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Feasibility study of technology for Pu solution monitoring including FP; Development of gamma spectra detector for high active liquid waste

FPを含むPu溶液モニタリング技術のための適用性調査研究; 高放射性溶液用ガンマスペクトル検出器の開発

関根 恵; 松木 拓也; 所 颯; 蔦木 浩一; 北尾 貴彦; 中村 仁宣; 富川 裕文

Sekine, Megumi; Matsuki, Takuya; Tokoro, Hayate; Tsutagi, Koichi; Kitao, Takahiko; Nakamura, Hironobu; Tomikawa, Hirofumi

再処理施設においては、プルトニウム(Pu)モニタリングのさらなる適用拡大を図るため、核分裂生成物(FP)を含むPu溶液中のPu量を測定可能な検出器開発が必要である。Puモニタリングに適用可能な$$gamma$$線を調べるため、高線量下、広範囲のエネルギーが測定可能かつ高い分解能を持つCe:GAGG (Ce:Gd$$_{3}$$Al$$_{2}$$Ga$$_{3}$$O$$_{12}$$)シンチレータを装備した検出器(対象:高放射性廃液)を新たに設計・開発した。その検出器を用いて東海再処理施設の高放射性廃液のコンクリートセル内で、同廃液に対し800keV以上の$$gamma$$線スペクトル測定を実施したところ、Eu-154由来と考えられるピークを検出した。この測定結果は、中性子の測定結果とMCNPシミュレーションを組み合わせ、Puモニタリング技術開発へ適用していく。本発表では、検出器の選定,設計、$$gamma$$線スペクトル測定結果、Puモニタリングへの適用性評価について報告する。本技術開発は、文部科学省核セキュリティ補助金事業の一環として実施している。

In a reprocessing facility, it is necessary to develop a detector which can measure plutonium (Pu) content in the Pu solutions containing fission products (FP) in order to expand the application of Pu monitoring. In order to establish this technology, JAEA has studied a system measure $$gamma$$-rays was utilized since it applicable for Pu monitoring. Ce:GAGG (Ce:Gd$$_{3}$$Al$$_{2}$$Ga$$_{3}$$O$$_{12}$$) scintillator detector can measure a wide energy range in a high-dose environment and has reasonable resolution. $$gamma$$-ray measurements were performed inside of the concrete cell containing the High Active Liquid Waste tank at the Tokai reprocessing plant. In the spectra, the two significant peaks were measured by the GAGG above 800 keV and were considered to be from Eu-154. There $$gamma$$-ray measurements will be combined with previous neutron measurements and both will be compared to MCNP models for future Pu monitoring technology. This presentation will describe the detector selection, the design system, the results of $$gamma$$-ray spectral measurements and the applicability for Pu monitoring. This project has been carried out under the support of the Ministry of Education, Culture, Sports, Science and Technology (MEXT) of the Japanese government.

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