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Journal Articles

Experiment and numerical simulation of pulsation flow in single channel for Li-7 enrichment technology development by MCCCE method

Horiguchi, Naoki; Yoshida, Hiroyuki; Kitatsuji, Yoshihiro; Hasegawa, Makoto*; Kishimoto, Tadafumi*

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 7 Pages, 2023/05

From the viewpoint of energy security in Japan and reduction of the environmental load, continuous operation of light water reactors is essential. Since a pH adjuster with enriched Li-7 ions is required for water quality control on PWR, the development of Li-7 enrichment technology is one of the key issues. The multi-channel counter-current electrophoresis (MCCCE) method has been developed as the technology with a low environmental load. To put this method into practical use, it is necessary to understand Li-7 ion behavior in the channel flow and optimize the experimental condition to separate Li-7 and its isotope. In this paper, to understand Li-7 ion behavior in a single channel of the experimental apparatus, a numerical simulation method based on a computational fluid dynamics (CFD) code with a particle tracking method, TPFIT-LPT, was developed. In the method, the motion of multiple ions under the electric field was simulated as a particle with an added velocity by the electric field. The difference in the isotopes was represented by changing of the magnitude of the added velocity. We also considered that although it is impossible to measure the behavior of each ion, it is important to measure the flow velocity of the bulk fluid for the validation of the numerical simulation. We developed a lab-scale experimental apparatus in which the single channel of the actual apparatus was simplified to measure the flow velocity by Particle Image Velocimetry (PIV). We set a pulsation flow condition on the lab-scale experiment, which is one of difficult conditions for the numerical simulation, and measured the velocity. As the result, we confirmed that the pulsation flow was reproduced. We set the measured data as the inlet boundary condition of the numerical simulation and conducted it. As the numerical result, we confirmed the ions affected by the electric field moved upstream with pulsation. We also confirmed the effect of the electric field on the motion of the isotope.

JAEA Reports

Interim activity status report of "the group for investigation of reasonable safety assurance based on graded approach" (from September, 2019 to September, 2020)

Yonomoto, Taisuke; Nakashima, Hiroshi*; Sono, Hiroki; Kishimoto, Katsumi; Izawa, Kazuhiko; Kinase, Masami; Osa, Akihiko; Ogawa, Kazuhiko; Horiguchi, Hironori; Inoi, Hiroyuki; et al.

JAEA-Review 2020-056, 51 Pages, 2021/03

JAEA-Review-2020-056.pdf:3.26MB

A group named as "The group for investigation of reasonable safety assurance based on graded approach", which consists of about 10 staffs from Sector of Nuclear Science Research, Safety and Nuclear Security Administration Department, departments for management of nuclear facility, Sector of Nuclear Safety Research and Emergency Preparedness, aims to realize effective graded approach (GA) about management of facilities and regulatory compliance of JAEA. The group started its activities in September, 2019 and has had discussions through 10 meetings and email communications. In the meetings, basic ideas of GA, status of compliance with new regulatory standards at each facility, new inspection system, etc were discussed, while individual investigation at each facility were shared among the members. This report is compiled with expectation that it will help promote rational and effective safety management based on GA by sharing contents of the activity widely inside and outside JAEA.

JAEA Reports

Safety measures in the melting facilities of The Advanced Volume Reduction Facilities; Document collection of discussion meetings related to melting facilities

Iketani, Shotaro; Yokobori, Tomohiko; Ishikawa, Joji; Yasuhara, Toshiyuki*; Kozawa, Toshiyuki*; Takaizumi, Hirohide*; Momma, Takeshi*; Kurosawa, Shingo*; Iseda, Hirokatsu; Kishimoto, Katsumi; et al.

