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Journal Articles

Interaction of solute manganese and nickel atoms with dislocation loops in iron-based alloys irradiated with 2.8 MeV Fe ions at 400 $$^{circ}$$C

Nguyen, B. V. C.*; Murakami, Kenta*; Chena, L.*; Phongsakorn, P. T.*; Chen, X.*; Hashimoto, Takashi; Hwang, T.*; Furusawa, Akinori; Suzuki, Tatsuya*

Nuclear Materials and Energy (Internet), 39, p.101639_1 - 101639_9, 2024/06

Journal Articles

Molecular geochemistry of radium; A key to understanding cation adsorption reaction on clay minerals

Yamaguchi, Akiko; Kurihara, Yuichi*; Nagata, Kojiro*; Tanaka, Kazuya; Higaki, Shogo*; Kobayashi, Toru; Tanida, Hajime; Ohara, Yoshiyuki*; Yokoyama, Keiichi; Yaita, Tsuyoshi; et al.

Journal of Colloid and Interface Science, 661, p.317 - 332, 2024/05

 Times Cited Count:0 Percentile:0.01(Chemistry, Physical)

no abstracts in English

Journal Articles

A Systematic approach for the adequacy analysis of a set of experimental databases: Application in the framework of the ATRIUM activity

Baccou, J.*; Glantz, T.*; Ghione, A.*; Sargentini, L.*; Fillion, P.*; Damblin, G.*; Sueur, R.*; Iooss, B.*; Fang, J.*; Liu, J.*; et al.

Nuclear Engineering and Design, 421, p.113035_1 - 113035_16, 2024/05

 Times Cited Count:0

Journal Articles

Comprehensive estimation of nuclide production cross sections using a phenomenological approach

Iwamoto, Hiroki; Meigo, Shinichiro; Sugihara, Kenta*

Physical Review C, 109(5), p.054610_1 - 054610_12, 2024/05

Nuclide production cross sections are crucial in nuclear research, development, space exploration, and astrophysical investigations. Despite their importance, limited experimental data availability restricts the practicality of phenomenological approaches to comprehensive cross-section estimation. To address this, we propose a Gaussian process-based machine learning (ML) model capable of transferring knowledge from elements with abundant data to those with limited or no experimental data. Our ML model not only enables comprehensive cross-section estimations for various elements but also demonstrates predictive capabilities akin to physics models, even in regions with scarce training data.

Journal Articles

Production rates of long-lived radionuclides $$^{10}$$Be and $$^{26}$$Al under direct muon-induced spallation in granite quartz and its implications for past high-energy cosmic ray fluxes

Sakurai, Hirohisa*; Kurebayashi, Yutaka*; Suzuki, Soichiro*; Horiuchi, Kazuho*; Takahashi, Yui*; Doshita, Norihiro*; Kikuchi, Satoshi*; Tokanai, Fuyuki*; Iwata, Naoyoshi*; Tajima, Yasushi*; et al.

Physical Review D, 109(10), p.102005_1 - 102005_18, 2024/05

Secular variations of galactic cosmic rays (GCRs) are inseparably associated with the galactic activities and should reflect the environments of the local galactic magnetic field, interstellar clouds, and nearby supernova remnants. The high-energy muons produced in the atmosphere by high-energy GCRs can penetrate deep underground and generate radioisotopes in the rock. As long lived radionuclides such as $$^{10}$$Be and $$^{26}$$Al have been accumulating in these rocks, concentrations of $$^{10}$$Be and $$^{26}$$Al can be used to estimate the long-term variations in high-energy muon yields, corresponding to those in the high-energy GCRs over a few million years. This study measured the production cross sections for muon induced $$^{10}$$Be and $$^{26}$$Al by irradiating positive muons with the momentum of 160 GeV/c on the synthetic silica plates and the granite core at the COMPASS experiment line in CERN SPS. In addition, it the contributions of the direct muon spallation reaction and the nuclear reactions by muon-induced particles on the production of long lived radionuclides in the rocks were clarified.

Journal Articles

Characteristics of temporal variability of long-duration bursts of high-energy radiation associated with thunderclouds on the Tibetan plateau

Tsuchiya, Harufumi; Hibino, Kinya*; Kawata, Kazumasa*; Onishi, Munehiro*; Takita, Masato*; Munakata, Kazuoki*; Kato, Chihiro*; Shimoda, Susumu*; Shi, Q.*; Wang, S.*; et al.

