Present status of the JAEA-AMS-TONO (2022FY)

Fujita, Natsuko; Miyake, Masayasu; Matsubara, Akihiro*; Ishii, Masahiro*; Watanabe, Takahiro; Jinno, Satoshi; Nishio, Tomohiro*; Ogawa, Yumi; Kimura, Kenji; Shimada, Akiomi; et al.

Dai-35-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.17 - 19, 2024/03

The JAEA-AMS-TONO facility at the Tono Geoscience Center, JAEA has three accelerator mass spectrometers. We report the present status of the JAEA-AMS-TONO.

Status report of JAEA-AMS-TONO; Research and technical development in the last four years

Kokubu, Yoko; Fujita, Natsuko; Watanabe, Takahiro; Matsubara, Akihiro; Ishizaka, Chika; Miyake, Masayasu*; Nishio, Tomohiro*; Kato, Motohisa*; Ogawa, Yumi*; Ishii, Masahiro*; et al.

Nuclear Instruments and Methods in Physics Research B, 539, p.68 - 72, 2023/06

https://doi.org/10.1016/j.nimb.2023.03.005

The JAEA-AMS-TONO facility at the Tono Geoscience Center, JAEA has an accelerator mass spectrometer (JAEA-AMS-TONO-5MV). The spectrometer enabled us to use a multi-nuclide AMS of carbon-14 (C), beryllium-10, aluminium-26 and iodine-129, and we have recently been proceeding test measurement of chlorine-36. In response to an increase of samples, we installed a state-of-the-art multi-nuclide AMS with a 300 kV Tandetron accelerator in 2020. Recently, we are driving the development of techniques of isobar separation in AMS and of sample preparation. Ion channeling is applied to remove isobaric interference and we are building a prototype AMS based on this technique for downsizing of AMS. The small sample graphitization for C has been attempted using an automated graphitization equipment equipped with an elemental analyzer.

Present status of the JAEA-AMS-TONO (2022FY)

Fujita, Natsuko; Miyake, Masayasu; Matsubara, Akihiro*; Ishii, Masahiro*; Watanabe, Takahiro; Jinno, Satoshi; Nishio, Tomohiro*; Ogawa, Yumi; Yamamoto, Yusuke; Kimura, Kenji; et al.

Dai-23-Kai AMS Shimpojiumu Hokokushu, p.1 - 4, 2022/12

The JAEA-AMS-TONO facility at the Tono Geoscience Center, JAEA has three accelerator mass spectrometers. We report the present status of the JAEA-AMS-TONO.

atomic X-ray spectroscopy using a counter-emulsion hybrid method

Fujita, Manami; Hasegawa, Shoichi; Hosomi, Kenji; Ichikawa, Masaya; Ichikawa, Yudai; Kim, S.; Nanamura, Takuya; Sako, Hiroyuki; Tamura, Hirokazu; Yamamoto, Takeshi; et al.

Progress of Theoretical and Experimental Physics (Internet), 2022(12), p.123D01_1 - 123D01_17, 2022/12

https://doi.org/10.1093/ptep/ptac156

Measurement of differential cross sections for elastic scattering in the momentum range 0.44-0.80 GeV/c

Nanamura, Takuya; Fujita, Manami; Hasegawa, Shoichi; Ichikawa, Masaya; Ichikawa, Yudai; Imai, Kenichi*; Naruki, Megumi; Sato, Susumu; Sako, Hiroyuki; Tamura, Hirokazu; et al.

Progress of Theoretical and Experimental Physics (Internet), 2022(9), p.093D01_1 - 093D01_35, 2022/09

https://doi.org/10.1093/ptep/ptac101

Development of emergency monitoring system for alpha-particle-emitting radionuclides in the air