JAEA-Review 2018-016, 46 Pages, 2018/12

JAEA-Review-2018-016.pdf:12.79MB

Japan Atomic Energy Agency (JAEA) adopts melting process for the waste processing and packaging method of radioactive miscellaneous solid waste in NSRI because melting process is effective in radioactivity evaluation, volume reduction, and stabilization treatment. Metal melting processing facilities, Incinerator, and Nonmetal melting processing facilities (hereinafter referred to as melting process facilities) have taken lots of safety measures, including measures for preventing the recurrence of the fire accidents. To exchange opinions and discuss the validity of these measures and so on with internal personnel and external experts, "Discussions on Melting Process Facilities" was held. As a document collection, this paper summarizes presentation materials of discussion meetings. Presentation materials describe "Outline of AVRF", "Safety measures in the melting facilities in WVRF", "Operation management of the melting facilities in WVRF", "Comparison of the past accident cases between facilities in and outside Japan and WVRF", and "Introduction of past accident cases and safety measures in other facilities from each committee".

JAEA Reports

Pretreatment works for disposal of radioactive wastes produced by research activities, 1

Ishihara, Keisuke; Yokota, Akira; Kanazawa, Shingo; Iketani, Shotaro; Sudo, Tomoyuki; Myodo, Masato; Irie, Hirobumi; Kato, Mitsugu; Iseda, Hirokatsu; Kishimoto, Katsumi; et al.

JAEA-Technology 2016-024, 108 Pages, 2016/12

JAEA-Technology-2016-024.pdf:29.74MB

Radioactive isotope, nuclear fuel material and radiation generators are utilized in research institutes, universities, hospitals, private enterprises, etc. As a result, various low-level radioactive wastes (hereinafter referred to as non-nuclear radioactive wastes) are produced. Disposal site for non-nuclear radioactive wastes have not been settled yet and those wastes are stored in storage facilities of each operator for a long period. The Advanced Volume Reduction Facilities (AVRF) are built to produce waste packages so that they satisfy requirements for shallow underground disposal. In the AVRF, low-level beta-gamma solid radioactive wastes produced in the Nuclear Science Research Institute are mainly treated. To produce waste packages meeting requirements for disposal safely and efficiently, it is necessary to cut large radioactive wastes into pieces of suitable size and segregate those depending on their types of material. This report summarizes activities of pretreatment to dispose of non-nuclear radioactive wastes in the AVRF.

Journal Articles

Contrast variation by dynamic nuclear polarization and time-of-flight small-angle neutron scattering, 1; Application to industrial multi-component nanocomposites

Noda, Yohei*; Koizumi, Satoshi*; Masui, Tomomi*; Mashita, Ryo*; Kishimoto, Hiromichi*; Yamaguchi, Daisuke; Kumada, Takayuki; Takata, Shinichi; Oishi, Kazuki*; Suzuki, Junichi*

Journal of Applied Crystallography, 49(6), p.2036 - 2045, 2016/12

 Times Cited Count:19 Percentile:78.21(Chemistry, Multidisciplinary)

Journal Articles

Effects of ultra-intense laser driven proton beam on the hydriding property of palladium

Abe, Hiroshi; Orimo, Satoshi; Kishimoto, Masahiko*; Aone, Shigeo*; Uchida, Hirohisa*; Daido, Hiroyuki; Oshima, Takeshi

Nuclear Instruments and Methods in Physics Research B, 307, p.218 - 220, 2013/07

 Times Cited Count:1 Percentile:11.48(Instruments & Instrumentation)

We investigated the structure changes of a hydrogen storage alloy by ion irradiations, and its absorption property in order to obtain basic data and to elucidate relevant mechanisms of hydrogen absorption by the influence of the irradiation. In previous studies, the induction of vacancies in a hydrogen absorption alloy was found to be effective to increase in the hydrogen absorption rate. As well known, the rate of hydrogen absorption strongly depends upon the surface state of a hydrogen storage alloy because the dissociation of hydrogen molecules or water molecules needs electron change with the surface in the H$$_{2}$$ gas or electrochemical reaction process. In this study, ion irradiations were made at a room temperature using the laser driven proton beam method, at Kansai Photon Science Institute, Japan Atomic Energy Agency. The beam treatment has several unique properties such as short pulse duration, high peak current, low transverse emittance, and wide energy range from KeV to MeV. The irradiation was used to modify the alloy surface using this equipment. From obtained results, the initial hydrogen absorption rate was found improved by the laser driven proton beam rather more effectively than a mono-energetic proton beam. Discussion is made on the correlation among proton irradiation (laser driven proton or mono-energetic proton) and the initial hydrogen absorption rate of the alloy. We argue about the usefulness of an energy spread beam.

