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JAEA Reports

Improvement of load control unit in material irradiation test system (Contract research)

Okada, Yuji; Magome, Hirokatsu; Matsui, Yoshinori

JAEA-Technology 2022-014, 113 Pages, 2022/09

JAEA-Technology-2022-014.pdf:15.79MB

Material irradiation test system had been newly installed in JMTR (Japan Materials Testing Reactor) with taking 5 years which was from 2008 through 2013. The aim of material irradiation test system is to conduct IASCC (Irradiation Assisted Stress Corrosion Cracking) evaluation study. This system is mainly consist of water control unit, which can simulate elevated temperature and pressure of the light water reactor environment in the reactor, and load control unit, which can perform the crack propagation examination under irradiation. This load control unit gives a load to CT (Compact Tension) specimen, and perform the crack propagation examination. The principle of loading to CT specimen is using pressure difference between pressure generated by high temperature and high pressure water by water control unit in capsule and pressure generated by load gas pressure supplied by helium gas cylinder in bellows installed in load control unit. In 2013, the commissioning of material irradiation test system was carried out for adjustment. During this commissioning, the correlation between the differential pressure in load control unit and the load was confirmed by using the test container connected to load control unit with load cell. From the results of commissioning, the problem, which the load change speeds at loading and unloading were different due to different pressure change speeds by the piping resistance performance in the periodic loading test in which load from minimum to maximum repeatedly applied, was confirmed. This report summarizes the problem of load change speed due to the piping resistance performance, which was confirmed in 2013, the improvement and performance test of load control unit for solving the problem described above, which were carried out from 2014 to 2015, and operating procedure.

JAEA Reports

Development of coupled mass-transport and chemical-reaction calculation code for alteration of engineered barrier

Sasagawa, Tsuyoshi; Mukai, Masayuki; Sawaguchi, Takuma

JAEA-Data/Code 2021-012, 122 Pages, 2022/01

JAEA-Data-Code-2021-012.pdf:3.87MB

Reducing public dose is required when radioactive wastes such as high-level and from reactor core internals etc. are disposed of by means of multi barrier system consist of engineered and natural barriers. In these barriers, engineered barrier is expected to bring out confinement function of waste's radionuclides in the barrier. Materials used as the engineered barriers are altered and performances of the barrier materials are degraded in course of time. To estimate properly the degraded performances, analytical evaluation of long-term change of the engineered barrier state is important. Change state of the engineered barrier is given by mass-transport and geochemical-reaction inside the barrier materials and these phenomena are interrelated, it is necessary to calculate the state by means of coupled analysis procedure. We have developed a coupled mass-transport and geochemical-reaction calculation code (MC- BUFFER) to evaluate alteration of engineered barrier specially targeted for water permeability of bentonite buffer material as one of most important performances to engineered barrier. This report describes functions expected for the engineered barrier, influence parameters for the functions, implementation models in MC-BUFFER, structure and functions of MC-BUFFER, input file format and output examples, execution method of MC-BUFFER, and sample run with MC-BUFFER.

Journal Articles

Heat conduction analyses on rewetting front propagation during transients beyond anticipated operational occurrences for BWRs

Yonomoto, Taisuke; Shibamoto, Yasuteru; Satou, Akira; Okagaki, Yuria

Journal of Nuclear Science and Technology, 53(9), p.1342 - 1352, 2016/09

AA2015-0497.pdf:1.05MB

 Times Cited Count:3 Percentile:28.28(Nuclear Science & Technology)

Our previous study investigated the rewetting behavior of dryout fuel surface during transients beyond anticipated operational occurrences (AOOs) for BWRs, which indicated the rewetting velocity was significantly affected by the precursory cooling defined as cooling immediately before rewetting. The present study further investigated the previous experiments by conducting additional experimental and numerical heat conduction analyses to characterize the precursory cooling. For the characterization, the precursory cooling was firstly defined quantitatively based on evaluated heat transfer rates; the rewetting velocity was investigated as a function of the cladding temperature immediately before the onset of the precursory cooling. The results indicated that the propagation velocity appeared to be limited by the maximum heat transfer rate near the rewetting front. This limitation was consistent with results of the heat conduction analysis.

