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JAEA Reports

Verification of alternative dew point hygrometer for CV-LRT in MONJU; Short- and long-term verification for capacitance-type dew point hygrometer (Translated document)

Ichikawa, Shoichi; Chiba, Yusuke; Ono, Fumiyasu; Hatori, Masakazu; Kobayashi, Takanori; Uekura, Ryoichi; Hashiri, Nobuo*; Inuzuka, Taisuke*; Kitano, Hiroshi*; Abe, Hisashi*

JAEA-Research 2017-001, 40 Pages, 2017/03

JAEA-Research-2017-001.pdf:5.19MB

In order to reduce the influence on a plant schedule of the MONJU by the maintenance of dew point hygrometers, The JAEA examined a capacitance type dew point hygrometer as an alternative dew point hygrometer for a lithium-chloride type dew point hygrometer which had been used at the CV-LRT in the MONJU. As a result of comparing a capacitance type dew point hygrometer with a lithium-chloride type dew point hygrometer at the CV-LRT (Atmosphere: nitrogen, Testing time: 24 hours), there weren't significant difference between a capacitance type dew point hygrometer and a lithium-chloride type dew point hygrometer. As a result of comparing a capacitance dew point hygrometer with a high-mirror-surface type dew point hygrometer for long term verification (Atmosphere: air, Testing time: 24 months), the JAEA confirmed that a capacitance type dew point hygrometer satisfied the instrument specification ($$pm$$2.04$$^{circ}$$C) required by the JEAC4203-2008.

JAEA Reports

Measurement of rock mass deformation around the closure test drift during groundwater recovery experiment at 500m depth of Mizunami Underground Research Laboratory

Kuwabara, Kazumichi*; Aoyagi, Yoshiaki; Ozaki, Yusuke; Matsui, Hiroya

JAEA-Research 2017-002, 39 Pages, 2017/03

JAEA-Research-2017-002.pdf:3.58MB

Authors developed a displacement meter using optical fiber sensor. The displacement meter can be set at any locations in a borehole and guarantee the measurement accuracy up to 5MPa. Total twelve displacement meters were installed in three boreholes to measure the rock mass displacement during groundwater recovery test. The measurement of the rock mass displacement was stated on March, 27, FY 2014. During the first and second groundwater recovery experiments, compressive displacements were observed close to the closure test drift wall. Magnitude of the measured displacements, except vicinity of test drift wall, was smaller than that of calculated under the assumption of it is an isotropic elastic material.

JAEA Reports

Research of the tasks on risk communication enforcement in fiscal year 2015 (Contract research)

Tanaka, Masaru*; Aoyama, Isao*; Ishizaka, Kaoru*; Ohata, Yuki*; Fukuike, Iori*; Kawase, Keiichi; Watanabe, Masanori; Tokizawa, Takayuki; Miyagawa, Hiroshi*; Ishimori, Yuu

JAEA-Research 2017-003, 65 Pages, 2017/06

JAEA-Research-2017-003.pdf:2.92MB

JAEA Ningyo-toge Environmental Engineering Center and Fukushima Environmental Safety Center have same challenges in risk communication. As reference, similar domestic cases were investigated by our two Centers, and requirements for building long-term relationship were clarified. As follows; (1) Develop new relationship with various stakeholders in the region. (2) Make better use of existing resources (personnel, land and facilities, etc.). (3) Make a concerted effort to create new values with local stakeholders. (4) Make an opportunity which local stakeholders confirm safety and build confidence to the project. These efforts will enhance the opportunities for operators and residents to learn about environment management and environmental protection.

JAEA Reports

A Study of the evaluation of the excavation damaged zone in the Horonobe Underground Research Laboratory, 2; Investigation in the 250 m gallery (Joint research)

Aoyagi, Kazuhei; Kubota, Kenji*; Nakata, Eiji*; Suenaga, Hiroshi*; Nohara, Shintaro*

