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Kokubun, Yuji; Hosomi, Kenji; Inoue, Kazumi; Koike, Yuko; Uchiyama, Rei; Sasaki, Kazuki; Maehara, Yushi; Matsuo, Kazuki; Uesugi, Misaki; Yamashita, Daichi; et al.
JAEA-Review 2025-057, 168 Pages, 2026/03
JAEA-Review-2025-057.pdf:2.43MB
The Nuclear Fuel Cycle Engineering Laboratories conducts environmental radiation monitoring around the reprocessing plant in accordance with the "Safety Regulations for Reprocessing Plant of JAEA, Part IV: Environmental Monitoring". This report summarizes the results of environmental radiation monitoring conducted during the period from April 2024 to March 2025 and the results of dose calculations for the surrounding public due to the release of radioactive materials from the plant into the atmosphere and ocean. In the results of the above environmental radiation monitoring, several items were affected by radioactive materials emitted from the accident at the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Company, Incorporated (changed to Tokyo Electric Power Holdings, Inc. on April 1, 2016), which occurred in March 2011. Also included as appendices are an overview of the environmental monitoring plan, an overview of measurement methods, measurement results and their changes over time, meteorological statistics results, radioactive waste release status, and an evaluation of the data which deviated of the normal range.
Kokubun, Yuji; Hosomi, Kenji; Nagaoka, Mika; Seya, Natsumi; Inoue, Kazumi; Koike, Yuko; Uchiyama, Rei; Sasaki, Kazuki; Maehara, Yushi; Matsuo, Kazuki; et al.
JAEA-Review 2024-054, 168 Pages, 2025/03
JAEA-Review-2024-054.pdf:2.73MB
The Nuclear Fuel Cycle Engineering Laboratories conducts environmental radiation monitoring around the reprocessing plant in accordance with the "Safety Regulations for Reprocessing Plant of JAEA, Part IV: Environmental Monitoring". This report summarizes the results of environmental radiation monitoring conducted during the period from April 2023 to March 2024 and the results of dose calculations for the surrounding public due to the release of radioactive materials from the plant into the atmosphere and ocean. In the results of the above environmental radiation monitoring, several items were affected by radioactive materials emitted from the accident at the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Company, Incorporated (changed to Tokyo Electric Power Holdings, Inc. on April 1, 2016), which occurred in March 2011. In addition, environmental monitoring plan, analysis and measurement methods, monitoring data and their chronological change, meteorological data after statistical processing, status of radioactive waste release and evaluation results of the data over the normal range are included as appendices.
Uchida, Shunsuke; Hata, Kuniki; Hanawa, Satoshi
JAEA-Data/Code 2024-003, 119 Pages, 2025/01
JAEA-Data-Code-2024-003.pdf:11.29MB
JAEA-Data-Code-2024-003-appendix(CD-ROM).zip:0.28MB
The calculation code for determining corrosive circumstance in light water reactors, WRAC-JAEA, has been developed based on water radiolysis calculation codes for BWR. The code has involved several new calculation functions to apply it for PWR, i.e., (1) high temperature pH (pH
), (2) pH effects on water radiolysis, (3) electrochemical corrosion potential (ECP) based on the mixed potential theory, and (4) ECP based on the water radiolysis calculation results. Moderation of corrosive conditions in the primary cooling systems is one of the promising procedures to mitigate the loss of reliabilities of major components in the systems, especially in aging plants. However, water chemistry control for corrosive environment mitigation procedures are much different in BWRs and PWRs. In BWRs, intergranular stress corrosion cracking (IGSCC) of stainless steel is the dominant causes for determining plant reliability. It is difficult to increase pH and injected hydrogen amounts due to direct power cycle operation. So, precise control of hydrogen injection with supported by water radiolysis and ECP analyses has been carried out to keep material reliability. In PWRs, it is possible to maintain stable control of corrosive circumstances with higher pH and sufficiently large hydrogen concentration. Recently, it was pointed out that one of the major causes of primary water stress corrosion cracking (PWSCC) of nickel alloys was hydrogen. The optimal hydrogen concentration should be evaluated to mitigate ECP without increasing hydrogen concentration. For this, a combined water radiolysis and ECP analysis code is required to determine the suitable hydrogen concentration and ECP. WRAC-JAEA can contribute not only to evaluation of corrosive conditions each of BWR and PWR, but also to prepare for suitable countermeasures for both BWR and PWR by cross-talking the knowledge and experience with assistance of the code results.
