the on-line dedicated aerosols measurements as well as sampling aerosols, to conduct initial FD simulants and aerosols post-trial analyses. This paper focuses on the initial FD simulant and aerosols chemical and microstructural analyses. Results on an ex-vessel composition of FD, named VF-U3, are given.

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