JAEA-Research 2017-004, 91 Pages, 2017/06

JAEA-Research-2017-004.pdf:6.07MB

In this study, we performed seismic tomography, seismic refraction survey, resistivity tomography, and hydraulic tests to investigate the hydro-mechanical property of the excavation damaged zone (EDZ) in the 250 m gallery of the Horonobe Underground Research Laboratory. As a result of seismic tomography, seismic velocity is significantly decreased within 1 m from the gallery wall. The decrease of seismic velocity is related to the density of fracture induced around the gallery wall as a result of the gallery excavation. Thus the extent of the fractures induced by gallery excavation, i.e., EDZ fractures is clarified to be within 1.0 m from the gallery wall. The enhanced hydraulic conductivity was detected within 0.5 to 1.0 m from the gallery wall on the basis of the result of hydraulic tests. This is almost consistent with the extent of the region that seismic velocity is significantly decreased. Therefore, it is estimated that EDZ fractures induced around the gallery leads to the increase of hydraulic conductivity. In addition, the desaturation zone around the gallery is not induced as a result of resistivity tomography. From these results, the hydro-mechanical property of the EDZ is clarified in detail. Also, the in situ tests and evaluation method applied in this study are appropriate to investigate the EDZ in detail.

JAEA Reports

XAFS measurement of simulated waste borosilicate glass samples (Joint research)

Nagai, Takayuki; Kobayashi, Hidekazu; Sasage, Kenichi; Ayame, Yasuo; Okamoto, Yoshihiro; Shiwaku, Hideaki; Yamanaka, Keisuke*; Ota, Toshiaki*

JAEA-Research 2017-005, 54 Pages, 2017/06

JAEA-Research-2017-005.pdf:16.17MB

Addition of radioactive waste to a borosilicate frit affects the local structures of boron (B) and waste elements in a waste glass. Synchrotron XAFS measurement was applied to investigate the local structural changes by using simulated waste borosilicate glass samples. Following results were obtained by the B K-edge XAFS analysis. It was confirmed that B K-edge XAFS analysis enables us to discriminate sp$$^{2}$$ type boron (BO$$_{3}$$) from sp$$^{3}$$ type boron (BO$$_{4}$$). Addition of waste elements to a glass frit increases the percentage of BO$$_{3}$$ and decreases that of BO$$_{4}$$. By decreasing the SiO$$_{2}$$/Al$$_{2}$$O$$_{3}$$ ratio or increasing the (SiO$$_{2}$$+B$$_{2}$$O$$_{3}$$)/Al$$_{2}$$O$$_{3}$$ ratio in the glass composition, the BO$$_{3}$$ percentage increases and the BO$$_{4}$$ percentage decreases. Addition of P$$_{2}$$O$$_{5}$$ decreases the BO$$_{3}$$ percentage and increases the BO$$_{4}$$ percentage. Following results were obtained from XAFS measurement of the waste elements. Cerium (Ce) valence is more reduced with the increase of the B$$_{2}$$O$$_{3}$$ content. Addition of P$$_{2}$$O$$_{5}$$ has a tendency to reduce the Ce valence and to enhance deposition of Zr oxide. Deposition of ruthenium compounds separated from glass phase can not be improved by changing the B$$_{2}$$O$$_{3}$$ content. This study was performed as a part of the project, "Improvement of vitrification process of high-level radioactive liquid wastes" on the foundation business of the Agency for Natural Resources and Energy.

JAEA Reports

Development of separation process for Pd by extraction with 5,8-diethyl-7-hydroxy-6-dodecanone oxime

Morita, Yasuji; Yamagishi, Isao

JAEA-Research 2017-006, 27 Pages, 2017/06

JAEA-Research-2017-006.pdf:1.83MB

Separation of Pd by extraction with 5,8-diethyl-7-hydroxy-6-dodecanone oxime (DEHDO) was examined by batch and continuous tests for the purpose of developing Pd separation process. Batch extraction tests using n-dodecane solution of DEHDO revealed that Pd, Zr and Mo were extracted from simulated high-level radioactive liquid wastes (HLLW) and other elements were not, and also showed that the extraction rate was a little slow and a white precipitate appeared in the aqueous phase but its formation could be avoided by raising temperature. The extracted Pd was found to be back-extracted with sodium nitrite. In the continuous extraction tests with simulated HLLW without Zr and Mo, about 98% of Pd were extracted with DEHDO-n-dodecane and 95% of the extracted Pd were back-extracted with sodium nitrite and nitric acid. Continuous extraction test with simulated HLLW with Zr and Mo showed the possibility of the simultaneous separation of Pd and Mo by DEHDO extraction.