Cu
Oy thin films under longitudinal magnetic field by using heavy-ion irradiationSueyoshi, Tetsuro*; Enokihata, Ryusei*; Yamaguchi, Hiroshi*; Semboshi, Satoshi*; Ozaki, Toshinori*; Sakane, Hitoshi*; Nishizaki, Terukazu*; Ishikawa, Norito
Superconductor Science and Technology, 37(7), p.075010_1 - 075010_7, 2024/06
Times Cited Count：1 Percentile：14.28(Physics, Applied)We attempted to improve the critical current density (Jc) under a longitudinal magnetic field (LMF) by using columnar defects (CDs) tilted toward the transport current, where the CDs were produced with 80 MeV Xe ions at an incident angle(s) up to 87.5 degree relative to the c-axis of YBaCuOy thin films. The formation of CDs extending throughout the film was confirmed by cross-sectional transmission electron microscopy. The CDs tilted at 87.5 degree weakened the magnetic field dependence of Jc under the LMF, providing a Jc higher than that of the unirradiated film in a high magnetic field. This is the first study to demonstrate that CDs and/or irradiation defects contribute to flux pinning under the LMF in high-Tc superconductors.
Hata, Kuniki; Hanawa, Satoshi; Chimi, Yasuhiro; Uchida, Shunsuke
Journal of Nuclear Science and Technology, 61(4), p.448 - 458, 2024/04
Times Cited Count：1 Percentile：15.37(Nuclear Science & Technology)no abstracts in English
Hata, Kuniki; Hanawa, Satoshi; Chimi, Yasuhiro; Uchida, Shunsuke; Lister, D. H.*
Journal of Nuclear Science and Technology, 60(8), p.867 - 880, 2023/08
Times Cited Count：2 Percentile：22.44(Nuclear Science & Technology)One of the major subjects for evaluating the corrosive conditions in the PWR primary coolant was to determine the optimal hydrogen concentration for mitigating PWSCC without any adverse effects on major structural materials. As suitable procedures for evaluating the corrosive conditions in PWR primary coolant, a couple of procedures, i.e., water radiolysis and ECP analyses, were proposed. The previous article showed the radiolysis calculation in the PWR primary coolant, which was followed by an ECP study here. The ECP analysis, a couple of a mixed potential model and an oxide layer growth model, was developed originally for BWR conditions, which was extended to PWR conditions with adding Li
(Na) and H effects on the anodic polarization curves. As a result of comparison of the calculated results with INCA in-pile-loop experiment data as well as other experimental data, it was confirmed that the ECPs calculated with the coupled analyses agreed with the measured within 
100mV discrepancies.
