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JAEA Reports

Procedure on confirmation of completion of decommissioning of nuclear facilities (Contract research)

Shimada, Taro; Shimada, Asako; Miwa, Kazuji*; Nabekura, Nobuhide*; Sasaki, Toshihisa*; Takai, Shizuka; Takeda, Seiji

JAEA-Research 2024-004, 115 Pages, 2024/06

JAEA-Research-2024-004.pdf:6.02MB

We have studied the confirmation method for the termination of decommissioning of nuclear facilities based on the site release flow presented at the Nuclear Regulation Authority (NRA) study team meeting in 2017, and organized it as a procedure for the site soil. First, the effects of radionuclides released by the Fukushima Daiichi Nuclear Power Station accident are excluded as background radioactivity, and the distribution of radioactivity concentration of facility origin on the site is evaluated using geostatistical method kriging. Then, considering the downstream transport of sediment by surface runoff generated by rainfall that exceeds the infiltration capacity of the ground surface, a series of evaluation procedures are presented to evaluate the exposure dose reflecting future changes from the evaluated radioactivity concentration distribution, and a comparison method with the assumed 0.01 mSv/y as a dose criterion is proposed. Furthermore, an example of the procedure for evaluating the distribution of contamination in the subsurface was also presented for the case where groundwater is affected.

Journal Articles

Development of risk assessment code for dismantling of radioactive components in decommissioning stage of nuclear reactor facilities

Shimada, Taro; Sasagawa, Tsuyoshi; Miwa, Kazuji; Takai, Shizuka; Takeda, Seiji

Proceedings of International Conference on Environmental Remediation and Radioactive Waste Management (ICEM2023) (Internet), 7 Pages, 2023/10

Nuclear regulatory inspection should be performed on the basis of the risk information during the decommissioning phase of the nuclear power plant. However, it is difficult because the methodology for quantitatively assessing the radiation exposure risk during decommissioning activities has not been established. Therefore, a decommissioning risk assessment code, DecAssess-R, has been developed based on the decommissioning safety assessment code, DecAssess, which creates event trees from initiating events and evaluates the radiation risk resulting from public exposure dose for each accident sequence. The assessment took into account that mobile radioactive inventories that can be easily dispersed in the work area, such as radioactive dust accumulated in HEPA filters attached to a contamination control enclosure, will fluctuate with the progress of the decommissioning work. Initiating events were selected based on the investigation of accidents and malfunctions during dismantling, disassembly, and component replacement activities around the world, and event trees were created from the initiating events to indicate the progress scenario. The frequencies of occurrence were determined with reference to general industry data in addition to the above accidents and malfunctions, and the probabilities of event progression were determined with reference to failure data during the operation phase. The exposure risks during dismantling of components in the reference BWR were evaluated. As a result, the public exposure dose was maximum in case of fire during dismantling of reactor internals and fire spread to combustibles and filters, including radioactivity temporarily stored in the work area. The exposure risk was also maximum because the probability of occurrence of this accident sequence was greater than that of other scenarios.

Journal Articles

Laboratory experiment on runoff of particles deposited on land surface by rainfall at accidents in the decommissioning stage

Shimada, Taro; Namekawa, Masakazu*; Miwa, Kazuji; Takeda, Seiji

Proceedings of Waste Management Symposia 2023 (WM2023) (Internet), 8 Pages, 2023/02

It is supposed that radioactive dust deposited at the land surface will be moved downstream and concentrated at the depression by overland flow at heavy rain after the accidental release of radioactive dusts accumulated at the filters in the decommissioning stage of nuclear facilities. The authors are developing a calculation code to evaluate distribution changes of radioactivity on the surface and public dose considering the conditions such as rainfall, topography and types of cover surface. It is necessary to construct methods for setting parameter values used for the calculations based on the actual situation. Therefore, the parameter values were obtained by the experiments where Fe$$_3$$O$$_4$$ powder spread on the cover surface such as smooth and aged-asphalt, concrete and bare soil, was eroded by overland flow and raindrops and they were collected at the lower end of the slope at a minute interval. The collected weights of overland flow and Fe$$_3$$O$$_4$$ powder were measured. Based on the Manning's roughness coefficient for smooth asphalt already known as a fixed value, the erosion velocity coefficient was evaluated. Then Manning's roughness coefficients for other cover surfaces were obtained using the erosion velocity coefficient. Manning's roughness coefficients were slightly smaller than the range of literature values. In addition, elevations for the cover surface were measured by 3D scanner as point cloud data, and the surface roughness were evaluated. The values of surface roughness and Manning's roughness coefficients had a correlation. It indicated a possibility to utilize the surface roughness to set the Manning's roughness coefficient for the evaluation of radioactivity distribution change by heavy rainfall.