JAEA Reports

Development of LEAP-III code for evaluation of long-time event progress under tube failure accident in steam generators

Uchibori, Akihiro; Yanagisawa, Hideki*; Takata, Takashi; Kurihara, Akikazu; Hamada, Hirotsugu; Ohshima, Hiroyuki

JAEA-Research 2017-007, 61 Pages, 2017/07

JAEA-Research-2017-007.pdf:4.3MB

For safety assessment of a steam generator of sodium-cooled fast reactors, it is necessary to evaluate the possibility of occurring tube failure propagation and of water leak rate under sodium-water reaction accident. In the previous studies, a computer code called LEAP-II calculating a wastage-type failure propagation and the water leak rate during long-time event progress was developed. In this study, a numerical method to evaluate the possibility of occurring overheating rupture was introduced into the LEAP-II code to expand application range of this code. The completed code is called LEAP-III. The test analysis on a tube bundle configuration demonstrated that the overheating rupture model could provide conservative prediction.

JAEA Reports

Expansion characteristics of particles in ablation plume measured with resonance absorption spectroscopy; Comparison of neutral atoms of titanium and hafnium

Jung, K.; Miyabe, Masabumi; Akaoka, Katsuaki; Oba, Masaki; Wakaida, Ikuo

JAEA-Research 2017-008, 26 Pages, 2017/08

JAEA-Research-2017-008.pdf:5.99MB

We are developing an analytical method using laser ablation absorption spectroscopy (LAAS) to analyze radioactive waste mixed with zirconium, uranium and so on. It is essential to evaluate the characteristics of the plume formed by the objective particles for LAAS analysis. Therefore, in this study, titanium and hafnium whose chemical properties are similar to those of Zr were chosen as analytical object. And the difference in expanding behavior of the plume due to the weight of the particles was investigated. As a result of changing the height of the probe beam and applying the optical time-of-flight method to the plume, it was found that the influence of the background gas is larger for Ti than Hf. The meaning of the resonance absorption signal of the waste sample mixed with nuclear fuel materials and nuclear reactor materials was understood by this study and basic knowledge to optimize experimental conditions were also obtained.

JAEA Reports

Study on effects of coupled phenomenon on long-term behavior for crystalline rock (Joint research)

Kimoto, Kazushi*; Ichikawa, Yasuaki*; Matsui, Hiroya

JAEA-Research 2017-009, 18 Pages, 2017/11

JAEA-Research-2017-009.pdf:6.5MB

JAEA has started this study as joint research with Okayama University from 2016. In fiscal year 2016, several kinds of elastic wave velocity were measured using ultra sonic sensors and laser Doppler vibrometer to evaluate the anisotropy of different elastic wave in granite. The velocity measurements were carried out focused on transmitted wave and surface wave. The results showed that strong anisotropy was observed in transmitted P- wave velocity while weak anisotropy was observed in transmitted S-wave and group velocity estimated by surface velocity measurement. In addition, data obtained from surface velocity measurement was partitioned into transmitted and reflected waves and analyzed them in detail. It resulted that elastic wave due to mineral particles consist of granite was dispersed; however, significant dispersion was only observed at specific location.

JAEA Reports

Study on crystalline rock aiming at evaluation method of long-term behavior of rock mass (Joint research)

Fukui, Katsunori*; Hashiba, Kimihiro*; Matsui, Hiroya

JAEA-Research 2017-010, 61 Pages, 2017/11

JAEA-Research-2017-010.pdf:16.86MB

JAEA has started this study as a collaboration study with Tokyo University from 2016. In the fiscal year of 2016, creep testing on Tage tuff was continuously conducted. Existing theory of rate process and stochastic process was modified to be applied to evaluate effects of water, and then the modified theory was validated based on the results of strength and creep tests performed under dry and wet conditions. Furthermore, effects of water contents on stress-strain curves were examined by uniaxial compression testing under various water content conditions.

JAEA Reports

Cladding tube burst experiment assumed MA fuel pin for transmutation physics experimental facility

Sugawara, Takanori; Tsujimoto, Kazufumi

JAEA-Research 2017-011, 35 Pages, 2017/10

JAEA-Research-2017-011.pdf:4.88MB

The construction of Transmutation Physics Experimental Facility (TEF-P) is planned in the J-PARC project. TEF-P is a critical assembly and it will treat minor actinide (MA) fuel in the experiment. The temperature when the air cooling for the TEF-P core would stop was estimated but there were no data to evaluate the soundness of the MA fuel pin. To set a tentative limit temperature for the TEF-P core, cladding tube burst experiment was performed. As the result, the cladding tube burst occurred at 660$$^{circ}$$C as the severest case. Through these results and the estimation of creep rupture time, the tentative limit temperature for the TEF-P core was set to 600$$^{circ}$$C.