Progress of Earth and Planetary Science (Internet), 11, p.26_1 - 26_14, 2024/05

Journal Articles

Combining muon spin relaxation and DFT simulations of hydrogen trapping in Al$$_{6}$$Mn

Shimizu, Kazuyuki*; Nishimura, Katsuhiko*; Matsuda, Kenji*; Akamaru, Satoshi*; Nunomura, Norio*; Namiki, Takahiro*; Tsuchiya, Taiki*; Lee, S.*; Higemoto, Wataru; Tsuru, Tomohito; et al.

Scripta Materialia, 245, p.116051_1 - 116051_6, 2024/05

 Times Cited Count:0

Hydrogen at the mass ppm level causes hydrogen embrittlement in metallic materials, but it is extremely difficult to experimentally elucidate the hydrogen trapping sites. We have taken advantage of the fact that positive muons can act as light isotopes of hydrogen to study the trapping state of hydrogen in matter. Zero-field muon spin relaxation experiments and the density functional theory (DFT) calculations for hydrogen trapping energy are carried out for Al$$_{6}$$Mn. The DFT calculations for hydrogen in Al$$_{6}$$Mn have found four possible trapping sites in which the hydrogen trapping energies are 0.168 (site 1), 0.312 (site 2), 0.364 (site 3), and 0.495 (site 4) in the unit of eV/atom. Temperature variations of the deduced dipole field width ($$Delta$$) indicated step-like changes at temperatures, 94, 193, and 236 K. Considering their site densities, the observed $$Delta$$ change temperatures are interpreted by trapping muons at sites 1, 3, and 4.

Journal Articles

Determination of $$^{90}$$Sr in highly radioactive aqueous samples via conversion to a kinetically stable 1,4,7,10-tetraazacyclododecane-1,4,7,10-tetraacetic acid complex followed by concentration-separation-fractionation based on capillary electrophoresis-liquid scintillation

Ouchi, Kazuki; Haraga, Tomoko; Hirose, Kazuki*; Kurosawa, Yuika*; Sato, Yoshiyuki; Shibukawa, Masami*; Saito, Shingo*

Analytica Chimica Acta, 1298, p.342399_1 - 342399_7, 2024/04

 Times Cited Count:0

Given that conventional methods of high-dose sample analysis pose substantial exposure risks and generate large amounts of secondary radioactive waste, faster procedures allowing for decreased radiation emission are highly desirable. To address this need, we developed a $$^{90}$$Sr$$^{2+}$$ quantitation technique that is based on liquid scintillation counting-coupled capillary transient isotachophoresis (ctITP) with two-point detection and relies on the rapid concentration, separation, and fractionation of 1,4,7,10-tetraazacyclododecane-1,4,7,10-tetraacetic acid (DOTA)-complexed $$^{90}$$Sr$$^{2+}$$ in a single run. This method, which allows for the handling of high-dose radioactive specimens at the microliter level and is substantially faster than conventional ion-exchange protocols, was used to selectively quantify $$^{90}$$Sr$$^{2+}$$ in real high-dose waste. The successful concentration-separation in ctITP was ascribed to the inertness of the Sr-DOTA complex to dissociation.

Journal Articles

Evaluation of thermal neutron scattering law of nuclear-grade isotropic graphite

Nakayama, Shinsuke; Iwamoto, Osamu; Kimura, Atsushi

EPJ Web of Conferences, 294, p.07001_1 - 07001_6, 2024/04

Graphite is a candidate of moderator in innovative nuclear reactors such as molten salt reactors. Scattering of thermal neutrons by the moderator material has a significant impact on the reactor core design. To contribute to the development of innovative nuclear reactors, an evaluation method of thermal neutron scattering law for reactor grade graphite was studied. The inelastic scattering component due to lattice vibration was evaluated based on the phonon density of states computed with first-principles lattice dynamics simulations. The simulations were performed for ideal crystalline graphite. The coherent elastic scattering component due to crystal structure was evaluated based on neutron transmission and scattering experiments recently performed in the J-PARC/MLF facility. In comparison with the neutron transmission experiments, it was found that the quantification of small-angle neutron scattering due to structures larger than crystal, such as pores in graphite, is important. Based on the above methods, thermal neutron scattering law data for reactor-grade graphite at room temperature were evaluated.