Hata, Kuniki; Uchida, Shunsuke; Hanawa, Satoshi; Chimi, Yasuhiro; Sato, Tomonori
Proceedings of 21st International Conference on Environmental Degradation of Materials in Nuclear Power Systems - Water Reactors (Internet), 14 Pages, 2023/08
Hata, Kuniki; Uchida, Shunsuke; Hanawa, Satoshi; Chimi, Yasuhiro
Proceedings of International Symposium on Contribution of Materials Investigations and Operating Experience to LWRs' Safety, Performance and Reliability (Fontevraud 10) (Internet), 11 Pages, 2022/00
Hanawa, Satoshi; Hata, Kuniki; Chimi, Yasuhiro; Kasahara, Shigeki
Proceedings of 21st International Conference on Water Chemistry in Nuclear Reactor Systems (Internet), 12 Pages, 2019/09
Kasahara, Shigeki; Chimi, Yasuhiro; Hata, Kuniki; Hanawa, Satoshi
Zairyo To Kankyo, 68(9), p.240 - 247, 2019/09
In order to study environment assisted cracking mechanism of stainless steel under BWR primary coolant condition, effects of applied load on oxidation in the vicinity of crack tips of CT specimens were evaluated. Loaded CT specimens were immersed in an aqueous condition at 290
C as a simulated BWR coolant condition, and microstructural observation on oxide near the tips of pre-cracks was carried out. Oxide inner layers, which consisted of fine grain magnetite containing Fe and Cr were formed, and oxide outer layers consisting of large grains of FeO
were observed to cover the inner layers. FEM analysis of stress and strain in the loaded CT specimen suggests that both of dislocations due to localized plastic deformation and elastic strain could play important roles to accelerate inner oxide formation in the vicinity of the crack tip of the specimens.
Kim, J.*; Yamanaka, Satoru*; Nakajima, Akira*; Kato, Takanori*; Kim, Y.*; Fukuda, Tatsuo; Yoshii, Kenji; Nishihata, Yasuo; Baba, Masaaki*; Takeda, Masatoshi*; et al.
Advanced Sustainable Systems (Internet), 2(11), p.1800067_1 - 1800067_8, 2018/11
Times Cited Count：8 Percentile：24.99(Green & Sustainable Science & Technology)Moro, Takuya*; Kim, J.*; Yamanaka, Satoru*; Murayama, Ichiro*; Kato, Takanori*; Nakayama, Tadachika*; Takeda, Masatoshi*; Yamada, Noboru*; Nishihata, Yasuo; Fukuda, Tatsuo; et al.
Journal of Alloys and Compounds, 768, p.22 - 27, 2018/11
Times Cited Count：20 Percentile：61.68(Chemistry, Physical)
and Br and its effect on corrosion of a low-alloy steelHata, Kuniki; Inoue, Hiroyuki*; Kojima, Takao*; Kasahara, Shigeki; Hanawa, Satoshi; Ueno, Fumiyoshi; Tsukada, Takashi; Iwase, Akihiro*
Proceedings of Symposium on Water Chemistry and Corrosion in Nuclear Power Plants in Asia 2017 (AWC 2017) (USB Flash Drive), p.304 - 314, 2017/09
A model simulation of 
radiolysis of mixed solutions of NaCl and NaBr was carried out. The simulation result agreed well with the experimental result, and Br played an important role in determining the amounts of products from water radiolysis. The simulation result also showed that, in highly pure NaCl solutions, the steady-state concentration of a radolytic product, HO, was mainly controlled by three reactions (Cl + 
OH 
ClOH
, ClOH Cl + OH, and ClOH + H Cl + HO), which indicated that accurate evaluation of the rate constants of these reactions was very important in improving the radiolysis simulation of solutions containing Cl. An immersion test using a low-alloy steel, SQV2A, in the mixed solutions was also carried out under irradiation. The corrosion rate increased or decreased depending on the pH or the concentrations of the halide ions in a similar way to the change in concentration of HO produced from water radiolysis, which is affected by the presence of Cl and Br. However, at high pH values (
12), the corrosion rate was almost zero even though the concentration of HO was high. This could be attributed to enhancement of the passivity of test specimens at higher pH values.
Kim, J.*; Yamanaka, Satoru*; Nakajima, Akira*; Kato, Takanori*; Kim, Y.*; Fukuda, Tatsuo; Yoshii, Kenji; Nishihata, Yasuo; Baba, Masaaki*; Takeda, Masatoshi*; et al.
Ferroelectrics, 512(1), p.92 - 99, 2017/08
Times Cited Count：15 Percentile：52.27(Materials Science, Multidisciplinary)Yamanaka, Satoru*; Kim, J.*; Nakajima, Akira*; Kato, Takanori*; Kim, Y.*; Fukuda, Tatsuo; Yoshii, Kenji; Nishihata, Yasuo; Baba, Masaaki*; Yamada, Noboru*; et al.
