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$$gamma$$ radiolysis of an extractant for minor actinides, Hexaoctyl-nitrilotriacetamide (HONTA), in dodecane diluent

Toigawa, Tomohiro   ; Suzuki, Hideya; Ban, Yasutoshi  ; Ishii, Sho*; Matsumura, Tatsuro  

Radiolytic stability of an extractant, N,N,N',N',N'',N''-hexaoctyl-nitrilotriacetamide (HONTA), for separation between minor actinides and rare-earth elements were investigated by using $$gamma$$-ray emitting from cobalt-60. Degradation amount of HONTA and its products yields were obtained by gas chromatographic analysis. Our results showed the cleavage sites in HONTA radiolysis and suggested that the radiolysis of HONTA was ruled by different mechanism depending on the absorbed dose.

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