Journal Articles

Distribution coefficients of iodine and tin on granodiorite and tuffaceous sandstone specimens

Hemmi, Ko; Yamaguchi, Tetsuji; Iida, Yoshihisa

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 22(1), p.3 - 10, 2015/06

Iodine and tin are important elements in performance assessment of geological disposal of radioactive wastes. Sorption experiments of iodine were carried out under varying nitrate concentration with a range of 0 to 5 mol dm$$^{-3}$$ at neutral pH range in order to determine the distribution coefficient of iodine was zero or non-zero value. The experimental results with estimated statistical errors showed non-zero values for tuffaceous sandstone except for NaNO$$_{3}$$ concentration 0.5 mol dm$$^{-3}$$. Non-zero values were also obtained under NaNO$$_{3}$$ concentrations higher than 0.5 mol dm$$^{-3}$$ for granodiorite. Sorption experiments of tin were carried out at high pH range in order to check whether the distribution coefficient of tin decreases significantly with pH as a result of formation of anionic hydrolysis species of tin. The distribution coefficients of tin on granodiorite decreased from 9.79$$times$$10$$^{-2}$$ m$$^{3}$$ kg$$^{-1}$$ at pH10.4 to 2.46$$times$$10$$^{-3}$$ m$$^{3}$$ kg$$^{-1}$$ at pH12.4. The distribution coefficient of tin on tuffaceous sandstone was about one order of magnitude higher (about 2$$times$$10$$^{-2}$$ m$$^{3}$$ kg$$^{-1}$$) than that of granodiorite at pH around 12.4.

Journal Articles

Improvement and testing of radiation source models in DecDose for public dose assessments during decommissioning of nuclear facilities

Shimada, Taro; Sukegawa, Takenori

Journal of Nuclear Science and Technology, 52(3), p.396 - 415, 2015/03

 Times Cited Count:1 Percentile:9.74(Nuclear Science & Technology)

Radiation source models in DecDose code for assessing public and worker exposure doses during the decommissioning of nuclear facilities were improved in this study. A segmentation model evaluating the length, volume, and surface area of kerfs in the object to be dismantled was improved to deal with seven shapes of objects simulating most of the components and the structures in nuclear facilities. Models for the evaluation of the external dose by direct and skyshine radiation were also improved to deal with the distribution of waste containers temporarily placed in the building and the quantity of radionuclides stored in the individual container. Good agreement was observed between actual and calculated kerf volumes in cutting some components such as the reactor pressure vessel of the Japan Power Demonstration Reactor. It is an indication of the validity of the model improved in this study. On the other hand, some discrepancies were observed between actual and calculated quantities of radionuclides discharged into the ocean, indicating the necessity of further validation of the model.

Journal Articles

Construction of evaluation model for rainwater cultivation amount

Munakata, Masahiro; Amano, Kenji; Tanaka, Tadao

JNES-RE-2013-9032, p.63 - 78, 2014/02

no abstracts in English

Journal Articles

Effect of partial welding on the residual stress and structural integrity of piping welds

Katsuyama, Jinya; Masaki, Koichi; Onizawa, Kunio

Journal of Pressure Vessel Technology, 135(6), p.061403_1 - 061403_8, 2013/12

 Times Cited Count:0 Percentile:0.01(Engineering, Mechanical)

When weld defects are observed during an inspection after welding, repair welding is performed after removing the defects. However, partial repair welding can potentially complicate the weld residual stress distribution. In this study, we performed thermal-elastic-plastic analyses to evaluate the weld residual stress produced by repair welding after pipe butt-welding. In addition, based on the analysis results for varying repair-welding conditions, we also performed structural integrity assessments related to stress corrosion cracking using the probabilistic fracture mechanics analysis code PASCAL-SP. It was clearly observed that the tensile stress in the repair-welded region increased and that compressive stresses occurred outside the repair-welded region. A deeper mechanical cutting depth caused larger increases in the tensile residual stress of the repair-welded region. It was also clarified that partial repair welding may favorably affect the break probability of piping welds.

Journal Articles

Assessment of residual stress due to overlay-welded cladding and structural integrity of a reactor pressure vessel

Katsuyama, Jinya; Nishikawa, Hiroyuki*; Udagawa, Makoto; Nakamura, Mitsuyuki*; Onizawa, Kunio

Journal of Pressure Vessel Technology, 135(5), p.051402_1 - 051402_9, 2013/10

 Times Cited Count:26 Percentile:72.37(Engineering, Mechanical)

The residual stresses generated within the weld-overlay cladding and base material of reactor pressure vessel (RPV) steel was evaluated for as-welded and post-welded heat-treated conditions using thermo-elastic plastic creep analyses considering phase transformation. By comparing the analytical results with the experimentally determined values, we found a good agreement for the residual stress distribution within the cladding and the base material. It was shown that considering phase transformation during welding was important for improving the accuracy of residual stress analysis. Using the calculated residual stress distribution, we performed fracture mechanics analyses for an RPV during pressurized thermal shock events. We evaluated the effect of the weld residual stress on the structural integrity of an RPV. The results indicated that consideration of residual stress produced by weld-overlay cladding and PWHT is important for assessing the structural integrity of RPV.

