Study on microwave power dependency of electron spin resonance spectrum of carbonate radicals in teeth

Iwami, Satone*; Yamashita, Takuma*; Mitsuyasu, Yusuke*; Ono, Kenta*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.

KEK Proceedings 2024-6, p.91 - 95, 2024/12

We aim to improve the detection limit of the ESR dosimetry method. In this study, the saturation behavior of each radical was investigated by varying the microwave power during ESR measurement. Based on the difference in spin relaxation time between carbonate radicals and native radicals, it is expected that the signal-to-noise ratio improves and the detection limit can be lowered when the microwave power is increased to 4.0 mW.

Measurement of the longitudinal bunch-shape distribution for a high-intensity negative hydrogen ion beam in the low-energy region

Kitamura, Ryo; Futatsukawa, Kenta*; Hayashi, Naoki; Hirano, Koichiro; Kondo, Yasuhiro; Kosaka, Satoshi*; Miyao, Tomoaki*; Morishita, Takatoshi; Nemoto, Yasuo*; Oguri, Hidetomo

Physical Review Accelerators and Beams (Internet), 26(3), p.032802_1 - 032802_12, 2023/03

https://doi.org/10.1103/PhysRevAccelBeams.26.032802

A bunch-shape monitor (BSM) is a useful device for performing longitudinal beam tuning using the pointwise longitudinal phase distribution measured at selected points in the beam transportation. To measure the longitudinal phase distribution of a low-energy negative hydrogen (H) ion beam, highly oriented pyrolytic graphite (HOPG) was adopted for the secondary-electron-emission target to mitigate the thermal damage due to the high-intensity beam loading. The HOPG target enabled the measurement of the longitudinal phase distribution at the center of a 3-MeV H ion beam with a high peak current of about 50 mA. The longitudinal bunch width was measured using HOPG-BSM at the test stand, which was consistent with the beam simulation. The correlation measurement between the beam transverse and longitudinal planes was demonstrated using HOPG-BSM. The longitudinal Twiss and emittance measurement with the longitudinal Q-scan method was conducted using HOPG-BSM.

Detection limit of electron spin resonance for Japanese deciduous tooth enamel and density separation method for enamel-dentine separation

Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; Osaka, Ken*; Sasaki, Keiichi*; et al.

Journal of Radiation Research (Internet), 63(4), p.609 - 614, 2022/07

AA2021-0724.pdf:0.68MB

https://doi.org/10.1093/jrr/rrac033

Electron spin resonance (ESR) dosimetry is one of the most powerful tools for radiation dose reconstruction. The detection limit of this technique using human teeth is reported to be 56 mGy or 67 mGy; however, the absorbed dose of Fukushima residents after the Fukushima Daiichi Nuclear Power Plant (FNPP) accident was estimated to be lower than this detection limit. Our aim is to assess the absorbed radiation dose of children in Fukushima Prefecture after the accident; therefore, it is important to estimate the detection limit for their teeth. The detection limit for enamel of deciduous teeth of Japanese children separated by the mechanical method is estimated to be 115.0 mGy. The density separation method can effectively separate enamel from third molars of Japanese people. As we have collected thousands of teeth from children in Fukushima, the present technique may be useful to examine their external absorbed dose after the FNPP accident.

Rapid analysis of Sr in cattle bone and tooth samples by inductively coupled plasma mass spectrometry

Koarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Yanagisawa, Kayo*; Terashima, Motoki; Fujiwara, Kenso; Kino, Yasushi*; Oka, Toshitaka; Takahashi, Atsushi*; Suzuki, Toshihiko*; et al.

Journal of Analytical Atomic Spectrometry, 36(8), p.1678 - 1682, 2021/08

https://doi.org/10.1039/D1JA00086A

Rapid analysis of Sr in bone and tooth samples of cattle were achieved by an inductively coupled plasma mass spectrometry (ICP-MS) coupled with mass shift and solid phase extraction techniques. Limit of detection (LOD) in the ICP-MS measurement of 0.1 g samples was lower than that of the radioactivity measurement. Analytical time of the ICP-MS method was reduced from 20 days to 11 hours, compared with the radiometric method. Therefore, the ICP-MS method can be rapid and useful procedure of Sr in small bone and tooth samples derived from terrestrial animals.

Bunch-size measurement of the high-intensity H beam with 3 MeV by the bunch-shape monitor

Kitamura, Ryo; Futatsukawa, Kenta*; Hayashi, Naoki; Hirano, Koichiro; Kondo, Yasuhiro; Kosaka, Satoshi*; Miyao, Tomoaki*; Nemoto, Yasuo*; Morishita, Takatoshi; Oguri, Hidetomo

JPS Conference Proceedings (Internet), 33, p.011012_1 - 011012_6, 2021/03

https://doi.org/10.7566/JPSCP.33.011012

The new bunch shape monitor (BSM) is required to measure the bunch size of the high-intensity H beam with 3 MeV at the front-end section in the J-PARC linac. The carbon-nano tube wire and the graphene stick are good candidates for the target wire of the BSM, because these materials have the enough strength to detect the high-intensity beam. However, since the negative high voltage of more than a few kV should be applied to the wire in the BSM, the suppression of the discharge is the challenge to realize the new BSM. After the high-voltage test to investigate the effect of the discharge from the wire, the detection of the signal from the BSM was successful at the beam core with the peak current of 55 mA using the graphene stick. The preliminary result of the bunch-size measurement is reported in this presentation.