Journal Articles

Development of the X-ray interferometer and the method of spatial and temporal synchronization of XRL and optical pulse

Hasegawa, Noboru; Ochi, Yoshihiro; Kawachi, Tetsuya; Terakawa, Kota*; Tomita, Takuro*; Yamamoto, Minoru; Nishikino, Masaharu; Oba, Toshiyuki; Kaihori, Takeshi; Imazono, Takashi; et al.

X-Ray Lasers 2010; Springer Proceedings in Physics, Vol.136, p.353 - 358, 2011/12

The understanding of the dynamics of the initial process is important for the micro processing and welding by the ultra-short laser pulse. The X-ray laser is suitable for probing this initial process because it has short wavelength (Ni-like Ag, 13.9 nm) and short duration (7 ps). For this investigation, the origin of time of the pumping pulse is quite important. In this study, we used the scintillation plate and the plasma gate technique to realize the spatial and temporal synchronization of the pump and probe pulses. For the spatial alignment, a CsI scintillation plate that was set at the sample position was illuminated by both the X-ray laser pulse, and the fluorescence light were detected by the CCD camera. For the temporal synchronization, we set a thin foil at the sample position. We measured the transmission of the X-ray laser while changing a temporal delay of the pumping laser with respect to the time of X-ray laser pulse to obtain the origin of the irradiation time.

Journal Articles

Source development and novel applications of laser-driven plasma X-ray lasers in JAEA

Kawachi, Tetsuya; Hasegawa, Noboru; Nishikino, Masaharu; Ishino, Masahiko; Imazono, Takashi; Oba, Toshiyuki; Kaihori, Takeshi; Kishimoto, Maki; Ochi, Yoshihiro; Tanaka, Momoko; et al.

X-Ray Lasers 2010; Springer Proceedings in Physics, Vol.136, p.15 - 24, 2011/12

This paper reviews recent improvement in the source development of laser-driven X-ray lasers and the applications in the research fields of material science, laser processing, X-ray imaging, and radiation damage in biological cells. In the application for material science, we have firstly observed temporal correlation between the domain structures of ferro-electric substance under the Curie temperature. In the laser processing, new X-ray laser interferometer reveals us the nano-scale surface distortion of substance pumped by a femto-second optical pulse. In the X-ray diffraction image, we have taken several static images of micro-structure of samples: now we are trying to extend the objective to nano-scale dynamics using pump and probe method. In the radiation damage of biological cells, we observed double strand break in DNA using X-ray laser exposure; this results are compared with the case using incoherent several KeV X-ray exposure.

JAEA Reports

Clearance of concrete generated from modification activities of JRR-3; Method for measuring and evaluating of radioactivity concentration

Satoyama, Tomonori; Kishimoto, Katsumi; Hoshi, Akiko; Takaizumi, Hirohide; Tsutsumi, Masahiro; Inanobe, Hiroshi; Yoshimori, Michiro

JAEA-Technology 2011-003, 53 Pages, 2011/03

JAEA-Technology-2011-003.pdf:1.6MB

In Nuclear Science Research Institute, clearance activities for extremely low-level radioactive concrete debris, which were generated from the modification activities of JRR-3 from FY 1985 to FY 1989 and now are stored in the waste storage facility NL, have been carried out in order to plan reasonable disposal and effectively reusing of concrete waste, moreover to secure storage capacity at the waste storage facilities. Method for measuring and evaluating of radioactivity concentration was applied for approval of Minister of MEXT on November 8, 2007, approved on July 25, 2008. After that the necessary equipments for clearance works were equipped and operational safety progress and manuals for clearance works were prepared. So clearance works were started in FY 2009. This report summarizes the method for measuring and evaluating of radioactivity concentration for concrete generated from modification activities of JRR-3.

