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Zhang, A.*; Deng, K.*; Sheng, J.*; Liu, P.*; Kumar, S.*; 島田 賢也*; Jiang, Z.*; Liu, Z.*; Shen, D.*; Li, J.*; et al.
Chinese Physics Letters, 40(12), p.126101_1 - 126101_8, 2023/12
被引用回数：2 パーセンタイル：57.37(Physics, Multidisciplinary)In a Dirac semimetal, the massless Dirac fermion has zero chirality, leading to surface states connected adiabatically to a topologically trivial surface state as well as vanishing anomalous Hall effect. Recently, itis predicted that in the nonrelativistic limit of certain collinear antiferromagnets, there exists a type of chiral "Dirac-like" fermion, whose dispersion manifests four-fold degenerate crossing points formed by spin-degenerate linear bands, with topologically protected Fermi arcs. Here, by combining with neutron diffraction and first-principles calculations, we suggest a multidomain collinear antiferromagnetic configuration, rendering the existence of the Fermi-arc surface states induced by chiral Dirac-like fermions.
Hu, Q.*; Wang, Q. M.*; Zhang, T.*; Zhao, C.*; Iltaf, K. H.*; Liu, S. Q.*; 深津 勇太
Energy Reports (Internet), 9, p.3661 - 3682, 2023/12
被引用回数：4 パーセンタイル：73.72(Energy & Fuels)This study evaluates petrophysical properties of representative geological rocks in the context of injectivity, storage space, and caprock integrity for effective utilization and long-term storage of carbon dioxide. A total of 10 geological rocks were selected as representative storage media for consideration as saline aquifers & depleted oil and gas reservoirs, basalts, and cap rocks, as well as utilization in organic-rich shale and coal seams. An integrated suite of laboratory tests, including liquid immersion porosimetry, gas expansion porosimetry, grain size distribution, mercury intrusion porosimetry, and gas diffusion, were performed on these various rock samples. The results exhibit a disparity of petrophysical properties among two broad groups of rocks: rocks selected for possible storage of CO
have porosities of 
10-25%, permeabilities of 10
-10
m
, 
m-sized pore-throat size distribution, and mostly good pore connectivity; in contrast, the potential caprocks have porosities of 0.5-5%, permeabilities of 10
-10
m, pore throat sizes of 
50 nm, and probably poorly connected pore networks. An understanding of the measured facets of pore structure and contribution of fractures is also critical in the context of different testing principles and data interpretation of petrophysical analyses, as well as observational scales in the laboratory and field, and therefore reliable confidence of CO storage and utilization performance. Our work further illustrates the controlling influence of grain size distribution and geological processes on pore size distribution and pore connectivity for a wide range of rock types and lithologies, and particularly presents the extent and behavior of CO gas diffusion with a custom-designed apparatus for a holistic understanding of various petrophysical attributes of widely different geological rocks.
Fe
intermetallic compoundCao, Y.*; Zhou, H.*; Khmelevskyi, S.*; Lin, K.*; Avdeev, M.*; Wang, C.-W.*; Wang, B.*; Hu, F.*; 加藤 健一*; 服部 高典; et al.