Journal Articles

Sensitivity analysis for the scenarios on deterioration or loss of safety functions expected in disposal system due to human error on application of engineering technology

Takeda, Seiji; Inoue, Yoshihisa; Kimura, Hideo

Materials Research Society Symposium Proceedings, Vol.1518, p.237 - 242, 2013/10

The sensitive analysis of radionuclide migration for the scenarios on deterioration or loss of safety functions expected in HLW disposal system due to the human error (initial defective scenarios) is performed in this study. Release rates for Cs-135 and Se-79 are estimated from Monte Carlo-based analysis. Maximum release rates of radionuclides for initial defective scenarios, buffer (colloidal transport case) and sealing plugs (pathway of short-circuit), are about one or two order magnitude higher than that normal scenario. From a viewpoint of future safety review, these results especially indicate the need to understand the feasibility on two types of initial defective scenario for the buffer and sealing plugs, leading to the loss of restraint of colloidal migration in the buffer and the loss of restraint with the plugs from migration through dominant pathway in tunnels and their vicinity.

Journal Articles

Fracture mechanics evaluation using PASCAL3 for current structural integrity assessment method for reactor pressure vessel

Nishikawa, Hiroyuki*; Masaki, Koichi*; Katsuyama, Jinya; Onizawa, Kunio

Nihon Genshiryoku Gakkai Wabun Rombunshi, 12(3), p.211 - 221, 2013/09

Probabilistic fracture mechanics analysis code PASCAL3 has been developed at JAEA to support the validation of the codes and standards which provide the structural integrity assessment method of reactor pressure vessels (RPVs) during pressurized thermal shock. Previous version of PASCAL2 has many functions including the evaluation method for an embedded crack, PTS transient database, non-destructive inspection models. This code has been improved mainly focusing on cladding on the inner surface of RPV. Using the PASCAL3 code, effects of the initiation and growth model for a surface flaw have been analyzed to determine the standard condition of PASCAL3. Deterministic and probabilistic evaluation using PASCAL3 for current structural integrity assessment method for RPV has also been conducted. The results show that the consideration of warm pre-stress effect decreases the conditional probability

Journal Articles

Study on the structural integrity of RPV using PFM analysis concerning inhomogeneity of the heat-affected zone

Masaki, Koichi; Katsuyama, Jinya; Onizawa, Kunio

E-Journal of Advanced Maintenance (Internet), 5(2), p.85 - 92, 2013/08

In order to obtain the technical basis to judge the needs of surveillance test specimens from HAZ materials, the features of inhomogeneity of HAZ in RPV steels were investigated. Concerning on the fracture toughness in HAZ, HAZ materials close to weld metal indicated higher toughness than that of base metal due to high-toughness phase, while HAZ materials close to base metal were equivalent or slightly lower toughness than that of base metal due to the same phase as base metal. A structural integrity assessment method concerning such inhomogeneous distribution of fracture toughness for HAZ materials was developed and incorporated into PFM analysis code PASCAL3. Case studies on postulated flaws distribution and chemical composition were performed by using PASCAL3. It was shown that in highly irradiated conditions, CPI and CPF in HAZ close to weld metal are lower than base metal, while those in HAZ close to base metal were almost equivalent to base metal.

Journal Articles

Corrosion rate of zircaloy-4 in deoxidized deionized water at 80-120$$^{circ}$$C

Maeda, Toshikatsu; Chiba, Noriaki; Tateishi, Tsuyoshi*; Yamaguchi, Tetsuji

Nihon Genshiryoku Gakkai Wabun Rombunshi, 12(2), p.158 - 164, 2013/06

no abstracts in English

Journal Articles

Diffusion of Cs, Np, Am and Co in compacted sand-bentonite mixtures; Evidence for surface diffusion of Cs cations

Sawaguchi, Takuma; Yamaguchi, Tetsuji; Iida, Yoshihisa; Tanaka, Tadao; Kitagawa, Isamu