Journal Articles

Total and double differential scattering cross-section measurements of isotropic graphite

Kimura, Atsushi; Endo, Shunsuke; Nakamura, Shoji

EPJ Web of Conferences, 294, p.01002_1 - 01002_7, 2024/04

Journal Articles

Impact of irradiation side on muon-induced single-event upsets in 65-nm Bulk SRAMs

Deng, Y.*; Watanabe, Yukinobu*; Manabe, Seiya*; Liao, W.*; Hashimoto, Masanori*; Abe, Shinichiro; Tampo, Motonobu*; Miyake, Yasuhiro*

IEEE Transactions on Nuclear Science, 71(4), p.912 - 920, 2024/04

With the miniaturization of semiconductors and the decrease in operating voltage, there is a growing interest and discussion in whether the muons in cosmic rays may be the source of single event upsets (SEUs). In the case of neutron-induced SEUs, it was reported that the irradiation side has the impact on SEU cross sections. Here, to investigate the impact of irradiation direction on muon-induced SEUs, we have measured and simulate muon-induced SEUs in 65-nm bulk SRAMs with different muon irradiation directions. It was found that the peak SEU cross section for the package side irradiation is about twice large as that for the board side irradiation. We also revealed that the difference in observed SEU cross sections between the package side and the board side irradiation is caused by differences in energy straggling due to changes in penetration depth depending on the incident direction.

Journal Articles

Estimating the corrosion rate of stainless steel R-SUS304ULC in nitric acid media under concentrating operation

Irisawa, Eriko; Kato, Chiaki

Journal of Nuclear Materials, 591, p.154914_1 - 154914_10, 2024/04

 Times Cited Count:0 Percentile:0.08(Materials Science, Multidisciplinary)

The amount of corrosion of austenitic stainless-steel R-SUS304ULC was evaluated considering the changes in solution composition and boiling during actual concentration operations. Austenitic stainless-steel R-SUS304ULC is the structural material of the highly radioactive liquid waste concentrator in Japanese spent fuel reprocessing plant, which treats highly corrosive nitric acid solutions during enrichment operations. The study results show that it is necessary to focus on nitric acid concentrations, oxidizing metal ion concentrations, and decompression boiling as factors that accelerate the corrosion rate of stainless steel because of cathodic reaction activation.

Journal Articles

Generation and verification of ORIGEN and ORIGEN-S activation cross-section libraries of JENDL-5 and JENDL/AD-2017

Konno, Chikara; Kochiyama, Mami; Hayashi, Hirokazu

Mechanical Engineering Journal (Internet), 11(2), p.23-00386_1 - 23-00386_11, 2024/04

Activation cross-section libraries for the ORIGEN and ORIGEN-S codes have been generated from JENDL-5 and JENDL/AD-2017. The ORIGEN activation cross-section libraries of the 200 and 48 group structures were generated with the AMPX-6 code, while the ORIGEN-S activation cross-section libraries with a MAXS format of the 199 group structure were done with the PREPO2018 code. Activation calculations for JPDR were carried out in order to validate the produced ORIGEN and ORIGEN-S activation cross-section libraries. The following comparisons were performed: the ORIGEN calculation results with the produced activation cross-section libraries and bundled ones, the 200 group and 48 group ORIGEN calculations, the ORIGEN and ORIGEN-S calculations with the JENDL-5 activation cross-section libraries, etc. Most of the differences of the calculation results were less than 20%, which demonstrated that the libraries were produced adequately.

Journal Articles

Stochastic ray tracing for Fresnel diffraction

Seto, Keita

Optics Express (Internet), 32(10), p.16999 - 17011, 2024/04

Journal Articles

Spin dependence in the $$p$$-wave resonance of $$^{139}$$$overrightarrow{textrm{La}}$+$overrightarrow{n}$

Okudaira, Takuya*; Nakabe, Rintaro*; Auton, C. J.*; Endo, Shunsuke; Fujioka, Hiroyuki*; Gudkov, V.*; Ide, Ikuo*; Ino, Takashi*; Ishikado, Motoyuki*; Kambara, Wataru*; et al.

Physical Review C, 109(4), p.044606_1 - 044606_9, 2024/04

Journal Articles

High sensitivity of a future search for effects of $$P$$-odd/$$T$$-odd interactions on the 0.75 eV $$p$$-wave resonance in $$overrightarrow{n}$$+$$^{139}overrightarrow{textrm{La}}$$ forward transmission determined using a pulsed neutron beam

Nakabe, Rintaro*; Auton, C. J.*; Endo, Shunsuke; Fujioka, Hiroyuki*; Gudkov, V.*; Hirota, Katsuya*; Ide, Ikuo*; Ino, Takashi*; Ishikado, Motoyuki*; Kambara, Wataru*; et al.

Physical Review C, 109(4), p.L041602_1 - L041602_4, 2024/04

JAEA Reports

Utilization of gamma ray irradiation at the WASTEF Facility

Sano, Naruto; Yamashita, Naoki; Watanabe, Masaya; Tsukada, Manabu*; Hoshino, Kazutoyo*; Hirai, Koki; Ikegami, Yuta*; Tashiro, Shinsuke; Yoshida, Ryoichiro; Hatakeyama, Yuichi; et al.