Journal Articles

Development of dose evaluation method considering radionuclides migration on the surface of the site for confirmation of completion of decommissioning

Miwa, Kazuji; Namekawa, Masakazu*; Shimada, Taro; Takeda, Seiji

MRS Advances (Internet), 7(7-8), p.165 - 169, 2022/03

We have developed evaluation method of radiocesium (RCs) migration by surface runoff and soil erosion in considering vertical distribution of RCs in initial contaminated soil and concentration of RCs in different particle size. RCs migration on ground surface during single year has been evaluated in virtual site contaminated uniformly by Cs-137. As a result, RCs has concentrated in the impoundment, and 0.18% of total inventory in the site migrated into the sea. These results suggest that surface migration of RCs effects increasing of external exposure at impoundment and internal exposure from ingestion of marine product.

Journal Articles

Vertical distributions of Iodine-129 and iodide in the Chukchi Sea and Bering Sea

Miwa, Kazuji; Obata, Hajime*; Suzuki, Takashi

Journal of Nuclear Science and Technology, 57(5), p.537 - 545, 2020/05

 Times Cited Count:2 Percentile:20.94(Nuclear Science & Technology)

This study investigated the vertical distribution of Iodine-129 ($$^{129}$$I) which is mainly produced by European nuclear reprocessing plants in the Chukchi Sea and Bering Sea. $$^{129}$$I was found to be distributed almost uniformly in fallout level, and an increasing in $$^{129}$$I concentration levels caused by high $$^{129}$$I water inflow from the Atlantic Ocean was not observed. Additionally, we revealed the vertical distribution of iodide, one chemical form of iodine, from the Bering Shelf area to the Chukchi Sea for the first time. The increasing tendency of iodide near sea bottom was observed.

Journal Articles

Development of dose estimation system integrating sediment model for recycling radiocesium-contaminated soil to coastal reclamation

Miwa, Kazuji; Takeda, Seiji; Iimoto, Takeshi*

Radiation Protection Dosimetry, 184(3-4), p.372 - 375, 2019/10

 Times Cited Count:0 Percentile:0.01(Environmental Sciences)

The Ministry of the Environment has indicated the policy of recycling the contaminated soil generated by decontamination activity after the Fukushima accident. By recycling to coastal reclamation which is one of effective recycling application, dissolved radiocesium and absorbed radiocesium on soil particles will flow out to the ocean by construction, therefore evaluating radiocesium transition in ocean considering the both types of radiocesium is important for safety assessment. In this study, the radiocesium outflow during constructing and after constructing is modeled, and radiocesium transition in ocean is evaluated by Sediment model suggested in OECD/NEA. The adaptability of sediment model is confirmed by reproducing evaluation of the coastal area of Fukushima. We incorporate the sediment model to PASCLR2 code system to evaluate the doses from radiocesium in ocean.

Journal Articles

Student and Young researcher's view of research on health physics and environment science

Miwa, Kazuji; Terasaka, Yuta; Ochi, Kotaro; Futemma, Akira; Sasaki, Miyuki; Hirouchi, Jun

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 61(9), p.687 - 691, 2019/09

This report summarizes the contents of the session of the Health Physics and Environment Science Division, which was held in Atomic Energy Society of Japan 2019 Spring Meeting. In this session, six students and young researchers who engaged in the field of nuclear energy and radiation gave a lecture about health physics and environmental science research through their expertise. After the all presentations end, we took discussion time about the issues and future development in this field with all attendees. In this report, we summarized each lecture outline and discussion contents.

Journal Articles

Current status and issues for clearance, 5; Concept of restricted use of contaminated rubbles in the Fukushima Daiichi NPS

Shimada, Taro; Miwa, Kazuji; Takeda, Seiji

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 61(7), p.531 - 534, 2019/07

Rubbles less than 5 $$mu$$Sv/h of surface dose rate, which are stored outdoor in the Fukushima Daiichi NPS (1F) site, will be recycled and applied in a restricted reuse only within 1F site in the future. However, there is no precedent for establishing the reference values such as dose and/or concentration for reuse or recycling under the existing exposure situation. In this study, we suggested a concept for establishing the reference radioactive concentration of recycling material for the restricted use in the 1F site. In addition, based on the concept, we calculated the reference radiocesium concentrations of the recycling material used for paved roads and the bases of concrete building.