JAEA Reports

Development of measurement system of radioactive plume using unmanned airplane in the fiscal year 2016 (Contract research)

Ishizaki, Azusa; Sanada, Yukihisa; Nishizawa, Yukiyasu*; Futemma, Akira; Munakata, Masahiro

JAEA-Research 2017-012, 58 Pages, 2018/03

JAEA-Research-2017-012.pdf:9.36MB

At the accident of nuclear facilities, a prediction of behavior of released radioactive plume is indispensable for the decision of the refuge plan of inhabitants. Currently, prediction system which is based on atmospheric dispersion simulation has been implemented for as a tool of the atomic energy disaster prevention. However, direct measurement method of radioactive plume has not existed. In this study, some component technologies were developed for establishment of direct measurement methods of radioactive plume using unmanned aerial vehicle whose technological innovation is remarkable. In addition, algorism of making flight plan was developed based on prediction model of radioactive plume. This report summarized the outcome of the first year with plan of three years.

JAEA Reports

Study on characterisation of colloidal silica grout under condition of sea water

Toguri, Satohito*; Okihara, Mitsunobu*; Tsuji, Masakuni*; Nakashima, Hitoshi*; Sugiyama, Hirokazu*; Saito, Akira*; Sato, Toshinori; Aoyagi, Kazuhei; Masunaga, Kosuke

JAEA-Research 2017-013, 131 Pages, 2018/02

JAEA-Research-2017-013.pdf:8.49MB

The discussions on scientifically promising site for the geological disposal has been made at the council of studying group on techniques for geological disposal of radioactive wastes, which is held by Resources and Energy Agency. From the aspect of ensuring safety during the transportation of disposal waste, the coastal area is discussed to be a more suitable area. This report shows the result of the first year of this project as following items; Study on the state-of-art technology and remain tasks; laboratory tests on characterization of colloidal silica grout under sea water; Study on the development of grouting technology (design and the evaluation method of influence on the rock mass).

JAEA Reports

Visualization of fractures in an Excavation Damaged Zone in the Horonobe Underground Research Laboratory (Joint research)

Aoyagi, Kazuhei; Chen, Y.*; Sakurai, Akitaka; Ishii, Eiichi; Ishida, Tsuyoshi*

JAEA-Research 2017-014, 49 Pages, 2018/01

JAEA-Research-2017-014.pdf:16.29MB

In this research, we performed the resin injection experiment at the 350 m gallery of the Horonobe Underground Research Laboratory in order to identify the three dimensional distribution of fractures induced around the gallery owing to excavation. To this end, the low viscosity resin mixed with a fluorescent substance was developed and applied to the in situ resin injection experiment. As a result, the resin was successfully penetrated into the fractures around the gallery without disturbing their situation and then fixed within them. After the experiment, the rock cores around the injection borehole were drilled for the observation. The observation under ultraviolet light revealed that the extent of the development of fractures was about 0.9 m into the borehole wall. In addition, the aperture of the fractures distributed within 0.3 m from the gallery wall was ranged 1 to 2 mm, and that distributed from 0.3 to 0.9 m was less than 1 mm. On the other hand, in the borehole televiewer (BTV) survey, only one fracture within 0.2 m from the wall could be detected owing to the resolution of the survey system. Thus, it is expected that the BTV survey underestimate the extent of the development of fractures.

JAEA Reports

Development of correlation of gaseous ruthenium transfer rate to condensed water in accident of evaporation to dryness by boiling of reprocessed high level liquid waste in Fuel Reprocessing Facilities

Yoshida, Kazuo; Tamaki, Hitoshi; Yoshida, Naoki; Amano, Yuki; Abe, Hitoshi

JAEA-Research 2017-015, 18 Pages, 2018/01

JAEA-Research-2017-015.pdf:3.08MB

An accident of evaporation to dryness by boiling of high level liquid waste is postulated as one of the severe accidents at a fuel reprocessing facility. It was observed at the experiments that a large amount of ruthenium (Ru) is volatilized and transfer to the vapor phase in the tank. The nitric acid and water mixed vapor released from the tank is condensed. Volatilized Ru is expected to transfer into the condensed water at the compartments in the building. Quantitative estimation of the amount of Ru transferred condensed water is key issues to evaluate the reduction the amount of Ru through leak path in the facility building. This report presents that a correlation has been developed for Ru transfer rate to condensed water with vapor condensing rate based on the experimental results and additional thermal-hydraulic simulation of the experiments. Applicability of the correlation has been also demonstrated with the accident simulation of typical facilities in full-scale.

