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particle diameters using an alpha-particle imaging detectorMorishita, Yuki; Sagawa, Naoki; Takada, Chie; Momose, Takumaro; Takasaki, Koji
Radiation Protection Dosimetry, 199(13), p.1376 - 1383, 2023/08
Times Cited Count：0 Percentile：0.01(Environmental Sciences)It is very important to evaluate the diameters (activity median aerodynamic diameter) of Plutonium dioxide (PuO) particles for internal exposure dose evaluation. In this study, a method of evaluating PuO particle diameters using an alpha-particle imaging detector was developed. PuO particles with different diameters were modeled by Monte Carlo simulation, and the change in the shape of the energy spectrum for each particle diameter was evaluated. Two different patterns were modeled, namely, the case of 
PuO and the case of PuO (including isotopic composition of Pu). Multiple regression analysis was performed to determine the PuO particle diameter from the obtained parameters. The simulated diameters and the diameters obtained with the regression model were in good agreement. The advantage of using the alpha-particle imaging detector is to measure the alpha energy spectrum for individual particle, and this allows accurate measurement of particle diameter distribution.
-tetradodecyldiglycolamide (TDdDGA) by using mixer-settler extractors in a hot cellBan, Yasutoshi; Suzuki, Hideya; Hotoku, Shinobu; Kawasaki, Tomohiro*; Sagawa, Hiroshi*; Tsutsui, Nao; Matsumura, Tatsuro
Solvent Extraction and Ion Exchange, 37(1), p.27 - 37, 2019/00
Times Cited Count：22 Percentile：66.01(Chemistry, Multidisciplinary)A continuous counter-current experiment using TDdDGA was performed using mixer-settler extractors installed in a hot cell. Nitric acid containing minor actinides (MAs: Am and Cm), rare earths (REs: Y, La, Nd, and Eu), and other fission products (Sr, Cs, Zr, Mo, Ru, Rh, and Pd) was fed to the extractor. TDdDGA effectively extracted MAs and REs from the feed, while other fission products were barely extracted. The extracted MAs and REs were back-extracted by bringing them in contact with 0.02 mol/dm
nitric acid, and they were collected as the MA-RE fraction. The proportions of MA and RE in the MA-RE fraction were 
98% and 86%, respectively. These results demonstrated the applicability of TDdDGA as an extractant for MAs and REs.
Suzuki, Hideya; Tsubata, Yasuhiro; Kurosawa, Tatsuya*; Sagawa, Hiroshi*; Matsumura, Tatsuro
Journal of Nuclear Science and Technology, 54(11), p.1163 - 1167, 2017/11
Times Cited Count：26 Percentile：93.1(Nuclear Science & Technology)A highly practical diamide-type extractant, which is an alkyl diamide amine with 2-ethylhexyl alkyl chains (ADAAM(EH)), was investigated for mutual separation of Am(III) and Cm(III). ADAAM(EH) is a multidentate ligand with one soft N-donor atom and two hard O-donor atoms in its central frame. This tridentate arrangement of donor atoms provides selective binding to Am(III) compared to that with Cm(III) in highly acidic media, resulting in separation factors of up to 5.5. A continuous liquid-liquid extraction and stripping test was conducted using a multistage countercurrent mixer-settler extractor with ADAAM(EH) in n-dodecane. In this test, separation of Am(III) and Cm(III) was achieved with very high yield.
,-di(2-ethylhexyl)octanamide from nitric acid mediumTsutsui, Nao; Ban, Yasutoshi; Sagawa, Hiroshi; Ishii, Sho; Matsumura, Tatsuro
Solvent Extraction and Ion Exchange, 35(6), p.439 - 449, 2017/08
Times Cited Count：5 Percentile：19.71(Chemistry, Multidisciplinary)Solvent extraction of uranium from a nitric acid medium was performed with ,-di(2-ethylhexyl)octanamide (DEHOA) by a single-stage batch method, and the distribution ratio equation of U(VI) was derived as 
= 1.1![$$[rm NO^{-}_{3}]^{1.6}_{rm aq}[{rm DEHOA}]^{2}_{rm org}$$](/search/images/ERNVY2TNEBHE4XT1FV4V44ZTPVOV24ZRFY1H0X11LRZG0IDBOF4VW402OJWSARCFJBHUC5K3LZ3TE5K5PNOHE1JAN3ZGO5JE.gif)
. Furthermore, the nitric acid distribution was also evaluated, and the distribution ratio equation 
= 0.12![$$[rm H^{+}]^{0.76}_{rm aq}[{rm DEHOA_{rm Free}}]_{rm H}$$](/search/images/ERNVY2TNEBEF24ZLPVOV24ZQFY1TM5K5PNOHE1JAMFYX0W11LRZG0ICEIVEE4QK5PNOHE1JAIZZGKZL3PVOV4402OJWSASD3EQ.gif)
was obtained. Batch experiments to evaluate the time dependence of U(VI) extraction and the U(VI) loading capacity of DEHOA were also performed. It was revealed that U(VI) extraction by DEHOA reached an equilibrium state within a few minutes, and the loading capacity was 0.71 mol/dm (M) when the concentrations of DEHOA and nitric acid were 1.5 and 3.0 M, respectively.