Journal Articles

Joint meeting of young researchers in the field of radiation protection and radiation biology

Kataoka, Noriaki*; Nakajima, Junya; Miwa, Kazuji; Hirota, Seiko*; Tsubota, Yoichi; Yamada, Ryohei; Fujimichi, Yuki*; Ishikawa, Junya*; Sunaoshi, Masaaki*

Hoken Butsuri (Internet), 54(2), p.140 - 145, 2019/06

It is the written report of the joint meeting of young researchers in the field of radiation protection and radiation biology.

Journal Articles

Study on restricted use of contaminated rubble on Fukushima Daiichi NPS site, 1; Estimation of reference radiocesium concentration for recycling materials

Shimada, Taro; Miwa, Kazuji; Takeda, Seiji

Progress in Nuclear Science and Technology (Internet), 6, p.203 - 207, 2019/01

Rubbles less than 5 $$mu$$Sv/h of surface dose rate, which are stored outdoor in the Fukushima Daiichi NPS (1F) site, will be recycled and applied in a restricted reuse only within 1F site in the future. In this study, we suggested a concept for establishing the reference radioactive concentration of recycling material for the restricted use in the 1F site. Reference radiocesium concentration is calculated so that increased dose rate by restricted reuse does not exceed 1 $$mu$$Sv/h which is the minimum value of dose rate map in the 1F entire site. In order to justify the restricted reuse under the reference concentration calculated, additional occupational dose, dose rate at the site boundary and groundwater concentration at the outlet to the ocean are evaluated and confirmed that the values are below 2 mSv/y, 1 mSv/y and 1 Bq/cm$$^{3}$$ of $$^{134}$$Cs and $$^{137}$$Cs, respectively. And then calculated the reference radiocesium concentrations of the recycling material used for paved roads and the bases of concrete building.

Journal Articles

Study on restricted use of contaminated rubble on Fukushima Daiichi NPS site, 2; Validation of reference radiocesium concentration for recycling materials

Miwa, Kazuji; Shimada, Taro; Takeda, Seiji

Progress in Nuclear Science and Technology (Internet), 6, p.166 - 170, 2019/01

In this study, in order to validate the restricted use of recycling material at the reference radiocesium concentration (determined in series report (1)), we evaluated worker annual doses, air dose rate at the site boundary and impact of migrated radiocesium into groundwater. Firstly, we evaluated the additional annual dose for workers, on the assumption that typical workers coming in contact with the source after construction (Road: 1.2 mSv/y, Building: 1.3 mSv/y). Secondly, we evaluated the air dose rates by distance from road and building including recycling material, and investigated the distance for not exceeding 1 mSv/y (including additional dose rate by recycling and background dose rate of 0.6 mSv/y) at the site boundary (Road: 25 m, Building: 1 m). Thirdly, we evaluated the Cs migration in groundwater, and investigated the distance required for satisfying the operation target value ($$^{134}$$Cs: 1 Bq/L, $$^{137}$$Cs: 1 Bq/L) at the boundary (coastal line) (Road: 10 m, Building: 10 m).

Oral presentation

Development of dose evaluation method for confirmation of completion of decommissioning, 3; Development of dose estimation method considering changes in surface soil contamination distribution

Miwa, Kazuji; Namekawa, Masakazu*; Shimada, Taro; Takeda, Seiji

no journal, , 

The distribution of surface soil contamination on the site of nuclear facilities after confirmation of the decommissioning may be changed by rainfall. In this study, the radionuclides migration model is developed to evaluate the radiation dose to the public including radionuclides distribution change. The result of radionuclides migration estimation on virtual site condition suggests that radionuclides which is migrated by surface water and soil migration gather in depression area. It is also shown that radionuclides migration on surface is more significant path to the ocean than radionuclides migration in groundwater. Based on these findings, it is suggested that the radiation dose considering change of radionuclides distribution may be larger than that from initial radionuclides distribution.