Chemistry of Materials, 35(8), p.3249 - 3255, 2023/04
被引用回数：1 パーセンタイル：45.8(Chemistry, Physical)静水圧や化学圧力は、結晶構造を変化させる効率的な刺激であり、材料科学において電気的、磁気的特性のチューニングによく利用されている。しかし、化学圧力は定量化が困難であり、これら両者の定量的な対応関係はまだよくわかっていない。本研究では、負の熱膨張(NTE)を持つ永久磁石の候補である金属間化合物を調べた。放射光X線その場観察により、AlをドープしたHoFeに負の化学圧力があることを明らかにし、単位セル体積の温度・圧力依存性を用いそれを定量的に評価した。また、磁化測定と中性子回折測定を組み合わせることで、磁気秩序に対する化学圧力と静水圧の違いを比較した。興味深いことに、圧力はNTEの抑制と増強を制御するために使用することができた。電子状態計算から、圧力がFermiレベル(EF)に対する主要バンドの上部に影響を与えたことを示しており、これは磁気安定性に影響を与え、それが磁気とNTEを調節する上で重要な役割を果たしていることがわかった。本研究は、圧力の影響を理解し、それを利用して機能性材料の特性を制御する良い例を示している。
Ao, N.*; Zhang, H.*; Xu, H. H.*; Wu, S. C.*; Liu, D.*; 徐 平光; Su, Y. H.; Kang, Q. H.*; Kang, G. Z.*
Engineering Fracture Mechanics, 281, p.109166_1 - 109166_14, 2023/03
被引用回数：5 パーセンタイル：87.64(Mechanics)Considering the complex service environments that high-speed railway axles are subjected to, the fatigue crack growth (FCG) behavior of a structurally gradient axle steel with different pre-crack depths both in air and corrosive medium was investigated at a frequency of 5 Hz. The results indicated that in the high 
region, FCG rate was dramatically accelerated by corrosion, but the gap narrows as decreased. The accelerated corrosion FCG rate was a comprehensive result of the acceleration effect of the anodic dissolution, hydrogen-enhanced localized plasticity and the retardation effect of corrosion-induced crack-tip blunting. Despite the fact that the corrosion resistance gradually decreased as the pre-crack depth increased, the FCG rate in the corrosive medium gradually decreased. This was because fatigue loading played a more important role than corrosion in accelerating the corrosion FCG rate.
BaCo(PO
)Sheng, J.*; Wang, L.*; Candini, A.*; Jiang, W.*; Huang, L.*; Xi, B.*; Zhao, J.*; Ge, H.*; Zhao, N.*; Fu, Y.*; et al.
Proceedings of the National Academy of Sciences of the United States of America, 119(51), p.e2211193119_1 - e2211193119_9, 2022/12
被引用回数：4 パーセンタイル：56.47(Multidisciplinary Sciences)Although considerable progress has been made in the theoretical understanding of the low-dimensional frustrated quantum magnets, experimental realizations of a well-established scaling analysis are still scarce. This is particularly true for the two-dimensional antiferromagnetic triangular lattices. Owing to the small exchange strength, the newly discovered compound NaBaCo(PO) provides a rare opportunity for clarifying the quantum criticality in an ideal triangular lattice with quantum spin S=1/2. In addition to the establishment of the complete phase diagrams, the spin Hamiltonian with a negligible interplane interaction has been determined through the spin wave dispersion in the polarized state, which is consistent with the observation of a two-dimensional quantum critical point with the Bose-Einstein condensation of diluted free bosons.
Liu, B.*; Feng, R.*; Busch, M.*; Wang, S.*; Wu, H.*; Liu, P.*; Gu, J.*; Bahadoran, A.*; 松村 大樹; 辻 卓也; et al.
ACS Nano, 16(9), p.14121 - 14133, 2022/09
被引用回数：51 パーセンタイル：98.66(Chemistry, Multidisciplinary)Pt single-atom materials possess an ideal atom economy but suffer from limited intrinsic activity and side reaction of producing HO in catalyzing the oxygen reduction reaction (ORR). Here, we demonstrate that anchoring platinum alloys on single-atom Pt-decorated carbon (Pt- SAC) surmounts their inherent deficiencies, thereby enabling a complete four-electron ORR pathway catalysis with high efficiency and durability. Pt
Co@Pt-SAC demonstrates an exceptional mass and specific activities 1 order of magnitude higher than those of commercial Pt/C. They are durable throughout 50000 cycles, showing only a 10 mV decay in halfwave potential. The superior durability is attributed to the shielding effect of the Pt-SAC coating, which significantly mitigates the dissolution of PtCo cores.
Fe(n,
)
Fe cross section from the surrogate ratio method and its effect on the Fe nucleosynthesisYan, S. Q.*; Li, X. Y.*; 西尾 勝久; Lugaro, M.*; Li, Z. H.*; 牧井 宏之; Pignatari, M.*; Wang, Y. B.*; Orlandi, R.; 廣瀬 健太郎; et al.
