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Report No.
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Experimental study on U-Pu cocrystallization reprocessing process

Shibata, Atsuhiro ; Oyama, Koichi; Yano, Kimihiko ; Nomura, Kazunori ; Koyama, Tomozo; Nakamura, Kazuhito; Kikuchi, Toshiaki*; Homma, Shunji*

A new reprocessing system with 2-stage crystallization process has been developed. In the first stage of the system, U and Pu are recovered from dissolver solution by U-Pu co-crystallization. Laboratory scale experiments were carried out with U and Pu mixed solution and irradiated fuel dissolver solution to obtain fundamental data on U-Pu co-crystallization process. Pu co-crystallized with U, but crystallization yields of Pu were lower than those of U. FPs were separated from U and Pu by co-crystallization, and decontamination factors of Cs and Eu to U in crystal were over 100.

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Category:Nuclear Science & Technology

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