,-di(2-ethylhexyl)octanamide toward uranium from nitric acidTsutsui, Nao; Ban, Yasutoshi; Sagawa, Hiroshi; Ishii, Sho; Matsumura, Tatsuro
Proceedings of 5th International Conference on Asian Nuclear Prospects 2016 (ANUP 2016) (CD-ROM), 2 Pages, 2016/10
Extraction properties of ,-di(2-ethylhexyl)octanamide (DEHOA) toward uranium from nitric acid were studied using single-stage batch method. The results revealed that DEHOA effectively extracted uranium when the nitrate ion concentration was 2.0-3.0 mol/dm.
Hayafune, Hiroki; Kato, Atsushi; Chikazawa, Yoshitaka; Okubo, Tsutomu; Sagawa, Hiroshi*; Shimakawa, Yoshio*
Proceedings of International Conference on Fast Reactors and Related Fuel Cycles; Safe Technologies and Sustainable Scenarios (FR-13) (USB Flash Drive), 11 Pages, 2013/03
Evaluation of earthquake and tsunami on JSFR has been analyzed. For seismic design, safety components are confirmed to maintain their functions even against recent strong earthquakes. As for Tsunami, some parts of reactor building might be submerged including component cooling water system whose final heat sink is sea water. However, in the JSFR design, safety grade components are independent from component cooling water system (CCWS). The JSFR emergency power supply adopts a gas turbine system with air cooling, since JSFR does not basically require quick start-up of the emergency power supply thanks to the natural convection DHRS. Even in case of long station blackout, the DHRS could be activated by emergency batteries or manually and be operated continuously by natural convection.
Chikazawa, Yoshitaka; Enuma, Yasuhiro; Kisohara, Naoyuki; Yamano, Hidemasa; Kubo, Shigenobu; Hayafune, Hiroki; Sagawa, Hiroshi*; Okamura, Shigeki*; Shimakawa, Yoshio*
Proceedings of 2012 International Congress on Advances in Nuclear Power Plants (ICAPP '12) (CD-ROM), p.677 - 686, 2012/06
Evaluation of Earthquake and Tsunami on JSFR has been analyzed. For seismic design, safety components are confirmed to maintain their functions even against recent strong Earthquakes. As for Tsunami, some parts of reactor building might be submerged including component cooling water system whose final heat sink is sea water. However, in the JSFR design, safety grade components are independent from component cooling water system (CCWS). The JSFR emergency power supply adopts a gas turbine system with air cooling, since JSFR does not basically require quick start-up of the emergency power supply thanks to the natural convection DHRS. Even in case of long station blackout, the DHRS could be activated by emergency batteries or manually and be operated continuously by natural convection.
Shinohara, Masanori; Yanagi, Shunki; Tochio, Daisuke; Shimazaki, Yosuke; Nojiri, Naoki; Owada, Hiroyuki; Sato, Nao; Sagawa, Hiroshi; Umeda, Masayuki
JAEA-Technology 2011-029, 39 Pages, 2011/12
JAEA-Technology-2011-029.pdf:3.03MB
JAEA plans and performs the safety demonstration test using the HTTR to develop High Temperature Gas Reactor technologies. Cold test of the loss of forced cooling was conducted prior to the safety demonstration test, to check test procedure and plant behavior. Cold test consists of two phases, Phase1, 1 or 2 Vessel Cooling System (VCS) terminates, in the Phase2, all 3 Gas circulators and 1 VCS terminates. Cold test could confirm test process, and obtain data necessary to analysis and 2-dimensional horizontal sectional model analysis was verified to simulate actual measurement value.