Astrophysical Journal, 919(2), p.84_1 - 84_7, 2021/10
被引用回数：1 パーセンタイル：8.53(Astronomy & Astrophysics)The long-lived Fe (with a half-life of 2.62 Myr) is a crucial diagnostic of active nucleosynthesis in the Milky Way galaxy and in supernovae near the solar system. The neutron-capture reaction Fe(n,)Fe on Fe (half-life=44.5 days) is the key reaction for the production of Fe in massive stars. This reaction cross section has been previously constrained by the Coulomb dissociation experiment, which offered partial constraint on the E1 -ray strength function but a negligible constraint on the M1 and E2 components. In this work, for the first time, we use the surrogate ratio method to experimentally determine the Fe(n,)Fe cross sections in which all the components are included. We derived a Maxwellian-averaged cross section of 27.5
3.5 mb at 
= 30 keV and 13.41.7 mb at = 90 keV, roughly 10%-20% higher than previous estimates. We analyzed the impact of our new reaction rates in nucleosynthesis models of massive stars and found that uncertainties in the production of Fe from the Fe(n,)Fe rate are at most 25
. We conclude that stellar physics uncertainties now play a major role in the accurate evaluation of the stellar production of Fe.
Lai, W.-H.*; Wang, H.*; Zheng, L.*; Jiang, Q.*; Yan, Z.-C.*; Wang, L.*; 吉川 浩史*; 松村 大樹; Sun, Q.*; Wang, Y.-X.*; et al.
Angewandte Chemie; International Edition, 59(49), p.22171 - 22178, 2020/12
被引用回数：79 パーセンタイル：95.7(Chemistry, Multidisciplinary)Herein, we report a comprehensive strategy to synthesize a full range of single-atom metals on carbon matrix, including V, Mn, Fe, Co, Ni, Cu, Ge, Mo, Ru, Rh, Pd, Ag, In, Sn, W, Ir, Pt, Pb, and Bi. The extensive applications of various single-atom catalysts (SACs) are manifested via their ability to electro-catalyze typical hydrogen evolution reactions (HER) and conversion reactions in novel room-temperature sodium sulfur batteries (RT-Na-S). The enhanced performances for these electrochemical reactions arisen from the ability of different single active atoms on local structures to tune their electronic configuration. Significantly, the electrocatalytic behaviors of diverse SACs, assisted by density functional theory calculations, are systematically revealed by in situ synchrotron X-ray diffraction and in situ transmission electronic microscopy, providing a strategic library for the general synthesis and extensive applications of SACs in energy conversion and storage.
decay of 
USun, M. D.*; Liu, Z.*; Huang, T. H.*; Zhang, W. Q.*; Andreyev, A. N.; Ding, B.*; Wang, J. G.*; Liu, X. Y.*; Lu, H. Y.*; Hou, D. S.*; et al.
Physics Letters B, 800, p.135096_1 - 135096_5, 2020/01
被引用回数：11 パーセンタイル：78.75(Astronomy & Astrophysics)Fine structure in the decay of U was observed in the fusion-evaporation reaction 
Re(
Ar,p3n) by using fast digital pulse processing technique. Two -decay branches of U feeding the ground state and 244 keV excited state of 
Th were identified by establishing the decay chain U
Th
Ra
Rn. The -particle energy for the ground-state to ground-state transition of U was determined to be 8993(17) keV, 213 keV higher than the previous value, the half-life was updated to be 62
s. Evolution of nuclear structure for 
=131 even-
isotones from Po to U was discussed in the frameworks of nuclear mass and reduced -decay width, a weakening octupole deformation in the ground state of U relative to its lighter isotones Ra and Th was suggested.
Tang, C.*; Song, Q.*; Chang, C.-Z.*; Xu, Y.*; 大沼 悠一; 松尾 衛*; Liu, Y.*; Yuan, W.*; Yao, Y.*; Moodera, J. S.*; et al.
Science Advances (Internet), 4(6), p.eaas8660_1 - eaas8660_6, 2018/06
被引用回数：30 パーセンタイル：84.16(Multidisciplinary Sciences)This work demonstrates markedly modified spin dynamics of magnetic insulator (MI) by the spin momentum-locked Dirac surface states of the adjacent topological insulator (TI). As the Bi concentration 
is systematically tuned in 5-nm-thick (Bi
Sb
)Te TI films, the weight of the surface relative to bulk states peaks at = 0.32 when the chemical potential approaches the Dirac point. At this concentration, the Gilbert damping constant of the precessing magnetization in 10-nm-thick YFe
O
MI films in the MI/TI heterostructures is enhanced by an order of magnitude, the largest among all concentrations. In addition, the MI acquires additional strong magnetic anisotropy that favors the in-plane orientation with similar Bi concentration dependence. These extraordinary effects of the Dirac surface states distinguish TI from other materials such as heavy metals in modulating spin dynamics of the neighboring magnetic layer.
