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Report No.

Development of ${it spatiotemporal}$ measurement and analysis techniques in X-ray photoelectron spectroscopy; From NAP-HARPES to 4D-XPS

Toyoda, Satoshi*; Yamamoto, Tomoki*; Yoshimura, Masashi*; Sumida, Hirosuke*; Mineoi, Susumu*; Machida, Masatake*; Yoshigoe, Akitaka ; Suzuki, Satoru*; Yokoyama, Kazushi*; Ohashi, Yuji*; Kurosawa, Shunsuke*; Kamada, Kei*; Sato, Hiroki*; Yamaji, Akihiro*; Yoshino, Masao*; Hanada, Takashi*; Yokota, Yui*; Yoshikawa, Akira*

We have developed ${it spatiotemporal}$ measurement and analysis techniques in X-ray photoelectron spectroscopy. To begin with, time-division depth profiles of gate stacked film interfaces have been achieved by NAP-HARPES (Near Ambient Pressure Hard X-ray Angle-Resolved Photo Emission Spectroscopy) data. We then have promoted our methods to quickly perform peak fittings and depth profiling from time-division ARPES data, which enables us to realize 4D-XPS analysis. It is found that the traditional maximum entropy method (MEM) combined with Jackknife averaging of sparse modeling in NAP-HARPES data is effective to perform dynamic measurement of depth profiles with high precision.



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