Oral presentation

Radiation protection perspectives needed for discussions of recycling radionuclides contaminated materials

Miwa, Kazuji

no journal, , 

There are large amount of radionuclides contaminated soil and debris in Fukushima Prefecture after Fukushima Daiichi Nuclear Power Station accident. It is difficult to dispose the entire amount of soil and debris as radioactive waste from the view point of preparing the disposal site. Therefore, we focused on the recycling as one of the way to reduce the quantity of the radionuclides contaminated materials. In this study, we organised the issues when assuming recycling in the current concept of radiation protection, and propose the way of applying the concept of radiation protection to the regulation in the field. Specifically, we proposed five ways of applying the reference level in radiation protection from radionuclides contaminated material in existing exposure situation. In addition, we calculated radionuclides concentrations for two model case of recycling applying proposed radiation protection concept.

Oral presentation

Development of dose evaluation method for confirmation of completion of decommissioning, 1; Development of radioactivity distribution evaluation combined with scoping survey and sampling measurement

Shimada, Taro; Nabekura, Nobuhide*; Miwa, Kazuji; Takeda, Seiji

no journal, , 

It is necessary for confirmation of completion of decommissioning of nuclear facilities to comply with dose criteria for public using the land after site release, based on the radioactivity distribution at the land of the site. We are developing a methodology of public dose evaluation based on the survey results of evaluation of the radioactivity distribution. In this report, the external drift kriging method combined with scoping survey and sampling measurement were applied to 1km square area, and a cross validation method was applied to validate the evaluated distribution. Index of Mean Absolute Error is appropriate to evaluate the difference between evaluation and measurement. In addition, upper limit of 95% single side confidence interval for the evaluation of non-measured point was suggested to input for dose evaluation.

Oral presentation

Development of dose evaluation method for confirmation of completion of decommissioning, 1; Study on validation method for evaluated radioactivity distribution

Shimada, Taro; Miwa, Kazuji; Sasaki, Toshihisa*; Takeda, Seiji

no journal, , 

The authors are developing a methodology for confirming that public dose using the site after site release will be in compliance with the dose criteria based on the radioactivity distribution at the termination of the decommissioning of nuclear facilities. In a previous study, it was confirmed that kriging with external drift combined with scoping survey and representative measurement could evaluate the radioactivity distribution. However, the issue that evaluated distribution should be validated from the viewpoint of sufficiency on points of representative measurement remained. Therefore, we developed the method for the validation, that mean absolute error (MAE) between each measured value and evaluated value is less than a reference value of MAE between an average of measured values and each measured value. The method was applied to supposed distributions and it was confirmed that some of the evaluated distributions were validated.

Oral presentation

Development of risk assessment methodology for nuclear power plants in decommissioning phase, 1; Overview of risk assessment and selection of initiating events

Shimada, Taro; Sasagawa, Tsuyoshi; Miwa, Kazuji; Takai, Shizuka; Takeda, Seiji

no journal, , 

It is necessary to develop the methodology for risk assessment during decommissioning so as to select the components or tasks based on the risk-informed at the nuclear regulation inspection. The characteristic is that the radioactive contamination that may be released in the event of an accident fluctuates spatially and temporally as the dismantling work progresses. We have started to construct a methodology for the risk assessment in decommissioning phase. And an outline of risk assessment based on the characteristics of the dismantling work was created. The risk is defined as the product of exposure dose and frequency in this study. As a result of investigating cases of decommissioning and similar trouble events during periodic inspection work, many cases related to fire during cutting work at dismantling were found. Based on the results, quality engineering methods such as FMEA (Failure Mode and Effects Analysis) were used to select the initiating events due to human error. In addition, event trees were created assuming that the events progress due to the failure of mitigation measures for those initiating events.

Oral presentation

Estimation of radionuclide migration considering sorption to suspended particles and soil near spring water points in a coastal zone

Sawaguchi, Takuma; Miwa, Kazuji*; Shimada, Taro; Takeda, Seiji

no journal, , 

In the previous dose assessment for the radioactive waste disposal, the dissolved radionuclides leaking from the repository were assumed to flow directly into the living environment (ocean, lake, river, etc.) through natural barriers. However, based on the knowledge after the Fukushima Daiichi Nuclear Power Plant accident, it was considered that radionuclides via groundwater could sorb and desorb with soil near spring water points, and that radiocesium was mainly transferred as sorbed to suspended particles in the living environment. In this study, in order to contribute to the dose assessment for intermediate-depth disposal, we analytically understood the influence on the migration in the living environment with or without consideration of the nuclide sorption on the seabed soil during spring water inflow into a coastal zone. In addition, the effects were also evaluated for the presence or absence of the nuclide sorption/desorption on suspended particles and the particle sedimentation. As a result, the radioactivity concentrations in seabed soil and seawater immediately above the seabed were higher in the estimate that considered the sorption/desorption and the sedimentation than in the estimate that did not. These results indicate that it is important to consider the radionuclide sorption on the seabed soil and the migration of radionuclides sorbed on suspended particles in the estimation of radionuclide migration in the living environment because these phenomena could cause the increase of radionuclide concentrations in the interface layer and the seabed soil and the higher exposure due to benthic fish and shellfish ingestion, etc.