JAEA Reports

High density electric survey around the Horonobe Underground Research Laboratory, 3

Nakamura, Takahiro; Sanada, Hiroyuki; Sugita, Yutaka; Teshima, Minoru*; Kasagi, Toshio*; Kishimoto, Munemaru*; Deguchi, Tomonori*; Makuuchi, Ayumu*

JAEA-Research 2010-006, 68 Pages, 2010/06

JAEA-Research-2010-006.pdf:33.19MB

The present document is to report the result of geophysical survey by electric survey around a site proposed for the Horonobe Underground Research Laboratory Project at Horonobe-cho, Hokkaido by the Japan Atomic Energy Agency. This Electric survey using pole-pole array in Horonobe Underground Research Laboratory Area was the third survey. Resistivity distribution near surface was about 20 $$Omega$$$$cdot$$m and it become to about 2 $$Omega$$$$cdot$$m as the depth increasing. Resistivity distribution was good agreement with existing survey results and existing electrical resistivity log data. By comparing resistivity model with hydrology model, it was confirmed that resistivity reflected the density of salinity. The range and distribution trends of apparent resistivity in this year were similar to the results of last year. It is thought that the data in which reproducibility is high is acquired in this survey. The influence on the underground water flow by construction is not admitted now.

Journal Articles

Demonstration of submicroJoule, spatially coherent soft-X-ray laser pumped by 0.1 Hertz, 10 Joule, picosecond laser

Ochi, Yoshihiro; Kawachi, Tetsuya; Hasegawa, Noboru; Nishikino, Masaharu; Oba, Toshiyuki; Tanaka, Momoko; Kishimoto, Maki; Kaihori, Takeshi; Nagashima, Keisuke; Sugiyama, Akira

Japanese Journal of Applied Physics, 48(12), p.120212_1 - 120212_3, 2009/12

 Times Cited Count:31 Percentile:73.37(Physics, Applied)

We have demonstrated the fully spatial coherent 13.9-nm laser with output energy of submicroJoule by means of the double target geometry by using new driver system. The power amplifiers providing tow beams with 10-J energy and picoseconds duration at the repetition rate of 0.1 Hz. The obtained 13.9-nm laser pulse with 10$$^{10}$$ coherent photons will enable us to make single-shot pump-probe observation of non-periodic ultrafast phenomena.

Journal Articles

High-precision measurement of the spectral width of the nickel-like molybdenum X-ray laser

Hasegawa, Noboru; Kawachi, Tetsuya; Sasaki, Akira; Yamatani, Hiroshi; Kishimoto, Maki; Ochi, Yoshihiro; Tanaka, Momoko; Nishikino, Masaharu; Kunieda, Yuichi; Nagashima, Keisuke; et al.

Journal of Physics; Conference Series, 163(1), p.012062_1 - 012062_4, 2009/06

 Times Cited Count:2 Percentile:66.91(Physics, Multidisciplinary)

The precise knowledge about the wavelength and the spectral width of the lasing line is important for the applications of X-ray lasers, and especially for the spectral width, it is good benchmark of the atomic code because it depends on the electron collisional excitation and de-excitation rate coefficient. Only a few measurements of the spectral width of the laser line have been reported, because the spectral width of the X-ray laser is so narrow that the required spectral resolution is quite high. In this study, we took the nickel-like molybdenum X-ray laser as an example, and measure the spectral width by use of the high resolution spectrometer in order to compare it with a theoretical one.

JAEA Reports

High density electric survey around the Horonobe Underground Research Laboratory, 2

Nakamura, Takahiro; Sanada, Hiroyuki; Sugita, Yutaka; Teshima, Minoru*; Kishimoto, Munemaru*; Matsuo, Koichi*

JAEA-Research 2008-102, 58 Pages, 2009/03

JAEA-Research-2008-102.pdf:48.97MB

The present document is to report the result of geophysical survey by electric survey around a site proposed for the Horonobe Underground Research Laboratory Project at Horonobe-cho, Hokkaido by the Japan Atomic Energy Agency. This Electric survey using pole-pole array in Horonobe Underground Research Laboratory Area was the second survey. Resistivity distribution near surface was about 20 ohm-m and it become to about 2 ohm-m as the depth increasing. Resistivity distribution was good agreement with existing survey results and existing electrical resistivity log data. By comparing resistivity model with hydrology model, it was confirmed that resistivity reflected the density of salinity. The range and distribution trends of apparent resistivity in this year were similar to the results of last year. It is thought that the data in which reproducibility is high is acquired in this survey. The influence on the underground water flow by construction is not admitted now.