Takasaki, Koji; Sagawa, Naoki; Kurosawa, Shigeyuki; Mizuniwa, Harumi
Journal of Nuclear Science and Technology, 48(6), p.911 - 918, 2011/06
Times Cited Count：12 Percentile：66.68(Nuclear Science & Technology)An autoradiographical method using an imaging plate (IP) was developed to analyze the plutonium contamination in the plutonium handling facility and was applied to the monitoring of the workplace in a practical uranium-plutonium mixed oxide (MOX) fuel fabrication facility. A good relationship between the photo stimulated luminescence (PSL) intensities of IP and radioactivities measured by a radiation counter was obtained by the least-square fitting, taking the fading effect into consideration. The 
-radioactivities of plutonium contamination were derived from the PSL image in this IP method, and their relative errors were evaluated from exposure time.
Sagawa, Naoki; Yamazaki, Takumi; Kurosawa, Shigeyuki*; Izaki, Kenji; Mizuniwa, Harumi; Takasaki, Koji
JAEA-Technology 2010-051, 35 Pages, 2011/03
JAEA-Technology-2010-051.pdf:1.83MB
The image analysis method using a imaging plate (IP) is recent technique, and this method can get the information of radioactivity distribution by the unit of Photo Simulated Luminescence (PSL). We have investigated the PSL images obtained by measuring some plutonium samples which are radiation protection samples in order to apply imaging plate to the radiation protection at the MOX fuel facility. Plutonium spots were extracted from the PSL image extracted by the threshold, in which about 99% of the back ground was excluded, and identified by the additional requirement that the spot size is more than 40 pixels. The average background is subtracted from PSL strength of the spot area identified as Pu, and the radioactivity of the Pu spot was evaluated by multiplying the conversion calculation that is in consideration of fading.
Onozawa, Atsushi; Harada, Akio; Honda, Junichi; Nakata, Masahito; Kanazawa, Hiroyuki; Sagawa, Tamio
JAEA-Conf 2008-010, p.325 - 332, 2008/12
The measurement technique for hydrogen concentration using Backscattered Electron Image analysis (BEI method) had been developed by Studsvik Nuclear AB. The hydride in claddings is identified using BEIs with SEM and the hydrogen concentration is calculated from the area fractions of the hydride in those BEIs. In the RFEF, the sample polishing techniques and image processing procedure for BEI method were improved to measure the hydrogen concentration in the irradiated fuel claddings more precisely. In the previous tests using the un-irradiated fuel claddings, it is confirmed improved BEI method has high reliability. The radial and axial hydrogen concentration profiles of the irradiated fuel claddings were measured with improved BEI method. As the results of these measurements, the local hydrogen concentration could be indicated more precisely with the improved BEI method compared to the other methods for the hydrogen concentration measurement and observation.
Takasaki, Koji; Sagawa, Naoki; Kurosawa, Shigeyuki*; Shioya, Satoshi; Suzuki, Kazunori; Horikoshi, Yoshinori; Mizuniwa, Harumi
JAEA-Technology 2008-028, 73 Pages, 2008/03
JAEA-Technology-2008-028.pdf:5.88MB
Recently, an imaging plate (IP) was developed. Pu analysis by an IP was studied in the JAEA Cooperative Research Scheme on the Nuclear Fuel Cycle, and the availability about detection of Pu and discrimination with radon progenies was shown. In order to apply these results to the radiation control, this research aims at evaluation of radioactivity, discrimination with radon progenies, and evaluation of AMAD by an IP. In the conventional autoradiography (ARG) by a ZnS and Polaroid film, Contamination of Pu can only be grasped by viewing. Since the digital data of the radiation and location is obtained by an IP, Pu can be detected quantitatively and radioactivity can be evaluated. As a result of this research, the image of alpha emitter on an IP is the same as that of the conventional ARG, and can be applied also to the ARG of beta and 
emitter. In measurement of Pu, the function of Image J (image-analysis software) was very available. Pu radioactivity was evaluated by an IP.