Clay Minerals, 48(2), p.411 - 422, 2013/05

 Times Cited Count:2 Percentile:6.52(Chemistry, Physical)

Diffusive transport of Cs$$^{+}$$ in compacted sand-bentonite mixtures was studied by a through diffusion method. Experiments were performed under variable aqueous compositions. Effective diffusivity ($$D$$$$_{e}$$) values of 5.2E-10$$ sim$$ 5.9E-9 m$$^{2}$$ s$$^{-1}$$ were obtained. The variation was somewhat large in the $$D$$$$_{e}$$ values. Apparent diffusivity ($$D$$$$_{a}$$) values, on the other hand, were 2.0E-12 $$sim$$ 6.2E-12 m$$^{2}$$ s$$^{-1}$$, which shows small variation. The results indicate that, in applying Fick's 1st law of diffusion, diffusive flux is proportional to the apparent concentration gradient of Cs in the sand-bentonite mixture rather than the gradient of Cs concentration in pore water. Since the apparent concentration gradient in sand-bentonite mixtures is nearly equal to the gradient of adsorbed Cs, diffusion of Cs under adsorbed state would be the main mechanism of diffusion of Cs in sand-bentonite mixtures.

Journal Articles

Development of a reactive transport code MC-CEMENT ver.2 and its verification using 15-year ${it in-situ}$ concrete/clay interactions at the Tournemire URL

Yamaguchi, Tetsuji; Kataoka, Masaharu; Sawaguchi, Takuma; Mukai, Masayuki; Hoshino, Seiichi; Tanaka, Tadao; Marsal, F.*; Pellegrini, D.*

Clay Minerals, 48(2), p.185 - 197, 2013/05

 Times Cited Count:3 Percentile:9.54(Chemistry, Physical)

Highly alkaline environments induced by cement based materials are likely to deteriorate the physical and/or chemical properties of the bentonite buffer materials in radioactive waste repositories. Predicting long-term alteration of concrete/clay systems requires physico-chemical models and a number of input parameters. In order to provide reliability to the long-term prediction of bentonite buffer performance under disposal conditions, it is necessary to develop and verify reactive transport codes for concrete/clay systems. In this study, a PHREEQC-based, reactive transport analysis code (MC-CEMENT ver.2) was developed and was verified by comparing results of the calculations with ${it in situ}$ observations of the mineralogical evolution at the concrete/argillite interface. The calculation reproduced the observations such as the mineralogical changes limited within one cm in thickness, formation of CaCO$$_{3}$$ and CSH, dissolution of quartz, decrease of porosity in argillite and increase in concrete. These agreements indicate possibility that the models based on lab-scale ($$sim$$ 1 y) experiments can be applied to longer time scale. The fact that the calculation did not reproduce the dissolution of clays and the formation of gypsum indicates that there is still room for improvement in our model.

Journal Articles

Changes in hydraulic conductivity of sand-bentonite mixtures accompanied by alkaline alteration

Yamaguchi, Tetsuji; Sawaguchi, Takuma; Tsukada, Manabu; Kadowaki, Mitsushi*; Tanaka, Tadao

Clay Minerals, 48(2), p.403 - 410, 2013/05

 Times Cited Count:8 Percentile:23.68(Chemistry, Physical)

Montmorillonite is the main constituent of bentonite clay buffer materials in radioactive waste repositories. Highly alkaline environments induced by cement based materials are likely to alter montmorillonite, and to deteriorate the physical and/or chemical properties of the buffer materials. The deterioration may cause variation in hydraulic conductivity of the buffer and induce major uncertainties in the radionuclide migration analysis. Empirical data on the variation of hydraulic conductivity are, however, scarce mainly because the alteration of compacted buffer materials, sand-bentonite mixture specimen, is extremely slow. In this study, laboratory experiments were performed to observe changes in hydraulic conductivity of sand-bentonite mixtures accompanied with their alkaline alteration using NaOH based solutions at 80-90 $$^{circ}$$C. Three types of experiments proved that the alkaline alteration of bentonite buffer can increase the hydraulic conductivity. The data obtained in this study are useful for verification of the code that will be used for assessing the alteration.