Journal Articles

High-resolution spectroscopy of the nickel-like molybdenum X-ray laser toward the generation of circularly polarized X-ray laser

Hasegawa, Noboru; Sasaki, Akira; Yamatani, Hiroshi; Kishimoto, Maki; Tanaka, Momoko; Ochi, Yoshihiro; Nishikino, Masaharu; Kunieda, Yuichi; Kawachi, Tetsuya; Yoneda, Hitoki*; et al.

Journal of the Optical Society of Korea, 13(1), p.60 - 64, 2009/03

 Times Cited Count:5 Percentile:29.39(Optics)

The precise knowledge about the spectral width of the X-ray laser line is important to generate the circularly polarized X-ray laser. There are three magnetic sub-levels at lower state of the collisional excitation X-ray laser transition of the nickel-like ion X-ray laser medium. The polarization of each transition is circular or linear. Therefore the circularly polarized X-ray laser could be extracted by the influence of the Zeeman effect if the X-ray laser medium was under the external magnetic field. The strength of the magnetic field required for the circularly polarized X-ray laser is determined by the spectral width of the X-ray laser. Only a few measurements of the spectral width of the laser line have been reported, because the spectral width of the X-ray laser is so narrow that the required spectral resolution is quite high. In this study, we took the nickel-like molybdenum X-ray laser as an example and succeeded the measurement of the spectral width of the X-ray laser.

Journal Articles

Frequency filter of seed X-ray by use of X-ray laser medium; Toward the generation of the temporally coherent X-ray laser

Hasegawa, Noboru; Kawachi, Tetsuya; Kishimoto, Maki; Sukegawa, Kota*; Tanaka, Momoko; Tai, R. Z.*; Ochi, Yoshihiro; Nishikino, Masaharu; Nagashima, Keisuke; Kato, Yoshiaki*

Japanese Journal of Applied Physics, 48(1), p.012503_1 - 012503_6, 2009/01

 Times Cited Count:6 Percentile:26.26(Physics, Applied)

We evaluate the characteristics of a higher-order harmonics light as a seed X-ray amplified through the laser-produced X-ray amplifier. Narrow spectral bandwidth of the X-ray amplifier works as the frequency filter of the seed X-ray, resulting in that only the temporally coherent X-ray is amplified. Experimental investigation using the 29th-order harmonic light of the Ti:sapphire laser at a wavelength of 26.9 nm together with the neon-like manganese X-ray laser medium shows obvious spectral narrowing of the seed X-ray and amplification without serious diffraction effects on the propagation of the amplified X-ray beam. This implies that the present combination is potential to realize temporally coherent X-ray lasers, with the expected duration of several 100 fs.

Journal Articles

New driver laser system for double target X-ray lasers at JAEA

Ochi, Yoshihiro; Hasegawa, Noboru; Kawachi, Tetsuya; Nishikino, Masaharu; Tanaka, Momoko; Kishimoto, Maki; Oba, Toshiyuki

X-Ray Lasers 2008; Springer Proceedings in Physics, Vol.130, p.161 - 166, 2009/00

Journal Articles

Development of driver laser system for 0.1-Hz X-ray laser

Ochi, Yoshihiro; Kawachi, Tetsuya; Hasegawa, Noboru; Nagashima, Keisuke; Nishikino, Masaharu; Kishimoto, Maki; Tanaka, Momoko