Sr
CuOLin, J. Q.*; Liu, X.*; Blackburn, E.*; 脇本 秀一; Ding, H.*; Islam, Z.*; Sinha, S. K.*
Physical Review Letters, 120(19), p.197001_1 - 197001_6, 2018/05
被引用回数：3 パーセンタイル：29(Physics, Multidisciplinary)X線散漫散乱の観測により、銅酸化物高温超伝導体La
SrCuO中の不純物Srにより生じるナノスケールの格子歪みを観測した。この結果は、これまで議論となっていた不純物による歪みの性質を明らかにしたとともに、STMで観測されているギャップの不均一性の原因ではないことを明らかにした。
Zr(
)
Zr cross section from the surrogate ratio method and its effect on 
-process nucleosynthesisYan, S. Q.*; Li, Z. H.*; Wang, Y. B.*; 西尾 勝久; Lugaro, M.*; Karakas, A. I.*; 牧井 宏之; Mohr, P.*; Su, J.*; Li, Y. J.*; et al.
Astrophysical Journal, 848(2), p.98_1 - 98_8, 2017/10
被引用回数：5 パーセンタイル：21.26(Astronomy & Astrophysics)The Zr()Zr reaction cross section is crucial in the modelling of -process nucleosynthesis in asymptotic giant branch stars because it controls the operation of the branching point at the unstable Zr and the subsequent production of Zr. We have carried out the measurement of the 
Zr(
O,
O) and 
Zr(O,O) reactions and obtained the -decay probability ratio of 
Zr
and Zr to determine the Zr()Zr reaction cross sections with the surrogate ratio method. We tested our deduced maxwellian-averaged cross section in stellar models with masses between 2 and 6 
and metallicities 0.014 and 0.03. The largest changes - up 80 % variations in Zr - are seen in the models of 3-4 , where the 
Ne neutron source is mildly activated. The new rate can still provide a match to data from meteoritic stardust silicon carbide grains, provided the maximum mass of the parent stars is below 4 , for a metallicity of 0.03.
Zr(n,)Zr cross section with 
Zr(O,O)
Zr reactionsYan, S. Q.*; Li, Z. H.*; Wang, Y. B.*; 西尾 勝久; 牧井 宏之; Su, J.*; Li, Y. J.*; 西中 一朗; 廣瀬 健太郎; Han, Y. L.*; et al.
Physical Review C, 94(1), p.015804_1 - 015804_5, 2016/07
被引用回数：6 パーセンタイル：44.35(Physics, Nuclear)The relative -decay probability ratios of the neutron resonance states in Zr and Zr populated via two neutron transfer reactions, Zr(O,O)Zr and Zr(O,O)Zr, have been measured to test the validity of the surrogate ratio method (SRM) in determining the (n,) reaction cross section. The cross sections of the Zr(n,)Zr reaction are derived from the experimentally obtained ratios and the cross sections of the 
Zr(n,)Zr reaction in the equivalent neutron energy range of 
= 0 - 8 MeV. The deduced cross sections of Zr(n,)Zr reaction agree with the directly measured ones in the low-energy region, and with the evaluated ENDF/B-VII.1 data at higher energies of 
3 MeV. The agreement supports the concept of the SRM method to indirectly determine the (n,) reaction cross sections.
/SrTiO (110) interfaceAnnadi, A.*; Zhang, Q.*; Renshaw Wang, X.*; Tuzla, N.*; Gopinadhan, K.*; L
, W. M.*; Roy Barman, A.*; Liu, Z. Q.*; Srivastava, A.*; Saha, S.*; et al.
Nature Communications (Internet), 4, p.1838_1 - 1838_7, 2013/05
被引用回数：97 パーセンタイル：94.61(Multidisciplinary Sciences)We report the observation of unexpected conductivity at the LaAlO/SrTiO interface prepared on (110)-oriented SrTiO, with a LaAlO-layer thickness-dependent metal-insulator transition. Density functional theory calculation reveals that electronic reconstruction, and thus conductivity, is still possible at this (110) interface by considering the energetically favourable (110) interface structure, that is, buckled TiO/LaO, in which the polarization discontinuity is still present. The conductivity was further found to be strongly anisotropic along the different crystallographic directions with potential for anisotropic superconductivity and magnetism, leading to possible new physics and applications.