Advanced Sustainable Systems (Internet), 1(3-4), p.1600020_1 - 1600020_6, 2017/04
no abstracts in English
Wu, H.-Y.*; Takahashi, Shigeo*; Miyamura, Hiroko; Ozahata, Satoshi*; Nakao, Akihiro*
Electronic Imaging, 2017(1), p.118 - 130, 2017/01
Extracting hierarchical structures from networks provides us with an effective means of visualizing them, especially when they contain complicated node connectivities such as those in traffic and distributed networks. This paper presents an algorithm for inferring such partial orders by optimizing the network hierarchies along flow paths that are given as input. We study several network examples to demonstrate the feasibility of the proposed approach including course dependency charts, railway networks, and P2P networks.
Wu, H.-Y.*; Takahashi, Shigeo*; Miyamura, Hiroko; Ozahata, Satoshi*; Nakao, Akihiro*
Journal of Imaging Science and Technology, 60(6), p.060407_1 - 060407_13, 2016/11
Times Cited Count：0 Percentile：0.00(Imaging Science & Photographic Technology)Extracting hierarchical structures from networks provides us with an effective means of visualizing them, especially when they contain complicated node connectivities such as those in traffic and distributed networks. This paper presents an algorithm for inferring such partial orders by optimizing the network hierarchies along flow paths that are given as input. We study several network examples to demonstrate the feasibility of the proposed approach including course dependency charts, railway networks, and P2P networks.
Hanawa, Satoshi; Uchida, Shunsuke; Hata, Kuniki; Chimi, Yasuhiro; Kasahara, Shigeki*; Nishiyama, Yutaka
Proceedings of 20th Nuclear Plant Chemistry International Conference (NPC 2016) (USB Flash Drive), 11 Pages, 2016/10
ECP is the exclusive index to evaluate corrosion condition directly at the points of interest in the mixing of neutron and -ray environment. ECP can be calculated through the combination of water radiolysis and ECP model. A water radiolysis model have been applied to experiments performed in in-pile loops in the experimental reactors and applicability was confirmed. An ECP model based on the Butler-Volmer equation was also prepared. ECP of stainless steel was measured under well controlled water chemistry condition in in-pile loop in the Halden reactor, and the model was applied to evaluate ECP measured in the Halden reactor. The measured data were well explained by the water radiolysis calculation and ECP model. Accumulation of in-pile ECP data are expected for further validation of the models.
Hanawa, Satoshi; Uchida, Shunsuke; Hata, Kuniki; Chimi, Yasuhiro; Kasahara, Shigeki*; Nishiyama, Yutaka
Proceedings of 20th Nuclear Plant Chemistry International Conference (NPC 2016) (USB Flash Drive), 10 Pages, 2016/10
The authors proposed and ECP evaluation model introducing irradiation-induced diffusion in the oxide layer to simulate neutron irradiation effect, and predicted with this model that ECP is started to depress from the neutron flux of about ten to the fourteenth per square meter. As the JMTR has in-pile loops applicable to water chemistry experiments, degree of irradiation effect on ECP appears in the in-pile loop was estimated by the model. Under oxygen injected condition, ECP in a capsule becomes constant along the vertical direction due to the presence of high amount of oxygen and hydrogen peroxide in a capsule. However, if neutron irradiation depress ECP, ECP in a capsule along vertical direction wouldn't become constant, and the degree to the decrement is detectable by experiments.
Hata, Kuniki; Sato, Tomonori; Motooka, Takafumi; Ueno, Fumiyoshi; Hanawa, Satoshi; Kasahara, Shigeki; Tsukada, Takashi
Journal of Nuclear Science and Technology, 53(8), p.1183 - 1191, 2016/08
Times Cited Count：8 Percentile：53.71(Nuclear Science & Technology)