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Journal Articles

Negative correlation between electrical response and domain size in a Ti-composition-gradient Pb[(Mg$$_{1/3}$$Nb$$_{2/3}$$)$$_{1-x}$$Ti$$_{x}$$]O$$_{3}$$ crystal near the morphotropic phase boundary

Shimizu, Daisuke*; Tsukada, Shinya*; Matsuura, Masato*; Sakamoto, Junya*; Kojima, Seiji*; Namikawa, Kazumichi*; Mizuki, Junichiro; Owada, Kenji

Physical Review B, 92(17), p.174121_1 - 174121_5, 2015/11

 Times Cited Count:13 Percentile:50.04(Materials Science, Multidisciplinary)

The phase diagram and the relationship between the crystal coherence length and electrical response of Pb[(Mg$$_{1/3}$$Nb$$_{2/3}$$)$$_{1-x}$$Ti$$_{x}$$]O$$_{3}$$ (PMN-xPT) near the morphotropic phase boundary (MPB) have been precisely investigated using a single crystal with a Ti composition gradient by synchrotron X-ray diffraction and inelastic light scattering at room temperature. The crystal has two boundaries at Ti compositions of 29.0 mol% and 34.7 mol% which correspond to the phase boundaries between the monoclinic B (MB) and C (MC) phases and between the MC and tetragonal (T) phases, respectively. It is shown that there is a strong negative correlation between the electrical response and the crystal coherence length at the sub-$$mu$$m scale. The results are explained by the size effects of domains near the MPB.

Journal Articles

Contribution of intermediate submicrometer structures to physical properties near $$T$$$$_{rm c}$$ in Pb(Zn$$_{1/3}$$Nb$$_{2/3}$$)O$$_{3}$$-9%PbTiO$$_{3}$$PbTiO$$_{3}$$

Owada, Kenji; Mizuki, Junichiro; Namikawa, Kazumichi*; Matsushita, Mitsuyoshi*; Shimomura, Susumu*; Nakao, Hironori*; Hirota, Kazuma*

Physical Review B, 83(22), p.224115_1 - 224115_7, 2011/06

 Times Cited Count:8 Percentile:36.17(Materials Science, Multidisciplinary)

Complementary use of coherent X-ray diffraction (CXD), X-ray diffuse scattering, conventional X-ray diffraction techniques and dielectric measurements has enabled us to investigate Pb(Zn$$_{1/3}$$Nb$$_{2/3}$$)O$$_{3}$$-9%PbTiO$$_{3}$$ with a multiple-length-scale approach from the macroscale (lattice constants, bulk averaged) and microscale to the nanoscale (polar nanoregions (PNRs)) and discuss the contribution of each scale to the dielectric permittivity.

Journal Articles

X-ray photon correlation spectroscopy study in valence fluctuation compound Eu$$_{3}$$S$$_{4}$$

Nakao, Hironori*; Owada, Kenji; Shimomura, Susumu*; Ochiai, Akira*; Namikawa, Kazumichi*; Mizuki, Junichiro; Mimura, Hidekazu*; Yamauchi, Kazuto*; Murakami, Yoichi*

AIP Conference Proceedings 1234, p.935 - 938, 2010/06

 Times Cited Count:2 Percentile:66.93(Physics, Applied)

Journal Articles

X-ray intensity fluctuation spectroscopy using nanofocused hard X-rays; Its application to study of relaxor ferroelectrics

Owada, Kenji; Namikawa, Kazumichi*; Shimomura, Susumu*; Nakao, Hironori*; Mimura, Hidekazu*; Yamauchi, Kazuto*; Matsushita, Mitsuyoshi*; Mizuki, Junichiro

Japanese Journal of Applied Physics, 49(2), p.020216_1 - 020216_3, 2010/02

 Times Cited Count:3 Percentile:14.99(Physics, Applied)

Oral presentation

Recent progress in X-ray laser research in JAEA

Kawachi, Tetsuya; Kishimoto, Maki; Kado, Masataka; Tanaka, Momoko; Hasegawa, Noboru; Ochi, Yoshihiro; Nishikino, Masaharu; Ishino, Masahiko; Imazono, Takashi; Kunieda, Yuichi; et al.

no journal, , 

Recent progress in X-ray laser research in Japan Atomic Energy Agency is reviewed. Using the nickel-like silver soft X-ray laser at the wavelength of 13.9 nm, the application experiments have been conducted in the research fields such as material science, high-density plasma diagnostics, XRL ablation, XRL imaging using single-shot holography and atomic physics. The repetition rate of the XRL beam has been improved from each 10-20 minutes to 0.1 Hz by using new driver laser system with Nd: glass zigzag slab amplifier, and we are now constructing new beam line for the pump-probe measurement of the surface phase-transition by the method of X-ray laser interferometer. In the research activity on the extension of the wavelength region of the X-ray lasers, firstly, the demonstration of novel coherent X-ray generation by "flying mirror" technique is reported. The second is theoretical investigation of the resonance photo-pumping scheme toward water-window region.

Oral presentation

Configuration dependence of domain contribution to the dielectric properties of relaxor

Owada, Kenji; Mizuki, Junichiro; Namikawa, Kazumichi*; Matsushita, Mitsuyoshi*; Shimomura, Susumu*; Nakao, Hironori*; Hirota, Kazuma*

no journal, , 

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