[503] band of 
PtLi, G. S.*; Zhou, X. H.*; Zhang, Y. H.*; Zheng, Y.*; Liu, M. L.*; Hua, W.*; Zhou, H. B.*; Ding, B.*; Wang, H. X.*; Lei, X. G.*; et al.
Journal of Physics G; Nuclear and Particle Physics, 38(9), p.095105_1 - 095105_9, 2011/09
被引用回数：1 パーセンタイル：11.74(Physics, Nuclear)Ptの高スピン状態をタンデム加速器と多重線検出装置GEMINI-IIを用いて調べた。低スピン指標逆転現象が7/2[503]バンドで観測された。この現象は、中性子が7/2[503]軌道から7/2[514]軌道に移ることによって起こるという解釈は、DonauとFrauendorfの反古典的近似による計算結果によって支持された。
Deng, Z.*; Jin, C. Q.*; Liu, Q. Q.*; Wang, X. C.*; Zhu, J. L.*; Feng, S. M.*; Chen, L. C.*; Yu, R. C.*; Arguello, C.*; 後神 達郎*; et al.
Nature Communications (Internet), 2, p.1425_1 - 1425_5, 2011/08
被引用回数：160 パーセンタイル：93.76(Multidisciplinary Sciences)(Ga,Mn)Asは典型的な強磁性III-V族半導体として知られている。これは3価のGa原子を2価のMnで置き換えたものであるが、化学的溶解度が限られているため準安定であり、薄膜でしか製作できないものであった。また電子ドープも行うことができなかった。この困難な条件を超えるため、Masekらは理論的にI-II-V族半導体LiZnAsを提案した。この物質では原子価が等しい(Zn,Mn)の置き換えによる磁性の発現とLi濃度を過剰あるいは不足させることによるキャリアードープを独立に制御可能である。本研究では世界で初めてバルクな状態でのLi
(ZnMn
)Asの合成に成功した。わずかにLiを過剰にすることで、50Kまでの温度で強磁性が現れること、またp型のキャリアーを持つことが観測され、これらの結果を報告した。
Hender, T. C.*; Wesley, J. C.*; Bialek, J.*; Bondeson, A.*; Boozer, A. H.*; Buttery, R. J.*; Garofalo, A.*; Goodman, T. P.*; Granetz, R. S.*; Gribov, Y.*; et al.
Nuclear Fusion, 47(6), p.S128 - S202, 2007/06
被引用回数：921 パーセンタイル：100(Physics, Fluids & Plasmas)本論文は、1999年の"ITER Physics Basis"の刊行以降に世界各国の装置で得られた重要な成果について記述したものであり、本章ではMHD安定性及びディスラプションに関する成果が記述されている。MHD安定性に関しては、(1)鋸歯状振動,(2)新古典テアリングモード,(3)抵抗性壁モード,(4)誤差磁場,(5)先進シナリオにおけるMHD安定性に関する成果が記述されていて、ディスラプションに関しては、(1)ディスラプションの特徴・原因・頻度,(2)サーマルクエンチによるエネルギーの損失と堆積,(3)電流クエンチのダイナミクス,(4)ディスラプションにより発生する逃走電子,(5)統合モデルとシミュレーション,(6)ディスラプションの回避・予測・緩和に関する成果が記述されている。
Chen, L.-M.; 小瀧 秀行; 中島 一久*; Koga, J. K.; Bulanov, S. V.; 田島 俊樹; Gu, Y. Q.*; Peng, H. S.*; Wang, X. X.*; Wen, T. S.*; et al.
Physics of Plasmas, 14(4), p.040703_1 - 040703_4, 2007/04
被引用回数：36 パーセンタイル：75.41(Physics, Fluids & Plasmas)レーザーの自己導波の調査のため、長いunderdenseのプラズマと100TWレーザーパルスの相互作用実験を行い、レイリー長の約20倍の10mmという非常に長いプラズマチャネルを観測した。レーザーパルスがチャネル中で曲がること、及び電子キャビティ形成が実験的に初めて観測された。