JAEA Reports

The In-situ experiment for performance confirmation of engineered barrier system at Horonobe Underground Research Laboratory; Consideration of concrete-type plug composition

Nakayama, Masashi; Niunoya, Sumio*; Miura, Norihiko*; Takeda, Nobufumi*

JAEA-Research 2017-016, 62 Pages, 2018/01

JAEA-Research-2017-016.pdf:19.99MB

The Horonobe URL Project has being pursued by JAEA to enhance the reliability of relevant disposal technologies through investigations of the deep geological environment within the host sedimentary formation at Horonobe, Hokkaido. The URL Project consists of 2 major research areas, "Geoscientific Research" and "Research and Development on Geological Disposal Technologies", and proceeds in 3 overlapping phases, over a period of around 20 years. Phase III (Investigations in the underground facilities) investigation was started in 2010 FY. The in-situ experiment for performance confirmation of engineered barrier system (EBS experiment) had started 2013 at GL-350 m gallery, and heating by electric heater in simulated overpack had started in January, 2015. One of objectives of the EBS experiment is acquiring data concerned with THMC coupled behavior. These data will be used in order to confirm the performance of engineered barrier system. This report shows consideration of concrete-type plug composition. The low alkaline cement developed by JAEA, called HFSC, was used for the plug. HFSC has used in construction test at the gallery as shotcrete in Horonobe URL.

JAEA Reports

Confirmation tests for Warm Pre-stress (WPS) effect in reactor pressure vessel steel (Contract research)

Chimi, Yasuhiro; Iwata, Keiko; Tobita, Toru; Otsu, Takuyo; Takamizawa, Hisashi; Yoshimoto, Kentaro*; Murakami, Takeshi*; Hanawa, Satoshi; Nishiyama, Yutaka

JAEA-Research 2017-018, 122 Pages, 2018/03

JAEA-Research-2017-018.pdf:44.03MB

Warm pre-stress (WPS) effect is a phenomenon that after applying a load at a high temperature fracture does not occur in unloading during cooling, and then the fracture toughness in reloading at a lower temperature increases effectively. Engineering evaluation models to predict an apparent fracture toughness in reloading are established using experimental data with linear elasticity. However, there is a lack of data on the WPS effect for the effects of specimen size and surface crack in elastic-plastic regime. In this study, fracture toughness tests were performed after applying load-temperature histories which simulate pressurized thermal shock transients to confirm the WPS effect. The experimental results of an apparent fracture toughness tend to be lower than the predictive results using the engineering evaluation models in the case of a high degree of plastic deformation in preloading. Considering the plastic component of preloading can refine the engineering evaluation models.

JAEA Reports

Analysis of post irradiation examination of used BWR fuel with SWAT4.0

Kikuchi, Takeo; Tada, Kenichi; Sakino, Takao; Suyama, Kenya

JAEA-Research 2017-021, 56 Pages, 2018/03

JAEA-Research-2017-021.pdf:2.15MB
JAEA-Research-2017-021(errata).pdf:0.13MB

The criticality management of the fuel debris is one of the most important research issues in Japan. The current criticality management adopts the fresh fuel assumption. The adoption of the fresh fuel assumption for the criticality control of the fuel debris is difficult because the k$$_{rm eff}$$ of the fuel debris could exceed 1.0 in most of cases which the fuel debris contains water and does not contain neutron absorbers such as gadolinium. Therefore, the adoption of the burnup credit is considered. The prediction accuracy of the isotopic composition of used nuclear fuel must be required to adopt the burnup credit for the treatment of the fuel debris. JAEA developed a burnup calculation code SWAT4.0 to obtain reference calculation results of the isotopic composition of the used nuclear fuel. This code is used to evaluate the composition of fuel debris. In order to investigate the prediction accuracy of SWAT4.0, we analyzed the PIE of BWR obtained from 2F2DN23.

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