Chijimatsu, Masakazu*; Neyama, Atsushi*; Ishihara, Yoshinao*; Amemiya, Kiyoshi*; *; Iwata, Hiroshi*; Sagawa, Hiroshi*
JNC TJ8400 2002-004, 83 Pages, 2002/02
JNC-TJ8400-2002-004.pdf:0.91MB
In order to realize a coupling analysis in the near field of the geological disposal system, this study has been studied on the addition of the mass transport model to the coupled thermo-hydro-mechanical analysis code (THAMES) and preliminary coupling analysis by using development environmental tool (Diffpack) for numerical analysis. (1) In order to prepare the strategy on the addition of the mass transport model to the coupled thermo-hydro-mechanical analysis code (THAMES), we have studied on the requirement of THAMES-Transport and methodology of coupling analysis. After that we set out modification plan by the Eulerian-Lagrangian (EL) method. (2) Based on the document of modification plan, we have done addition of the mass transport model to the coupled thermo-hydro-mechanical analysis code (THAMES) and carried out verification analysis in order to confirm on the accuracy of THAMES-Transport. (3) In order to understand on the behavior of NaCl in the porewater under the coupled thermo-hydro-mechanical phenomena in the HLW engineered barrier system, we have calculated coupling phenomenon by using THAMES-Transport. Transportation and concentration phenomena of NaCl are calculated but precipitation of NaCl is not occurred under the analysis conditions in this report. (4) In order to confirm about feasibility of coupling analysis under the development environmental tool (Diffpack) for numerical analysis, we have carried out on the design work and writing program of the preliminary coupling system. In this study, we have adopted existing transport model (HYDROGEOCHEM) and geochemical model (phreeqe60) for preliminary coupling system. (5) In order to confirm program correctness of preliminary coupling system, we have carried out benchmarking analysis by using existing reactive-transport analysiscode (HYDROGEOCHEM). (6)We have been prepared short-range development plan based on through the modification study of THAMES and writing program of the preliminary coupling ...
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into Molten Pb-Bi eutecticSano, Hiroyuki*; Fujisawa, Toshiharu*; Sagawa, Yosuke*; Furukawa, Tomohiro; Aoto, Kazumi
no journal, ,
no abstracts in English
Mizuniwa, Harumi; Takasaki, Koji; Horikoshi, Yoshinori; Suzuki, Kazunori; Shioya, Satoshi; Sagawa, Naoki; Kurosawa, Shigeyuki*
no journal, ,
no abstracts in English
Sagawa, Naoki; Kurosawa, Shigeyuki*; Takasaki, Koji; Mizuniwa, Harumi
no journal, ,
no abstracts in English
Kato, Atsushi; Chikazawa, Yoshitaka; Yamano, Hidemasa; Kubo, Shigenobu; Hayafune, Hiroki; Sagawa, Hiroshi*; Okamura, Shigeki*; Nakata, Shuhei*
no journal, ,
Earthquake and Tsunami proof of the Sodium-cooled Fast Reactor (SFR) has been evaluated. As for seismic design, safety grade components are confirmed to maintain their functions even against recent strong earthquakes. As for Tsunami, in the SFR design, safety grade components are independent from component cooling water system. A gas turbine system with air cooling is adopted for emergency power supply, since the SFR does not basically require quick start-up of the emergency power supply thanks to the natural convection Decay Heat Removal System (DHRS). Even in case of long station blackout, the DHRS could be activated by emergency batteries or manually and be operated continuously by natural convection.
Suzuki, Hideya; Tsubata, Yasuhiro; Shibata, Mitsunobu; Kurosawa, Tatsuya; Kawasaki, Tomohiro; Sagawa, Hiroshi; Matsumura, Tatsuro
no journal, ,
JAEA continues to carry out the development of the ADS(Double-strata). Mutual separation of MA and Ln is important for the development of the partitioning process. The separation is particularly difficult, because they have the analogous chemical behavior. New reagent was synthesized and examined. The results of separation factors (SF) of Am against Eu are more than 25, SFAm/Cm = 5.5. The reagent is very stable chemically, high extraction capacity, fully miscible with hydrocarbon diluents, fast chemical kinetics, and following the CHON-principle.
Matsumura, Tatsuro; Suzuki, Hideya; Tsubata, Yasuhiro; Shibata, Mitsunobu; Kurosawa, Tatsuya; Kawasaki, Tomohiro; Sagawa, Hiroshi
no journal, ,
no abstracts in English
Suzuki, Hideya; Tsubata, Yasuhiro; Shibata, Mitsunobu; Kurosawa, Tatsuya; Kawasaki, Tomohiro; Sagawa, Hiroshi; Matsumura, Tatsuro
no journal, ,
JAEA continues to carry out the development of the ADS(Double-strata). Mutual separation of Am(III) and Cm(III) is important for the development of the partitioning process. The separation is particularly difficult, because they have the analogous chemical behavior. Alkyl diamide amine (ADAAM), a new high-performance reagent with a simple structure, was examined for the mutual separation of Am(III) and Cu(III). The combination of ADAAM and N,N,N',N'-tetraethyldiglycolamide (TEDGA) as a masking agent shows selectivity for Am(III) over Cm(III) in highly acidic media with separation factors up to 41.