Hokama, Tomonori; Fujita, Hiroki; Nakano, Masanao; Iimoto, Takeshi*

Radiation Protection Dosimetry, 196(3-4), p.136 - 140, 2021/11

https://doi.org/10.1093/rpd/ncab139

During the early phase of a nuclear accident, major radioactive materials are released into the environment, necessitating the prompt deployment of various protective actions to avoid or reduce radiation exposure. To implement these actions, the levels of radioactivity in the environment should be determined. However, the radioactivity concentrations of artificial alpha-particle-emitting radionuclides such as plutonium are difficult to measure in airborne samples, because they are interfered with natural radionuclides such as uranium decay products. Therefore, chemical separation is required to measure the concentrations. This study presents a new emergency monitoring system for airborne samples, which performs multiple-pulse time-interval analysis (MTA) without chemical separation. The system is used in conjunction with an alpha/beta-particle survey meter and adopted an analysis method focusing on the detected time interval of each particle. Its features are that a short time to output measurement result, easy handling and nondestructive. The estimated detection limit of the system was 9.510 Bq m. The MTA-based monitoring system could be useful in situations requiring prompt measurement and screening of samples.

Measurement of the differential cross sections of the elastic scattering in momentum range 470 to 850 MeV/

Miwa, Koji*; Fujita, Manami; Hasegawa, Shoichi; Hosomi, Kenji; Ichikawa, Yudai; Imai, Kenichi*; Nanamura, Takuya; Naruki, Megumi; Sako, Hiroyuki; Sato, Susumu; et al.

Physical Review C, 104(4), p.045204_1 - 045204_20, 2021/10

https://doi.org/10.1103/PhysRevC.104.045204

Manufacture of substitutive assemblies for MONJU reactor decommissioning

Sakakibara, Hiroshi; Aoki, Nobuhiro; Muto, Masahiro; Otabe, Jun; Takahashi, Kenji*; Fujita, Naoyuki*; Hiyama, Kazuhiko*; Suzuki, Hirokazu*; Kamogawa, Toshiyuki*; Yokosuka, Toru*; et al.

JAEA-Technology 2020-020, 73 Pages, 2021/03

JAEA-Technology-2020-020.pdf:8.26MB

The decommissioning is currently in progress at the prototype fast breeder reactor Monju. Fuel assemblies will be taken out of its core for the first step of the great task. Fuel assemblies stand on their own spike plugged into a socket on the core support plate and support with adjacent assemblies through their housing pads each other, resulting in steady core structure. For this reason, some substitutive assemblies are necessary for the purpose of discharging the fuel assemblies of the core. Monju side commissioned, therefore, Plutonium Fuel Development Center to manufacture the substitutive assemblies and the Center accepted it. This report gives descriptions of design, manufacture, and shipment in regard to the substitutive assemblies.

Study of identification method by the reaction for a scattering experiment at J-PARC

Sakao, Tamao*; Fujita, Manami; Hasegawa, Shoichi; Hosomi, Kenji; Ichikawa, Masaya; Ichikawa, Yudai; Imai, Kenichi*; Nanamura, Takuya; Naruki, Megumi; Sako, Hiroyuki; et al.

JPS Conference Proceedings (Internet), 33, p.011133_1 - 011133_6, 2021/03

https://doi.org/10.7566/JPSCP.33.011133

Supercritical water pretreatment method for analysis of strontium and uranium in soil (Andosols)

Nagaoka, Mika; Fujita, Hiroki; Aida, Taku*; Guo, H.*; Smith, R. L. Jr.*

Applied Radiation and Isotopes, 168, p.109465_1 - 109465_6, 2021/02

https://doi.org/10.1016/j.apradiso.2020.109465

The radioactivities in the environmental samples are analyzed to monitor the nuclear power facilities. The pretreatment of radioactive nuclides of alpha and beta emitters in the environmental samples is performed with acid to decompose organic matter and extract object nuclide such as Sr, U and Pu. However, the pretreatment methods are time-consuming and used many concentrated acid solutions that are unsafe and hazardous. Therefore, we develop to the new pretreatment method using supercritical water instead of acid. Hydrothermal pretreatment of soils (Andosols) from Ibaraki prefecture (Japan) was used to improve methods for monitoring radioactive Sr and U. Calcined samples were pretreated with subcritical or supercritical water (SCW) followed by extraction with 0.5 M HNO solutions. With SCW pretreatment, recoveries of Sr and U were 70% and 40%, respectively. Experimental recoveries obtained can be described by a linear relationship in water density. The proposed method is robust and can lower environmental burden of routine analytical protocols.