Journal Articles

Corrosion modeling for carbon steel under oxygen depleted underground environment

Shibata, Toshio*; Watanabe, Masatoshi; Taniguchi, Naoki; Shimizu, Akihiko*

Zairyo To Kankyo, 62(2), p.70 - 77, 2013/02

In the oxygen depleted underground environment, carbon steel reacts with H$$_{2}$$O, producing H$$_{2}$$ gas and forming corrosion film on the steel surface. Corrosion rate is controlled by diffusion of reaction species through corrosion film. Diffusion constants of some species working in the corrosion process were obtained from literatures. However, no data were found on the diffusion constant of H$$_{2}$$O in iron oxides based on an appropriate assumption. Mass transfer model for the corrosion rate was used to simulate the corrosion rate of carbon steel. Liquid phase diffusion model of Fe$$^{2+}$$ or H$$_{2}$$O through pores in the corrosion film and solid phase diffusion model of H$$_{2}$$O through corrosion film itself were examined by Excel simulation. Change in corrosion current density and corrosion loss with time and pH and temperature dependence of corrosion current density were examined. By comparing the results, it is suggested that the solid phase diffusion of H$$_{2}$$O in the corrosion film controls the corrosion rate of carbon steel in oxygen depleted environment.

Journal Articles

Product analysis for polyethylene degradation by radiation and thermal ageing

Sugimoto, Masaki; Shimada, Akihiko; Kudo, Hisaaki*; Tamura, Kiyotoshi; Seguchi, Tadao*

Radiation Physics and Chemistry, 82, p.69 - 73, 2013/01

 Times Cited Count:61 Percentile:97.76(Chemistry, Physical)

The oxidation products formed by thermal and radiation ageing of crosslinked polyethylene for cable insulation were analyzed by FTIR-ATR spectrometry. The most of products were composed of carboxylic acid, carboxylic ester, and carboxylic anhydride. The carboxylic acid was the primal product, and the others were the secondary products by the thermal reaction of carboxylic acids. The carboxylic acid as the primal oxidation product supports the proposed new oxidation mechanisms that the main chain scission should occur directly by oxidation of polyethylene radicals.

JAEA Reports

Study of cable ageing mechanism for nuclear power plant (Contract research)

Seguchi, Tadao*; Tamura, Kiyotoshi*; Watashi, Katsumi; Suzuki, Masahide; Shimada, Akihiko; Sugimoto, Masaki; Idesaki, Akira; Yoshikawa, Masahito; Oshima, Takeshi; Kudo, Hisaaki*

JAEA-Research 2012-029, 158 Pages, 2012/12

JAEA-Research-2012-029.pdf:9.4MB

The degradation mechanisms of ethylene-propylene rubber (EPR), crosslinked polyethylene (XLPE), polyvinylchloride (PVC), and silicone rubber (SiR) as the cable insulation materials were investigated for the cable ageing research of the nuclear power plant. The materials as same insulations for the practical cable (practical formulation) and as the model formulation containing specific additive were selected. They were exposed to the accelerated radiation and thermal environments. The mechanical properties, the crosslinking and chain scission, and the distribution of antioxidant and of oxidative products were measured and analyzed.

Journal Articles

Investigation on highly alkaline plume spreading over host rock of geological disposal of TRU waste by reactive transport analysis

Takeda, Seiji; Nishimura, Yuki; Munakata, Masahiro; Sawaguchi, Takuma; Kimura, Hideo

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 19(2), p.23 - 38, 2012/12

In safety assessments of the geological disposal of TRU waste, it is important to understand the possibility and extents of influence of hyperalkaline groundwater derived from the degradation of cementitious materials that are used as forms for the containment of waste and as constructional materials in the disposal facilities of TRU waste. In this research, reactive transport analyses of hyperalkaline plume induced by cementitious materials were performed to clarify the extent of the hyperalkaline groundwater spreading and the type of alterations occurring with or without considering the precipitation of zeolite. The effect of the groundwater velocities on the spread of hyperalkaline groundwater was also examined. The analysis results indicate that whether zeolites precipitate or not significantly affect extent of hyperalkaline groundwater and the amount of precipitation of secondary minerals. In the case that groundwater velocity was 10 times higher, hyperalkaline groundwater spread broader than the original groundwater velocity case. It might be due to our kinetic dissolution model of host rock minerals, which limits chemical reactions neutralizing hyperalkaline groundwater.

Journal Articles

Improvement of the center boring device for the irradiated fuel pellets

Toyokawa, Takuya; Usami, Koji; Shiina, Hidenori; Onozawa, Atsushi

Proceedings of 49th Conference on Hot Laboratories and Remote Handling (HOTLAB 2012) (Internet), 6 Pages, 2012/09

379 (Records 1-20 displayed on this page)