Oral presentation

Distribution and source of I-129 in Chukchi Sea and Bering Sea

Miwa, Kazuji; Obata, Hajime*; Suzuki, Takashi; Otosaka, Shigeyoshi

no journal, , 

I-129 in a global environment is originated from the European nuclear fuel reprocessing plants (NFRP), Sellafield in U.K. and La Hague in France, and it is observed a large amount of I-129 inflows from European NFRP into the eastern and central Arctic Ocean. Previous studies on I-129 at surface indicated seawater with high I-129 concentration does not inflow from eastern and central Arctic Ocean to Chukchi Sea, located in western Arctic Ocean. However, there is a possibility of inflow of I-129 because the vertical distribution of I-129 has not observed at the ocean. The purpose of this study is to identify the inflow of seawater with high I-129 concentration from eastern and central Arctic Ocean by observing the vertical distribution of I-129 and water mass structure in Chukchi Sea and Bering Sea. Seawater with high temperature at surface of southern Chukchi Sea (- 66$$^{circ}$$N) and with low temperature at bottom of the northern Chukchi Sea (69$$^{circ}$$N -) were observed. The seawater with low temperature might include high I-129 concentration. However, I-129 concentration in some points was observed ranging from 0.79 to 2.89 (10$$^{7}$$ atoms/L), which was two orders of magnitude lower than that in the eastern and central Arctic Ocean. And no significant difference of I-129 concentration between seawater at surface and at bottom was shown. Therefore, we could not identify the inflow of seawater with high I-129 concentration from eastern and central Arctic Ocean to Chukchi Sea.

Oral presentation

Development of exposure risk assessment code at decommissioning stage of nuclear power station, DecAssess-R

Shimada, Taro; Miwa, Kazuji; Sasagawa, Tsuyoshi; Takai, Shizuka; Takeda, Seiji

no journal, , 

For risk-informed implementation of nuclear regulatory inspections during the decommissioning phase of nuclear power plants, we are developing DecAssess-R, a code that evaluates changes in exposure risk over time according to the decommissioning process based on exposure dose and occurrence probability by accident sequence for each component to be dismantled. Event trees have been constructed from the initiating events that occurred during the decommissioning phase, and the occurrence frequency and accident progress probability of the events have been developed from past trouble cases. Using the developed risk assessment method, we evaluated the exposure risks due to fire as an example of dismantling of a 1.1 MW BWR in the United States. As a result, it was confirmed that the method can provide risk information according to the decommissioning process, not only the quantity of the residual radioactivity inventory, such as the result that the exposure risk is larger for a fire that occurs during air dismantling of peripheral equipment in the reactor building, which has a smaller radioactivity inventory, than for a fire that occurs during underwater dismantling of in-core structures, which has a larger radioactivity inventory. The results confirmed that the information on the risk according to the decommissioning process can be provided.

Oral presentation

Iodine speciation and iodine-129 distribution in the Chukchi Sea and Bering Sea

Obata, Hajime*; Miwa, Kazuji*; Kondo, Yoshiko*; Gamo, Toshitaka*; Otosaka, Shigeyoshi; Suzuki, Takashi

no journal, , 

Distributions chemical species of iodine (iodide, iodate and organic iodine) in seawater were investigated in the Chukchi Sea and Bering Sea, Arctic northern marginal seas. $$^{129}$$I, which is a good tracer for anthropogenically released iodine to the marine environments, were also revealed by this study. Iodide concentrations in seawater often increased toward the seafloor. This tendency was remarkable with iodide and organic iodine, indicating that these iodine species are released from the sediments of the continental shelf. Concentrations of $$^{129}$$I ranged from 0.79 to 2.89$$times$$10$$^{7}$$ atom/L. While this level was several times higher than those in the North Pacific, significant increase of $$^{129}$$I concentration due to seawater inflow from the North Atlantic was not observed. Considering latitudinal range of this study area, it can be estimated that most $$^{129}$$I detected by this study was derived by atmospheric deposition of $$^{129}$$I originates from Europe.

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