Reza Kenkyu, 36(APLS), p.1136 - 1138, 2008/12

We have developed a chirped pulse amplification laser with flash lamp pumped zigzag slab Nd:glass amplifiers for pumping the TCE X-ray lasers at 0.1-Hz repetition rate at the Japan Atomic Energy Agency. The laser provided 7 J/1.6 ps main pulse and 1/8 intensity pre-pulse at 1.2 ns before the main pulse. An energy fluctuation at 0.1-Hz operation was 20% (RMS), which was comparable with our present laser using rod amplifiers. The line focus on the target surface was 20 $$mu$$m in the width and 0.8 cm in the length. By using this laser, gain saturated Ni-like silver laser ($$lambda$$ = 13.9 nm) with energy output of $$>$$1 $$mu$$J was obtained. In this case, the gain coefficient (G) was 41.9 cm$$^{-1}$$ up to the plasma length (L) of 0.39 cm, resulting G $$times$$ L = 16.3. The beam divergence of the Ni-like silver laser was $$sim$$3 mrad. Consequently, the peak spectrum brilliance was estimated to be $$>$$10$$^{27}$$ photons/s/mm$$^{2}$$/mrad2/0.1%BW.

Journal Articles

Direct measurement of the temporal profile of the amplification gain of the transient collisional excitation neonlike manganese X-ray laser medium

Hasegawa, Noboru; Kawachi, Tetsuya; Sasaki, Akira; Kishimoto, Maki; Sukegawa, Kota; Tanaka, Momoko; Tai, R. Z.*; Ochi, Yoshihiro; Nishikino, Masaharu; Nagashima, Keisuke; et al.

Physical Review A, 76(4), p.043805_1 - 043805_5, 2007/10

 Times Cited Count:20 Percentile:66.75(Optics)

We firstly demonstrated the measurement of temporal profile of the amplification gain of the transient collisional excitation (TCE) X-ray laser with the solid target by use of X-ray diagnostic beam injection technique. In this experiment, higher-order harmonic light at a wavelength of 26.9 nm was injected into the neon-like manganese plasma as X-ray laser medium, and the amplified signal was observed. The obtained buildup time of the amplification gain was 23 ps measured from the time of the main pumping laser pulse, and the lifetime of the amplification gain was 27 ps. This result was in good agreement with the theoretical simulation by using an atomic kinetics code.

Journal Articles

Enhancement of double auger decay probability in xenon clusters irradiated with a soft-X-ray laser pulse

Namba, Shinichi*; Hasegawa, Noboru; Nishikino, Masaharu; Kawachi, Tetsuya; Kishimoto, Maki; Sukegawa, Kota; Tanaka, Momoko; Ochi, Yoshihiro; Takiyama, Ken*; Nagashima, Keisuke

Physical Review Letters, 99(4), p.043004_1 - 043004_4, 2007/07

 Times Cited Count:32 Percentile:77.84(Physics, Multidisciplinary)

The interaction of large Xe clusters with a soft X-ray laser pulse having a wavelength of 13.9 nm and an intensity of up to 2$$times$$10$$^{10}$$W/cm$$^{2}$$ was investigated using a time-of-flight ion mass spectrometer. It was found that Xe$$^{3+}$$ ions (which result from double Auger decay of 4d vacancies) became the dominant final ionic product with increasing cluster size and X-ray intensity. This is in contrast to the results of synchrotron radiation experiments involving free Xe atoms, in which Xe$$^{2+}$$ is the dominant resultant ion species. Possible mechanisms responsible for the enhancement of the double Auger transition probability in X-ray laser and cluster interaction are discussed.

Journal Articles

Nuclear resonant scattering of synchrotron radiation by Yb nuclides

Masuda, Ryo*; Higashitaniguchi, Satoshi*; Kitao, Shinji*; Kobayashi, Yasuhiro*; Seto, Makoto*; Mitsui, Takaya; Yoda, Yoshitaka*; Haruki, Rie*; Kishimoto, Shunji*

Journal of the Physical Society of Japan, 75(9), p.094716_1 - 094716_4, 2006/09

 Times Cited Count:2 Percentile:19.42(Physics, Multidisciplinary)

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132 (Records 1-20 displayed on this page)