External exposure dose estimation by electron spin resonance technique for wild Japanese macaque captured in Fukushima Prefecture

Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Mitsuyasu, Yusuke*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; Osaka, Ken*; et al.

Radiation Measurements, 134, p.106315_1 - 106315_4, 2020/06

https://doi.org/10.1016/j.radmeas.2020.106315

The relationship between the CO radical intensity and the absorbed dose (dose response curve) of tooth enamel of Japanese macaque was observed by electron spin resonance and the detection limit of our system was estimated to be 33.5 mGy, which is comparable to the detection limit for human molar teeth. Using the dose response curve, external exposure dose for seven wild Japanese macaques captured in Fukushima prefecture were examined. The results suggest that the external exposure dose for the wild Japanese macaques were ranged between 45 mGy to 300 mGy.

Development of evaluation method for variability of groundwater flow conditions associated with long-term topographic change and climate perturbations

Onoe, Hironori; Kosaka, Hiroshi*; Matsuoka, Toshiyuki; Komatsu, Tetsuya; Takeuchi, Ryuji; Iwatsuki, Teruki; Yasue, Kenichi

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 26(1), p.3 - 14, 2019/06

https://doi.org/10.3327/jnuce.26.1_3

In this study, it is focused on topographic changes due to uplift and denudation, also climate perturbations, a method which is able to assess the long-term variability of groundwater flow conditions using the coefficient variation based on some steady-state groundwater flow simulation results was developed. Spatial distribution of long residence time area which is not much influenced due to long-term topographic change and recharge rate change during the past one million years was able to estimate through the case study of the Tono area, Central Japan. By applying this evaluation method, it is possible to identify the local area that has low variability of groundwater flow conditions due to topographic changes and climate perturbations from the regional area quantitatively and spatially.

Development of methodology for the characterisation of the long-term geosphere evolution, 2; Estimation of the long-term evolution of groundwater flow conditions in a Tono area case study

Kosaka, Hiroshi; Saegusa, Hiromitsu; Yasue, Kenichi; Kusano, Tomohiro; Onoe, Hironori

Proceedings of 19th International Conference on Nuclear Engineering (ICONE-19) (CD-ROM), 9 Pages, 2011/10

The methodology for estimation of the long-term evolution of groundwater flow conditions are being developed using approaches on the basis of deductive and inductive methods in the case of Tono area. Based on the studies using the approach on the basis of deductive method, it has been confirmed that the method combining physical modeling of topographic change and groundwater flow simulations is useful for estimating of changes in groundwater flow conditions in the future due to topographic and climatic perturbations. Existing information for estimation of surface hydrological conditions, which are to be used for assignment of boundary conditions for the groundwater flow simulation, has been gathered from many sources and reviewed based on modern-analogue methods. In the studies using the approach on the basis of inductive method, paleo-hydrogeological studies have been carried out on several spatial and time scales. Through the study on the largest spatial scale, a methodology needed to understand changes of groundwater flow conditions due to long-term topographic change is proposed to efficiently identify the area to be carried out site characterization involving field investigations. And then, information to estimate the paleo-topography and paleo-climate has been obtained from literature surveys and field investigations. Through these studies, it has been confirmed that these two approaches are useful for estimation of the long-term evolution of deep groundwater flow conditions.

External exposure dose of Japanese macaque captured in Fukushima prefecture

Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Mitsuyasu, Yusuke*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; Osaka, Ken*; et al.

no journal, , 

Due to the Fukushima Daiichi Nuclear Power Plant accident, the exposure dose estimation for human is examined by the whole body counter or by the Fukushima Health Management Survey, however, the precise estimated dose cannot obtained by such methods. We applied electron spin resonance (ESR) dosimetry for the external dose estimation using tooth enamel of human/animal. As we reported last year, we improved the detection limit of ESR dosimetry down to 43 mGy. We used this improved ESR dosimetry system and attempted to estimate the external dose of wild Japanese macaque capture in Fukushima prefecture, however, the metal component which may obstruct the ESR measurement was observed, so that we cannot estimate the external dose. In this work, we investigated how to remove such metal components, obtain the clear ESR spectrum, and estimate the external dose.

Dose estimation for animals exposed low dose using their teeth

Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.

no journal, , 

The improvement of the ESR dosimetry is required to apply that for the low-dose exposure of wild animals. We will report our progress of the improvement, and compare the external exposure dose estimated by the ESR dosimetry technique and the calculated result based on the external exposure dose rate of the captured point.