JAEA-Technology 2023-029, 36 Pages, 2024/03

JAEA-Technology-2023-029.pdf:2.47MB

At the Waste Safety Testing Facility (WASTEF), the gamma ray irradiation device "Gamma Cell 220" was relocated from the 4th research building of the Nuclear Science Research Institute in FY2019, and the use of gamma ray irradiation has begun. Initially, Fuel Cycle Safety Research Group, Fuel Cycle Safety Research Division, Nuclear Safety Research Center, Sector of Nuclear Safety Research and Emergency Preparedness, the owner of this device, conducted the tests as the main user, but since 2022, other users, including those outside the organization, have started using it. The gamma ray irradiation device "Gamma Cell 220" is manufactured by Nordion International Inc. in Canada. Since it was purchased in 1989, the built-in 60Co radiation source has been updated once, and safety research related to nuclear fuel cycles, etc. It is still used for this purpose to this day. This report summarizes the equipment overview of the gamma ray irradiation device "Gamma Cell 220", its permits and licenses at WASTEF, usage status, maintenance and inspection, and future prospects.

JAEA Reports

Development of an electrochemical measurement method for carbon steels in radiation source dissolved solution and a corroded specimen analysis method using an imaging plate

Yamashita, Naoki; Aoyama, Takahito; Kato, Chiaki; Sano, Naruto; Tagami, Susumu

JAEA-Technology 2023-028, 22 Pages, 2024/03

JAEA-Technology-2023-028.pdf:1.9MB

At the Fukushima Daiichi Nuclear Power Station (1F), which is currently undergoing decommissioning, there is growing interest in the effects of radiation-emitting radionuclides such as $$^{90}$$Sr and $$^{137}$$Cs on the structural integrity. In particular, the corrosion behavior of carbon steel, which is used in many parts of 1F, is known to change depending on metal cations in solution, but the effects of $$^{90}$$Sr and $$^{137}$$Cs on corrosion are not yet understood. In addition, it is important to investigate the distribution of $$^{90}$$Sr and $$^{137}$$Cs in the rust layer in order to understand the corrosion behavior, but the method has not yet been established. In this study, a glove box was prepared to conduct corrosion tests of carbon steel in NaCl containing $$^{90}$$Sr and $$^{137}$$Cs in the glove box. In addition, in order to clarify the influence of $$^{90}$$Sr and $$^{137}$$Cs, which exist as metal cations in the solution, on the corrosion behavior of carbon steel, we attempted to establish a detection method for radioactive materials in the rust layer using an imaging plate.

Journal Articles

Application of transition-edge sensors for micro-X-ray fluorescence measurements and micro-X-ray absorption near edge structure spectroscopy; a case study of uranium speciation in biotite obtained from a uranium mine

Yomogida, Takumi; Hashimoto, Tadashi; Okumura, Takuma*; Yamada, Shinya*; Tatsuno, Hideyuki*; Noda, Hirofumi*; Hayakawa, Ryota*; Okada, Shinji*; Takatori, Sayuri*; Isobe, Tadaaki*; et al.

Analyst, 149(10), p.2932 - 2941, 2024/03

In this study, we successfully applied a transition-edge sensor (TES) spectrometer as a detector for microbeam X-ray measurements from a synchrotron X-ray light source to determine uranium (U) distribution at the micro-scale and its chemical species in biotite obtained from the U mine. It is difficult to separate the fluorescent X-ray of the U L$$alpha$$$$_{1}$$ line at 13.615 keV from that of the Rb K$$alpha$$ line at 13.395 keV in the X-ray fluorescence spectrum with an energy resolution of approximately 220 eV of the conventional silicon drift detector (SDD). Meanwhile, the fluorescent X-rays of U L$$alpha$$$$_{1}$$ and Rb K$$alpha$$ were fully separated by TES with 50 eV energy resolution at the energy of around 13 keV. The successful peak separation by TES led to an accurate mapping analysis of trace U in micro-X-ray fluorescence measurements and a decrease in the signal-to-background ratio in micro-X-ray absorption near edge structure spectroscopy.

Journal Articles

Studies on complex reactions of actinides in solution and development of analytical methods for small amounts of samples

Ouchi, Kazuki

Hosha Kagaku, (49), p.3 - 7, 2024/03

I introduce the elucidation of the deposition following the oxidation state of uranium and the electrochemical behavior of uranium(IV) chloride in an ionic liquid-organic mixture, as a basic study of in-solution reactions. In addition, I introduce the development of separation methods for actinides using a microchemical chip and polyacrylamide gel electrophoresis, as an applied study for quantitative analytical methods for small amounts of samples.

12036 (Records 1-20 displayed on this page)